Soil organic carbon enrichment of dust emissions: magnitude,mechanisms and its implications for the carbon cycle     

Nicholas P. Webb  Craig L. Strong  Adrian Chappell  Samuel K. Marx  Grant H. McTainsh 《地球表面变化过程与地形》2013,38(14):1662-1671

Soil erosion is an important component of the global carbon cycle. However, little attention has been given to the role of aeolian processes in influencing soil organic carbon (SOC) flux and the release of greenhouse gasses, such as carbon dioxide (CO₂), to the atmosphere. Understanding the magnitude and mechanisms of SOC enrichment in dust emissions is necessary to evaluate the impact of wind erosion on the carbon cycle. This research examines the SOC content and enrichment of dust emissions measured using Big Spring Number Eight (BSNE) wind‐vane samplers across five land types in the rangelands of western Queensland, Australia. Our results show that sandy soils and finer particulate quartz‐rich soils are more efficient at SOC emission and have larger SOC dust enrichment than clay‐rich aggregated soils. The SOC enrichment ratios of dusts originating from sites with sand‐rich soil ranged from 2·1–41·9, while the mean enrichment ratio for dusts originating from the clay soil was 2·1. We hypothesize that stronger inter‐particle bonds and the low grain density of the aggregated clay soil explain its reduced capacity to release SOC during saltation, relative to the particulate sandy soils. We also show that size‐selective sorting of SOC during transport may lead to further enrichment of SOC dust emissions. Two dust samples from regional transport events were found to contain 15–20% SOC. These preliminary results provide impetus for additional research into dust SOC enrichment processes to elucidate the impact of wind erosion on SOC flux and reduce uncertainty about the role of soil erosion in the global carbon cycle. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

Maximizing Net Extraction Using an Injection‐Extraction Well Pair in a Coastal Aquifer     

Chunhui Lu  Adrian D. Werner  Craig T. Simmons  Neville I. Robinson  Jian Luo 《Ground water》2013,51(2):219-228

In this study, we examine the maximum net extraction rate from the novel arrangement of an injection‐extraction well pair in a coastal aquifer, where fresh groundwater is reinjected through the injection well located between the interface toe and extraction well. Complex potential theory is employed to derive a new analytical solution for the maximum net extraction rate and corresponding stagnation‐point locations and recirculation ratio, assuming steady‐state, sharp‐interface conditions. The injection‐extraction well‐pair system outperforms a traditional single extraction well in terms of net extraction rate for a broad range of well placement and pumping rates, which is up to 50% higher for an aquifer with a thickness of 20 m, hydraulic conductivity of 10 m/d, and fresh water influx of 0.24 m²/d. Sensitivity analyses show that for a given fresh water discharge from an inland aquifer, a larger maximum net extraction is expected in cases with a smaller hydraulic conductivity or a smaller aquifer thickness, notwithstanding physical limits to drawdown at the pumping well that are not considered here. For an extraction well with a fixed location, the optimal net extraction rate linearly increases with the distance between the injection well and the sea, and the corresponding injection rate and recirculation ratio also increase. The analytical analysis in this study provides initial guidance for the design of well‐pair systems in coastal aquifers, and is therefore an extension beyond previous applications of analytical solutions of coastal pumping that apply only to extraction or injection wells.  相似文献   

Impact of loading displacements on SLR-derived parameters and on the consistency between GNSS and SLR results   总被引：5，自引：4，他引：1  

Krzysztof Sośnica  Daniela Thaller  Rolf Dach  Adrian Jäggi  Gerhard Beutler 《Journal of Geodesy》2013,87(8):751-769

Displacements of the Earth’s surface caused by tidal and non-tidal loading forces are relevant in high-precision space geodesy. Some of the corrections are recommended by the international scientific community to be applied at the observation level, e.g., ocean tidal loading (OTL) and atmospheric tidal loading (ATL). Non-tidal displacement corrections are in general recommended not to be applied in the products of the International Earth Rotation and Reference Systems Service, in particular atmospheric non-tidal loading (ANTL), oceanic and hydrological non-tidal corrections. We assess and compare the impact of OTL, ATL and ANTL on SLR-derived parameters by reprocessing 12 years of SLR data considering and ignoring individual corrections. We show that loading displacements have an influence not only on station long-term stability, but also on geocenter coordinates, Earth Rotation Parameters, and satellite orbits. Applying the loading corrections reduces the amplitudes of annual signals in the time series of geocenter and station coordinates. The general improvement of the SLR station 3D coordinate repeatability when applying OTL, ATL and ANTL corrections are 19.5 %, 0.2 % and 3.3 % respectively, w.r.t. the solutions without loading corrections. ANTL corrections play a crucial role in the combination of optical (SLR) and microwave (GNSS, VLBI, DORIS) space geodetic observation techniques, because of the so-called Blue-Sky effect: SLR measurements can be carried out only under cloudless sky conditions—typically during high air pressure conditions, when the Earth’s crust is deformed, whereas microwave observations are weather-independent. Thus, applying the loading corrections at the observation level improves SLR-derived products as well as the consistency with microwave-based results. We assess the Blue-Sky effect on SLR stations and the consistency improvement between GNSS and SLR solutions when ANTL corrections are included. The omission of ANTL corrections may lead to inconsistencies between SLR and GNSS solutions of up to 2.5 mm for inland stations. As a result, the estimated GNSS–SLR coordinate differences correspond better to the local ties at the co-located stations when applying ANTL corrections.  相似文献   

