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61.
The study of trace metal speciation has benefited from a great deal of interest leading to the development and the diversification of sequential extraction schemes (SES), which triggered the need for harmonization by the standard, measurements and testing programme (SM & T). However, some uncertainties still persist in the application of the harmonized 3-step protocol, because of the difficulty in conceptualizing a technique that can be applied to environmental samples irrespective of their nature. The alternative method proposed in this study is based on the solubility of the sample components progressively dissolved during the course of an acidimetric titration by 1 mol L−1 HCl. The major HCl-reactive mineralogical components are identified using mass balance calculation of H+ consumed by their dissolution together with the amount of major elements released into solution. The speciation of minor and trace elements is investigated by comparing their titrations to those of the major elements. This approach is much simpler than SES because it uses simple non-selective H+ at room temperature instead of a complex experimental design of so-called specific reagents. The different mineral components of the solid are no longer operationally defined and the problem of selectivity is irrelevant to the titration approach. The method was applied to several sediment samples from the Scheldt estuary and the particulate phase was further examined by Scanning Electron Microprobe and X-ray Diffraction techniques. The nearly complete consumption of H+ in the suspension is balanced by the total dissolution of carbonates and Fe-oxyhydroxides. In contrast to the speciation inferred from the Tessier SES, the acidimetric titration has demonstrated that the carbonate phase does not significantly contain trace metals with the exceptions of 40% of the Mn and 30% of the Co. In contrast, the Fe-oxyhydroxides seem to play a major role and account for 70% of Pb and 20% of Cr, in addition to 60% of P and additional amounts of 20% Co and 40% Mn. 70% of the Cu also occur in the oxyhydroxide phase, more likely coprecipitated with gibbsite. 90% of the Cd and 85% of Zn can be attributed to the Acid Volatile Sulfide (AVS) phase as evidenced from S titration. The acidimetric titration method not only provides information on the speciation of trace metals but also allows the quantification of their reactivity and mobility, if one considers that the titration roughly mimics pH changes that may occur as a result of chemical disequilibrium in the environment. The results demonstrate the potential of the acidimetric titration as an alternative to SES protocols in geochemical and environmental regulation studies. This method is applicable to a wide variety of environmental materials with little or minor adjustments. 相似文献
62.
K.Y. Chang S.S. He C.C. Chou S.L. Kao A.S. Chiou 《International journal of geographical information science》2013,27(8):1375-1393
To plan undeveloped optimal routes between Asia and Europe via the Arctic Northeast Passages using a 3D geographic information system (GIS), voyage paths are simulated in a 3D visual form. This ensures that the distances are calculated accurately, and that other voyage data such as water depths, sea ice distribution, and seashore topology are also easily deciphered, giving a more direct and clear demonstration compared to simplified presentations on an Electronic Chart Display & Information System (ECDIS). This article also implements a higher-geometry maze router in ice zone areas to obtain the optimal path in relation to safety and costs. This article compares the optimal Arctic Northeast Passages with traditional routes through the Suez Canal for dynamic analyses of the cost efficiency (including time costs, fuel costs, and other factors) of travel between major ports in Asia and Europe. The average benefit assessment is around 30–45% in a bulk carrier comparison. Thus, a 3D GIS can easily obtain and demonstrate safe navigation routes, providing a very convenient tool for initial planning. 相似文献
63.
Silva Vinicius Oliveira de Mello Carlos Rogério Chou Sin Chan 《Theoretical and Applied Climatology》2022,148(3-4):1289-1302
Theoretical and Applied Climatology - South of Minas Gerais state, in Southeast Brazil, is known for the coffee crop production (more than 30% of country’s production) and hydroelectricity... 相似文献
64.
Jian Chen Guijian Liu Mengmeng JiangChen-Lin Chou Hui LiBin Wu Liugen ZhengDongdong Jiang 《International Journal of Coal Geology》2011,88(1):41-54
To study the geochemical characteristics of 11 environmentally sensitive trace elements in the coals of the Permian Period from the Huainan coalfield, Anhui province, China, borehole samples of 336 coals, two partings, and four roof and floor mudstones were collected from mineable coal seams. Major elements and selected trace elements were determined by inductively coupled plasma optical emission spectrometry (ICP-OES), inductively coupled plasma mass spectrometry (ICP-MS), and hydride generation atomic absorption spectrometry (HAAS). The depositional environment, abundances, distribution, and modes of occurrence of trace elements were investigated. Results show that clay and carbonate minerals are the principal inorganic constituents in the coals. A lower deltaic plain, where fluvial channel systems developed successively, was the likely depositional environment of the Permian coals in the Huainan coalfield. All major elements have wider variation ranges than those of Chinese coals except for Mg and Fe. The contents of Cr, Co, Ni, and Se are higher than their averages for Chinese coals and world coals. Vertical variations of trace elements in different formations are not significant except for B and Ba. Certain roof and partings are distinctly higher in trace elements than underlying coal bench samples. The modes of occurrence of trace elements vary in different coal seams as a result of different coal-forming environments. Vanadium, Cr, and Th are associated with aluminosilicate minerals, Ba with carbonate minerals, and Cu, Zn, As, Se, and Pb mainly with sulfide minerals. 相似文献
65.
