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71.
72.
Natural and synthetic chemicals are essential to our daily lives, food supplies, health care, industries and safe sanitation. At the same time protecting marine ecosystems and seafood resources from the adverse effects of chemical contaminants remains an important issue. Since the 1970s, monitoring of persistent, bioaccumulative and toxic (PBT) chemicals using analytical chemistry has provided important spatial and temporal trend data in three important contexts; relating to human health protection from seafood contamination, addressing threats to marine top predators and finally providing essential evidence to better protect the biodiversity of commercial and non-commercial marine species. A number of regional conventions have led to controls on certain PBT chemicals over several years (termed ‘legacy contaminants’; e.g. cadmium, lindane, polycyclic aromatic hydrocarbons [PAHs] and polychlorinated biphenyls [PCBs]). Analytical chemistry plays a key role in evaluating to what extent such regulatory steps have been effective in leading to reduced emissions of these legacy contaminants into marine environments. In parallel, the application of biomarkers (e.g. DNA adducts, CYP1A-EROD, vitellogenin) and bioassays integrated with analytical chemistry has strengthened the evidence base to support an ecosystem approach to manage marine pollution problems. In recent years, however, the increased sensitivity of analytical chemistry, toxicity alerts and wider environmental awareness has led to a focus on emerging chemical contaminants (defined as chemicals that have been detected in the environment, but which are currently not included in regulatory monitoring programmes and whose fate and biological impacts are poorly understood). It is also known that natural chemicals (e.g. algal biotoxins) may also pose a threat to marine species and seafood quality. Hence complex mixtures of legacy contaminants, emerging chemicals and natural biotoxins in marine ecosystems represent important scientific, economic and health challenges. In order to meet these challenges and pursue cost-effective scientific approaches that can provide evidence necessary to support policy needs (e.g. the European Marine Strategy Framework Directive), it is widely recognised that there is a need to (i) provide marine exposure assessments for priority contaminants using a range of validated models, passive samplers and biomarkers; (ii) integrate chemical monitoring data with biological effects data across spatial and temporal scales (including quality controls); and (iii) strengthen the evidence base to understand the relationship between exposure to complex chemical mixtures, biological and ecological impacts through integrated approaches and molecular data (e.g. genomics, proteomics and metabolomics). Additionally, we support the widely held view that (iv) that rather than increasing the analytical chemistry monitoring of large number of emerging contaminants, it will be important to target analytical chemistry towards key groups of chemicals of concern using effects-directed analysis. It is also important to evaluate to what extent existing biomarkers and bioassays can address various classes of emerging chemicals using the adverse outcome pathway (AOP) approach now being developed by the Organization for Economic Cooperation and Development (OECD) with respect to human toxicology and ecotoxicology. 相似文献
73.
The purpose of this study was to quantify relationships between season, sediment availability, sediment transport pathways, and beach/foredune morphology at Greenwich Dunes, PEI. This was done for periods ranging from a few days to multiple decades using erosion pins, bedframe measurements, annual surveys, and digital photogrammetry using historical aerial photographs. The relative significance of seasonal/annual processes versus response of the foredune system to broader geomorphic controls (e.g. relative sea level rise, storms, etc.) was also assessed. The data show that there are clear seasonal differences in the patterns of sand supply from the beach to the foredune at Greenwich and that there are differences in sediment supply to the foredune between the east and west reaches of the study area, resulting in ongoing differences in foredune morphology. They also demonstrate that models that incorporate wind climate alone, or even models that include other factors like beach moisture, would not be able to predict the amount of sediment movement from the beach to the foredune in this environment unless there were some way to parameterize system morphology, especially the presence or absence of a dune ramp. Finally, the data suggest that the foredune can migrate landward while maintaining its form via transfers of sediment from the stoss slope, over the crest, and onto the lee slope. Although the rate of foredune development or recovery after disturbance changes over time due to morphological feedback, the overall decadal evolution of the foredune system at Greenwich is consistent with, and supports, the Davidson‐Arnott (2005) conceptual model of dune transgression under rising sea level. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
74.