The nature and genesis of marginal Cu–PGE–Au sulphide mineralisation in Paleogene Macrodykes of the Kangerlussuaq region, East Greenland     

David A. Holwell  Thomas Abraham-James  Reid R. Keays  Adrian J. Boyce 《Mineralium Deposita》2012,47(1-2):3-21

The Kangerlussuaq region of East Greenland hosts a variety of early Tertiary extrusive and intrusive igneous rocks related to continental break up and the passage of the ancestral Iceland plume. These intrusive bodies include a number of gabbroic macrodykes, two of which—the Miki Fjord Macrodyke, and the newly discovered Togeda Macrodyke—contain Cu–PGE–Au sulphide mineralisation along their margins. Sulphides occur as disseminated interstitial blebs and rounded globules of chalcopyrite and pyrrhotite with some Fe–Ti oxides and platinum-group minerals, comprising largely Pd bismuthides and tellurides. The globules are interpreted to have formed from fractionation of trapped droplets of an immiscible Cu- and Pd-rich sulphide melt and show geopetal indicators. Sulphur isotopes imply a local crustal source of S in these from pyritic sediments of the Kangerlussuaq Basin. Thus, generation of these sulphide occurrences was controlled by local country rock type. Low Ni/Cu and Pt/Pd ratios, also present in the Platinova reefs in the Skaergaard Intrusion, indicate that early fractionation of olivine may have depleted the magma of Ni and suggest the likely presence of a large magma chamber at depth. Xenoliths of Ni-rich olivine cumulates in the Miki Fjord Macrodyke may have been sourced from such a body. The location of thus far unidentified conduit or feeder zones to the macrodykes beneath the present day surface may represent potential targets for more massive sulphide orebodies.  相似文献   

Impact of Berm Breaching on Hyperbenthic Macroinvertebrate Communities in Intermittently Closed Estuaries   总被引：1，自引：0，他引：1  

Adrian W. T. Lill  Gerard P. Closs  Marc Schallenberg  Candida Savage 《Estuaries and Coasts》2012,35(1):155-168

Berm breaching of intermittently closed estuaries, either naturally or due to management practices, results in a physicochemical disturbance due to the flushing of water, material and biota into the ocean and the subsequent tidal influx. In 2007 and 2008 comparative and controlled studies were employed in three New Zealand estuaries: Sawmill Creek (46°04′ S 170°12′ E), Otokia Creek (45°57′ S 179°20′ E) and Kaikorai Lagoon (45°56′ S 170°23′ E), to investigate the impact of berm breaching on the hyperbenthic macroinvertebrate community in intermittently closed estuaries. Significant changes in community structure occurred in both the weekly comparative and the controlled studies (ANOSIM P < 0.01). Furthermore, the catch per unit effort of both total and key invertebrate taxa significantly increased after breaching (ANOVA P < 0.01). However, substantial numbers of individuals were expelled into the ocean (5,800 individuals, 20-min sample) while new taxa immigrated into the estuaries. Along with migration-related changes to community structure, berm breaches also resulted in the loss of ∼80% of inundated habitat and the concentration of existing populations. Consequently, the management of intermittent estuary connections to the ocean has implications for the ecology of individual, managed estuaries and also for regional coastal populations of epibenthic invertebrates.  相似文献   

Meshless BEM and overlapping Schwarz preconditioners for exterior problems on spheroids     

Adrian Costea  Quoc T. Le Gia  Ernst P. Stephan  Thanh Tran 《Studia Geophysica et Geodaetica》2011,55(3):465-477

We consider the exterior Neumann problem of the Laplacian with boundary condition on spheroids. We propose to use spherical radial basis functions in the solution of the boundary integral equation arising from the Dirichlet-to-Neumann map. Our meshless approach with radial basis functions is particularly suitable for handling scattered satellite data. We also propose a preconditioning technique based on an overlapping domain decomposition method to deal with ill-conditioned matrices arising from the approximation problem.  相似文献   

Validation of a Numerical Indicator of Microbial Contamination for Karst Springs   总被引：1，自引：0，他引：1  

Christoph Butscher  Adrian Auckenthaler  Stefan Scheidler  Peter Huggenberger 《Ground water》2011,49(1):66-76

