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11.
James M. Kaste Benjamin C. Bostick Eiliv Steinnes 《Geochimica et cosmochimica acta》2011,75(6):1642-1661
High concentrations of metals in organic matter can inhibit decomposition and limit nutrient availability in ecosystems, but the long-term fate of metals bound to forest litter is poorly understood. Controlled experiments indicate that during the first few years of litter decay, Al, Fe, Pb, and other metals that form stable complexes with organic matter are naturally enriched by several hundred percent as carbon is oxidized. The transformation of fresh litter to humus takes decades, however, such that current datasets describing the accumulation and release of metals in decomposing organic matter are timescale limited. Here we use atmospheric 210Pb to quantify the fate of metals in canopy-derived litter during burial and decay in coniferous forests in New England and Norway where decomposition rates are slow and physical soil mixing is minimal. We measure 210Pb inventories in the O horizon and mineral soil and calculate a 60-630 year timescale for the production of mobile organo-metallic colloids from the decomposition of fresh forest detritus. This production rate is slowest at our highest elevation (∼1000 m) and highest latitude sites (>63°N) where decomposition rates are expected to be low.We calculate soil layer ages by assuming a constant supply of atmospheric 210Pb and find that they are consistent with the distribution of geochemical tracers from weapons fallout, air pollution, and a direct 207Pb application at one site. By quantifying a gradient of organic matter ages with depth in the O horizon, we describe the accumulation and loss of metals in the soil profile as organic matter transforms from fresh litter to humus. While decomposition experiments predict that Al and Fe concentrations increase during the initial few years of decay, we show here that these metals continue to accumulate in humus for decades, and that enrichment occurs at a rate higher than can be explained by quantitative retention during decomposition alone. Acid extractable Al and Fe concentrations are higher in the humus layer of the O horizon than in the mineral soil immediately beneath this layer: it is therefore unlikely that physical soil mixing introduces significant Al and Fe to humus. This continuous enrichment of Al and Fe over time may best be explained by the recent suggestion that metals are mined from deeper horizons and brought into the O horizon via mycorrhizal plants. In sharp contrast to Al and Fe, we find that Mn concentrations in decomposing litter layers decrease exponentially with age, presumably because of leaching or rapid uptake, which may explain the low levels of acid extractable Mn in the mineral soil. This study quantifies how metals are enriched and lost in decomposing organic matter over a longer timescale than previous studies have been able to characterize. We also put new limits on the rate at which metals in litter become mobile organo-metallic complexes that can migrate to deeper soil horizons or surface waters. 相似文献
12.
Lead has been exploited by man over thousands of years for a variety of metallurgical, medicinal, and industrial purposes. The cumulative output of Pb from mining is estimated to be 260 million metric tonnes and 85% of this has occurred over the last two centuries. Global annual production of Pb from mining was about 3 million tonnes at the turn of the millenium. Terrestrial ecosystems all over Norway have been contaminated moderately to strongly by Pb and other trace elements from atmospheric deposition. With the aim of developing a method for mapping the accumulated content of anthropogenic Pb and how deep in the soil profile the atmospherically deposited Pb has penetrated, the concentration of Pb and the 206Pb/207Pb ratio has been studied in podzolic forest soils at four locations with different lithology, i.e. age and type of bedrock, in the Oslo area. The concentrations of Pb in the soil profiles are 6.6–38.1 mg/kg (median 10.3). The 206Pb/207Pb ratio ranges between 1.168 and 1.314 (median 1.267) over the entire profile. In the upper 5 cm the range is 1.168–1.191, similar to ratios determined in recent atmospheric deposition. Applying three different methods, the amount of anthropogenically deposited Pb is estimated at 1–6 t/km2. 相似文献
13.
