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71.
Anna M. Dymshits Peter I. Dorogokupets Igor S. Sharygin Konstantin D. Litasov Anton Shatskiy Sergey V. Rashchenko Eiji Ohtani Akio Suzuki Yuji Higo 《Physics and Chemistry of Minerals》2016,43(6):447-458
A new synchrotron X-ray diffraction study of chromium oxide Cr2O3 (eskolaite) with the corundum-type structure has been carried out in a Kawai-type multi-anvil apparatus to pressure of 15 GPa and temperatures of 1873 K. Fitting the Birch–Murnaghan equation of state (EoS) with the present data up to 15 GPa yielded: bulk modulus (K 0,T0), 206 ± 4 GPa; its pressure derivative K′0,T , 4.4 ± 0.8; (?K 0,T /?T) = ?0.037 ± 0.006 GPa K?1; a = 2.98 ± 0.14 × 10?5 K?1 and b = 0.47 ± 0.28 × 10?8 K?2, where α 0,T = a + bT is the volumetric thermal expansion coefficient. The thermal expansion of Cr2O3 was additionally measured at the high-temperature powder diffraction experiment at ambient pressure and α 0,T0 was determined to be 2.95 × 10?5 K?1. The results indicate that coefficient of the thermal expansion calculated from the EoS appeared to be high-precision because it is consistent with the data obtained at 1 atm. However, our results contradict α 0 value suggested by Rigby et al. (Brit Ceram Trans J 45:137–148, 1946) widely used in many physical and geological databases. Fitting the Mie–Grüneisen–Debye EoS with the present ambient and high-pressure data yielded the following parameters: K 0,T0 = 205 ± 3 GPa, K′0,T = 4.0, Grüneisen parameter (γ 0) = 1.42 ± 0.80, q = 1.82 ± 0.56. The thermoelastic parameters indicate that Cr2O3 undergoes near isotropic compression at room and high temperatures up to 15 GPa. Cr2O3 is shown to be stable in this pressure range and adopts the corundum-type structure. Using obtained thermoelastic parameters, we calculated the reaction boundary of knorringite formation from enstatite and eskolaite. The Clapeyron slope (with \({\text{d}}P/{\text{d}}T = - 0.014\) GPa/K) was found to be consistent with experimental data. 相似文献
72.
73.
74.
Alberto Escudero Nobuyoshi Miyajima Falko Langenhorst 《Chemie der Erde / Geochemistry》2012,72(1):25-30
The chemical composition and microstructure of rutile grains in a ultra-high pressure metamorphic gneiss of the Saxonian Erzgebirge, Germany have been studied by Raman spectroscopy, SEM, EMPA and TEM. Rutile inclusions in garnet contain free dislocations, iron-enriched dislocations and exsolved ilmenite lamellae, while subgrain boundaries are observed in rutile grains of the rock matrix. The previously reported α-PbO2 type TiO2 phase could not be confirmed by our TEM observations. On the basis of Zr solubility in the rutile and the presence of microdiamonds, minimum metamorphic peak conditions of 3.95 GPa and 915 °C are estimated. 相似文献
75.
New and previous versions of the high-resolution 20- and 60-km-mesh Meteorological Research Institute atmospheric general circulation models are used to investigate potential future changes in tropical cyclone (TC) activity in the North Indian Ocean (NIO). Fifteen ensemble experiments are performed under the International Panel on Climate Change A1B scenario. Most of the ensemble future (2075–2099) experiments do not project significant future changes in the basin-scale TC genesis number; however, they commonly show a substantial increase (by 46 %) in TC frequency over the Arabian Sea and a decrease (by 31 %) in the Bay of Bengal. Projected future changes in TC genesis frequency show a marked seasonal variation in the NIO: a significant and robust reduction during the pre-monsoon season, an increase during the peak-monsoon season, and a westward shift during the post-monsoon season. Several large-scale thermodynamic and dynamical parameters are analysed to elucidate the physical mechanism responsible for the future changes in TC activity; this analysis reveals a seasonal dependence of the relative contribution of these parameters to the projected future changes in TC genesis frequency. 相似文献
76.
