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11.
The effect of iron on montmorillonite stability. (I) Background and thermodynamic considerations 总被引:1,自引:0,他引:1
It is envisaged that high-level nuclear waste (HLW) will be disposed of in underground repositories. Many proposed repository designs include steel waste canisters and bentonite backfill. Natural analogues and experimental data indicate that the montmorillonite component of the backfill could react with steel corrosion products to produce non-swelling Fe-rich phyllosilicates such as chamosite, berthierine, or Fe-rich smectite. In K-bearing systems, the alteration of montmorillonite to illite/glauconite could also be envisaged. If montmorillonite were altered to non-swelling minerals, the swelling capacity and self-healing properties of the bentonite backfill could be reduced, thereby diminishing backfill performance. The main aim of this paper was to investigate Fe-rich phyllosilicate mineral stability at the canister-backfill interface using thermodynamic modelling. Estimates of thermodynamic properties were made for Fe-rich clay minerals in order to construct approximate phase-relations for end-member/simplified mineral compositions in logarithmic activity space. Logarithmic activity diagrams (for the system Al2O3-FeO-Fe2O3-MgO-Na2O-SiO2-H2O) suggest that if pore waters are supersaturated with respect to magnetite in HLW repositories, Fe(II)-rich saponite is the most likely montmorillonite alteration product (if fO2(g) values are significantly lower than magnetite-hematite equilibrium). Therefore, the alteration of montmorillonite may not be detrimental to nuclear waste repositories that include Fe, as long as the swelling behaviour of the Fe-rich smectite produced is maintained. If fO2(g) exceeds magnetite-hematite equilibrium, and solutions are saturated with respect to magnetite in HLW repositories, berthierine is likely to be more stable than smectite minerals. The alteration of montmorillonite to berthierine could be detrimental to the performance of HLW repositories. 相似文献
12.
Polar and neutral isopranyl glycerol ether lipids as biomarkers of archaea in near-surface sediments from the Nankai Trough 总被引:1,自引:0,他引:1
The molecular and carbon isotopic compositions of polar isopranyl glycerol ether lipids, which are direct indicators of viable archaea, and neutral isopranyl glycerol ether lipids, which are derived from polar lipids via hydrolysis, in near-surface sediments from a methane seep in the Nankai Trough (off central Japan) were investigated. Procedures for extracting, separating and derivatizing polar and neutral ether lipids for detection using gas chromatography were first examined with one sediment sample and a cultivated methanogen. For all sediment samples, archaeol and hydroxyarchaeol were detected in both the polar and neutral ether lipid fractions. Acyclic and cyclic biphytanes were also detected in both types of lipid fractions after treatment with HI/LiAlH4 for ether cleavage and alkylation. The δ13C values of archaeol, sn-2-hydroxyarchaeol, and sn-3-hydroxyarchaeol in the sample from 0.82 m below the seafloor were lower than −100‰ relative to PDB, indicating that diverse living methanotrophic archaea are present in the seep sediments. Biphytanes released from polar ether lipids in the same sample were less depleted in δ13C (−71‰ to −36‰). The wide range of δ13C values suggests that the biphytanes were derived not only from methanotrophic but also from non-methanotrophic archaea, and that the relative contributions of the methanotrophic and non-methanotrophic archaea differed, depending on the biphytane compound. The vertical profiles and δ13C values of the neutral ether lipids were similar to those of the intact polar ether lipids, suggesting that neutral ether lipids derived from fossil archaea in the samples had mainly been lost by the time of sampling. 相似文献
13.
Geological and geomorphological characteristics of landslides triggered by the 2004 Mid Niigta prefecture earthquake in Japan 总被引:8,自引:0,他引:8
The 2004 Mid Niigta prefecture earthquake (MJMA 6.8) triggered more than one thousand landslides in the Miocene to Quaternary sedimentary rocks in Japan. The most common landslides were shallow disrupted landslides on steep slopes, which has been common in many previous disastrous earthquakes in the world. The Mid Niigta prefecture earthquake also triggered more than one hundred deep landslides, providing valuable information on the conditions for their occurrence. A field investigation and the interpretation of aerial photographs taken before and after the earthquake suggest that reactivation of existing landslides and undercutting of slopes are the most important factors for deep landslides to be triggered by earthquakes. In addition, planar sliding surfaces seem to be essential for the generation of catastrophic landslides triggered by this earthquake. Planar bedding–parallel sliding surfaces were formed at the boundary between the overlying permeable sandstone and underlying siltstone or along the bedding planes of alternating beds of sandstone and siltstone. Sliding surfaces along the slope-parallel oxidation front were formed in the area of black mudstone. New landslides (rockslide-avalanches) occurred with the sliding surfaces in a several-cm thick tuff interbedded in siltstone. One rockslide-avalanche occurred on a slope where buckling deformation preceded the earthquake. Gentle valley bottom sediments were mobilized in many locations, probably because they were saturated and partial liquefaction had occurred due to the earthquake shaking. 相似文献
14.
