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91.
Norbert?A.?GajosEmail author Craig?C.?Lundstrom Alexander?H.?Taylor 《Contributions to Mineralogy and Petrology》2016,171(11):93
We present new Fe and Si isotope ratio data for the Torres del Paine igneous complex in southern Chile. The multi-composition pluton consists of an approximately 1 km vertical exposure of homogenous granite overlying a contemporaneous 250-m-thick mafic gabbro suite. This first-of-its-kind spatially dependent Fe and Si isotope investigation of a convergent margin-related pluton aims to understand the nature of granite and silicic igneous rock formation. Results collected by MC-ICP-MS show a trend of increasing δ56Fe and δ30Si with increasing silica content as well as a systematic increase in δ56Fe away from the mafic base of the pluton. The marginal Torres del Paine granites have heavier Fe isotope signatures (δ56Fe = +0.25 ± 0.02 2se) compared to granites found in the interior pluton (δ56Fe = +0.17 ± 0.02 2se). Cerro Toro country rock values are isotopically light in both Fe and Si isotopic systems (δ56Fe = +0.05 ± 0.02 ‰; δ30Si = ?0.38 ± 0.07 ‰). The variations in the Fe and Si isotopic data cannot be accounted for by local assimilation of the wall rocks, in situ fractional crystallization, late-stage fluid exsolution or some combination of these processes. Instead, we conclude that thermal diffusion or source magma variation is the most likely process producing Fe isotope ratio variations in the Torres del Paine pluton. 相似文献
93.
Emissions of biogenic volatile organic compounds (BVOC) were measured using a relaxed eddy accumulation (REA) technique on an above-canopy tower in a temperate forest (Changbai Mountain, Jilin province, China) during the 2010 and 2011 summer seasons. Solar global radiation and photosynthetically active radiation (PAR) were also measured. Based on PAR energy dynamic balance, an empirical BVOC emission and PAR transfer model was developed that includes the processes of BVOC emissions and PAR transfer above the canopy level, including PAR absorption and consumption, and scattering by gases, liquids, and particles (GLPs). Simulated emissions of isoprene and monoterpenes were in agreement with observations. The averages of the relative estimator biases for the flux were 39.3 % for isoprene, and 27.1 % for monoterpenes in the 2010 and 2011 growing seasons, with NMSE (normalized mean square error) values of 0.133 and 0.101, respectively. The observed and simulated mean diurnal variations of isoprene and monoterpenes in the 2010 and 2011 growing seasons were evaluated for the validation of the empirical model. Under observed atmospheric conditions, the sensitivity analysis showed that emissions of isoprene and monoterpenes were more sensitive to changes in PAR than to water vapor content or to the magnitude of the scattering factor. The emissions of isoprene and monoterpenes in the 2010 and 2011 growing seasons (from June to September) were estimated using this empirical model along with hourly observational data, with mean hourly emissions of 1.71 and 1.55 mg m?2 h?1 for isoprene, and 0.48 and 0.47 mg m?2 h?1 for monoterpenes in 2010 and 2011, respectively. As formaldehyde (HCHO) is considered as the main oxidation product of isoprene and monoterpenes, it is necessary to investigate the link between HCHO and BVOC emissions. GOME-2 HCHO vertical column densities (VCDs) can be used to estimate BVOC emission fluxes in the Changbai Mountain temperate forest. 相似文献
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Joong-Bae Ahn Sera Jo Myoung-Seok Suh Dong-Hyun Cha Dong-Kyou Lee Song-You Hong Seung-Ki Min Seong-Chan Park Hyun-Suk Kang Kyo-Moon Shim 《Asia-Pacific Journal of Atmospheric Sciences》2016,52(2):223-236
The change of extreme precipitation is assessed with the HadGEM2-AO - 5 Regional Climate Models (RCMs) chain, which is a national downscaling project undertaken cooperatively by several South Korean institutes aimed at producing regional climate change projection with fine resolution (12.5 km) around the Korean Peninsula. The downscaling domain, resolution and lateral boundary conditions are held the same among the 5 RCMs to minimize the uncertainties from model configuration. Climatological changes reveal a statistically significant increase in the mid-21st century (2046- 2070; Fut1) and the late-21st century (2076-2100; Fut2) precipitation properties related to extreme precipitation, such as precipitation intensity and average of upper 5 percentile daily precipitation, with respect to the reference period (1981-2005). Changes depending on the intensity categories also present a clear trend of decreasing light rain and increasing heavy rain. In accordance with these results, the change of 1-in-50 year maximum precipitation intensity over South Korea is estimated by the GEV method. The result suggests that the 50-year return value (RV50) will change from -32.69% to 72.7% and from -31.6% to 96.32% in Fut1 and from -31.97% to 86.25% and from -19.45% to 134.88% in Fut2 under representative concentration pathway (RCP) 4.5 and 8.5 scenarios, respectively, at the 90% confidence level. This study suggests that multi-RCMs can be used to reduce uncertainties and assess the future change of extreme precipitation more reliably. Moreover, future projection of the regional climate change contains uncertainties evoked from not only driving GCM but also RCM. Therefore, multi-GCM and multi-RCM studies are expected to provide more robust projection. 相似文献
98.
