Interannual and Decadal Changes in Tropospheric Ozone in China and the Associated Chemistry–Climate Interactions: A Review     

Yu FU  Hong LIAO  Yang YANG 《大气科学进展》2019,36(9):975-993

China has been experiencing widespread air pollution due to rapid industrialization and urbanization in recent decades.The two major concerns of ambient air quality in China are particulate matter(PM) and tropospheric ozone(O_3). With the implementation of air pollution prevention and control actions in the last five years, the PM pollution in China has been substantially reduced. In contrast, under the conditions of the urban air pollution complex, the elevated O_3 levels in city clusters of eastern China, especially in warm seasons, have drawn increasing attention. Emissions of air pollutants and their precursors not only contribute to regional air quality, but also alter climate. Climate change in turn can change chemical processes, long-range transport, and local meteorology that influence air pollution. Compared to PM, less is known about O_3 pollution and its climate effects over China. Here, we present a review of the main findings from the literature over the period 2011–18 with regard to the characteristics of O_3 concentrations in China and the mechanisms that drive its interannual to decadal variations, aiming to identify robust conclusions that may guide decision-making for emissions control and to highlight critical knowledge gaps. We also review regional and global modeling studies that have investigated the impacts of tropospheric O_3 on climate, as well as the projections of future tropospheric O_3 owing to climate and/or emission changes.  相似文献   

CWRF模式在中国夏季极端降水模拟的误差订正          下载免费PDF全文

董晓云  余锦华  梁信忠  马圆 《应用气象学报》2019,30(2):223-232

利用1980—2015年6—8月我国逐日降水观测数据评估CWRF模式（Climate-Weather Research and Forecasting model）多种参数化方案对我国夏季日降水的模拟能力,并考察累积概率变换偏差订正法（CDFt）的订正效果。通过将广义帕累托分布（GPD）引入到偏差订正模型中,提出针对极端降水的累积概率变换偏差订正法（XCDFt）,检验和评估其对极端降水订正的适用性。结果显示:CWRF模式微物理过程选用Morrison-aerosol参数化方案组合对我国降水场的模拟较好,CDFt订正效果良好;XCDFt偏差订正模型能够较好地提取模式建模与验证时期变化信号,订正后相比订正前与观测极端降水的概率分布更为接近;经过XCDFt订正后华南、华中和华北地区20年一遇的极端降水重现水平较模拟值更接近观测值,可为CWRF模式提高极端降水的业务预测水平提供参考。  相似文献   

基于不同分辨率和参数化方案的新疆区域数值模式性能初步评估     

杜娟  李曼  于晓晶  辛渝 《沙漠与绿洲气象(新疆气象)》2019,(3):57-65

基于中尺度数值模式WRF,选取新疆两次强降水过程,设计3个试验方案,其中试验1为控制试验,试验2提高分辨率,试验3提高分辨率并调整物理参数化方案,初步评估不同分辨率和参数化方案对新疆区域2m温度、10m风速、降水预报的影响。结果表明:(1)提高分辨率对2m温度、10m风速模拟精度均有提高,2m温度预报精度提高约0.5℃,降低了日间温度模拟冷偏差;10m风速预报精度提高约0.5m/s,降低了风速模拟正偏差;但提高分辨率后,模式出现虚假降水预报的情况。(2)提高分辨率并调整物理参数化方案后,2m温度模拟误差略有减小,模拟偏差减小约0.2℃;10m风速模拟误差增大约0.5m/s,模拟偏差增大超过0.5m/s;对降水落区、量级的模拟精度显著提高,减小了降水中心的模拟强度,对虚假降水预报有一定修正。  相似文献   

加强新疆锂资源规范管理和助力产业延伸的对策分析     

曹伟伟  段星星  陈世忠  邢浩  米宝昕  杨振  周玉 《地质论评》2024,70(S1):323-324

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Selection of sand models and identification of parameters using an enhanced genetic algorithm          下载免费PDF全文

