Pressure and temperature dependence of the viscosity of a NaAlSi<Subscript>2</Subscript>O<Subscript>6</Subscript> melt     

Akio Suzuki  Eiji Ohtani  Hidenori Terasaki  Keisuke Nishida  Hiromi Hayashi  Tatsuya Sakamaki  Yuki Shibazaki  Takumi Kikegawa 《Physics and Chemistry of Minerals》2011,38(1):59-64

The viscosity of a silicate melt of composition NaAlSi₂O₆ was measured at pressures from 1.6 to 5.5 GPa and at temperatures from 1,350 to 1,880°C. We employed in situ falling sphere viscometry using X-ray radiography. We found that the viscosity of the NaAlSi₂O₆ melt decreased with increasing pressure up to 2 GPa. The pressure dependence of viscosity is diminished above 2 GPa. By using the relationship between the logarithm of viscosity and the reciprocal temperature, the activation energies for viscous flow were calculated to be 3.7 ± 0.4 × 10² and 3.7 ± 0.5 × 10² kJ/mol at 2.2 and 2.9 GPa, respectively.  相似文献   

Importance of intracellular Fe pools on growth of marine diatoms by using unialgal cultures and on the Oyashio region phytoplankton community during spring     

Koji Sugie  Kenshi Kuma  Satoshi Fujita  Satomi Ushizaka  Koji Suzuki  Tsutomu Ikeda 《Journal of Oceanography》2011,67(2):183-196

We report on the ability for luxury Fe uptake and the potential for growth utilizing intracellular Fe pools for 4 coastal centric diatom isolates and in situ phytoplankton assemblages, mainly composed of diatoms. Iron uptake of the diatom isolates and natural phytoplankton assemblages in the Oyashio region during spring blooms were prevented by adding hydroxamate siderophore desferrioxamine B (DFB). After the addition of DFB, intracellular Fe in the diatom isolates supported 2.4–4.2 cell divisions with 1.2–2.6 Chl a doublings. The intracellular Fe was primarily used for cell generation rather than Chl a production, leading to a reduction in the Chl a cell quota in the Fe-starved cells with time. The metabolic properties of the Fe-starved cells with their cell morphologies were different among species or genera. An on-deck incubation experiment also exhibited 1.9 cell divisions and 0.81 Chl a doublings of phytoplankton after the addition of DFB, also indicating the preference of cell generation over Chl a production. A decrease in the level of cellular Chl a, a main light-harvesting pigment in Fe-starved diatoms, may become a superior survival strategy to protect the cells from high irradiance that can cause photo-oxidative damages through photosynthesis. Such relatively low-Fe with high-light conditions could often occur in surface waters of the Oyashio region from spring to summer.  相似文献   

Formation process of pyrite polyframboid based on the heavy-metal analysis by micro-PIXE     

Hisanari Sugawara  Masayuki Sakakibara  David Belton  Tetsuya Suzuki 《Environmental Earth Sciences》2013,69(3):811-819

Pyrite framboid in sedimentary rocks could be concerned with arsenic contamination in groundwater of acidic environment and has been studied for the formation process of its unique morphology. However, not much has been discussed about the formation process based on the heavy-metal distribution in pyrite framboids and their aggregates. To reveal the formation process of pyrite framboids and their aggregates, mudstone from the Late Cretaceous Hakobuchi Group, central Hokkaido, Japan, are investigated for mode, petrographical, mineralogical, and micro-PIXE (particle-induced X-ray emission) analysis in this study. Spherical and sub-spherical pyrite framboids observed in polyframboids can be divided into two types based on the diameter of framboids (D) and the average diameter of microcrystals (d) within framboids: type 1, ranging from 2 to 9 μm and from 0.4 to 0.9 μm, respectively, and type 2, ranging from 8 to 50 μm and from 0.5 to 1.8 μm, respectively. Based on the quantitative traverse analyses and 2-D elemental mapping results by micro-PIXE, heterogeneities in the concentrations of heavy metals within the analyzed aggregations of pyrite are exhibited. On the basis of the As and Pb zoning patterns, the time range and chronological stages of pyrite-aggregation growth are revealed.  相似文献   

A study of the morphology of winter sprites in the Hokuriku area of Japan in relation to cloud charge height     

K. Myokei  Y. Matsudo  T. Asano  T. Suzuki  Y. Hobara  K. Michimoto  M. Hayakawa 《Journal of Atmospheric and Solar》2009,71(5):597-602

