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741.
Thomas A. M. Pugh James Ryder A. Robert MacKenzie Sarah J. Moller James D. Lee Carole Helfter Eiko Nemitz Douglas Lowe C. Nicholas Hewitt 《Journal of Atmospheric Chemistry》2010,65(2-3):89-110
Measurements of atmospheric composition have been made over a remote rainforest landscape. A box model has previously been demonstrated to model the observed daytime chemistry well. However the box model is unable to explain the nocturnal measurements of relatively high [NO] and [O3], but relatively low observed [NO2]. It is shown that a one-dimensional (1-D) column model with simple O3-NOx chemistry and a simple representation of vertical transport is able to explain the observed nocturnal concentrations and predict the likely vertical profiles of these species in the nocturnal boundary layer (NBL). Concentrations of tracers carried over from the end of the night can affect the atmospheric chemistry of the following day. To ascertain the anomaly introduced by using the box model to represent the NBL, vertically-averaged NBL concentrations at the end of the night are compared between the 1-D model and the box model. It is found that, under low to medium [NOx] conditions (NOx?<?1 ppbv), a simple parametrisation can be used to modify the box model deposition velocity of ozone, in order to achieve good agreement between the box and 1-D models for these end-of-night concentrations of NOx and O3. This parametrisation would could also be used in global climate-chemistry models with limited vertical resolution near the surface. Box-model results for the following day differ substantially if this effective nocturnal deposition velocity for ozone is implemented; for instance, there is a 9% increase in the following days peak ozone concentration. However under medium to high [NOx] conditions (NOx > 1 ppbv), the effect on the chemistry due to the vertical distribution of the species means no box model can adequately represent chemistry in the NBL without modifying reaction rate coefficients. 相似文献
742.
Jeffrey L. Collett Jr. Pierre Herckes Sarah Youngster Taehyoung Lee 《Atmospheric Research》2008,87(3-4):232
Considerable effort has been put into characterizing the ionic composition of fogs and clouds over the past twenty-five years. Recently it has become evident that clouds and fogs often contain large concentrations of organic material as well. Here we report findings from a series of studies examining the organic composition of radiation fogs in central California. Organic compounds in these fogs comprise a major fraction of total solute mass, with total organic carbon sometimes reaching levels of several tens of mg/L. This organic matter is comprised of a wide variety of compounds, ranging from low molecular weight organic acids to high molecular weight compounds with molecular masses approaching several hundred to a thousand g/mole. The most abundant individual compounds are typically formic acid, acetic acid, and formaldehyde. High concentrations are also observed of some dicarboxylic acids (e.g., oxalate) and dicarbonyls (e.g., glyoxal and methylglyoxal) and of levoglucosan, an anhydrosugar characteristically emitted by biomass combustion. Many other compounds have been identified in fog water by GC/MS, including long chain n-alkanoic acids, n-alkanes, PAH, and others, although these compounds typically comprise a total of only a few percent of fog TOC. Measurements of fog scavenging of organic and elemental carbon reveal preferential scavenging of organic carbon. Tracking of individual organic compounds utilized as source type markers suggests the fogs differentially scavenge carbonaceous particles from different source types, with more active processing of wood smoke than vehicle exhaust. Observations of high deposition velocities of fog-borne organic carbon, in excess of 1 cm/s, indicate that fogs in the region represent an important mechanism for cleansing the atmosphere of pollution. 相似文献
743.