Myoung-Seok Suh Seok-Geun Oh Young-Suk Lee Joong-Bae Ahn Dong-Hyun Cha Dong-Kyou Lee Song-You Hong Seung-Ki Min Seong-Chan Park Hyun-Suk Kang 《Asia-Pacific Journal of Atmospheric Sciences》2016,52(2):151-169
We projected surface air temperature changes over South Korea during the mid (2026-2050) and late (2076-2100) 21st century against the current climate (1981-2005) using the simulation results from five regional climate models (RCMs) driven by Hadley Centre Global Environmental Model, version 2, coupled with the Atmosphere- Ocean (HadGEM2-AO), and two ensemble methods (equal weighted averaging, weighted averaging based on Taylor’s skill score) under four Representative Concentration Pathways (RCP) scenarios. In general, the five RCM ensembles captured the spatial and seasonal variations, and probability distribution of temperature over South Korea reasonably compared to observation. They particularly showed a good performance in simulating annual temperature range compared to HadGEM2-AO. In future simulation, the temperature over South Korea will increase significantly for all scenarios and seasons. Stronger warming trends are projected in the late 21st century than in the mid-21st century, in particular under RCP8.5. The five RCM ensembles projected that temperature changes for the mid/late 21st century relative to the current climate are +1.54°C/+1.92°C for RCP2.6, +1.68°C/+2.91°C for RCP4.5, +1.17°C/+3.11°C for RCP6.0, and +1.75°C/+4.73°C for RCP8.5. Compared to the temperature projection of HadGEM2-AO, the five RCM ensembles projected smaller increases in temperature for all RCP scenarios and seasons. The inter-RCM spread is proportional to the simulation period (i.e., larger in the late-21st than mid-21st century) and significantly greater (about four times) in winter than summer for all RCP scenarios. Therefore, the modeled predictions of temperature increases during the late 21st century, particularly for winter temperatures, should be used with caution. 相似文献
99.
Dana?L.?DrewEmail author Ilya?N.?Bindeman Matthew?W.?Loewen Paul?J.?Wallace 《Contributions to Mineralogy and Petrology》2016,171(1):10
During the onset of caldera cluster volcanism at a new location in the Snake River Plain (SRP), there is an increase in basalt fluxing into the crust and diverse silicic volcanic products are generated. The SRP contains abundant and compositionally diverse hot, dry, and often low-δ18O silicic volcanic rocks produced through time during the formation of individual caldera clusters, but more H2O-rich eruptive products are rare. We report analyses of quartz-hosted melt inclusions from pumice clasts from the upper and lower Arbon Valley Tuff (AVT) to gain insight into the initiation of caldera cluster volcanism. The AVT, a voluminous, caldera-forming rhyolite, represents the commencement of volcanism (10.44 Ma) at the Picabo volcanic field of the Yellowstone hotspot track. This is a normal δ18O rhyolite consisting of early and late erupted members (lower and upper AVT, respectively) with extremely radiogenic Sr isotopes and unradiogenic Nd isotopes, requiring that ~50 % of the mass of these elements is derived from melts of Archean upper crust. Our data reveal distinctive features of the early erupted lower AVT melt including: variable F concentrations up to 1.4 wt%, homogenous and low Cl concentrations (~0.08 wt%), H2O contents ranging from 2.3 to 6.4 wt%, CO2 contents ranging from 79 to 410 ppm, and enrichment of incompatible elements compared to the late erupted AVT, subsequent Picabo rhyolites, SRP rhyolites, and melt inclusions from other metaluminous rhyolites (e.g., Bishop Tuff, Mesa Falls Tuff). We couple melt inclusion data with Ti measurements and cathodoluminescence (CL) imaging of the host quartz phenocrysts to elucidate the petrogenetic evolution of the AVT rhyolitic magma. We observe complex and multistage CL zoning patterns, the most critical being multiple truncations indicative of several dissolution–reprecipitation episodes with bright CL cores (higher Ti) and occasional bright CL rims (higher Ti). We interpret the high H2O, F, F/Cl, and incompatible trace element concentrations in the context of a model involving melting of Archean crust and mixing of the crustal melt with basaltic differentiates, followed by multiple stages of fractional crystallization, remelting, and melt extraction. This multistage process, which we refer to as distillation, is further supported by the complex CL zoning patterns in quartz. We interpret new Δ18O(Qz-Mt) isotope measurements, demonstrating a 0.4 ‰ or ~180 °C temperature difference, and strong Sr isotopic and chemical differences between the upper and lower AVT to represent two separate eruptions. Similarities between the AVT and the first caldera-forming eruptions of other caldera clusters in the SRP (Yellowstone, Heise and Bruneau Jarbidge) suggest that the more evolved, lower-temperature, more H2O-rich rhyolites of the SRP are important in the initiation of a caldera cluster during the onset of plume impingement. 相似文献
100.
Sunyurp Park 《地理信息系统科学与遥感》2016,53(5):634-650
Spatiotemporal characteristics and anthropogenic signals of aerosol optical thickness (AOT) distributions over Korea are investigated in this study using AOT time-series data from the Moderate Resolution Imaging Spectroradiometer (MODIS). AOT observations, a quantitative measure of the atmospheric quality, had significant geographical variations during the study period (2000–2010). Comparing metro cities or counties with similar populations, western regions showed higher AOT values than eastern regions. Particular matter with a diameter < 10 µm (PM10), including aeolian dust or yellow dust, is the primary component of atmospheric aerosols, and their transport into the region has shown a strong seasonal pattern with its peak from March to April and lows from July to September. These seasonal dust patterns, however, did not correspond well to temporal AOT records, which typically reached the maximum level in June nationwide. Rather, widespread regional fire events and humidity showed significant correlations with AOT time-series. This correlation rapidly increased as the range of fire occurrence was extended to the west as far as 115°E. The relative humidity also had a significant correlation with AOT during the month of June. In addition to urban emission of anthropogenic aerosols, regional biomass burning and secondary growth of hygroscopic aerosols are considered important contributors to the degradation of the atmospheric environment during the non-Asian Dust season over the Korean Peninsula. 相似文献