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31.
32.
Fog and rain water chemistry at Mt. Fuji: A case study during the September 2002 campaign 总被引:2,自引:0,他引:2
Koichi Watanabe Yusaku Takebe Nobuhiro Sode Yasuhito Igarashi Hiroshi Takahashi Yukiko Dokiya 《Atmospheric Research》2006,82(3-4):652
Measurements of fog and rain water chemistry at the summit of Mt. Fuji, the highest peak in Japan, as well as at Tarobo, the ESE slope of Mt. Fuji in September 2002. The pH of fog and rain water sampled at Mt. Fuji varied over a range of 4.0–6.8. Acidic fogs (pH < 5.0) were observed at the summit when the air mass came from the industrial regions on the Asian continent. The ratio of [SO42−]/[NO3−] in the fog water was lower at Tarobo than at the summit. High concentrations of Na+ and Cl− were determined in the rain water sampled at the summit, possibly because of the long-range transport of sea-salt particles raised by a typhoon through the middle troposphere. The vertical transport of sea-salt particles would influence the cloud microphysical properties in the middle troposphere. Significant loss of Mg2+ was seen in the rain water at the summit. The concentrations of peroxides in the fog and rain water were relatively large (10–105 μM). The potential capacity for SO2 oxidation seems to be strong from summer to early autumn at Mt. Fuji. The fog water peroxide concentrations displayed diurnal variability. The peroxide concentrations in the nighttime were significantly higher than those in the daytime. 相似文献
33.
Partitioning of Ni2+, Co2+, Fe2+, Mn2+ and Mg2+ between olivine and silicate melts: compositional dependence of partition coefficient 总被引:1,自引:0,他引:1
Eiichi Takahashi 《Geochimica et cosmochimica acta》1978,42(12):1829-1844
Partitioning of Ni2+, Co2+, Fe2+, Mn2+ and Mg2+ between olivine and silicate melts has been determined near the join (Mg0.5·-Fe0.5)2SiO4-K2O 4SiO2 and for seven different basaltic compositions. The experiments were made at 1 atm total pressure, 1500-1100°C, and under moderate to reducing oxygen fugacities. The concentration factor, defined as KMO = (MO)ol/(MO)liq (molar ratio), increases markedly for all the cations studied as the olivine component of the liquid decreases. Much of the increase in KMO is considered as due to the compositional effect of the coexisting liquid: the temperature effect on KMO is probably opposite to the compositional effect (KMO decreases as temperature decreases).The partition coefficient KMO-MgO = (MO/MgO)ol/(MO/MgO)liq for the reaction, Mol2+ + Mgliq2+ = Mliq2+ + Mgol2+. is relatively constant over a wide range of SiO2 content of the liquid, except in the case of Ni2+. The partition coefficients have similar ranges both in synthetic and natural rock systems: KNiO-MgO = 1.8–3.0, KCoO-MgO = 0.6–0.8, KFeO-MgO = 0.27–0.38, and KMnO-MgO = 0.23–0.32. There is a systematic variation in the partition coefficient KMO-MgO with the composition of liquid; KMO-MgO increases with increasing SiO2 content of melt. The partition coefficients for Co2+, Fe2+ and Mn2+ are useful to test the equilibration of olivine with magma of a wide compositional range. 相似文献
34.
Seasonal variability regarding the nature of precipitation and the activity of cumulus convection during the 1991 Meiyu season of Changjiang-Huaihe River Basin(Jianghuai)has been investigated by calculating apparent heat source/apparent moisture sink and analyzing TBB(cloud-top blackody radiation temperature)data.It is found that three periods of strong ascending motion during the Meiyu season lead to three episodes of heavy rain,and the latent heat due to the precipitation is of the sole heat source of the atmosphere.The nature of precipitation shows distinct seasonal variability,from frontal precipitation of the first episode to the extremely strong convective precipitation of the third episode.TBB field of East Asia may well reflect not only the intensity of convection and rainfall,but also the movement of rain belt and convection belt.In the whole Meiyu season.convection belt mainly stays in Jianghuai.but may shift within the domain of East Asia.Its locating in Jianghuai or not determines the maintenance or break of Meiyu.In the third episode,the narrow convection belt over Jianghuai is mainly caused by southwest monsoon which takes moist and convective atmosphere from tropical ocean. 相似文献
35.
36.