The concentrations of dissolved organic carbon and nitrogen (DOC and DON, respectively) were measured in Shiraho fringing
reef (Japan), using a high-temperature catalytic-oxidation method. When the seawater on the reef flat (shallow lagoon) was
isolated from the surrounding ocean due to the low tide, the concentrations of DOC and DON on the reef flat were 66–75 and
4.8–5.7 μmol l−1, respectively. The DOC and DON concentrations were higher than those of the adjacent outer ocean (57–58 and 3.8 μmol l−1, respectively), suggesting that the coral reef functioned as a net source of dissolved organic matter for the surrounding
ocean. In order to investigate long-term bacterial decomposition of the reef-derived DOC (RF-DOC), the seawater samples collected
on the reef flat and at the adjacent ocean were incubated in the dark for 1 year. Regression analysis using an exponential
curve that considered two degradability pools (labile and refractory) fitted the mineralization of the RF-DOC very well (r
2 > 0.89). According to the regression analysis, the DOC produced on the reef flat was composed of the labile fraction of 63–94%
(average 77%) and the refractory fraction of 6–37% (average 23%). It was concluded that some of the DOC that was produced
in the coral reef ecosystem was exported to the surrounding ocean if the reef flat had a water residence time less than several
months. The exported organic matter may support microbial communities in the ocean as an energy source. 相似文献
77.
Ryuji Tateyama Eiji Ohtani Hidenori Terasaki Keisuke Nishida Yuki Shibazaki Akio Suzuki Takumi Kikegawa 《Physics and Chemistry of Minerals》2011,38(10):801-807
The compositional dependence on the density of liquid Fe alloys under high pressure is important for estimating the amount
of light elements in the Earth’s outer core. Here, we report on the density of liquid Fe–Si at 4 GPa and 1,923 K measured
using the sink–float method and our investigation on the effect of the Si content on the density of the liquid. Our experiments
show that the density of liquid Fe–Si decreases from 7.43 to 2.71 g/cm3 non-linearly with increasing Si content (0–100 at%). The molar volume of liquid Fe–Si calculated from the measured density
gradually decreases in the compositional range 0–50 at% Si, and increases in the range 50–100 at% Si. It should be noted that
the estimated molar volume of the alloys shows a negative volume of mixing between Fe and Si. This behaviour is similar to
Fe–S liquid (Nishida et al. in Phys Chem Miner 35:417–423, 2008). However, the excess molar volume of mixing for the liquid Fe–Si is smaller than that of liquid Fe–S. The light element
contents in the outer core estimated previously may be an underestimation if we take into account the possible negative value
of the excess mixing volume of iron–light element alloys in the outer core. 相似文献
78.
Human impacts on sand-producing, large benthic foraminifers were investigated on ocean reef flats at the northeast Majuro Atoll, Marshall Islands, along a human population gradient. The densities of dominant foraminifers Calcarina and Amphistegina declined with distance from densely populated islands. Macrophyte composition on ocean reef flats differed between locations near sparsely or densely populated islands. Nutrient concentrations in reef-flat seawater and groundwater were high near or on densely populated islands. δ15N values in macroalgal tissues indicated that macroalgae in nearshore lagoons assimilate wastewater-derived nitrogen, whereas those on nearshore ocean reef flats assimilate nitrogen from other sources. These results suggest that increases in the human population result in high nutrient loading in groundwater and possibly into nearshore waters. High nutrient inputs into ambient seawater may have both direct and indirect negative effects on sand-producing foraminifers through habitat changes and/or the collapse of algal symbiosis. 相似文献
79.
