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71.
72.
Lower to Middle Devonian carbonates of the Prague Syncline, the Carnic Alps, the Montagne Noire, and the Cantabrian Mountains were investigated for δ13Ccarb and δ13Corg. These values were measured on bulk rocks, selected components and cements. Many carbonates exhibit primary marine values, but some are altered by diagenesis. A δ13C curve can be presented for the latest Pridolian to Emsian time interval. Several sharp or broad positive excursions are obvious in the woschmidti-postwoschmidti, sulcatus, kitabicus, Late serotinus, and kockelianus conodont zones. The excursion at the Silurian–Devonian boundary is known worldwide and therefore considered global in nature. Some of the others are described for the first time from central and southern Europe, and their global nature has to be verified by further investigations in other regions. Most excursions relate to and/or started during major regressions whereas sea-level highstands correspond to minimal δ13C values. Similar relationships between sea-level changes and δ13C have been observed from other early Palaeozoic intervals. The transgressive Chote? (?) and Ka?ák events are marked by positive isotope excursions, this type of combination is usually observed in late Palaeozoic to Cenozoic black shale events. 相似文献
73.
Matthew J. Wooller John W. Pohlman Benjamin V. Gaglioti Peter Langdon Miriam Jones Katey M. Walter Anthony Kevin W. Becker Kai-Uwe Hinrichs Marcus Elvert 《Journal of Paleolimnology》2012,48(1):27-42
Atmospheric contributions of methane from Arctic wetlands during the Holocene are dynamic and linked to climate oscillations. However, long-term records linking climate variability to methane availability in Arctic wetlands are lacking. We present a multi-proxy ~12,000?year paleoecological reconstruction of intermittent methane availability from a radiocarbon-dated sediment core (LQ-West) taken from a shallow tundra lake (Qalluuraq Lake) in Arctic Alaska. Specifically, stable carbon isotopic values of photosynthetic biomarkers and methane are utilized to estimate the proportional contribution of methane-derived carbon to lake-sediment-preserved benthic (chironomids) and pelagic (cladocerans) components over the last ~12,000?years. These results were compared to temperature, hydrologic, and habitat reconstructions from the same site using chironomid assemblage data, oxygen isotopes of chironomid head capsules, and radiocarbon ages of plant macrofossils. Cladoceran ephippia from ~4,000?cal?year BP sediments have ??13C values that range from ~?39 to ?31??, suggesting peak methane carbon assimilation at that time. These low ??13C values coincide with an apparent decrease in effective moisture and development of a wetland that included Sphagnum subsecundum. Incorporation of methane-derived carbon by chironomids and cladocerans decreased from ~2,500 to 1,500?cal?year BP, coinciding with a temperature decrease. Live-collected chironomids with a radiocarbon age of 1,640?cal?year BP, and fossil chironomids from 1,500?cal?year BP in the core illustrate that ??old?? carbon has also contributed to the development of the aquatic ecosystem since ~1,500?cal?year BP. The relatively low ??13C values of aquatic invertebrates (as low as ?40.5??) provide evidence of methane incorporation by lake invertebrates, and suggest intermittent climate-linked methane release from the lake throughout the Holocene. 相似文献
74.
Nikki Vercauteren Elie Bou-Zeid Marc B. Parlange Ulrich Lemmin Hendrik Huwald John Selker Charles Meneveau 《Boundary-Layer Meteorology》2008,128(2):205-228
We examine the dynamics of turbulence subgrid (or sub-filter) scales over a lake surface and the implications for large-eddy
simulations (LES) of the atmospheric boundary layer. The analysis is based on measurements obtained during the Lake-Atmosphere
Turbulent EXchange (LATEX) field campaign (August–October, 2006) over Lake Geneva, Switzerland. Wind velocity, temperature
and humidity profiles were measured at 20 Hz using a vertical array of four sonic anemometers and open-path gas analyzers.
The results indicate that the observed subgrid-scale statistics are very similar to those observed over land surfaces, suggesting
that the effect of the lake waves on surface-layer turbulence during LATEX is small. The measurements allowed, for the first
time, the study of subgrid-scale turbulent transport of water vapour, which is found to be well correlated with the transport
of heat, suggesting that the subgrid-scale modelling of the two scalars may be coupled to save computational resources during
LES. 相似文献
75.
Richard Ulrich 《Icarus》2009,201(1):127-134
Diffusion advection is an effect in diffusive multicomponent mass transfer that occurs when the flux vectors of the individual components do not add up to zero. This can be a significant effect for the mass transfer of water vapor from subsurface ice or liquid reservoirs through porous regolith at martian temperatures and pressures. Ignoring diffusion advection and using Fick's law alone to calculate the flux under these conditions will result in an erroneously small value while using a measured flux to calculate a diffusivity will result in an erroneously high value. The inaccuracy in both cases increases with temperature. The literature contains several examples of erroneous treatment of this effect. The correct approach is well-known from other applications of mass transfer and takes diffusion advection into account in the appropriate amount regardless of the temperature and pressure and reduces to the simple Fick's law when conditions warrant. In this way, there is no need to decide under what conditions diffusion advection is or is not important. It can be used in the transition region to pure Knudsen diffusion in a fashion similar to that used with the more limited Fickian approach. 相似文献
76.
