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201.
Silke Severmann Rachel A. Mills Jon P. Telling R. John Parkes 《Geochimica et cosmochimica acta》2006,70(7):1677-1694
A detailed geochemical and microbiological study of a ∼2 m sediment core from the inactive Alvin mounds within the TAG hydrothermal field was conducted to examine, for the first time, the role of prokaryotes in subsurface weathering of hydrothermal sediments. Results show that there has been substantial post-depositional remobilisation of metal species and diagenetic overprinting of the original high-temperature hydrothermal minerals, and aspects have involved prokaryotic processes. Prokaryotic enumeration demonstrates the presence of a population smaller than the average for deep sea sediments, probably due to the low organic carbon content, but not inhibited by (and hence adapted to) the metal rich environment. There was a small but significant increase in population size associated with the active redox boundary in an upper metal sulphide layer (50-70 cm) around which active metal remobilisation was concentrated (Cu, Au, Cd, Ag, U, Zn and Zn). Hence, subsurface prokaryotes were potentially obtaining energy from metal metabolism in this near surface zone. Close association of numbers of culturable Mn and Fe reducing prokaryotes with subsurface Fe2+ and Mn2+ pore water profiles suggested active prokaryotic metal reduction at depth in core CD102/43 (to ∼175 cm). In addition, a prokaryotic mechanism, which is associated with bacterial sulphate reduction, is invoked to explain the U enrichment on pyrite surfaces and Zn and Pb remobilisation in the upper sediment. Although prokaryotic populations are present throughout this metalliferous sediment, thermodynamic calculations indicated that the inferred low pH of pore waters and the suboxic/anoxic conditions limits the potential energy available from Fe(II) oxidation, which may restrict prokaryotic chemolithotrophic biomass. This suggests that intense prokaryotic Fe oxidation and weathering of seafloor massive sulphide deposits may be restricted to the upper portion of the deposit that is influenced by near neutral pH and oxic seawater unless there is significant subsurface fluid flow. 相似文献
202.
Norbert Hertkorn Ronald Benner Philippe Schmitt-Kopplin Karl Kaiser John I. Hedges 《Geochimica et cosmochimica acta》2006,70(12):2990-3010
Refractory carboxyl-rich alicyclic molecules (CRAM) are characterized in marine dissolved organic matter (DOM) using nuclear magnetic resonance spectroscopy and ultrahigh resolution mass spectrometry. CRAM are distributed throughout the water column and are the most abundant components of deep ocean DOM ever characterized. CRAM are comprised of a complex mixture of carboxylated and fused alicyclic structures with a carboxyl-C:aliphatic-C ratio of 1:2 to 1:7. CRAM are expected to constitute a strong ligand for metal binding, and multiple coordination across cations could promote aggregation and marine gel formation thereby affecting CRAM reactivity and the bioavailability of nutrients and trace metals. It appears CRAM are ultimately derived from biomolecules with structural similarities to sterols and hopanoids. The occurrence of CRAM in freshwater and terrestrial environments seems likely, considering the global distribution of biomolecules and the similarities of biogeochemical processes among environments. 相似文献
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205.
Pensacola Bay, Florida, was in the strong northeast quadrant of Hurricane Ivan when it made landfall on September 16, 2004
as a category 3 hurricane on the Saffir-Simpson scale. We present data describing the timeline and maximum height of the storm
surge, the extent of flooding of coastal land, and the magnitude of the freshwater inflow pulse that followed the storm. We
computed the magnitude of tidal flushing associated with the surge using a tidal prism model. We also evaluated hurricane
effects on water quality using water quality surveys conducted 20 and 50 d after the storm, which we compared with a survey
14 d before landfall. We evaluated the scale of hurricane effects relative to normal variability using a 5-yr monthly record.
