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151.
G. Diego Gatta Nicola Rotiroti Martin Fisch Milen Kadiyski Thomas Armbruster 《Physics and Chemistry of Minerals》2008,35(9):521-533
The elastic and structural behaviour of the synthetic zeolite CsAlSi5O12 (a = 16.753(4), b = 13.797(3) and c = 5.0235(17) Å, space group Ama2, Z = 2) were investigated up to 8.5 GPa by in situ single-crystal X-ray diffraction with a diamond anvil cell under hydrostatic conditions. No phase-transition occurs within the P-range investigated. Fitting the volume data with a third-order Birch–Murnaghan equation-of-state gives: V 0 = 1,155(4) Å3, K T0 = 20(1) GPa and K′ = 6.5(7). The “axial moduli” were calculated with a third-order “linearized” BM-EoS, substituting the cube of the individual lattice parameter (a 3, b 3, c 3) for the volume. The refined axial-EoS parameters are: a 0 = 16.701(44) Å, K T0a = 14(2) GPa (βa = 0.024(3) GPa?1), K′ a = 6.2(8) for the a-axis; b 0 = 13.778(20) Å, K T0b = 21(3) GPa (βb = 0.016(2) GPa?1), K′ b = 10(2) for the b-axis; c 0 = 5.018(7) Å, K T0c = 33(3) GPa (βc = 0.010(1) GPa?1), K′ c = 3.2(8) for the c-axis (K T0a:K T0b:K T0c = 1:1.50:2.36). The HP-crystal structure evolution was studied on the basis of several structural refinements at different pressures: 0.0001 GPa (with crystal in DAC without any pressure medium), 1.58(3), 1.75(4), 1.94(6), 3.25(4), 4.69(5), 7.36(6), 8.45(5) and 0.0001 GPa (after decompression). The main deformation mechanisms at high-pressure are basically driven by tetrahedral tilting, the tetrahedra behaving as rigid-units. A change in the compressional mechanisms was observed at P ≤ 2 GPa. The P-induced structural rearrangement up to 8.5 GPa is completely reversible. The high thermo-elastic stability of CsAlSi5O12, the immobility of Cs at HT/HP-conditions, the preservation of crystallinity at least up to 8.5 GPa and 1,000°C in elastic regime and the extremely low leaching rate of Cs from CsAlSi5O12 allow to consider this open-framework silicate as functional material potentially usable for fixation and deposition of Cs radioisotopes. 相似文献
152.
In situ strength measurements on natural upper-mantle minerals 总被引:1,自引:0,他引:1
Junji Yamamoto Jun-ichi Ando Hiroyuki Kagi Toru Inoue Akihiro Yamada Daisuke Yamazaki Tetsuo Irifune 《Physics and Chemistry of Minerals》2008,35(5):249-257
Using in situ strength measurements at pressures up to 10 GPa and at room temperature, 400, 600, and 700°C, we examined rheological
properties of olivine, orthopyroxene, and chromian-spinel contained in a mantle-derived xenolith. Mineral strengths were estimated
using widths of X-ray diffraction peaks as a function of pressure, temperature, and time. Differential stresses of all minerals
increase with increasing pressure, but they decrease with increasing temperature because of elastic strain on compression
and stress relaxation during heating. During compression at room temperature, all minerals deform plastically at differential
stress of 4–6 GPa. During subsequent heating, thermally induced yielding is observed in olivine at 600°C. Neither orthopyroxene
nor spinel shows complete stress relaxation, but both retain some stress even at 700°C. The strength of the minerals decreases
in the order of chromian-spinel ≈ orthopyroxene > olivine for these conditions. This order of strength is consistent with
the residual pressure of fluid inclusions in mantle xenoliths. 相似文献
153.
Emilia Palonen 《GeoJournal》2008,73(3):219-230
As in most parts of Central and Eastern Europe, there is a tradition in Hungary of changing street names and memorials in
the wake of major political transitions. This article focuses on the change of street names and memorials, i.e. the city-text,
in Hungary’s political capital, Budapest, between 1985 and 2001. The city-text in Budapest became a locus of dispute between
different political authorities, including the nation state, the metropolitan municipality, and the district, each bearing
different political ideals during and after the fall of communism. Discursive changes in the post-communist city-text emerged
expressing specific conceptions of national sovereignty, but the direction of the changes were debated. Different levels of
administration in Budapest and Hungary had divergent visions of what the new discourse on national sovereignty should be.
