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41.
Albrecht Spitz 《International Journal of Earth Sciences》1915,6(4-6):286-314
Ohne Zusammenfassung 相似文献
42.
Central European Cenozoic plume volcanism with OIB characteristics and indications of a lower mantle source 总被引:6,自引:0,他引:6
Average concentrations of incompatible elements and isotopes of radiogenic Sr, Nd and Pb in a 350 km long belt of Central
European volcanics (CECV) resemble those in OIB in general and in OIB from the N Atlantic in particular. This similarity allows
to infer comparable sources for CECV and OIB which might have been located in the lower mantle according to seismic tomography
and chemistry, with the latter unlike a MORB source. The incompatible element contribution of lower mantle origin can be modelled
from primitive mantle minus continental crust and upper mantle inventories. Alkali basaltic magmas from the modelled source
are close in composition to CECV and OIB. The continental crust contains almost half of the silicate Earth's content of Rb,
K, Pb, Ba, Th and U, which were mobilized to a major extent through dehydration of subducted ocean crust. Related losses from
the lower mantle had to be replaced by deep subductions of oceanic lithosphere recognized from their isotopic imprint. From
a balance based on Nd isotopes it can be concluded that average CECV contains 60% matter from residual primitive mantle and
40% from deeply subducted lithosphere (including some young upper mantle materials). Plume products from separate CECV regions
developed, within 45 Ma, from rather depleted to more primitive isotopic signatures. Four periods of volcanism from Eocene
to late Quaternary time are explained as four pulses of an almost stationary ultrafast plume uprise as modelled by Larsen
and Yuen (1997). Magma production has increased from the first to the third pulse with the peak during Miocene time in the
Vogelsberg region. The final pulse produced the Quaternary Eifel volcanoes. Tectonism from the Alpine orogen has probably
triggered the synchronous volcanism of CECV, Massif Central etc. The European lithospheric plate has moved under the control
of the opening Atlantic almost in an eastern direction with a velocity of 1 cm per year and has shifted extinct volcanoes
off their source channels.
Received: 10 July 1998 / Accepted: 10 February 1999 相似文献
43.
A study was conducted to evaluate monitored natural attenuation (MNA) as a remedy for arsenic in groundwater at a former phosphate mining and manufacturing facility. The mineralogy, speciation, and lability of arsenic in phosphatic wastes present in soils were characterized using sequential extraction procedures, leaching experiments, batch adsorption tests, and microchemical speciation analysis. A PHREEQC-based reactive transport model was also parameterized using these laboratory results, and it was used to evaluate the importance of identified attenuation mechanisms on arsenic concentrations along a vertical flow path from a shallow, alluvial aquifer to the underlying Floridan aquifer. Arsenic was found to occur in several chemical forms in phosphatic wastes, including unstable sulfide minerals, adsorbed surface complexes, and relatively insoluble phosphate and oxide minerals. Most arsenic was associated with stable minerals. The reactive transport model predicted that historical leaching of solid-phase waste materials in soils would not have generated enough arsenic to explain the concentrations observed in downgradient groundwater; instead, the source of arsenic to groundwater was likely acidic and saline process water that infiltrated though unlined ponds and ditches during historical manufacturing operations. A key factor affecting the long-term effectiveness of natural attenuation of arsenic in groundwater is the occurrence and stability of iron oxyhydroxides in aquifer sediments. According to laboratory and reactive transport model results, sufficient levels were found to be present at the site to effectively limit arsenic migration at concentrations exceeding drinking water standards in the future in the Floridan aquifer. This study presents the geochemical evaluations that are needed to satisfy EPA guidelines on determining whether or not MNA is an acceptable remedy for a site. It specifically details the characterization and modeling that were used to demonstrate effectiveness at a site where MNA was ultimately selected as the remedy for arsenic in groundwater. 相似文献
44.
45.
Exploring the impact of diagenesis on (isotope) geochemical and microstructural alteration features in biogenic aragonite
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Ann‐Christine Ritter Vasileios Mavromatis Martin Dietzel Ola Kwiecien Felix Wiethoff Erika Griesshaber Laura A. Casella Wolfgang W. Schmahl Jennifer Koelen Rolf D. Neuser Albrecht Leis Dieter Buhl Andrea Niedermayr Sebastian F. M. Breitenbach Stefano M. Bernasconi Adrian Immenhauser 《Sedimentology》2017,64(5):1354-1380
For the Quaternary and Neogene, aragonitic biogenic and abiogenic carbonates are frequently exploited as archives of their environment. Conversely, pre‐Neogene aragonite is often diagenetically altered and calcite archives are studied instead. Nevertheless, the exact sequence of diagenetic processes and products is difficult to disclose from naturally altered material. Here, experiments were performed to understand biogenic aragonite alteration processes and products. Shell subsamples of the bivalve Arctica islandica were exposed to hydrothermal alteration. Thermal boundary conditions were set at 100°C, 175°C and 200°C. These comparably high temperatures were chosen to shorten experimental durations. Subsamples were exposed to different 18O‐depleted fluids for durations between two and twenty weeks. Alteration was documented using X‐ray diffraction, cathodoluminescence, fluorescence and scanning electron microscopy, as well as conventional and clumped isotope analyses. Experiments performed at 100°C show redistribution and darkening of organic matter, but lack evidence for diagenetic alteration, except in Δ47 which show the effects of annealing processes. At 175°C, valves undergo significant aragonite to calcite transformation and neomorphism. The δ18O signature supports transformation via dissolution and reprecipitation, but isotopic exchange is limited by fluid migration through the subsamples. Individual growth increments in these subsamples exhibit bright orange luminescence. At 200°C, valves are fully transformed to calcite and exhibit purple‐blue luminescence with orange bands. The δ18O and Δ47 signatures reveal exchange with the aqueous fluid, whereas δ13C remains unaltered in all experiments, indicating a carbonate‐buffered system. Clumped isotope temperatures in high‐temperature experiments show compositions in broad agreement with the measured temperature. Experimentally induced alteration patterns are comparable with individual features present in Pleistocene shells. This study represents a significant step towards sequential analysis of diagenetic features in biogenic aragonites and sheds light on reaction times and threshold limits. The limitations of a study restricted to a single test organism are acknowledged and call for refined follow‐up experiments. 相似文献
46.