L. H. Shih T. Y. Chou 《International Journal of Environmental Science and Technology》2011,8(3):523-532
Although solar power systems are considered as one of the most promising renewable energy sources, some uncertain factors as well as the high cost could be barriers which create customer resistance. Leasing instead of purchase, as one type of product service system, could be an option to reduce consumer concern on such issues. This study focuses on consumer concerns about uncertainty and willingness to pay for leasing solar power systems. Conjoint analysis method is used to find part worth utilities and estimate gaps of willingness to pay between attribute levels, including various leasing time lengths. The results show the part worth utilities and relative importance of four major attributes, including leasing time. Among concerns about uncertainties, government subsidy, electricity price, reliability, and rise of new generation solar power systems were found to be significantly related to the additional willingness-to-pay for a shorter leasing time. Cluster analysis is used to identify two groups standing for high and low concerns about uncertainty. People with more concerns tend to pay more for a shorter lease time. 相似文献
66.
Keh‐Chyuan Tsai Chung‐Che Chou Chi‐Lon Lin Pei‐Ching Chen Sheng‐Jhih Jhang 《地震工程与结构动力学》2008,37(4):627-645
This paper first presents the force–deformation relationship of a post‐tensioned (PT) steel beam‐to‐column connection constructed with bolted web friction devices (FDs). This paper then describes the test program conducted in the National Center for Research on Earthquake Engineering, Taiwan, on four bolted FDs and four full‐scale PT beam‐to‐column moment connection subassemblies using the FDs. Tests confirm that (1) the hysteretic behavior of four bolted FDs is very stable, (2) the friction coefficient between the steel plate and the brass shim is about 0.34, (3) the proposed force–deformation relationships reasonably predict the experimental responses of the PT connections under cyclically increasing deformations up to a beam peak rotation of 0.05 rad, and (4) the decompression moments do not degrade as beam cyclic deformations increase. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
67.
This paper introduces a risk-based decision process integrated into a drought early warning system (DEWS) for reservoir operation. It is to support policy making under uncertainty for drought management. Aspects of posterior risk, chances of option occurrences and the corresponding options to given chances, are provided to help decision makers to make better decisions. A new risk index is also defined to characterize decision makers’ attitudes toward risk. Decision makers can understand the inclination of attitude associated with any specific probability through accuracy assessment, and learn to adjust their attitudes in decision-making process. As a pioneering experiment, the Shihmen reservoir in northern Taiwan was tested. Over the simulation period (1964–2005), the expected overall accuracy approximated to 77%. The results show that the proposed approach is very practical and should find good use for reservoir operations. 相似文献
68.
69.
Acoustic imaging is a new method to construct the acoustic signal at a point on the solar surface or in the solar interior with the signals measured at the solar surface. The constructed signals contain both intensity information and phase information. The intensity is computed by summing the squared amplitude of the constructed signal over time. The phase of constructed signals can be studied by the cross-correlation function between the time series constructed with ingoing waves and outgoing waves. The location of the envelope peak of the cross-correlation function and the phase of the cross-correlation function contain different information on the physical conditions of the plasma along the wave path. From the constructed signals, one can form the two-dimensional outgoing intensity map, absorption map, phase-shift map, and envelope-shift map of a target region at different focal depths. The perturbed physical conditions caused by the magnetic fields of active regions manifest in these maps. The outgoing intensity is lower in magnetic regions than the quiet Sun. The group travel time and phase travel time are smaller in magnetic regions than in the quiet Sun. In this paper, we review the studies of active regions, including emerging flux regions, with acoustic imaging. 相似文献
70.
The typical loess on high slopes along the BaoLan High-speed Rail, China, was selected as the research object. The influence of the freeze-thaw cycle and dry-wet alternation on the shear-strength parameters of the unsaturated loess was investigated by laboratory experimental methods. Moreover, the temperature field, seepage field, and stability of slopes with different gradients were simulated under the effect of the freeze-thaw cycle and dry-wet alternation by using the geotechnical analysis software Geo-Studio. The research results showed(1) when the freeze-thaw cycle was repeated on the slope, with the frozen depth increasing, the melted depth did the same; besides, the closed loop of isotherms formed on the slope;(2) under the action of dry-wet circulation, the negative pore-water pressure and volumetric water content showed an upward tendency. However, owing to the different slope gradients, rainfall infiltration was not the same. As time went by, the differences of the negative pore-water pressure and volumetric water content between the slopes of different gradients continued to increase;(3) with the freeze-thaw cycle and dry-wet alternation increasing, the slope-safety factor decreased. Especially in the early period, the slope-safety factor changed remarkably. For slopes undergoing freeze-thaw action, the slope-safety factor was negatively correlated with the gradient. However, with regard to slopes undergoing dry-wet alternation, the result became more complex because the slope-safety factor was related to both seepage strength and slope grade. Accordingly, further research is needed to study the effect of seepage strength and slope grade on the stability of loess slopes. 相似文献