The changes, therefore, did not express a simple transition to an agreed-upon post-communist value system, but were the result
of a symbolic struggle between different levels of administration over what should be commemorated in the city-text. 相似文献
154.
Lars Olov Andersson 《Physics and Chemistry of Minerals》2008,35(9):505-520
The EPR spectra of Maxixe-type beryl contain a large number of overlapping signals. The angular dependence of the 1:3:3:1
signal typical for the CH3 radical shows that this radical is located at the center of the channel cavity with its symmetry axis parallel to the crystal
c-axis and is rotating around this axis. Its EPR spectrum is axially symmetric with g
// = 2.00263, g
⊥ = 2.00249 and A// = 2.288 mT, A⊥ = 2.256 mT. These anisotropies have the opposite signs of those found for surface-adsorbed methyl radicals. Hydrogen atoms
are located at position 2a at the center of the beryl cavity and the EPR parameters of the narrow doublet signal are A
0 = 1,407 MHz and g = 2.00230. Another doublet signal, which is broader and has axial symmetry with g
// = 2.00265, g
⊥ = 2.00625 and A// = 0.895 mT, A⊥ = 0.885 mT, could come from a HCO3 radical. One narrow and easily saturated signal with g
// = 2.00227 and g
⊥ = 2.00386 is interpreted to arise from a carbon monoxide radical in the beryl channel, oriented with its axis parallel to
the crystal c-axis. Additional weak doublet lines, which have similar g values as the carbon monoxide radical, are created by nearby hydrogens. A powder spectrum with g
// = 2.0017 and g
⊥ = 2.0004 appears upon UV irradiation of the single crystal and is easily saturated. This spectrum is interpreted to arise
from a carbon dioxide radical, which rotates around its symmetry axis. 相似文献
155.
An increasingly utilized strategy for expanding conservation in the developing world has been the promotion of protected areas
that supersede national borders. Alternatively known as transfrontier biosphere reserves, transfrontier or transboundary conservation
areas, or Peace Parks, these protected areas are aggressively advanced by conservation agencies for their purported ecological
and economic benefits. This article provides a comparative assessment of two case studies to understand the various impacts
of transboundary conservation. The Great Limpopo Transfrontier Park, which unites protected areas in South Africa, Mozambique
and Zimbabwe, is contrasted with efforts to protect jaguars along the United States–Mexico border. We argue that while these
cases are promising for the purposes of biodiversity protection, they demonstrate that transboundary conservation can minimize
political context, contributes to the hegemony of international conservation agendas, and remains closely linked to economic
neoliberalism and decentralization in the developing world.
相似文献
Brian KingEmail: |
156.
Until recently the traditional spatial configuration of the European geography was based upon the core-periphery model. The
‘pentagon’, broadly defined as lying between London, Paris, Milan, Munich and Hamburg, was seen as the core area characterised
by having the highest concentration of economic development in the European Union (EU), with the remainder of the European
territory viewed as peripheral, albeit to varying degrees. In a number of cases such peripheral areas equated with clear regional
disparities. The elaboration of the European Spatial Development Perspective (ESDP) (CEC, European spatial development perspective, towards balanced and sustainable development in the territory of the
European Union, 1999) challenged this core-periphery model. European spatial planning policies, aimed at encouraging social
and economic, and with ever increasing importance, territorial cohesion, seek amongst other aspects to encourage the development
of a balanced and polycentric urban system. This paper adopts a network analysis approach to the analysis of air passenger
flows between some 28 principal European metropolitan urban regions. The evaluation of these flows contributes to an enhanced
comprehension of the spatial dynamics of the European metropolitan territory which goes beyond that deriving from the more
standard analyses of the individual components of the urban system. Several indicators are used, deriving from gravitational
modelling techniques, to analyse the complexity of the air passenger flows. A multidimensional scaling (MDS) technique is
introduced in order to interpret and visualise the resulting spatial configuration and positioning of the different metropolitan
centres within the conceptual European ‘space of air passenger flows’, thereby contrasting with the more traditional map-based
geographical image of Europe, based upon Cartesian coordinates.