Bernard Bourdon Sarah Bureau Morten B. Andersen Eric Pili Amélie Hubert 《Chemical Geology》2009,258(3-4):275-287
This study investigates U-series, Sr isotopes, major and trace elements in a chalk aquifer system located in Eastern France. Soil and rock samples were collected along depth profiles down to 45 m in four localities as an attempt to investigate the weathering processes in the soil, the unsaturated zone and the saturated zone of the aquifer. Interstitial water was extracted from soils and rocks by a centrifugation technique. U-series offer a powerful tool to calculate weathering rates because the relative mobility of the U- and Th-isotopes can be precisely measured and it does not require the determination of a reference state as in other approaches. As expected, the data show very large mobile element depletion in the soil with large 230Th excess relative to 238U, while the rocks show more limited but not insignificant mobile element depletion. The U-series data have been used to constrain weathering rates based on a 1-D reactive transport model. Weathering rates in the near surface are about 10–100 times faster than at depth. However, when integrated over the depth of the cores, including the unsaturated and the saturated zones, this underground weathering represents more than 30% of the total weathering flux, assuming congruent dissolution of carbonates. The (234U/238U) ratios in interstitial water are consistent with solid samples showing 234U depletion near the surface and an excess 234U at depth. A leaching experiment performed on chalk shows that the excess 234U in natural waters percolating through carbonate rocks results both from preferential 234U leaching and direct recoil in the interstitial water. A new approach was used to derive the recoil ejection factor based on BET measurements and the fractal dimension of chalk surface. Consideration of preferential leaching and recoil allows a more accurate modeling of weathering rates. 相似文献
744.
Kunaljeet S. Tanwar Sarah C. Petitto Peter J. Eng 《Geochimica et cosmochimica acta》2009,73(15):4346-2587
The surface structure of α-Fe2O3(0 0 0 1) was studied using crystal truncation rod (CTR) X-ray diffraction before and after reaction with aqueous Fe(II) at pH 5. The CTR results show the unreacted α-Fe2O3(0 0 0 1) surface consists of two chemically distinct structural domains: an O-layer terminated domain and a hydroxylated Fe-layer terminated domain. After exposing the α-Fe2O3(0 0 0 1) surface to aqueous Fe(II), the surface structure of both co-existing structural domains was modified due to adsorption of Fe at crystallographic lattice sites of the substrate, resulting in six-coordinated adsorbed Fe at the surface. The average Fe-O bond lengths of the adsorbed Fe are consistent with typical Fe(III)-O bond lengths (in octahedral coordination), providing evidence for the oxidation of Fe(II) to Fe(III) upon adsorption. These results highlight the important role of substrate surface structure in controlling Fe(II) adsorption. Furthermore, the molecular scale structural characterization of adsorbed Fe provides insight into the process of Fe(II) induced structural modification of hematite surfaces, which in turn aids in assessing the effective reactivity of hematite surfaces in Fe(II) rich environments. 相似文献
745.
This paper introduces the special issue ‘organisational geographies of power’ by examining the theoretical and empirical context for debates. It does this, firstly, with reference to existing theoretical work on what power is and does as well as work on the construction of power relations. Building on this, the paper then, secondly, examines the way relational and production network approaches have incorporated power into work on transnational corporations before, thirdly, considering how work on neoliberalism has studied the construction of spatial power relations. In doing this the paper highlights four important questions for future research relating to the practices and spatiality of power, the exercising of power and the situated effects of power relations. 相似文献
746.
This paper presents sedimentary evidence for rapid englacial debris entrainment during jökulhlaups. Previous studies of jökulhlaup sedimentology have focused predominantly on proglacial impact, rather than depositional processes within glaciers. However, observations of supraglacial floodwater outbursts suggest that englacial sediment emplacement is possible during jökulhlaups. The November 1996 jökulhlaup from Skei?arárjökull, Iceland presented one of the first opportunities to examine englacial flood deposits in relation to former supraglacial outlets. Using observations from Skei?arárjökull, this paper identifies and explains controls on the deposition of englacial flood sediments and presents a qualitative model for englacial jökulhlaup deposition. Englacial jökulhlaup deposits were contained within complex networks of upglacier‐dipping fractures. Simultaneous englacial deposition of fines and boulder‐sized sediment demonstrates that englacial fracture discharge had a high transport capacity. Fracture geometry was an important control on the architecture of englacial jökulhlaup deposits. The occurrence of pervasively frozen flood deposits within Skei?arárjökull is attributed to freeze‐on by glaciohydraulic supercooling. Floodwater, flowing subglacially or through upglacier‐dipping fractures, would have supercooled as it was raised to the surface faster than its pressure‐melting point could increase as glaciostatic pressure decreased. Evidence for floodwater contact with the glacier bed is supported by the ubiquitous occurrence of sheared diamict rip‐ups and intra‐clasts of basal ice within jökulhlaup fractures, deposited englacially some 200–350 m above the bed of Skei?arárjökull. Evidence for fluidal supercooled sediment accretion is apparent within stratified sands, deposited englacially at exceptionally high angles of rest in the absence of post‐depositional disturbance. Such primary sediment structures cannot be explained unless sediment is progressively accreted to opposing fracture walls. Ice retreat from areas of former supraglacial outbursts revealed distinct ridges characterized by localized upwellings of sediment‐rich floodwater. These deposits are an important addition to current models of englacial sedimentation and demonstrate the potential for post‐jökulhlaup landform development. Copyright © 2001 John Wiley & Sons, Ltd. 相似文献
747.