Continuous observations of sprites in the Hokuriku area of Japan were performed from two optical sites during the three winter periods. The purpose of this observation is to study the major effect in the appearance of sprites and in determining the morphology of sprites (columns or carrots). Detailed analysis is performed based on the estimation of the height of ?10 °C at the time of sprite occurrence. When the height of ?10 °C is lower than 1800 m, the occurrence of sprites is infrequent, and the dominant shape is column. Then when it is increased (1800–3000 m), a new situation takes place, namely the occurrence of sprites is very enhanced and more spectacular shapes like carrots tend to be frequently observed in addition to column sprites. These sprite characteristics are first compared with those of parent lightning in the Hokuriku area and with our latest computer simulations on sprite initiation.  相似文献   

Three-dimensional EM computer simulation on sprite initiation above a horizontal lightning discharge     

T. Asano  T. Suzuki  M. Hayakawa  M.G. Cho 《Journal of Atmospheric and Solar》2009,71(8-9):983-990

The purpose of this paper is to study the three-dimensional (3D) effects of the source current and the electromagnetic (EM) pulse on the distribution of upper atmospheric electric field and ionization created. A new lightning model has been employed; i.e., we have included a horizontal channel in addition to the conventional vertical channel. The effects of the horizontal lightning channel are summarized as follows: (1) the effect of a vertical channel plays a fundamental role in the whole view of sprite initiation; (2) the position of a sprite is shifted from the position of its parent vertical channel in response to the length of a horizontal channel; and (3) we observe very fine structures with local maxima and minima in the “reduced” electric field (the electric field divided by the neutral gas density). These theoretical inferences are discussed and compared with the observational facts so far reported (such as lateral shift of sprites, morphological difference of sprites, etc.).  相似文献   

The Higo High-Grade Metamorphic Rocks in Japan as a Part of the Collisional Terrane Between the Sino-Korean and Yangtze Craton     

Yasuhito Osanai  Takuji Hamamoto  Hiroo Kagami  Kazuhiro Suzuki  Masaaki Owada  Atsushi Kamei   《Gondwana Research》1999,2(4):599-601

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Simulation of near source ground motion and its characteristics     

S. Suzuki  K. Asano 《Soil Dynamics and Earthquake Engineering》2000,20(1-4)

It is fact that the severe ground motions of shear waves have a strong effect on the dynamic behavior of buildings and civil structures. We simulate near source strong motions of a pure shear wave and synthesize small motions, using the parameters based on the recorded accelerograms at the site that is regarded as a base rock in the Osaka basin, Japan. By making use of a stochastic technique, we can easily introduce higher frequency contents in the motions and apply the technique to the synthesis of small waves regarding as a green function. We also introduce to the analysis the useful relationships among the time duration T_d, the seismic moment M₀, the corner frequency f_c and the high cutoff frequency f_max which were regressed by a simple representation scheme. Considering two active faults that may affect severe damage on buildings and civil structures, we try to predict strong ground motions in Osaka basin and show the characteristics of them.  相似文献   

Rapid Identification of Water-Conducting Fractures Using a Trace Methane Gas Measurement     

Masakazu Niwa Ph.D  Kenji Amano Ph.D  Ryuji Takeuchi Ph.D  Koji Shimada Ph.D 《Ground Water Monitoring & Remediation》2021,41(3):41-50

Identification of water-conducting fractures is important for the safety assessment of underground projects in crystalline rocks at geological disposal sites. We applied a portable methane gas analyzer by wavelength-scanned cavity ring-down spectroscopy to detect the water-conducting fractures in the underground tunnel of the Mizunami Underground Research Laboratory, central Japan. The tunnel is excavated in granite with CH₄-rich groundwater. Two approaches were taken to obtain the profile of CH₄ concentration along the gallery walls: (1) “Scan by walking” at the speed of 0.5 m/s and (2) monitoring for 30 s at 0.5 or 1 m intervals. In the Scan by walking approach, the peaks of the CH₄ concentration corresponded well with the occurrence of high water flow rate fractures. Thus, this method is useful for rapid identification of major water-conducting fractures. Monitoring at constant intervals takes more time than the Scan by walking approach; however, this method can largely detect occurrences of fractures with low fluid fluxes.  相似文献   

Laboratory detection of a new interstellar free radical CH2CN(2B1)     