Rapid changes in spring water quality in karst areas due to rapid recharge of bacterially contaminated water are a major concern for drinking water suppliers and users. The main objective of this study was to use field experiments with fecal indicators to verify the vulnerability of a karst spring to pathogens, as determined by using a numerical modeling approach. The groundwater modeling was based on linear storage models that can be used to simulate karst water flow. The vulnerability of the karst groundwater is estimated using such models to calculate criteria that influence the likelihood of spring water being affected by microbial contamination. Specifically, the temporal variation in the vulnerability, depending on rainfall events and overall recharge conditions, can be assessed and quantified using the dynamic vulnerability index (DVI). DVI corresponds to the ratio of conduit to diffuse flow contributions to spring discharge. To evaluate model performance with respect to predicted vulnerability, samples from a spring were analyzed for Escherichia coli, enterococci, Clostridium perfringens, and heterotrophic plate count bacteria during and after several rainfall events. DVI was shown to be an indication of the risk of fecal contamination of spring water with sufficient accuracy to be used in drinking water management. We conclude that numerical models are a useful tool for evaluating the vulnerability of karst systems to pathogens under varying recharge conditions  相似文献   

The degradation characteristics of microbial biomass in soil     

Adrian Spence  David J. Mcnally  Margaret V. McCaul  Brett Paull 《Geochimica et cosmochimica acta》2011,75(10):2571-2581

Soil microbial biomass is a primary source of soil organic carbon (SOC) and therefore plays a fundamental role in carbon and nitrogen cycling. However, little is known about the fate and transformations of microbial biomass in soil. Here we employ HR-MAS NMR spectroscopy to monitor ¹³C and ¹⁵N labeled soil microbial biomass and leachate degradation over time. As expected, there is a rapid loss of carbohydrate structures. However, diffusion edited HR-MAS NMR data reveals that macromolecular carbohydrates are more resistant to degradation and are found in the leachate. Aromatic components survive as dissolved species in the leachate while aliphatic components persist in both the biomass and leachate. Dissolved protein and peptidoglycan accumulate in the leachate and recalcitrant amide nitrogen and lipoprotein persists in both the degraded biomass and leachate. Cross-peaks that appear in ¹H-¹⁵N HR-MAS NMR spectra after degradation suggest that specific peptides are either selectively preserved or used for the synthesis of unknown structures. The overall degradation pathways reported here are similar to that of decomposing plant material degraded under similar conditions suggesting that the difference between recalcitrant carbon from different sources is negligible after decomposition.  相似文献   

Late Holocene Neoglacial conditions from the Lesotho highlands, southern Africa: phytolith and stable carbon isotope evidence from the archaeological site of Likoaeng     

Adrian G. Parker  Julia Lee-Thorp  Peter J. Mitchell 《Proceedings of the Geologists' Association. Geologists' Association》2011,122(1):201-211

The late Holocene environmental history of the Lesotho highlands, southern Africa, is poorly understood with few detailed studies to date. At Likoaeng, Senqu Valley, Lesotho, a 3 m stratified sedimentary sequence from an open-air archaeological site records vegetation development for the period 3400-1070 cal. BP. Phytolith analyses and bulk sediment organic matter δ¹³C indicate that C₄ grassland dominated the lower part of the sequence until approximately 2960 cal. BP when there was a switch to C₃ Pooid grassland (2960-2160 cal. BP). Also noted was a change from hunting mainly bovids to a dominance of fishing at the site. The change in grassland type and archaeological subsistence strategies corresponds with an episode of neoglacial cooling and the expansion of Alpine sourgrasses into lower altitudes. From 2160 to 1600 cal. BP grassland became a mix of C₃ and C₄ types and by 1600-1070 cal. BP there was a return to C₄ dominated grassland. During this latter phase there was a reversal from fishing to hunting again (and eventually some keeping of domestic livestock) at the site. These data outline the vegetation response to latitudinal shifts of frontal systems, and relatively strong atmospheric circulation variability, perhaps underpinned by variations of polar water into the Benguela Current during the late Holocene.  相似文献   

Understanding the fate of iron in a modern temperate estuary: Leirárvogur,Iceland     

Gemma M. Byrne  Richard H. Worden  David M. Hodgson  David A. Polya  Paul R. Lythgoe  Craig D. Barrie  Adrian J. Boyce 《Applied Geochemistry》2011

Fluvial dissolved Fe concentrations decrease upon mixing with seawater, resulting in the formation of Fe-floccules. However, a clear understanding of the fate of these floccules has yet to be established. Assessing how tidal processes affect the formation of Fe-colloids in the Leirárvogur estuary, SW Iceland, is an important step in understanding the formation and potential deposition of estuarine Fe-rich minerals within this estuarine system. The Leirárvogur estuary drains predominately Fe-rich basalt, increasing the likelihood of detecting changes in Fe-phases. Fluvial waters and local lake waters that drain into the estuary were compared and the effects of seasonal changes were considered, in an attempt to understand how varying end-members and external factors play a role in Fe-rich mineral formation. Aqueous and colloidal Fe concentrations were found to be greater towards the head of the Leirárvogur estuary, suggesting that potential Fe-rich minerals and complexes are forming at sites of fluvial input. Increasing suspended colloidal Fe towards the estuary mouth suggests that Fe-colloids are readily transported seaward.  相似文献