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Structural changes of synthetic opal by heat treatment 总被引：1，自引：0，他引：1
Akane Arasuna Masayuki Okuno Hiroki Okudera Tomoyuki Mizukami Shoji Arai Shin’ichi Katayama Mikio Koyano Nobuaki Ito 《Physics and Chemistry of Minerals》2013,40(9):747-755
The structural changes of synthetic opal by heat treatment up to 1,400 °C were investigated using scanning electron microscopy, X-ray diffraction, and Fourier transform infrared and Raman spectroscopies. The results indicate that the dehydration and condensation of silanol in opal are very important factors in the structural evolution of heat-treated synthetic opal. Synthetic opal releases water molecules and silanols by heat treatment up to 400 °C, where the dehydration of silanol may lead to the condensation of a new Si–O–Si network comprising a four-membered ring structure of SiO4 tetrahedra, even at 400 °C. Above 600 °C, water molecules are lost and the opal surface and internal silanol molecules are completely dehydrated by heat effect, and the medium-temperature range structure of opal may begin to thermally reconstruct to six-membered rings of SiO4 tetrahedra. Above 1,000 °C, the opal structure almost approaches that of silica glass with an average structure of six-membered rings. Above 1,200 °C, the opal changes to low-cristobalite; however, minor evidence of low-tridymite stacking was evident after heat treatment at 1,400 °C. 相似文献
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Marine Pliocene and Pleistocene beds of the Boso Peninsula are more than 3 km thick and contain abundant fauna and flora. Almost continuous deposition occurred at a high sedimentation rate from the early part of the last reversed geomagnetic polarity epoch to the middle part of the last normal polarity epoch. Several microbiostratigraphic marker horizons enable correlation with deep-sea sediments fully independent of magnetostratigraphic zonation. Globorotalia truncatulinoides first occurs below the normal polarity event BO-B-2, which is correlated with the Olduvai Event in deep-sea sediments, whereas the disappearance of discoasters and the first occurrence of Gephyrocapsa caribbeanica are recognized at the top of BO-B-2, and the first occurrence of Gephyrocapsa oceanica is recognized at the top of BO-B-1. Based on the correlation of the Boso section with Mediterranean stage stratotype sections, the transition from the Pliocene to Pleistocene is estimated to be in the lower part of the Kazusa Group. 相似文献
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Odair J. Manfroi Kuraji Koichiro Tanaka Nobuaki Suzuki Masakazu Michiko Nakagawa Tohru Nakashizuka Lucy Chong 《水文研究》2004,18(13):2455-2474
Stemflow volume generation in lowland tropical forests was measured over a 1‐year period in the Malaysian state of Sarawak. The stemflow volume generated by 66 free‐standing trees with a diameter at breast height (DBH) over 1 cm and a tree height over 1 m were measured daily in a representative 10 m × 10 m plot of the forest. Throughfall in the plot was also measured using 20 gauges in a fixed position. Of the 2292 mm of total rainfall observed during the year‐long period, stemflow accounted for 3·5%, throughfall for 82% and there was an interception loss of 14·5%. Understory trees (DBH < 10 cm) played an important role in stemflow generation, producing 77% of the overall stemflow volume and 90% during storms with less than 20 mm of rainfall. Also, owing to their efficiency at funneling rainfall or throughfall water received by their crowns, some understory trees noticeably reduced the catches of the throughfall gauges situated under the reach of their crown areas. During storms producing greater than 20 mm of rainfall, 80% of the total stemflow occurred; trees with a large DBH or height and for which the ratio between crown's diameter and depth is less than 1, tended to generate more stemflow volume in these storms. Mean areal stemflow as a fraction of rainfall in this lowland tropical forest was 3·4%, but may range from 1–10% depending upon the proportion of trees that are high or poor stemflow yielders. Trees with DBH greater than 10 cm were likely to contribute less than 1% of the 3·4% mean areal stemflow in the forest. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
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A three-dimensional, time-dependent hydrodynamic and suspended sediment transport model was performed and applied to the Danshuei
River estuarine system and adjacent coastal sea in northern Taiwan. The model was validated with observed time-series salinity
in 2001, and with salinity and suspended sediment distributions in 2002. The predicted results quantitatively agreed with
the measured data. A local turbidity maximum was found in the bottom water of the Kuan-Du station. The validated model then
was conducted with no salinity gradient, no sediment supply from the sediment bed, wind stress, and different freshwater discharges
from upstream boundaries to comprehend the influences on suspended sediment dynamics in the Danshuei River estuarine system.
The results reveal that concentrations of the turbidity maximum simulated without salinity gradient are higher than those
of the turbidity maximum simulated with salinity gradient at the Kuan-Du station. Without bottom resuspension process, the
estuarine turbidity maximum zone at the Kuan-Du station vanishes. This suggests that bottom sediment resuspension is a very
important sediment source to the formation of estuarine turbidity maximum. The wind stress with northeast and southwest directions
may contribute to decrease the suspended sediment concentration. When the freshwater discharges increase at the upstream boundaries,
the limits of salt intrusion pushes downriver toward river mouth. Suspended sediment concentrations increase at the upriver
reaches in the Danshuei River to Tahan Stream, while decrease at Kuan-Du station. 相似文献
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Takanori Sato Nobuaki Tanaka Anand Nainar Koichiro Kuraji Mie Gomyo Haruhiko Suzuki 《水文科学杂志》2020,65(13):2322-2335
ABSTRACT Many studies have focused on soil erosion in unmanaged Japanese cypress plantations because the sparse understory vegetation and litter covering the forest ground enhance soil erosion. In this study, soil erosion, litter, and overland flow measurements were conducted over 14 months to identify the spatio-temporal variation and examine the optimal sample size. Fifteen traps (each 0.25 m wide) were installed in line along the bottom of a 15-m-wide slope. Soil erosion and overland flow had large spatial variations as compared to litter. The temporal coefficient of variation of soil erosion and overland flow was highest during dry seasons, while smaller during wet seasons. The random sampling analysis showed that the rate of decrease in spatio-temporal variation became moderate as the sample size increased beyond six. This result indicated that the optimal sample size was five, the total width of which was equivalent to about 8% of the monitored slope width. 相似文献
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Nobuaki Niitsuma 《Island Arc》2004,13(1):306-317
Abstract Seven chronostratigraphic stages were established based on the correlation of magneto‐biostratigraphic marker horizons within the Deep Sea Drilling Project and Ocean Drilling Program cores from the forearc of the Japan Trench. Because the stages are coeval with changes in the rate of sedimentation, lithofacies, magnetic intensity and composition of fossil assemblages, they probably reflect the tectonic situation in the Japan Trench forearc and also in the arc–trench system. The stages correlate to the tectonic events of the Japanese Island Arcs; for example, evolution of the Boso triple junction, initiation of Philippine Sea Plate subduction and the Japan Sea opening. 相似文献