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41.
This paper explores the role of the secondary inorganic aerosol (SIA) species ammonium,NH4+,nitrate,NO3-,and sulfate,SO24-,during haze and fog events using hourly mass concentrations of PM2.5 measured at a suburban site in Hangzhou,China.A total of 546 samples were collected between 1 April and 8 May 2012.The samples were analyzed and classified as clear,haze or fog depending on visibility and relative humidity (RH).The contribution of SIA species to PM2.5 mass increased to ~50% during haze and fog.The mass contribution of nitrate to PM2.5 increased from 11% during clear to 20% during haze episodes.Nitrate mass exceeded sulfate mass during haze,while near equal concentrations were observed during fog episodes.The role of RH on the correlation between concentrations of SIA and visibility was examined,with optimal correlation at 60%-70% RH.The total acidity during clear,haze and fog periods was 42.38,48.38 and 45.51 nmol m-3,respectively,indicating that sulfate,nitrate and chloride were not neutralized by ammonium during any period.The nitrate to sulfate molar ratio,as a function of the ammonium to sulfate molar ratio,indicated that nitrate formation during fog started at a higher ammonium to sulfate molar ratio compared to clear and haze periods.During haze and fog,the nitrate oxidation ratio increased by a factor of 1.6-1.7,while the sulfur oxidation ratio increased by a factor of 1.2-1.5,indicating that both gaseous NO2 and SO2 were involved in the reduced visibility.  相似文献   
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We discuss the spatial and temporal characteristics of X-ray flares occurring in the active region NOAA2372 from April 6 to 13, 1980. The flares are seen to extend in most cases across the whole active complex, involving several magnetic features. They originate in an intermediate bipole, between the two main sunspots of the active region, where high magnetic shear was detected. A rapid expansion is seen in some cases, in conjunction with the start of the impulsive hard X-ray bursts. We also detect, in the late phases of some of the events, a large soft X-ray structure overlying the whole active region, which also shows up as a noise storm region at metric wavelengths. These large loops cool by heat conduction but, in some cases, Hα condensations seem to appear, probably as a result of magnetic compression and a condensation mode of the thermal instability. The topological aspects of the field configuration are discussed, in the context of flare models invoking magnetic reconnection at the site of the primary energy release. In such a model, the intermediate bipole is the natural site of initial magnetic reconnection, particle acceleration and heating. In one particular case of a flare observed at the limb, we find possible evidence of particle acceleration in a neutral sheet at the boundary between two clearly defined magnetic structures.  相似文献   
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Vasulkar  Amey  Verlaan  Martin  Slobbe  Cornelis  Kaleschke  Lars 《Ocean Dynamics》2022,72(8):577-597
Ocean Dynamics - One of the major challenges facing global hydrodynamic tidal models is the modelling of the interaction between sea ice and tides in high-latitude waters. Recent studies have shown...  相似文献   
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This work considers the spatial distribution and ages of western MOZ basin siliclastic sediments prior to providing insights into the diagenesis of degraded dune and alluvial fan sands. Previously published and new TL/OSL ages imply that extensive over-washing of dune sands took place at least 100 ka ago while ages on Okavango floodplains imply that the fan was formed ca. 40 ka and has since undergone periods of higher and lower flood regimes. Sediment analyses indicate that both dune and fan sands contain a diagenetic matrix of clay-enhanced amorphous silica (CEAS) which bonds weakly formed aggregates. The time of formation of diagenetic matrix products is inconclusive but may have been accelerated during or shortly after events dated using OSL/TL techniques. Hence earlier dune over-washing may have led to greater porewater of an acidic to near neutral nature which in turn promoted smectite formation and silicic acid precipitation > 100 000 years ago. The relatively abundant CEAS matrix in floodplain sands implies more recent semi-continuous flood events again of an acidic-near neutral nature leading to the formation of smectite. In this case the floodplain sediments are dated as having been deposited around 40 and 11 ka, when porewater content may have accelerated clay formation and silica dissolution. The dual nature of the CEAS in the islands reflects a changing environment from smectite-dominated flooding events to sepiolite-dominated desiccation events. Flooding may also correspond to TL/OSL ages over the past 40 000 years which contributed to accelerated CEAS formation. The sepiolite is associated with a Ca-rich matrix implying desiccation which may relate to drying events over the 40 000 year period or to riparian tree root pumping and selective salt accumulation. This work shows that sedimentation in incipient rifts is complex and rarely explained totally in terms of primary depositional events. The implications of different stages of sand diagenesis may be significant in enhancing palaeo-environmental interpretations in semi-arid fluvial environments.  相似文献   
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We assume that the motion field in the solar photosphere is described by a spectrum of turbulence, defined by suitably chosen parameters. For various values of the spectral parameters we compute average (i.e. averaged over a sufficiently large part of the photosphere) profiles of weak Fraunhofer lines. The resulting profiles which represent the distribution function of line-of-sight velocity components as modified by the transfer of radiation through the atmosphere, are thereupon still broadened by a function representing the influence of the distribution function of the granulation cell sizes. The resulting functions should be compared with the distribution function of line-of-sight velocity components as derived from observations, in order to arrive at an observational derivation of the parameters of the photospheric spectrum of turbulence.  相似文献   
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We present a model for high-energy solar flare explosions driven by 3-dimensional X-type current loop coalescence. The 3-dimensional X-type current loop coalescence, where two crossed flux-tubes interact at one point, is a fundamentally new process as compared to the 1-D and 2-D cases studied earlier. This process is studied by a first-order approach of the relevant variables near the point of coalescence; it appears to yield reliable information in a sufficiently large area around this point. It is shown that, following a strong plasma collapse due to the pinch effect, a point-like plasma explosion can be driven while fast magnetosonic shock waves can also be excited. We found that the conditions in the area producing the remarkable flare bursts of 21 May, 1984 were indeed such that the many flare spikes could have been due to 3-D explosive X-type current loop coalescence. We also show, by studying the conditions of shock formation in a gamma ray flare, that the time delay of -rays from the impulsive phase could be the time needed for the shock formation in the flaring region.We draw some general conclusions on the question why certain flares do emit -rays in the MeV energy range, and why other, apparently important and energetic flares, do not. We accentuate the fact that a well-developed high-energy flare has three phases of particle acceleration.  相似文献   
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