Yin‐Fu Jin  Zhen‐Yu Yin  Shui‐Long Shen  Pierre‐Yves Hicher 《国际地质力学数值与分析法杂志》2016,40(8):1219-1240

Numerous constitutive models of granular soils have been developed during the last few decades. As a consequence, how to select an appropriate model with the necessary features based on conventional tests and with an easy way of identifying parameters for geotechnical applications has become a major issue. This paper aims to discuss the selection of sand models and parameters identification by using genetic algorithm. A real‐coded genetic algorithm is enhanced for the optimization with high efficiency. Models with gradually varying features (elastic‐perfectly plastic modelling, nonlinear stress–strain hardening, critical state concept and two‐surface concept) are selected from numerous sand models as examples for optimization. Conventional triaxial tests on Hostun sand are selected as the objectives in the optimization. Four key points are then discussed in turn: (i) which features are necessary to be accounted for in constitutive modelling of sand; (ii) which type of tests (drained and/or undrained) should be selected for an optimal identification of parameters; (iii) what is the minimum number of tests that should be selected for parameter identification; and (iv) what is the suitable and least strain level of objective tests to obtain reliable and reasonable parameters. Finally, a useful guide, based on all comparisons, is provided at the end of the discussion. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

Influence of core property on multi-electron process in slow collisions of isocharged sequence ions with neon     

卢荣春  于得洋  邵曹杰  阮芳芳  蔡晓红 《海洋学报(英文版)》2010,29(11)

Influence of core property on multi-electron process in the collisions of q=6-9 and 11 isocharged sequence ions with Ne is investigated in the keV/u region. The cross-section ratios of double-, triple-, quadruple- and total multi-electron processes to the single electron capture process as well as the partial ratios of different reaction channels to the relevant multi-electron process are measured by using position-sensitive and time-of-flight techniques. The experimental data are compared with the theoretical predictions including the extended classical over-barrier model, the molecular Columbic barrier model and the semi-empirical scaling law. Results show a core effect on multi-electron process of isocharge ions colliding with Neon, which is consistent with the results of Helium we obtained previously.  相似文献   

Evaluating the spatiotemporal variations of water budget across China over 1951–2006 using IBIS model     

Qiuan Zhu  Hong Jiang  Xiaohua Wei  Changhui Peng  Xiuqing Fang  Shirong Liu  Guomo Zhou  Shuquan Yu  Weiming Ju 《水文研究》2010,24(4):429-445

The Integrated Biosphere Simulator is used to evaluate the spatial and temporal patterns of the crucial hydrological variables [run‐off and actual evapotranspiration (AET)] of the water balance across China for the period 1951–2006 including a precipitation analysis. Results suggest three major findings. First, simulated run‐off captured 85% of the spatial variability and 80% of the temporal variability for 85 hydrological gauges across China. The mean relative errors were within 20% for 66% of the studied stations and within 30% for 86% of the stations. The Nash–Sutcliffe coefficients indicated that the quantity pattern of run‐off was also captured acceptably except for some watersheds in southwestern and northwestern China. The possible reasons for underestimation of run‐off in the Tibetan plateau include underestimation of precipitation and uncertainties in other meteorological data due to complex topography, and simplified representations of the soil depth attribute and snow processes in the model. Second, simulated AET matched reasonably with estimated values calculated as the residual of precipitation and run‐off for watersheds controlled by the hydrological gauges. Finally, trend analysis based on the Mann–Kendall method indicated that significant increasing and decreasing patterns in precipitation appeared in the northwest part of China and the Yellow River region, respectively. Significant increasing and decreasing trends in AET were detected in the Southwest region and the Yangtze River region, respectively. In addition, the Southwest region, northern China (including the Heilongjiang, Liaohe, and Haihe Basins), and the Yellow River Basin showed significant decreasing trends in run‐off, and the Zhemin hydrological region showed a significant increasing trend. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