M. Chauvin H.-G. Florén M. Jackson T. Kamae T. Kawano M. Kiss M. Kole V. Mikhalev E. Moretti G. Olofsson S. Rydström H. Takahashi J. Lind J.-E. Strömberg O. Welin A. Iyudin D. Shifrin M. Pearce 《Experimental Astronomy》2016,41(1-2):17-41
In the 50 years since the advent of X-ray astronomy there have been many scientific advances due to the development of new experimental techniques for detecting and characterising X-rays. Observations of X-ray polarisation have, however, not undergone a similar development. This is a shortcoming since a plethora of open questions related to the nature of X-ray sources could be resolved through measurements of the linear polarisation of emitted X-rays. The PoGOLite Pathfinder is a balloon-borne hard X-ray polarimeter operating in the 25-240 keV energy band from a stabilised observation platform. Polarisation is determined using coincident energy deposits in a segmented array of plastic scintillators surrounded by a BGO anticoincidence system and a polyethylene neutron shield. The PoGOLite Pathfinder was launched from the SSC Esrange Space Centre in July 2013. A near-circumpolar flight was achieved with a duration of approximately two weeks. The flight performance of the Pathfinder design is discussed for the three Crab observations conducted. The signal-to-background ratio for the observations is shown to be 0.25 ±0.03 and the Minimum Detectable Polarisation (99 % C.L.) is (28.4 ±2.2) %. A strategy for the continuation of the PoGOLite programme is outlined based on experience gained during the 2013 maiden flight. 相似文献
37.
采用1979—2009年NCEP/NCAR再分析资料、NOAA向外长波辐射(outgoing long-wave radiation,简称OLR)及扩展重建海表面温度资料,对南海大气季节内振荡(Intra-seasonal Oscillation,简称ISO)特征及其与ENSO循环的关系进行了诊断分析。结果表明:1)南海大气ISO的30~60 d周期在5—10月均显著。一般年南海大气ISO的对流传播在纬向上存在东传和西传,在经向上具有南北半球季节性摆动的特征。以低频动能表征的南海大气ISO强度年代际变化特征明显,近31 a来趋势增强,年变化呈单峰结构,峰值在7—8月。2)南海大气ISO的对流与ENSO循环显著相关,其强度在El Nio(La Nia)年减弱(增强)。与一般年对比,南海大气ISO对流在El Nio和La Nia年均表现为西传减弱、北传显著。北传特征表现为强对流活跃带于春季(4—5月)北跳至北半球(在La Nia年最北可至35°N),但在北半球的传播方向与一般年相比存在显著差异。3)南海大气ISO强度与ENSO循环关系密切,在El Nio(La Nia)年减弱(增强),两者表现为约半年(6~8个月)的滞后相关。Nio3区海表面温度异常序列与南海大气ISO强度的相关在中西太平洋地区和El Nio成熟前的春、秋季最显著,同时相关中心伴随低频动能高值区东移。 相似文献
38.
Shinya Iwasaki Kozo Takahashi Yusuke Ogawa Seiichiro Uehara Christoph Vogt 《Journal of Oceanography》2014,70(3):241-249
Accurate knowledge of the extent of biogenic opal preservation in marine sediment cores is important for paleoceanographic reconstructions. The alkaline leaching method is widely employed for %biogenic opal analysis due to its ease and speed. In this study, a revised method for measuring %biogenic opal in sediment from arctic coring expedition samples was suggested. The studied middle Eocene sediments from the central Arctic Ocean presented a problem in insufficiently leaching biogenic opal with a Na2CO3 solution. Based on XRD analysis, it was suggested that such an alkaline resistance results from slight diagenesis of biogenic opal. In order to solve this problem, an alkaline leaching method utilizing a 2 M NaOH solution was suggested for the accurate measurement of %biogenic opal in the Eocene sediments from the central Arctic. Furthermore, dissolution rates from lithogenic matter by NaOH solution were measured in order to correct the %biogenic opal values. 相似文献
39.