Norikazu Matsuoka Cline E. Thomachot Chiaki T. Oguchi Tamao Hatta Masahiro Abe Hiroyuki Matsuzaki 《Geomorphology》2006,81(3-4):408-420
Rates and processes of rock weathering, soil formation, and mountain erosion during the Quaternary were evaluated in an inland Antarctic cold desert. The fieldwork involved investigations of weathering features and soil profiles for different stages after deglaciation. Laboratory analyses addressed chemistry of rock coatings and soils, as well as 10Be and 26Al exposure ages of the bedrock. Less resistant gneiss bedrock exposed over 1 Ma shows stone pavements underlain by in situ produced silty soils thinner than 40 cm and rich in sulfates, which reflect the active layer thickness, the absence of cryoturbation, and the predominance of salt weathering. During the same exposure period, more resistant granite bedrock has undergone long-lasting cavernous weathering that produces rootless mushroom-like boulders with a strongly Fe-oxidized coating. The red coating protects the upper surface from weathering while very slow microcracking progresses by the growth of sulfates. Geomorphological evidence and cosmogenic exposure ages combine to provide contrasting average erosion rates. No erosion during the Quaternary is suggested by a striated roche moutonnée exposed more than 2 Ma ago. Differential erosion between granite and gneiss suggests a significant lowering rate of desert pavements in excess of 10 m Ma− 1. The landscape has been (on the whole) stable, but the erosion rate varies spatially according to microclimate, geology, and surface composition. 相似文献
15.
In east Asia, acidic gases derived from fossil fuel combustion have increased in the past decades. On the other hand, the Asian dust, also called Kosa (yellow sand) is transported following windstorms from arid lands in the Asian continent. Many researchers have been interested in the reaction between acidic aerosols and Kosa aerosols as well as the long-range transport of these emissions. To investigate the characteristics of chemical components in precipitation on a long-term basis over Japan, precipitation was sequentially collected from April 1984 to March 1997 at Kanazawa located near the coast of the Sea of Japan. Precipitation samples were collected at 1 mm intervals for the first 5 mm rainfall and all volume of rainwater after 6 mm for all precipitation events with an automatic wet only precipitation collector. According to the analyses of precipitation including Kosa aerosols during Kosa periods, the reaction in the air between Kosa and acidic components during the long-range transport was discussed. 相似文献
16.
Abstract. Near-infrared (NIR) and visible light microthermometry was applied to the fluid inclusions in sphalerite from a possible southeast extension of the Toyoha polymetallic deposit. Sphalerite occurs as euhedral-subhedral crystals or collo-form aggregates with a variety of color, which contain a well-developed growth banding. Combined with morphological observations, fluid inclusions in dark-colored sphalerite were examined using a near-infrared light microscopic technique, whereas those in light-colored sphalerite and quartz were examined by a conventional visible light microscopy.
Salinities of fluid inclusions in dark-colored sphalerite have a wide variation (1.0–10.3 wt % NaCl equiv.) compared to that in light-colored sphalerite and quartz (0.0–3.4 wt % NaCl equiv.). These variations suggest that the conventional microthermometric data from light-colored sphalerite and quartz were inadequate to interpret the ore formation process. Dark-colored colloform sphalerite and a dark core of subhedral sphalerite formed from high-salinity fluids (6.5–10.3 wt % NaCl equiv.) under highly supersaturated conditions with respect to sphalerite.
The NIR and visible light microthermometry of fluid inclusions in sphalerite combined with its morphological observations is an invaluable method to infer the formation conditions of sphalerite. The NIR and visible light microthermometry is useful to reveal how the nature of ore fluids changed with time. 相似文献
Salinities of fluid inclusions in dark-colored sphalerite have a wide variation (1.0–10.3 wt % NaCl equiv.) compared to that in light-colored sphalerite and quartz (0.0–3.4 wt % NaCl equiv.). These variations suggest that the conventional microthermometric data from light-colored sphalerite and quartz were inadequate to interpret the ore formation process. Dark-colored colloform sphalerite and a dark core of subhedral sphalerite formed from high-salinity fluids (6.5–10.3 wt % NaCl equiv.) under highly supersaturated conditions with respect to sphalerite.
