Polyfluorinated compounds in waste water treatment plant effluents and surface waters along the River Elbe, Germany   总被引：4，自引：0，他引：4  

Lutz Ahrens  Sebastian Felizeter  Renate Sturm  Zhiyong Xie  Ralf Ebinghaus 《Marine pollution bulletin》2009,58(9):1326-1333

Polyfluorinated compounds (PFCs) were investigated in waste water treatment plant (WWTP) effluents and surface waters of the River Elbe from samples collected in 2007. Concentrations of various PFCs, including C₄–C₈ perfluorinated sulfonates (PFSAs), C₆ and C₈ perfluorinated sulfinates, 6:2 fluorotelomer sulfonate, C₅–C₁₃ perfluorinated carboxylic acids (PFCAs), C₄ and C₈ perfluoroalkyl sulfonamides and 6:2, 8:2 and 10:2 unsaturated fluorotelomercarboxylic acids were quantified. ∑PFC concentrations of the river water ranged from 7.6 to 26.4 ng L⁻¹, whereas ∑PFC concentrations of WWTP effluents were approximately 5–10 times higher (30.5–266.3 ng L⁻¹), indicating that WWTPs are potential sources of PFCs in the marine environment. PFC patterns of different WWTP effluents varied depending on the origin of the waste water, whereas the profile of PFC composition in the river water was relatively constant. In both kinds of water samples, perfluorooctanoic acid (PFOA) was the major PFC, whereas perfluorobutane sulfonate (PFBS) was the predominant PFSA.  相似文献   

Using global node-based velocity in random walk particle tracking in variably saturated porous media: application to contaminant leaching from road constructions   总被引：2，自引：0，他引：2  

Chan-Hee Park  Christof Beyer  Sebastian Bauer  Olaf Kolditz 《Environmental Geology》2008,55(8):1755-1766

Precise and efficient numerical simulation of transport processes in subsurface systems is a prerequisite for many site investigation or remediation studies. Random walk particle tracking (RWPT) methods have been introduced in the past to overcome numerical difficulties when simulating propagation processes in porous media such as advection-dominated mass transport. Crucial for the precision of RWPT methods is the accuracy of the numerically calculated ground water velocity field. In this paper, a global node-based method for velocity calculation is used, which was originally proposed by Yeh (Water Resour Res 7:1216–1225, 1981). This method is improved in three ways: (1) extension to unstructured grids, (2) significant enhancement of computational efficiency, and (3) extension to saturated (groundwater) as well as unsaturated systems (soil water). The novel RWPT method is tested with numerical benchmark examples from the literature and used in two field scale applications of contaminant transport in saturated and unsaturated ground water. To evaluate advective transport of the model, the accuracy of the velocity field is demonstrated by comparing several published results of particle pathlines or streamlines. Given the chosen test problem, the global node-based velocity estimation is found to be as accurate as the CK method (Cordes and Kinzelbach in Water Resour Res 28(11):2903–2911, 1992) but less accurate than the mixed or mixed-hybrid finite element methods for flow in highly heterogeneous media. To evaluate advective–diffusive transport, a transport problem studied by Hassan and Mohamed (J Hydrol 275(3–4):242–260, 2003) is investigated here and evaluated using different numbers of particles. The results indicate that the number of particles required for the given problem is decreased using the proposed method by about two orders of magnitude without losing accuracy of the concentration contours as compared to the published numbers.  相似文献   

Influence of the atmospheric conditions on PM<Subscript>10</Subscript> concentrations in Poznań, Poland     

Bartosz Czernecki  Marek Półrolniczak  Leszek Kolendowicz  Michał Marosz  Sebastian Kendzierski  Natalia Pilguj 《Journal of Atmospheric Chemistry》2017,74(1):115-139