Vertical ground motion (VGM) rates stand as crucial information, either for predicting the impact of the actual sea level rise along low-lying coasts or refining geodynamic problems. Because present day VGM rates have a magnitude smaller than 10 mm/yr, they remain challenging to quantify and often elusive. We focus on the quantification of global-scale VGM rates in order to identify global or regional trends. We computed VGM rates by combining tide gauges records and local satellite altimetry, which yield a new dataset of 634 VGM rates. We further compare this database to previous studies that use geodetic techniques and tide gauges records in order to evaluate the consistency of both our results and previous ones. The magnitudes differ by less than 5 mm/yr, and similar subsidence and uplift general tendencies appear. Even if the asset of our database stands in the greater number of sites, the combination of all studies, each with different pros and cons, yields a hybrid dataset that makes our attempt to extract VGM trends more robust than any other, independent study. Fennoscandia, the West coast of North America, and the eastern coast of Australia are uplifting, while the eastern coast of North America, the British Isles and Western Europe, the eastern Mediterranean Sea, Japan, and the western coast of Australia are subsiding. Glacial Isostatic Adjustment (GIA) is expected to provide a major contribution to the present-day signal. Aside from Fennoscandia, observed VGM often depart from the GIA model predictions of Peltier (2004). This either results from an underestimate of the model predictions or from the influence of other processes: indeed, the influence of the geodynamic setting appears in particular along the coasts of western North America or Japan, where the alternation of transform faults and subduction zones makes it possible to assign contrasted behaviours to the local geodynamic context. Local mechanisms like anthropogenic processes or sediment compaction, also contribute to VGM. This remains true for the critical cases of Venice, the Gulf of Mexico, the Ganges delta, and the Maldives, which are particularly exposed to the current sea level rise. 相似文献
75.
Jeffrey Chiarenzelli Robin Lock Carol Cady Adria Bregani Benn Whitney 《Environmental Earth Sciences》2012,67(1):189-204
Water from four north-flowing rivers (Oswegatchie, Grasse, Raquette, and West Branch of the St. Regis) traversing three distinct geologic terranes (Adirondack Highlands, Adirondack Lowlands, St. Lawrence Valley), originating in the acidified northern Adirondack region, display rapid spatial changes in downriver multi-element chemistry and physical parameters. Downriver, most soluble elements increase (Ba, Ca, Cu, K, Mg, Na, Rb, S, and Sr) while statistically significant decreases in insoluble elements (Al, Ce, Dy, Er, Fe, Gd, La, Mn, Nd, Pr, and Y) also occur. Lithium, Si, and Zr did not show a consistent increasing or decreasing trend. Concentrations of most elements measured on June 5, 2008 were greater than 7?weeks later; however, greater discharge and lower pH enhanced Al concentrations occurred during the later sampling date. Elemental ratios track changes in lithology, anthropogenic influence, and pH. The Raquette River shows the least variation in elemental concentrations because of storage in numerous hydropower reservoirs and has non-detectable concentrations of some redox sensitive elements such as Co, Ni, and V. Oswegatchie tributaries display similar geochemical trends dependent upon their location and local bedrock and show geochemical trends along the trunks of major rivers that are also evident in smaller drainage basins. Comparison with analytical results from the Western Adirondack Stream Survey also indicates acidification is prevalent in the Adirondack Highlands, particularly in the Oswegatchie headwaters during periods of high flow, but acidity is rapidly buffered downriver due to interaction with marble in the Adirondack Lowlands. 相似文献
76.
Thomas Genty Bruno Bussière Robin Potvin Mostafa Benzaazoua Gérald J. Zagury 《Environmental Earth Sciences》2012,66(8):2387-2401
Oxidation of sulphide mining waste can generate acid mine drainage (AMD) that has the potential to seriously affect the ecosystems. Acid mine drainage is characterised by a high acidity, high concentrations of sulphates and metals. To reduce the environmental impacts due to AMD, neutralisation using limestone drains is an option proposed in the literature and used around the world. The present study focuses on the influence of the carbonate rock mineralogy and their particle size on the neutralising capacity. The tests were performed in two different anoxic conditions: in batch reactors, and in columns having a hydraulic retention time of 15?h. The results showed that the neutralisation capacity of calcite was more important than for dolomitic rock, and smaller particle size gave higher alkalinity production (fine calcite dissolved faster in contact with AMD). A characterization of metal precipitate in sludge and in limestone coating was performed and demonstrated that gypsum, lepidocrocite and goethite were the predominant secondary minerals to be formed. Finally, this study underlines that anoxic limestone drain cannot be used alone to treat high iron concentrated AMD. 相似文献
77.