This study based on longitudinal Zeeman effect magnetograms and spectral line scans investigates the dependence of solar surface magnetic fields on the spectral line used and the way the line is sampled to estimate the magnetic flux emerging above the solar atmosphere and penetrating to the corona from magnetograms of the Mt. Wilson 150-foot tower synoptic program (MWO). We have compared the synoptic program λ5250 Å line of Fe?i to the line of Fe?i at λ5233 Å since this latter line has a broad shape with a profile that is nearly linear over a large portion of its wings. The present study uses five pairs of sampling points on the λ5233 Å line. Line profile observations show that the determination of the field strength from the Stokes V parameter or from line bisectors in the circularly polarized line profiles lead to similar dependencies on the spectral sampling of the lines, with the bisector method being the less sensitive. We recommend adoption of the field determined with the line bisector method as the best estimate of the emergent photospheric flux and further recommend the use of a sampling point as close to the line core as is practical. The combination of the line profile measurements and the cross-correlation of fields measured simultaneously with λ5250 Å and λ5233 Å yields a formula for the scale factor δ ?1 that multiplies the MWO synoptic magnetic fields. By using ρ as the center-to-limb angle (CLA), a fit to this scale factor is δ ?1=4.15?2.82sin?2(ρ). Previously δ ?1=4.5?2.5sin?2(ρ) had been used. The new calibration shows that magnetic fields measured by the MDI system on the SOHO spacecraft are equal to 0.619±0.018 times the true value at a center-to-limb position 30°. Berger and Lites (2003, Solar Phys. 213, 213) found this factor to be 0.64±0.013 based on a comparison using the Advanced Stokes Polarimeter. 相似文献
77.
Peter Foukal Luca Bertello William C. Livingston Alexei A. Pevtsov Jagdev Singh Andrey G. Tlatov Roger K. Ulrich 《Solar physics》2009,255(2):229-238
Spectroheliograms and disk-integrated flux monitoring in the strong resonance line of Ca ii (K line) provide the longest record of chromospheric magnetic plages. We compare recent reductions of the Ca ii K spectroheliograms obtained since 1907 at the Kodaikanal, Mt. Wilson, and US National Solar Observatories. Certain differences
between the individual plage indices appear to be caused mainly by differences in the spectral passbands used. Our main finding
is that the indices show remarkably consistent behavior on the multidecadal time scales of greatest interest to global warming
studies. The reconstruction of solar ultraviolet flux variation from these indices differs significantly from the 20th-century
global temperature record. This difference is consistent with other findings that, although solar UV irradiance variation
may affect climate through influence on precipitation and storm tracks, its significance in global temperature remains elusive. 相似文献
78.
79.
Jordi LLORCA Ignasi CASANOVA Josep M. TRIGO‐RODRÍGUEZ José M. MADIEDO Julia ROSZJAR Addi BISCHOFF Ulrich OTT Ian A. FRANCHI Richard C. GREENWOOD Matthias LAUBENSTEIN 《Meteoritics & planetary science》2009,44(2):159-174
Abstract— Puerto Lápice is a new eucrite fall (Castilla‐La Mancha, Spain, 10 May 2007). In this paper, we report its detailed petrography, magnetic characterization, mineral and bulk chemistry, oxygen and noble gas isotope systematics, and radionuclide data. Study of four thin sections from two different specimens reveal that the meteorite is brecciated in nature, and it contains basaltic and granulitic clasts, as well as recrystallized impact melt and breccia fragments. Shock veins are ubiquitous and show evidence of at least three different shock events. Bulk chemical analyses suggest that Puerto Lápice belongs to the main group of basaltic eucrites, although it has a significantly higher Cr content. Oxygen isotopes also confirm that the meteorite is a normal member of the HED suite. Noble gas abundances show typical patterns, with dominant cosmogenic and radiogenic contributions, and indicate an average exposure age of 19 ± 2 Ma, and a Pu‐fission Xe age well within typical eucrite values. Cosmogenic radionuclides suggest a preatmospheric size of about 20–30 cm in diameter. 相似文献
80.
Kai-Uwe Ulrich Eugene S. Ilton Jonathan O. Sharp Rizlan Bernier-Latmani John R. Bargar 《Geochimica et cosmochimica acta》2009,73(20):6065-7290
The long-term stability of biogenic uraninite with respect to oxidative dissolution is pivotal to the success of in situ bioreduction strategies for the subsurface remediation of uranium legacies. Batch and flow-through dissolution experiments were conducted along with spectroscopic analyses to compare biogenic uraninite nanoparticles obtained from Shewanella oneidensis MR-1 and chemogenic UO2.00 with respect to their equilibrium solubility, dissolution mechanisms, and dissolution kinetics in water of varied oxygen and carbonate concentrations. Both materials exhibited a similar intrinsic solubility of ∼10−8 M under reducing conditions. The two materials had comparable dissolution rates under anoxic as well as oxidizing conditions, consistent with structural bulk homology of biogenic and stoichiometric uraninite. Carbonate reversibly promoted uraninite dissolution under both moderately oxidizing and reducing conditions, and the biogenic material yielded higher surface area-normalized dissolution rates than the chemogenic. This difference is in accordance with the higher proportion of U(V) detected on the biogenic uraninite surface by means of X-ray photoelectron spectroscopy. Reasonable sources of a stable U(V)-bearing intermediate phase are discussed. The observed increase of the dissolution rates can be explained by carbonate complexation of U(V) facilitating the detachment of U(V) from the uraninite surface. The fraction of surface-associated U(VI) increased with dissolved oxygen concentration. Simultaneously, X-ray absorption spectra showed conversion of the bulk from UO2.0 to UO2+x. In equilibrium with air, combined spectroscopic results support the formation of a near-surface layer of approximate composition UO2.25 (U4O9) coated by an outer layer of U(VI). This result is in accordance with flow-through dissolution experiments that indicate control of the dissolution rate of surface-oxidized uraninite by the solubility of metaschoepite under the tested conditions. Although U(V) has been observed in electrochemical studies on the dissolution of spent nuclear fuel, this is the first investigation that demonstrates the formation of a stable U(V) intermediate phase on the surface of submicron-sized uraninite particles suspended in aqueous solutions. 相似文献