The concentrations of copper, zinc, cadmium, selenium and mercury were determined in eggs, muscle, liver, kidney and stomach content of nestilings and adults of the Antarctic petrel, Thalassoica antarctica, and its predator, the south polar skua, Chataracta maccormicki, from Svarthamaren, Dronning Maud Land, Antarctica. The dominant food of the petrels is krill, Euphausia superba. The results show relatively high levels of cadmium in krill, which is assumed to be the main reason for the high levels of cadmium in petrels and skuas. Cadmium is almost absent in eggs, but accumulates very rapidly with age in nestlings. The copper concentrations in livers of nestling petrels reach very high levels during growth. This may be seen in connection with physiological development processes. Mercury seems to be accumulated with age and between trophic levels. Among the nestlings, the mercury levels decrease with increasing age, which may be accomplished by the excretion of mercury through the growth of feathers and as a dilution effect during growth. Selenium and mercury are inversely correlated in nestlings. The levels of zinc were similar for different nestling stages and between nestlings and adults in skuas and petrels. 相似文献
14.
Eiliv Larsen Astrid Lyså Ármann Höskuldsson Jan G. Davidsen Marie J. Nadeau Michael Power Georgios Tassis Stefan Wastegård 《第四纪科学杂志》2021,36(2):180-190
We provide the first documentation of tectonic deformation resulting from a volcanic eruption on the island of Jan Mayen. Vertical displacement of about 14 m southwest of the stratovolcano Beerenberg is associated with an eruption in ad 1732 on its southeastern flank. The age of the uplift event is bracketed by radiocarbon-dated driftwood buried by material deposited due to uplift, and by tephra from this eruption. Constraints, inferred from radiocarbon ages alone, allow for the possibility that uplift was completed prior to the ad 1732 eruption. However, the occurrence of tephra in the sediment column indicates that some displacement was ongoing during the eruption but ceased before the eruption terminated. We attribute the tectonic deformation to intrusion of shallow magma associated with the volcanic eruption. Our results complement previous studies of volcanic activity on Jan Mayan by providing precise age constraints for past volcanic activity. Also, it raises new hypotheses regarding the nature, timing and prevalence of precursor tectonic events to Jan Mayan eruptions. The uplift caused the complete isolation of a coastal lake by closing its outlet to the sea, thus landlocking the facultative migratory fish species Arctic charr (Salvelinus alpinus). 相似文献
15.
Air Pollution Studies in Central Russia (Tver and Yaroslavl Regions) Using the Moss Biomonitoring Technique and Neutron Activation Analysis 总被引：1，自引：0，他引：1
E. V. Ermakova M. V. Frontasyeva S. S. Pavlov E. A. Povtoreiko E. Steinnes Ye N. Cheremisina 《Journal of Atmospheric Chemistry》2004,49(1-3):549-561
Data of 34 elements, including heavy metals, halogens, rare earth elements, U, and Th in 139 moss samples, collected in Central Russia in 2000–2002 in the Tver and Yaroslavl regions and in the northern part of the Moscow region, are presented. Factor analysis with VARIMAX rotation was applied to identify possible sources of the elements determined in the mosses. The seven resulting factors represent crust, vegetation and anthropogenic components. Some of the factors were interpreted as being associated with ferrous smelters (Fe, Zn, Sb, Ta); combination of non-ferrous smelters and other industries (Mn, Co, Mo, Cr, Ni, W); an oil-refining plant, and oil combustion at the thermal power plant (V, Ni). The geographical distribution patterns of the factor scores are also presented. Dependency equations of elemental content in mosses versus distance from the source were derived. 相似文献
16.
Reijo Salminen Anne Kousa Rolf Tore Ottesen Olle Selinus Eiliv Steinnes Timo Tarvainen Bjoern OEhlander 《《幕》》2008,31(1):155-162
The mining environment, medical geology and urban geochemistry form a group of related scientific disciplines that have developed strongly during recent years in the Nordic countries. Modern legislation controls the environmental issues. Close co-operation of researchers and legislators has improved the quality and safety of life in the societies of the Nordic countries. In mining environmental studies, methods that are suitable in Arctic conditions have been developed; in medical geology, the input from the Nordic countries has made it an appreciated scientific discipline throughout the world, and in the case of the urban environment, methods developed by our geochemists have especially improved the health conditions, particularly of children. 相似文献
17.