F. Reitsma J. Albrecht 《International journal of geographical information science》2013,27(10):1073-1090
The paper describes the development of a new methodological approach for simulating geographic processes through the development of a data model that represents a process. This methodology complements existing approaches to dynamic modelling, which focus on the states of the system at each time step, by storing and representing the processes that are implicit in the model. The data model, called nen, focuses existing modelling approaches on representing and storing process information, which provides advantages for querying and analysing processes. The flux simulation framework was created utilizing the nen data model to represent processes. This simulator includes basic classes for developing a domain specific simulation and a set of query tools for inquiring after the results of a simulation. The methodology is prototyped with a watershed runoff simulation. 相似文献
47.
Tewodros Alemayehu Albrecht Leis Anton Eisenhauer Martin Dietzel 《Chemie der Erde / Geochemistry》2011,(2):177-187
Isotopic and chemical composition of groundwater from wells and springs, and surface water from the basalt-dominated Axum area (northern Ethiopia) provides evidence for the origin of water and dissolved species. Shallow (depth < 40 m) and deep groundwater are distinguished by both chemical and isotopic composition. Deep groundwater is significantly enriched in dissolved inorganic carbon up to 40 mmol l−1 and in concentrations of Ca2+, Mg2+, Na+ and Si(OH)4 compared to the shallow type.The δ2H and δ18O values of all solutions clearly indicate meteoric origin. Shifts from the local meteoric water line are attributed to evaporation of surface and spring water, and to strong water–rock interaction. The δ13CDIC values of shallow groundwater between −12 and −7‰ (VPDB) display the uptake of CO2 from local soil horizons, whereas δ13CDIC of deep groundwater ranges from −5 to +1‰. Considering open system conditions with respect to gaseous CO2, δ13CDIC = +1‰ of the deep groundwater with highest PCO2 = 10−0.9 atm yields δ13CCO2(gas) ≈ −5‰, which is close to the stable carbon isotopic composition of magmatic CO2. Accordingly, stable carbon isotope ratios within the above range are referred to individual proportions of CO2 from soil and magmatic origin. The uptake of magmatic CO2 results in elevated cations and Si(OH)4 concentrations. Weathering of local basalts is documented by 87Sr/86Sr ratios of the groundwater from 0.7038 to 0.7059. Highest values indicate Sr release from the basement rocks. Besides weathering of silicates, neoformation of solids has to be considered, which results in the formation of, e.g., kaolinite and montmorillonite. In several solutions supersaturation with respect to calcite is reached by outgassing of CO2 from the solution leading to secondary calcite formation. 相似文献
48.
49.
Stiffness variations in carbonates may be described as resulting from different concentrations of flat compliant pores or cracks, which can have a significant effect on the effective stiffness and acoustic properties (e.g., velocities and attenuations) of dry as well as saturated carbonates, although they carry extremely little porosity. As shown in this paper, the effects of dual porosity and wave-induced fluid flow or pore pressure communication may also play a significant role. On the basis of a previously published T-matrix approach to model the effective viscoelastic properties of cracked porous media, we illustrate the (frequency-dependent) effects of wave-induced fluid flow (mainly squirt flow) or pore pressure communication for a model structure consisting of a mixture of fluid-saturated porous grains and fluid-saturated cavities (vugs, etc.) that are embedded in a solid matrix associated with carbonates. We assume that the pores within the porous grains are decoupled from the pores in the solid matrix (and possibly saturated with different fluids) but that each pore system at the micro and/or mesoscale may or may not be connected. For each of four different connectivity models, we present numerical results for four different cases of microstructure (that emphasize the importance of cracks and flat compliant pores). Our numerical results indicate that the velocity and attenuation spectra of carbonates vary significantly, even when the crack density and all other volume concentrations are constant. 相似文献
50.
We have studied the long-time dynamical evolution of a population of comets surrounding the Solar System at a large distance. Orbital changes are caused by random passing stars. We first emphasize the need for a new simulation because of the lack of completeness of previous analytical and numerical studies. Then the solar neighborhood is modeled by a sphere of 1 pc in radius, which stars cross at random in direction and distance. The geometry of the encounters allows us to compute the impulse gained by the star and the Sun, in the context of an impact approximation. Then we determine the change of orbital elements for a population of comets and follow the evolution of the frequency distribution for the five Keplerian elements. Clouds are selected in such a way that we test the two main hypotheses for the origin of the Oort cloud, and also the regions of stability in an aphelion-eccentricity diagram. We show that stellar perturbations randomize the cloud and prevent one from inferring the initial cloud configuration from the current distribution. Clouds are depleted by the diffusion of comets into the planetary regions, where they become planet-influenced comets or are ejected from the Solar System. The diffusion of aphelion toward interstellar regions proves to be the major source of cometary loss. Direct ejection to hyperbolic orbits amounts to 9% of the originally population over the age of the Solar System. Finally the current and original cloud populations are estimated at 1.8 × 1012 and 2 × 1013 comets and we discuss these results. 相似文献