The NIR and visible light microthermometry of fluid inclusions in sphalerite combined with its morphological observations is an invaluable method to infer the formation conditions of sphalerite. The NIR and visible light microthermometry is useful to reveal how the nature of ore fluids changed with time. 相似文献
17.
Hikari Hasegawa Takashi Mikouchi Akira Yamaguchi Masahiro Yasutake Richard C. Greenwood Ian A. Franchi 《Meteoritics & planetary science》2019,54(4):752-767
Northwest Africa (NWA) 6112, Miller Range (MIL) 090206 (plus its pairs: MIL 090340 and MIL 090405), and Divnoe are olivine‐rich ungrouped achondrites. We investigated and compared their petrography, mineralogy, and olivine fabrics. We additionally measured the oxygen isotopic compositions of NWA 6112. They show similar petrography, mineralogy, and oxygen isotopic compositions and we concluded that these five meteorites are brachinite clan meteorites. We found that NWA 6112 and Divnoe had a c axis concentration pattern of olivine fabrics using electron backscattered diffraction (EBSD). NWA 6112 and Divnoe are suggested to have been exposed to magmatic melt flows during their crystallization on their parent body. On the other hand, the three MIL meteorites have b axis concentration patterns of olivine fabrics. This indicates that the three MIL meteorites may be cumulates where compaction of olivine grains was dominant. Alternatively, they formed as residues and were exposed to olivine compaction. The presence of two different olivine fabric patterns implies that the parent body(s) of brachinite clan meteorites experienced diverse igneous processes. 相似文献
18.
19.
BALLOON-BORNE MEASUREMENTS OF AEROSOL VERTICAL DISTRIBUTIONS OVER BEIJING DURING THE SUMMER AND AUTUMN OF 1993 下载免费PDF全文
Zhou Jun Tan Kun Shao Shisheng Gong Zhiben Shi Guangyu Guo Jiandong Wang Biao Zhang Baowu Sun Baolai Yasunobu Iwasak Masahiko Hayashi Masahiro Hase 《Acta Meteorologica Sinica》1994,8(4):478-487
The results of two balloon soundings during the summer and autumn of 1993 from the Xianghe Observation Station are being utilized in a study of the temporal and spatial distribution of the atmospheric aerosols.The balloon,gondola,instrumentation and atmospheric conditions during the observation period are described.The temporal and spatial characteristics of aerosol concentration,size ratio,mixing ratio,and size distribution for both troposphere and strato-sphere are presented and analyzed. 相似文献
20.
Influence of surface and vegetation characteristics on C-band radar measurements for soil moisture content 总被引:1,自引:0,他引:1
Shakil Ahmad Romshoo Masahiro Koike Sadayukihir Onaka Taikan Oki Katumi Musiake 《Journal of the Indian Society of Remote Sensing》2002,30(4):229-244
Soil moisture estimation using microwave remote sensing faces challenges of the segregation of influences mainly from roughness and vegetation. Under static surface conditions, it was found that Radarsat C-band SAR shows reasonably good correlation and sensitivity with changing soil moisture. Dynamic surface and vegetation conditions are supposed to result in a substantial reduction in radar sensitivity to soil moisture. A C-band scatterometer system (5.2 GHz) with a multi-polarization and multi-angular configuration was used 12 times to sense the soil moisture over a tall vegetated grass field. A score of vegetation and soil parameters were recorded on every occasion of the experiment. Three radar backscattering models Viz., Integral Equation Model (IEM), an empirical model and a volume scattering model, have been used to predict the backscattering phenomena. The volume scattering model, using the Distorted Born Approximation, is found to predict the backscattering phenomena reasonably well. But the surface scattering models are expectedly found to be inadequate for the purpose. The temporal variation of soil moisture does show good empirical relationship with the observed radar backscattering. But as the vegetation biomass increases, the radar shows higher sensitivity to the vegetation parameters compared to surface characteristics. A sensitivity analysis of the volume scattering model for all the parameters also reveals that the radar is more sensitive to plant parameters under high biomass conditions, particularly vegetation water content, but the sensitivity to surface characteristics, particularly to soil moisture, is also appreciable. 相似文献