Ivan's 3.5 m storm surge inundated 165 km2 of land, increasing the surface area of Pensacola Bay by 50% and its volume by 230%. The model suggests that 60% of the Bay's
volume was flushed, initially increasing the average salinity of Bay waters from 23 to 30 and lowering nutrient and chlorophylla concentrations. Additional computations suggest that wind forcing was sufficient to completely mix the water column during
the storm. Freshwater discharge from the largest river increased twentyfold during the subsequent 4 d, stimulating a modest
phytoplankton bloom (chlorophyll up to 18 μg l−1) and maintaining hypoxia for several months. Although the immediate physical perturbation was extreme, the water quality
effects that persisted beyond the first several days were within the normal range of variability for this system. In terms
of water quality and phytoplankton productivity effects, this ecosystem appears to be quite resilient in the face of a severe
hurricane effect. 相似文献
206.
The release of methane from crater sites following meteorite impact is a possible consequence of the thermal alteration of organic matter, or tapping of reservoired gas of biogenic or abiogenic origin. At least the latter is feasible on Mars. Methane and higher hydrocarbons are susceptible to polymerization and precipitation by radioactive minerals. Where such minerals are present in impact target rocks, the craters can be a preferred site for carbon concentration, and the formation of complex organic molecules. On icy bodies, such as Titan and Europa, methane released by impact could be a fuel for prebiotic chemistry involving other forms of irradiation. 相似文献
207.
Darren F. Mark John Parnell Simon P. Kelley Sarah C. Sherlock 《Journal of Geochemical Exploration》2006,89(1-3):259
Integration of fluid inclusion analysis with high spatial resolution Ar–Ar dating of K-feldspar cements has been used to resolve and reconstruct palaeo-fluid flow. Fluid inclusion analysis allows discrimination of distinct cement phases, thereby identifying discrete episodes of fluid flow. Ar–Ar dating of the same cements via high spatial resolution laserprobe establishes absolute age constraints on the framework previously constructed. Integration of these two datasets yields temperature–composition–time data. 相似文献
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209.
The “region” and “regional change” have been elusive ideas within political and economic geography, and in essence require a greater understanding of their dynamic characteristics. Trailing in the backwaters of the devolution to the Celtic nations of Britain, the contemporary era of New Labour’s political-economic ideology, manifest through “third-way” governance in England places the region and its functional capacity into the heart of geographical inquiry. Drawing upon a new regionalist epistemology, this paper seeks to recover a sense of (regional) political economy through a critical investigation of the development and formulation of Blair’s “New Regional Policy” (NRP). I address how New Labour has attempted to marry economic regionalisation on the one hand, and democratic regionalism on the other. This paper specifically questions the wisdom of such a marriage of politically distinct ideologies through a critical investigation of the underlying contradictions of their strategy from both a theoretical and empirical standpoint. Demonstrated both in the North East “no” vote in 2004, and in the post-mortem undertaken by the ODPM Select Committee in 2005, the paper illustrates how a loss of political drive gradually undermined the capacity of devolution to deliver in England. Finally, I argue that through the lens of the NRP we can speculate on some of the wider issues and implications for the study of regional governance. 相似文献
210.
Robert Shcherbakov Jordan Van Aalsburg John B. Rundle Donald L. Turcotte 《Tectonophysics》2006,413(1-2):53
Correlations in space and time play a fundamental role in earthquake processes. One direct manifestation of the effects of correlations is the occurrence of aftershocks due to the stress transfer in the vicinity of a main shock. Less obvious and more speculative changes in correlations may occur in the background seismicity before large earthquakes. Using statistical physics it is possible to introduce a measure of spatial correlations through a correlation length. This quantity characterizes how local fluctuations can influence the occurrence of earthquakes over distances comparable with the correlation length. In this work, the physical basis of spatial correlations of earthquakes is discussed in the context of critical phenomena and the percolation problem. The method of two-point correlation function is applied to the seismicity of California. Well defined variations in time of the correlation length are found for aftershock sequences and background seismicity. The scaling properties of our obtained distributions are analyzed with respect to changes in several scaling parameters such as lower magnitude cutoff of earthquakes, the maximum time interval between earthquakes, and the spatial size of the area considered. This scaling behavior can be described in a unified manner by utilizing the multifractal fit. Utilizing the percolation approach the time evolution of clusters of earthquakes is studied with the correlation length defined in terms of the radius of gyration of clusters. This method is applied to the seismicity of California. 相似文献