相似文献
Malcolm C. BurnsEmail: |
157.
This paper explores the links between a strategic policy, urban consolidation, and house prices by examining the changes in
the mix of housing and in house price for the period 1991–2004. We contend that urban consolidation could be seen as a source
of additional supply, (which might be expected to be felt in lower prices and so contribute to a local policy objective) but
also as a stimulus to demand (by developers who could bid up the price of lots where it was understood more housing could
be built). Analyses were carried out at the metropolitan and sub-regional scales using correlation tests. The research finds
very weak statistical connections, and concludes that this policy has not been associated with price changes. 相似文献
158.
Corey Johnson 《GeoJournal》2008,72(1-2):75-89
As John Agnew (Political geography: a reader, 1997) has argued, political and economic change often occasions competing visions of the scales that are appropriate for organizing particular political and economic activities. Nowhere is this more evident than in the European Union, and eastern Germany offers compelling evidence of the contested nature of contemporary scalar politics. Yet a recent debate in human geography (see, e.g. Marston et al., Transactions of the Institute of British Geographers 30:416–432, 2005) calls into question the very concept of scale and rejects its hierarchical conceptualization. In light of this debate, it is appropriate to draw on real-world case studies to examine the ways in which geography figures into policy. Drawing on field work in Saxony, evidence is offered in the form of competing visions of regionalism in the EU context. The evidence presented complicates both hierarchical and flat notions of scale. The current process of querying space to identify those scales that are best-suited for the globalized economy offers insights into both the socially constructed nature of scale as well as the ways in which scalar lenses help to illuminate the geographical aspects (and consequences) of strategies for coping with structural changes. 相似文献
159.
通过对塔里木盆地库车坳陷南天山山前带克孜勒努尔沟与依奇克里克野外露头沉积相的精细研究,结合山前带大量地震剖面分析与迪那201井、东秋5井等多口钻井测井相和岩心精细描述,将古近系库姆格列木群划分为2个层序。层序2低位域以冲积扇沉积为主,自湖侵体系域始,研究区广泛发育退积与进积型扇三角洲沉积。库姆格列木群层序2湖侵体系域内扇三角洲平原砂体以正韵律沉积为主,砂砾岩占地层厚度的(68.4~87)%;扇三角洲前缘砂体正、反韵律均有分布,砂砾岩占地层的百分比有所降低,为(55.2~77)%。高位体系域内主要发育以反韵律砂体为主的扇三角洲前缘沉积。古近系苏维依组只发育一个层序,其低位体系域的砂体为扇三角洲平原与前缘的分流河道砂体,湖侵体系域内扇三角洲前缘砂体正、反韵律均发育,高位体系域内主要发育扇三角洲前缘沉积,以反韵律砂体为主,正韵律砂体相对较少。对比苏维依组不同体系域内砂体储集性,湖侵域内砂体优于高位域内砂体。扇三角洲沉积体中有利储集砂体首选为湖侵体系域内的扇三角洲前缘水下分流河道和河口坝砂体,次之为低位域扇三角洲前缘(平原)分流河道砂体,最后是高位域内的河口坝及席状砂沉积砂体。特别要指出:低位体系域或者湖侵体系域底部发育的扇三角洲前缘(平原)分流河道砂体(底砂砾岩)被快速湖侵的较厚的暗色泥岩所覆盖,可形成较好储集场所。 相似文献
160.
运用源控含油气系统理论与综合分析技术,按成藏“层次分析”方法,通过对生、储、盖、圈(闭)静态要素及其内生、排、运、聚、散(失)动态过程的综合研究,对松辽盆地中央坳陷的三肇凹陷葡萄花油层成藏条件进行探讨,提出了以次级凹陷为中心、不同类型的油气聚集带紧邻并围绕次级凹陷最低部位呈环带状分布的大型凹陷内成藏模式,并进一步提出永乐次级凹陷中心及其三级聚油环带及徐家围子次级凹陷以西为"网式"运聚特征;在凹陷级成藏模式的指导下,通过对大面积密井网开发区综合解剖,提出三级构造带中单个的局部构造圈闭(群)、单个的(局部构造——)岩性圈闭(群)控油和成藏规律,为认识本区基本控油单元、油水分布规律、油气勘探及扩大新探区提供重要的理论依据。 相似文献