Dialogue, metaphors of dialogue and understandings of geography 总被引:2,自引:0,他引:2
Increasingly, human and physical geographers alike describe their research practices as involving dialogue of some kind. However, the widespread popularity of the term belies some very different understandings of its meaning and methodological implications. In this paper we reflect on these different conceptions of 'dialogical' geography as a way, first, of illustrating the broad range of understandings of research methodology now current in the discipline and, second, of identifying their implications for three long–standing controversies in the discipline: relativism and the truth of geographical knowledge, the associated dualisms between subject/object, nature/society, and realism/constructionism, and the potential for unity between human and physical geography. We argue that, while dialogue is a potentially fruitful way of understanding and practising geography, that the defence of it, like the attacks on it, is often misconceived. 相似文献
748.
Hermann Albert J.; Hinckley Sarah; Megrey Bernard A.; Napp Jeffrey M. 《ICES Journal of Marine Science》2001,58(5):1030-1041
749.
Subsistence in coastal fisheries policy: What's in a word? 总被引:1,自引:2,他引:1
Consideration of subsistence fishing activities seems particularly relevant to coastal fisheries policy, yet formal recognition of subsistence fishing is often absent from associated policy frameworks. A critical problem is the very meaning of the term “subsistence.” A review of the literature on subsistence, dominated until recently by North American research, reveals a schism between interpretations emphasizing material aspects of subsistence and interpretations highlighting cultural aspects. The North American literature on the subject is heavily influenced by a focus on Arctic indigenous populations emphasizing cultural survival. Ultimately, subsistence can be a matter of survival in the belly, the soul, or both. International case studies suggest that different interpretations of subsistence are appropriate in different circumstances, and that appropriate policy can be fashioned only after the local context of subsistence is understood. 相似文献
750.
Plio-Pleistocene microtephra in DSDP site 231, Gulf of Aden 总被引:1,自引:0,他引:1
Sarah J. Feakins Francis H. Brown Peter B. deMenocal 《Journal of African Earth Sciences》2007,48(5):341-352
We reconstruct a Plio-Pleistocene microscopic tephrostratigraphy for DSDP Site 231 in the Gulf of Aden. Systematic microtephrostratigraphy increases the potential for identifying tephra horizons for regional stratigraphic correlation and age control, as well as providing information about eruptive histories. Microtephra reveal three main pulses of volcanism c. 4.0–3.2 Ma, 2.4 Ma and 1.7–1.3 Ma, corresponding to peaks in volcanic activity recorded in the East African Rift System. Previous studies of DSDP Site 231 have reported six visible tephra horizons (up to 25 cm thick) with geochemical compositions matching East African tuffs. We find 68 additional microtephra horizons through microscopic examination of 1050 samples (each integrating c. 3 ka) in over 200 m of marine sediments. We report the major and minor element geochemical compositions of individual glass shards in six of these microtephra horizons and establish a robust correlation at 168.73 m to the Lokochot Tuff (3.58 Ma), which together with previously identified tephra, provides a tightly constrained chronostratigraphy for the mid Pliocene. 相似文献