Performance assessment of three convective parameterization schemes in WRF for downscaling summer rainfall over South Africa 总被引:2,自引:1,他引:1
Satyaban B. Ratna J. V. Ratnam S. K. Behera C. J. deW. Rautenbach T. Ndarana K. Takahashi T. Yamagata 《Climate Dynamics》2014,42(11-12):2931-2953
Austral summer rainfall over the period 1991/1992 to 2010/2011 was dynamically downscaled by the weather research and forecasting (WRF) model at 9 km resolution for South Africa. Lateral boundary conditions for WRF were provided from the European Centre for medium-range weather (ECMWF) reanalysis (ERA) interim data. The model biases for the rainfall were evaluated over the South Africa as a whole and its nine provinces separately by employing three different convective parameterization schemes, namely the (1) Kain–Fritsch (KF), (2) Betts–Miller–Janjic (BMJ) and (3) Grell–Devenyi ensemble (GDE) schemes. All three schemes have generated positive rainfall biases over South Africa, with the KF scheme producing the largest biases and mean absolute errors. Only the BMJ scheme could reproduce the intensity of rainfall anomalies, and also exhibited the highest correlation with observed interannual summer rainfall variability. In the KF scheme, a significantly high amount of moisture was transported from the tropics into South Africa. The vertical thermodynamic profiles show that the KF scheme has caused low level moisture convergence, due to the highly unstable atmosphere, and hence contributed to the widespread positive biases of rainfall. The negative bias in moisture, along with a stable atmosphere and negative biases of vertical velocity simulated by the GDE scheme resulted in negative rainfall biases, especially over the Limpopo Province. In terms of rain rate, the KF scheme generated the lowest number of low rain rates and the maximum number of moderate to high rain rates associated with more convective unstable environment. KF and GDE schemes overestimated the convective rain and underestimated the stratiform rain. However, the simulated convective and stratiform rain with BMJ scheme is in more agreement with the observations. This study also documents the performance of regional model in downscaling the large scale climate mode such as El Niño Southern Oscillation (ENSO) and subtropical dipole modes. The correlations between the simulated area averaged rainfalls over South Africa and Nino3.4 index were ?0.66, ?0.69 and ?0.49 with KF, BMJ and GDE scheme respectively as compared to the observed correlation of ?0.57. The model could reproduce the observed ENSO-South Africa rainfall relationship and could successfully simulate three wet (dry) years that are associated with La Niña (El Niño) and the BMJ scheme is closest to the observed variability. Also, the model showed good skill in simulating the excess rainfall over South Africa that is associated with positive subtropical Indian Ocean Dipole for the DJF season 2005/2006. 相似文献
40.
Takeshi?KuritaniEmail author Takeyoshi?Yoshida Jun-Ichi?Kimura Toshiro?Takahashi Yuka?Hirahara Takashi?Miyazaki Ryoko?Senda Qing?Chang Yoshinori?Ito 《Contributions to Mineralogy and Petrology》2014,167(2):969
The conditions under which rear-arc magmas are generated were estimated using primary basalts from the Sannome-gata volcano, located in the rear of the NE Japan arc. Scoriae from the volcano occur with abundant crustal and mantle xenoliths, suggesting that the magma ascended rapidly from the upper mantle. The scoriae show significant variations in their whole-rock compositions (7.9–11.1 wt% MgO). High-MgO scoriae (MgO > ~9.5 wt%) have mostly homogeneous 87Sr/86Sr ratios (0.70318–0.70320), whereas low-MgO scoriae (MgO < ~9 wt%) have higher 87Sr/86Sr ratios (>0.70327); ratios tend to increase with decreasing MgO content. The high-MgO scoriae are aphyric, containing ~5 vol% olivine microphenocrysts with Mg# [100 × Mg/(Mg + Fe2+)] of up to 90. In contrast, the low-MgO scoriae have crustal xenocrysts of plagioclase, alkali feldspar, and quartz, and the mineralogic modes correlate negatively with whole-rock MgO content. On the basis of these observations, it is inferred that the high-MgO scoriae represent primary or near-primary melts, while the low-MgO scoriae underwent considerable interaction with the crust. Using thermodynamic analysis of the observed petrological features of the high-MgO scoriae, the eruption temperature of the magmas was constrained to 1,160–1,220 °C. Given that the source mantle was depleted MORB-source mantle, the primary magma was plausibly generated by ~7 % melting of a garnet-bearing spinel peridotite; taking this into consideration, and considering the constraints of multi-component thermodynamics, we estimated that the primary Sannome-gata magma was generated in the source mantle with 0.5–0.6 wt% H2O at 1,220–1,230 °C and at ~1.8 GPa, and that the H2O content of the primary magma was 6–7 wt%. The rear-arc Sannome-gata magma was generated by a lower degree of melting of the mantle at greater depths and lower temperatures than the frontal-arc magma from the Iwate volcano, which was also estimated to be generated by ~15 % melting of the source mantle with 0.6–0.7 wt% H2O at ~1,250 °C and at ~1.3 GPa. 相似文献