Saito S  Yamamoto S  Irvine WM  Ziurys LM  Suzuki H  Ohishi M  Kaifu N 《The Astrophysical journal》1988,334(2):L113-L116

An asymmetric-top free radical CH2CN, which as a 2B1 ground state, was detected for the first time by laboratory microwave spectroscopy. The radical was produced in a free-space absorption cell by a DC glow discharge in pure CH3CN gas. About 60 fine-structure components were observed for the N = 11-10 to 14-13 a-type rotational transitions in the frequency region of 220-260 GHz, and many hyperfine resolved components for the N = 4-3 and 5-4 transitions in the 80 and 100 GHz regions, respectively. The molecular constants, including the rotational constants, centrifugal distortion constants, and spin-rotation coupling constants with centrifugal distortion correction terms were determined from the fine-structure resolved transitions, and the hyperfine coupling constants due to the hydrogen and nitrogen nuclei were obtained from the low-N transitions. As a result we assigned U100602 and U80484 from Sgr B2, and U40240 and U20120 from TMC-1, to the N = 5-4, 4-3, 2-1, and 1-0 transitions with K-1 = 0 of the CH2CN radical.  相似文献   

Diverse Range of Mineralization Induced by Phase Separation of Hydrothermal Fluid: Case Study of the Yonaguni Knoll IV Hydrothermal Field in the Okinawa Trough Back-Arc Basin     

Ryohei Suzuki    Jun-Ichiro Ishibashi    Miwako Nakaseama    Uta Konno    Urumu Tsunogai    Kaul Gena  Hitoshi Chiba 《Resource Geology》2008,58(3):267-288

The Yonaguni Knoll IV hydrothermal vent field (24°51′N, 122°42′E) is located at water depths of 1370–1385 m near the western edge of the southern Okinawa Trough. During the YK03–05 and YK04–05 expeditions using the submersible Shinkai 6500, both hydrothermal precipitates (sulfide/sulfate/carbonate) and high temperature fluids (Tmax = 328°C) presently venting from chimney‐mound structures were extensively sampled. The collected venting fluids had a wide range of chemistry (Cl concentration 376–635 mmol kg^?1), which is considered as evidence for sub‐seafloor phase separation. While the Cl‐enriched smoky black fluids were venting from two adjacent chimney‐mound structures in the hydrothermal center, the clear transparent fluids sometimes containing CO₂ droplet were found in the peripheral area of the field. This distribution pattern could be explained by migration of the vapor‐rich hydrothermal fluid within a porous sediment layer after the sub‐seafloor phase separation. The collected hydrothermal precipitates demonstrated a diverse range of mineralization, which can be classified into five groups: (i) anhydrite‐rich chimneys, immature precipitates including sulfide disseminations in anhydrite; (ii) massive Zn‐Pb‐Cu sulfides, consisting of sphalerite, wurtzite, galena, chalcopyrite, pyrite, and marcasite; (iii) Ba‐As chimneys, composed of barite with sulfide disseminations, sometimes associated with realgar and orpiment overgrowth; (iv) Mn‐rich chimneys, consisting of carbonates (calcite and magnesite) and sulfides (sphalerite, galena, chalcopyrite, alabandite, and minor amount of tennantite and enargite); and (v) pavement, silicified sediment including abundant native sulfur or barite. Sulfide/sulfate mineralization (groups i–iii) was found in the chimney–mound structure associated with vapor‐loss (Cl‐enriched) fluid venting. In contrast, the sulfide/carbonate mineralization (group iv) was specifically found in the chimneys where vapor‐rich (Cl‐depleted) fluid venting is expected, and the pavement (group v) was associated with diffusive venting from the seafloor sediment. This correspondence strongly suggests that the subseafloor phase separation plays an important role in the diverse range of mineralization in the Yonaguni IV field. The observed sulfide mineral assemblage was consistent with the sulfur fugacity calculated from the FeS content in sphalerite/wurtzite and the fluid temperature for each site, which suggests that the shift of the sulfur fugacity due to participation of volatile species during phase separation is an important factor to induce diverse mineralization. In contrast, carbonate mineralization is attributed to the significant mixing of vapor‐rich hydrothermal fluid and seawater. A submarine hydrothermal system within a back‐arc basin in the continental margin may be considered as developed in a geologic setting favorable to a diverse range of mineralization, where relatively shallow water depth induces sub‐seafloor phase separation of hydrothermal fluid, and sediment accumulation could enhance migration of the vapor‐rich hydrothermal fluid.  相似文献