Stable remanent directions encountered in three oriented lake-sediment cores, covering 6 m of gyttja deposits, reveal declination swings with amplitudes of the order of ± 50°. Anomalously low inclinations, scattered around the horizontal in the upper 2 m of core, is attributed to compressional disturbances of the alignment of magnetic grains during the coring procedure. Four 14C dates obtained (1250, 1940, 4600 and 6330 y B.P.) have enabled a correlation with features ‘c’–‘g’ of the British Geomagnetic Master Curve). For the older part of the curve, features ‘h’ and ‘i’, the correlation is questionable. Magneto-mineralogical parameters and qualitative chemical analysis of individual grains by secondary X-ray emission analysis reveal the presence of pure magnetite grains. Scanning electron micrographs show a dominant proportion of concoidal slightly elongated grains (10–80 μm). A few almost-perfect octahedral magnetite crystals can be related to outcrops of augen gneisses in the vicinity confirming a detrital origin of these grains. 相似文献
18.
This study describes shoreline migration paths for late Quaternary sediments on the inner Barents Sea shelf between Kola and the Pechora Sea. The depositional geometries provide an example of stratigraphical architecture in a glacially influenced basin prone to isostatic movements as well as rapid and high-amplitude changes in eustatic sea level. The depositional geometries reflect asymmetrical relative sea level changes characterised by marine inundation upon deglaciation and prolonged forced regressions. Thus, all deposition occurs during the falling stage and lowstand systems tracts. The transgressive and highstand systems tracts are lacking and the maximum landward position of the shoreline is coinciding with the basal surface of forced regression. Shoreline migration is dominated by downward and seaward trajectories, but aggradation occurs on the falling limb of the relative sea level curve due to superimposed eustatic cycles of lower hierarchical order. Fluvial aggradation behind the shoreline takes place during the lowstand systems tract, but is also linked to high sediment supply and may also respond to superimposed lower order sea level fluctuations. Lateral variations in isostatic load due to asynchronous ice advances lead to regional variations in shoreline trajectories. Significant differences in sea level history exist across former ice margins leading to time-transgressive and laterally discontinuous stratigraphical surfaces. Sequence boundaries are not only diachronous along the depositional profile, but also laterally, and basal surfaces of forced regression are strongly diachronous across former ice margins. Absolute age control allows for estimates of the time differences along significant stratigraphical surfaces. 相似文献
19.
Maria A. Jensen Igor N. Demidov Eiliv Larsen Astrid Lyså 《Quaternary Science Reviews》2009,28(23-24):2489-2506
The modern Severnaya Dvina and Mezen river systems in the Arkhangelsk region, NW Russia, are located within extensive palaeovalley systems. The palaeovalleys form depressions in bedrock and have controlled the drainage systems in the area at least since the Last Interglacial. Vertically stacked marine to fluvial sediments reflect deposition during fluctuating climate and sea levels.A compilation of lithostratigraphical data collected during the last decade has been coupled with bedrock topography and geomorphology from satellite images in order to describe the valley fill architecture for the two valley systems. Each system has been divided into a number of depositional units (storeys) separated by incision/non-deposition and used to investigate the timing of aggradational versus incisional phases. Time constraints for each phase are provided by optically stimulated luminescence (OSL) ages, and aggradation and incision are linked to independent records of climate and sea level change.The pattern of aggradation and erosion is regional and primarily driven by episodes of increasing and decreasing sediment supply. Aggradation is correlated to times of deglaciation with high sediment supply from the ice margin, release of sediment from ice-dammed lakes and low vegetation and degradation of permafrost on the flood plain. Incision is related to cold intervals with low sediment supply, delayed incision due to isostatic uplift and drainage of ice-dammed lakes. Relative sea level change controls the distribution of marine deposits, which show significant regional variations due to variable isostatic response across the region. Sea level change plays a limited role for fluvial aggradation/incision in the study area. 相似文献
20.