Mouctar Kamara Rashila Deshar Sahadev Sharma Md. Kamruzzaman Akio Hagihara 《Journal of Oceanography》2012,68(6):851-856
Weller??s allometric model assumes that the allometric relationships of mean area occupied by a tree $ \bar{s} $ , i.e., the reciprocal of population density $ \rho $ , $ \bar{s}\left( { = {1 \mathord{\left/ {\vphantom {1 {\rho = g_{\varphi } \cdot \bar{w}^{\varphi } }}} \right. \kern-0em} {\rho = g_{\varphi } \cdot \bar{w}^{\varphi } }}} \right) $ , mean tree height $ \bar{H}\left( { = g_{\theta } \cdot \bar{w}^{\theta } } \right) $ , and mean aboveground mass density $ \bar{d}\left( { = g_{\delta } \cdot \bar{w}^{\delta } } \right) $ to mean aboveground mass $ \bar{w} $ hold. Using the model, the self-thinning line $ \left( {\bar{w} = K \cdot \rho^{ - \alpha } } \right) $ of overcrowded Kandelia obovata stands in Okinawa, Japan, was studied over 8?years. Mean tree height increased with increasing $ \bar{w} $ . The values of the allometric constant $ \theta $ and the multiplying factor $ g_{\theta } $ are 0.3857 and 2.157?m?kg???, respectively. The allometric constant $ \delta $ and the multiplying factor $ g_{\delta } $ are ?0.01673 and 2.685?m?3?kg1???, respectively. The $ \delta $ value was not significantly different from zero, showing that $ \bar{d} $ remains constant regardless of any increase in $ \bar{w} $ . The average of $ \bar{d} $ , i.e., biomass density $ \left( {{{\bar{w} \cdot \rho } \mathord{\left/ {\vphantom {{\bar{w} \cdot \rho } {\bar{H}}}} \right. \kern-0em} {\bar{H}}}} \right) $ , was 2.641?±?0.022?kg?m?3, which was considerably higher than 1.3?C1.5?kg?m?3 of most terrestrial forests. The self-thinning exponent $ \alpha \left( { = {1 \mathord{\left/ {\vphantom {1 {\varphi = }}} \right. \kern-0em} {\varphi = }}{1 \mathord{\left/ {\vphantom {1 {\left\{ {1 - \left( {\theta + \delta } \right)} \right\}}}} \right. \kern-0em} {\left\{ {1 - \left( {\theta + \delta } \right)} \right\}}}} \right) $ and the multiplying factor $ K\left( { = \left( {g_{\theta } \cdot g_{\delta } } \right)^{\alpha } } \right) $ were estimated to be 1.585 and 16.18?kg?m?2??, respectively. The estimators $ \theta $ and $ \delta $ are dependent on each other. Therefore, the observed value of $ \theta + \delta $ cannot be used for the test of the hypothesis that the expectation of the estimator $ \theta + \delta $ equals 1/3, i.e., $ \alpha = {3 \mathord{\left/ {\vphantom {3 2}} \right. \kern-0em} 2} $ , or 1/4, i.e., $ \alpha = {4 \mathord{\left/ {\vphantom {4 3}} \right. \kern-0em} 3} $ . The $ \varphi $ value was 0.6310, which is the same as the reciprocal of the self-thinning exponent of 1.585, and was not significantly different from 2/3 (t?=?1.860, df?=?191, p?=?0.06429), i.e., $ \alpha = {3 \mathord{\left/ {\vphantom {3 2}} \right. \kern-0em} 2} $ . Thus the self-thinning exponent is not significantly different from 3/2 based on the simple geometric model. On the other hand, the self-thinning exponent was significantly different from 3/4 (t?=?6.213, df?=?191, p?=?3.182?×?10?9), i.e., $ \alpha = {4 \mathord{\left/ {\vphantom {4 3}} \right. \kern-0em} 3} $ . Therefore, the self-thinning exponent is significantly different from 4/3 based on the metabolic model. 相似文献
80.
We have made a Monte Carlo simulation of the intergalactic absorption in order to model the Lyman continuum absorption, which is required to estimate the escape fraction of the Lyman continuum from distant galaxies. To input into the simulation, we derive an empirical distribution function of the intergalactic absorbers which reproduces recent observational statistics of the Lyman α forest, Lyman limit systems (LLSs) and damped Lyman α systems (DLAs) simultaneously. In particular, we assume a common functional form of the number evolution along the redshift for all types of absorbers. The Lyman series transmissions in our simulation reproduce the observed redshift evolution of the transmissions excellently, and the Lyman continuum transmission also agrees with an observed estimation which is still quite rare in the literature. The probability distribution of the Lyman α opacity in our simulation is lognormal with a tail towards a large opacity. This tail is produced by DLAs. The probability distribution of the Lyman continuum opacity in our simulation also shows a broad tail towards a large opacity. This tail is produced by LLSs. Because of the rarity of LLSs, we have a chance to have a clean line of sight in the Lyman continuum even for z ∼ 4 with a probability of about 20 per cent. Our simulation expects a good correlation between the Lyman continuum opacity and the Lyman α opacity, which may be useful to estimate the former from the latter for an individual line of sight. 相似文献