Developing coastal adaptation to climate change in the New York City infrastructure-shed: process, approach, tools, and strategies 总被引:1,自引:0,他引:1
Cynthia Rosenzweig William D. Solecki Reginald Blake Malcolm Bowman Craig Faris Vivien Gornitz Radley Horton Klaus Jacob Alice LeBlanc Robin Leichenko Megan Linkin David Major Megan O��Grady Lesley Patrick Edna Sussman Gary Yohe Rae Zimmerman 《Climatic change》2011,106(1):93-127
While current rates of sea level rise and associated coastal flooding in the New York City region appear to be manageable by stakeholders responsible for communications, energy, transportation, and water infrastructure, projections for sea level rise and associated flooding in the future, especially those associated with rapid icemelt of the Greenland and West Antarctic Icesheets, may be outside the range of current capacity because extreme events might cause flooding beyond today??s planning and preparedness regimes. This paper describes the comprehensive process, approach, and tools for adaptation developed by the New York City Panel on Climate Change (NPCC) in conjunction with the region??s stakeholders who manage its critical infrastructure, much of which lies near the coast. It presents the adaptation framework and the sea-level rise and storm projections related to coastal risks developed through the stakeholder process. Climate change adaptation planning in New York City is characterized by a multi-jurisdictional stakeholder?Cscientist process, state-of-the-art scientific projections and mapping, and development of adaptation strategies based on a risk-management approach. 相似文献
78.
Concentrations of polycyclic aromatic hydrocarbons were determined in species of commercial fish and lobsters following an oil-spill just off the protected Madagascan coastline. Samples were collected along the coastline within and outside the affected area. Summed PAH concentrations ranged from 1.9 μg kg−1 to 63 μg kg−1 wet weight, but with no higher molecular weight PAHs (>202 Da) being detected. All concentrations of benzo[a]pyrene, benz[a]anthracene and dibenz[a,h]anthracene were <0.1 μg kg−1 wet weight, well within the EU and UK set limits for the protection of human health. Additionally, samples were calculated as the benzo[a]pyrene toxic equivalency quotient (TEQ) and found to be well below the level of concern in relation to health of human consumers. Evaluation of the biota PAH data indicated the origin of PAH was predominantly petrogenic with >80% arising from oil sources. Profile studies indicate a low-level multisource petrogenic contamination probably representing a pre-spill background for the area. 相似文献
79.
80.
G. P. T. Spampinato L. Ailleres P. G. Betts R. J. Armit 《Australian Journal of Earth Sciences》2013,60(5):581-603
The basement rocks of the poorly understood Thomson Orogen are concealed by mid-Paleozoic to Upper Cretaceous intra-continental basins and direct information about the orogen is gleaned from sparse geological data. Constrained potential field forward modelling has been undertaken to highlight key features and resolve deeply sourced anomalies within the Thomson Orogen. The Thomson Orogen is characterised by long-wavelength and low-amplitude geophysical anomalies when compared with the northern and western Precambrian terranes of the Australian continent. Prominent NE- and NW-trending gravity anomalies reflect the fault architecture of the region. High-intensity Bouguer gravity anomalies correlate with shallow basement rocks. Bouguer gravity anomalies below –300 µm/s2 define the distribution of the Devonian Adavale Basin and associated troughs. The magnetic grid shows smooth textures, punctuated by short-wavelength, high-intensity anomalies that indicate magnetic contribution at different crustal levels. It is interpreted that meta-sedimentary basement rocks of the Thomson Orogen, intersected in several drill holes, are representative of a seismically non-reflective and non-magnetic upper basement. Short-wavelength, high-intensity magnetic source bodies and colocated negative Bouguer gravity responses are interpreted to represent shallow granitic intrusions. Long-wavelength magnetic anomalies are inferred to reflect the topography of a seismically reflective and magnetic lower basement. Potential field forward modelling indicates that the Thomson Orogen might be a single terrane. We interpret that the lower basement consists of attenuated Precambrian and mafic enriched continental crust, which differs from the oceanic crust of the Lachlan Orogen further south. 相似文献