Molecular and isotopic compositions of bitumens in Silurian tar sands from the Tarim Basin,NW China: Characterizing biodegradation and hydrocarbon charging in an old composite basin   总被引：1，自引：0，他引：1  

Wanglu Jia  Zhongyao Xiao  Chiling Yu  Ping'an Peng 《Marine and Petroleum Geology》2010

Biodegradation and oil mixing in Silurian sandstone reservoirs of the Tarim Basin, one of the largest composite basins in China, were investigated by analyzing the molecular characteristics and stable carbon isotopic signatures of low-molecular-weight (LMW) saturated hydrocarbons and high-molecular-weight (HMW) asphaltenes. Detection of 25-norhopanes and 17-nortricyclic terpanes in most Silurian tar sands from the Tabei Uplift in the Tarim Basin suggests a much greater degree of biodegradation here than in the Tazhong Uplift. This explains the relatively more abundant tricyclic terpanes, gammacerane, pregnane and diasteranes in tar sands from the Tabei Uplift than in those from the Tazhong Uplift. Hence, care must be taken when assigning oil source correlations using biomarkers in tar sands because of the biodegradation and mixing of oils derived from multiple sources in such an old composite basin. Asphaltenes in the tar sands seem to be part of the oil charge before biodegradation, depending on the relative anti-biodegradation characteristics of asphaltenes, the similarity in carbon isotopic signatures for asphaltenes and their pyrolysates, and the consistent product distribution for flash pyrolysis and for regular steranes in asphaltene pyrolysates, regardless of whether the tar sands were charged with fresh oil. According to the relative distributions of regular steranes and the relatively abundant 1,2,3,4-tetramethylbenzene significantly enriched in ¹³C, the oil sources for asphaltenes in the tar sands might be related to lower Paleozoic marine source rocks formed in euxinic conditions. Nevertheless, the relatively low abundance of gammacerane and C₂₈ regular steranes observed in asphaltene pyrolysates and residual hydrocarbons, within limited samples investigated in this work, made a direct correlation of oils originally charged into Silurian tar sands with those Cambrian source rocks, reported so far, seem not to be possible. Comparison of carbon isotopic signatures of n-alkanes in asphaltene pyrolysates with those of LMW saturated hydrocarbons is helpful in determining if the abundant n-alkanes in tar sands are derived from fresh oil charges after biodegradation. The limited carbon isotopic data for n-alkanes in LMW saturated hydrocarbons from the tar sands can be used to classify oils charged after biodegradation in the composite basin into four distinct groups.  相似文献   

A new method for platform design based on parametric technology     

Yan-Yun Yu  Ming Chen  Yan Lin  Zhuo-Shang Ji 《Ocean Engineering》2010,37(5-6):473-482

A new method for platform design, named parametric platform design method (PPDM), is presented in this paper in order to improve the mobile platform design efficiency. In this method, an integrated parametric system that fully considers the characteristics of the platform is developed, which significantly optimizes the design process with the top–bottom design concept. In the parametric system, the main geometric dimensions are taken as parameters, while the topology between the structure members, the function requirements and the safety requirements are converted into geometric constraints. By geometric constraint solving (GCS), a set of parameters that satisfy all the given constraints are determined, and then the design scheme is obtained by several core algorithms, such as parametric tank subdivision, 3D stability calculation, parametric structure design, FEM preprocessing, etc. The parametric method greatly increases the changeability and the reusability of the platform model, and concurrent design is well supported. As the model is driven by parameters, PPDM is an excellent method for optimization design. As a result, PPDM has incomparable advantages on the design efficiency over traditional methods.  相似文献   

Palaeozoic uplands and unconformity in the North China Block: constraints from zircon LA‐ICP‐MS dating and geochemical analysis of Bauxite     

Yu Wang  Liyun Zhou  Lijun Zhao  Mo Ji  Honglei Gao 《地学学报》2010,22(4):264-273

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