Size-resolved characteristics of inorganic ionic species in atmospheric aerosols at a regional background site on the South African Highveld     

Andrew D. Venter  Pieter G. van Zyl  Johan P. Beukes  Jan-Stefan Swartz  Miroslav Josipovic  Ville Vakkari  Lauri Laakso  Markku Kulmala 《Journal of Atmospheric Chemistry》2018,75(3):285-304

Aerosols consist of organic and inorganic species, and the composition and concentration of these species depends on their sources, chemical transformation and sinks. In this study an assessment of major inorganic ions determined in three aerosol particle size ranges collected for 1 year at Welgegund in South Africa was conducted. SO₄^2? and ammonium (NH₄⁺) dominated the PM₁ size fraction, while SO₄^2? and nitrate (NO₃) dominated the PM_1–2.5 and PM_2.5–10 size fractions. SO₄^2? had the highest contribution in the two smaller size fractions, while NO₃^? had the highest contribution in the PM_2.5–10 size fraction. SO₄^2? and NO₃^? levels were attributed to the impacts of aged air masses passing over major anthropogenic source regions. Comparison of inorganic ion concentrations to levels thereof within a source region influencing Welgegund, indicated higher levels of most species within the source region. However, the comparative ratio of SO₄^2? was significantly lower due to SO₄^2? being formed distant from SO₂ emissions and submicron SO₄^2? having longer atmospheric residencies. The PM at Welgegund was determined to be acidic, mainly due to high concentrations of SO₄^2?. PM₁ and PM_1–2.5 fractions revealed a seasonal pattern, with higher inorganic ion concentrations measured from May to September. Higher concentrations were attributed to decreased wet removal, more pronounced inversion layers trapping pollutants, and increases in household combustion and wild fires during winter. Back trajectory analysis also revealed higher concentrations of inorganic ionic species corresponding to air mass movements over anthropogenic source regions.  相似文献   

Developing a reduced-form ensemble of climate change scenarios for Europe and its application to selected impact indicators     

Martin Dubrovsky  Miroslav Trnka  Ian P. Holman  Eva Svobodova  Paula A. Harrison 《Climatic change》2015,128(3-4):169-186

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Radio-continuum study of the nearby sculptor group galaxies. Part 3: NGC 7793 at λ=12.2, 6 and 3 cm     

Timothy J. Galvin  Miroslav D. Filipović  Nicholas F. H. Tothill  Evan J. Crawford  Andrew N. O’Brien  Nicholas Seymour  Thomas G. Pannuti  Alekzander R. Kosakowski  Biswas Sharma 《Astrophysics and Space Science》2014,353(2):603-611

We re-examine a series of archived centimetre radio-continuum observations (λ=16, 6 and 3 cm) focusing on NGC?7793 using the Australia Telescope Compact Array. These new images are both very sensitive (σ=0.011 mJy/beam) and feature reasonably high angular resolution (down to <3″). Using these images, a total of 76 discrete radio sources are identified, of which 57 have been classified. We also studied the radio component of the micro-quasar NGC7793-S26 which shows two distinct regions of somewhat steep spectral index (α) between ?0.3 and ?0.7.  相似文献   

Temporal trends of bulk precipitation and stream water chemistry (1977–1997) in a small forested area,Krusné hory,northern Bohemia,Czech Republic     