This study investigates atmospheric conditions’ influence on the mean and extreme characteristics of PM₁₀ concentrations in Poznań during the period 2006–2013. A correlation analysis was carried out to identify the most important meteorological variables influencing the seasonal dynamics of PM₁₀ concentrations. The highest absolute correlation values were obtained for planetary boundary layer height (r = ?0.57), thermal (daily minimum air temperature: r = ?0.51), anemological (average daily wind speed: r = ?0.37), and pluvial (precipitation occurrence: r = ?0.36) conditions, however the highest correlations were observed for temporal autocorrelations (1 day lag: r = 0.70). As regulated by law, extreme events were identified on the basis of daily threshold value i.e. 50 μg m^?3. On average, annually there are approximately 71.3 days anywhere in the city when the threshold value is exceeded, 46.6 % of those occur in winter. Additionally, 83.7 % of these cases have been found to be continuous episodes of a few days, with the longest one persisting for 22 days. The analysis of the macro-scale circulation patterns led to the identification of an easy-to-perceive seasonal relations between atmospheric fields that favour the occurrence of high PM₁₀ concentration, as well as synoptic situations contributing to the rapid air quality improvement. The highest PM₁₀ concentrations are a clear reaction to a decrease in air temperature by over 3 °C, with simultaneous lowering of PBL height, mean wind speed (by around 1 m s^?1) and changing dominant wind directions from western to eastern sectors. In most cases, such a situation is related to the expansion of a high pressure system over eastern Europe and weakening of the Icelandic Low. Usually, air quality conditions improve along with an intensification of westerlies associated with the occurrence of low pressure systems over western and central Europe. Opposite relations are distinguishable in summer, when air quality deterioration is related to the inflow of tropical air masses originating over the Sahara desert.  相似文献   

Development of a New Method of Extraction of Interstitial Water from Low‐Porosity Consolidated Sediments Recovered During Super‐Deep Drilling Projects          下载免费PDF全文

Tomohiro Toki  Harue Masuda  Harunur Rashid  Sebastian Hammerschmidt  Ryuichi Shinjo 《Geostandards and Geoanalytical Research》2016,40(2):291-300

During the Integrated Ocean Drilling Program (IODP) Expedition 338, several methods were tested for the extraction of interstitial water in consolidated, low‐porosity deep‐sea sediments from Site C0002 in the Kumano Basin. On the basis of those tests, we propose a modified ground rock interstitial normative determination (GRIND) method of extraction of interstitial water. In separate runs of the new method, sediment samples were ground in a ball mill with either ultrapure water or a solution of HNO₃. The interstitial water was then extracted with a conventional squeezer. Sufficient solution was extracted by this method to analyse most major and a few minor components of interstitial water that were comparable to those previously reported for samples extracted by the conventional squeezing method. The new method requires much smaller amounts of sediment than that of the conventional method and will be useful for analysis of samples recovered during super‐deep drilling programmes.  相似文献   

Temperature-dependent dissolution of residual non-aqueous phase liquids: model development and verification     

Steffi Popp  Christof Beyer  Andreas Dahmke  Nicolas Koproch  Ralf Köber  Sebastian Bauer 《Environmental Earth Sciences》2016,75(11):953

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Perceptions of environmental change and migration decisions     

Vally Koubi  Sebastian Stoll  Gabriele Spilker 《Climatic change》2016,135(3-4):439-451

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Towards the assimilation of tree-ring-width records using ensemble Kalman filtering techniques     

Walter Acevedo  Sebastian Reich  Ulrich Cubasch 《Climate Dynamics》2016,46(5-6):1909-1920

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X-ray computed microtomography—a useful tool for petrophysical properties determination     

Jadwiga A. Jarzyna  Paulina I. Krakowska  Edyta Puskarczyk  Kamila Wawrzyniak-Guz  Jakub Bielecki  Konrad Tkocz  Jacek Tarasiuk  Sebastian Wroński  Marek Dohnalik 《Computational Geosciences》2016,20(5):1155-1167

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Interactive Knowledge Generation in Urban Green Building Transitions     

Bérénice Preller  Julia Affolderbach  Christian Schulz  Sebastian Fastenrath  Boris Braun 《The Professional geographer》2017,69(2):214-224

Knowledge coproduction between practitioners and scientists offers promising opportunities for the emerging research field of the geography of sustainability transitions. Drawing on experiences from an international research project on urban green building transitions, this article explores the potentials and challenges of interactive and collaborative knowledge generation methods in understanding sustainability transitions. Our results show that ongoing engagement with local experts and practitioners through interactive World Café workshops and follow-up exchanges allows for a better understanding of the research context and knowledge exchange to all participants involved in the research process.  相似文献   

Nondestructive density determination on marine sediment cores from gamma-ray attenuation measurements     

Sebastian Gerland  Heinrich Villinger 《Geo-Marine Letters》1995,15(2):111-118

We describe an improved nondestructive technique for density measurement based on gamma-ray absorption that permits construction of high-resolution density profiles of marine sediment cores. The system is capable of resolving vertical density variations with a spatial resolution of 4 mm and absolute accuracy of ± 1%. Comparison with conventional density determination on samples confirms the absolute accuracy. In addition to standard vertical profiling, a core rotation option is included to measure density as a function of rotation angle. This allows the quantification of the variability of density within a layer and detection of inhomogenities like icerafted debris or biogenic structures.  相似文献