N. E. Peters  Jiri Cerny  Miroslav Havel  Radovan Krejci 《水文研究》1999,13(17):2721-2741

The Krusné hory (Erzgebirge or Ore Mountains) has been heavily affected by high atmospheric pollutant deposition caused by fossil fuel combustion in an adjacent Tertiary coal basin. Long‐term routine sampling of bulk precipitation (1977–1996) and stream water (1977–1998) in a forested area on the south‐eastern slope of the mountains were used to evaluate trends and patterns in solute concentration and flux with respect to controlling processes. From 1977 to 1996, the annual volume‐weighted Ca²⁺ and SOconcentrations decreased in bulk precipitation. However, after 1989, when a pronounced and continuous decrease occurred in coal production, annual volume‐weighted concentrations decreased for most solutes, except H⁺. The concentration decreases were marked, with 1996 levels at or below 50% of those in 1989. The lack of a trend in H⁺ is attributed to similar decreases in both acid anions and neutralizing base cations. Stream water concentrations of most solutes, i.e. H⁺, Ca²⁺, Mg²⁺, SONOwere highest at the onset of sampling in 1977, decreased markedly from 1977 to 1983 and decreased more gradually from 1983 to 1998. The spruce forest die‐back and removal reduced dry deposition of these solutes by reducing the filtering action, which was provided by the forest canopy. A notable decrease in stream water Ca²⁺ concentrations occurred after 1995 and may be due to the depletion of Ca²⁺, which was provided by catchment liming in 1986, 1988 and 1989. Solute flux trends in bulk atmospheric deposition and stream water generally were not significant and the lack of trend is attributed to the large interannual variability in precipitation quantity and runoff, respectively. All solutes except Na⁺ varied seasonally. The average seasonal concentrations varied between the solutes, but for most solutes were highest in winter and spring and lowest in summer, correlating with the seasonal trend in runoff. For Ca²⁺, Mg²⁺ and SOthe concentration minimum occurs in September and the maximum occurs in February or March, correlating with the seasonal baseflow. These solutes are primarily controlled by the contribution of soil water and groundwater to stream flow. During snowmelt, the meltwater generally causes concentrations to decrease as soil water and groundwater are diluted. For NO₃ , average minimum concentrations occur in August at the end of the growing season concurrent with the lowest stream flow, and the maximum occurs in February and March with high stream flow during snowmelt. Seasonal stream water NOconcentration variations are large compared with the long‐term decrease. Copyright © 1999 John Wiley & Sons, Ltd.  相似文献   

Landslide-dammed lake sediment volume calculation using waterborne ERT and SONAR profiling     

Filip Hartvich  Petr Tábořík  Miroslav Šobr  Bohumír Janský  Zdeněk Kliment  Jakub Langhammer 《地球表面变化过程与地形》2020,45(14):3463-3474

Lake sediment volume calculation is a challenging task, namely in cases when detailed drilling is complicated, expensive, or impossible, information on the pre-sedimentation surface unavailable, and record of siltation rate non-existent or too short. This study shows how waterborne, non-invasive geophysical survey, such as electrical resistivity tomography (ERT) can be very effective in acquiring the missing data, namely when combined with sound navigation ranging (SONAR) water depth measurements and supported by information from auxiliary sources. However, ERT surveying in water environment requires specific approaches, as we illustrate on the case of the Mladotice lake study. The lake was created after a landslide in May 1872, and since its formation, the depth has gradually decreased due to sedimentation. We have reconstructed the original surface, calculated the sediment volume, and compiled information on sedimentation to estimate its remaining life span. To achieve this, we measured nine waterborne ERT profiles across the lake. To reach the necessary depth, all ERT profiles were extended on land and crossed the lake using custom-built flotation pads. ERT profiling was combined with SONAR depth measurements, historical bathymetric surveys, borehole core analysis, sediment flux measurements, volumetric calculations, and water conductivity probing. The study has achieved three main results. First, practical applicability and advantages of stationary waterborne ERT profiling in combination with bathymetric sounding were demonstrated. Second, the original lake volume and accumulated sediment was calculated. We estimate that the volume of lake sediment is 187 000 m³, two-thirds of the original lake volume (over 275 000 m³). Finally, based on three volumetric data sets from 1972, 2003, and 2017, and recent monitoring of the sediment inflow, we propose scenarios of lake filling and its future development. Most interestingly, the sedimentation rate has decreased significantly in the last 20 years, suggesting that the lake may survive much longer than hitherto expected. © 2020 John Wiley & Sons, Ltd.  相似文献