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101.
Concentrations of polycyclic aromatic hydrocarbons were determined in species of commercial fish and lobsters following an oil-spill just off the protected Madagascan coastline. Samples were collected along the coastline within and outside the affected area. Summed PAH concentrations ranged from 1.9 μg kg−1 to 63 μg kg−1 wet weight, but with no higher molecular weight PAHs (>202 Da) being detected. All concentrations of benzo[a]pyrene, benz[a]anthracene and dibenz[a,h]anthracene were <0.1 μg kg−1 wet weight, well within the EU and UK set limits for the protection of human health. Additionally, samples were calculated as the benzo[a]pyrene toxic equivalency quotient (TEQ) and found to be well below the level of concern in relation to health of human consumers. Evaluation of the biota PAH data indicated the origin of PAH was predominantly petrogenic with >80% arising from oil sources. Profile studies indicate a low-level multisource petrogenic contamination probably representing a pre-spill background for the area. 相似文献
102.
Adrian Spence David J. Mcnally Margaret V. McCaul Brett Paull 《Geochimica et cosmochimica acta》2011,75(10):2571-2581
Soil microbial biomass is a primary source of soil organic carbon (SOC) and therefore plays a fundamental role in carbon and nitrogen cycling. However, little is known about the fate and transformations of microbial biomass in soil. Here we employ HR-MAS NMR spectroscopy to monitor 13C and 15N labeled soil microbial biomass and leachate degradation over time. As expected, there is a rapid loss of carbohydrate structures. However, diffusion edited HR-MAS NMR data reveals that macromolecular carbohydrates are more resistant to degradation and are found in the leachate. Aromatic components survive as dissolved species in the leachate while aliphatic components persist in both the biomass and leachate. Dissolved protein and peptidoglycan accumulate in the leachate and recalcitrant amide nitrogen and lipoprotein persists in both the degraded biomass and leachate. Cross-peaks that appear in 1H-15N HR-MAS NMR spectra after degradation suggest that specific peptides are either selectively preserved or used for the synthesis of unknown structures. The overall degradation pathways reported here are similar to that of decomposing plant material degraded under similar conditions suggesting that the difference between recalcitrant carbon from different sources is negligible after decomposition. 相似文献
103.
104.
Jian-Yang Li Lucille Le Corre Stefan E. Schröder Vishnu Reddy Brett W. Denevi Bonnie J. Buratti Stefano Mottola Martin Hoffmann Pablo Gutierrez-Marques Andreas Nathues Christopher T. Russell Carol A. Raymond 《Icarus》2013
Dawn spacecraft orbited Vesta for more than one year and collected a huge volume of multispectral, high-resolution data in the visible wavelengths with the Framing Camera. We present a detailed disk-integrated and disk-resolved photometric analysis using the Framing Camera images with the Minnaert model and the Hapke model, and report our results about the global photometric properties of Vesta. The photometric properties of Vesta show weak or no dependence on wavelengths, except for the albedo. At 554 nm, the global average geometric albedo of Vesta is 0.38 ± 0.04, and the Bond albedo range is 0.20 ± 0.02. The bolometric Bond albedo is 0.18 ± 0.01. The phase function of Vesta is similar to those of S-type asteroids. Vesta’s surface shows a single-peaked albedo distribution with a full-width-half-max ∼17% relative to the global average. This width is much smaller than the full range of albedos (from ∼0.55× to >2× global average) in localized bright and dark areas of a few tens of km in sizes, and is probably a consequence of significant regolith mixing on the global scale. Rheasilvia basin is ∼10% brighter than the global average. The phase reddening of Vesta measured from Dawn Framing Camera images is comparable or slightly stronger than that of Eros as measured by the Near Earth Asteroid Rendezvous mission, but weaker than previous measurements based on ground-based observations of Vesta and laboratory measurements of HED meteorites. The photometric behaviors of Vesta are best described by the Hapke model and the Akimov disk-function, when compared with the Minnaert model, Lommel–Seeliger model, and Lommel–Seeliger–Lambertian model. The traditional approach for photometric correction is validated for Vesta for >99% of its surface where reflectance is within ±30% of global average. 相似文献
105.
Robin S. Keir Oliver Schmale Maren Walter Jürgen Sültenfuß Richard Seifert Monika Rhein 《Earth and Planetary Science Letters》2008,270(3-4):338-348
Hydrothermal emission of mantle helium appears to be directly related to magma production rate, but other processes can generate methane and hydrogen on mid-ocean ridges. In an on-going effort to characterize these processes in the South Atlantic, the flux and distribution of these gases were investigated in the vicinity of a powerful black smoker recently discovered at 8°17.9' S, 13°30.4' W. The vent lies on the shoulder of an oblique offset in the Mid-Atlantic Ridge and discharges high concentrations of methane and hydrogen. Measurements during expeditions in 2004 and 2006 show that the ratio of CH4 to 3He in the neutrally buoyant plume is quite high, 4 × 108. The CTD stations were accompanied by velocity measurements with lowered acoustic Doppler current profilers (LADCP), and from these data we estimate the methane transport to have been 0.5 mol s− 1 in a WSW-trending plume that seems to develop during the ebb tidal phase. This transport is an order of magnitude greater than the source of CH4 calculated from its concentration in the vent fluid and the rise height of the plume. From this range of methane fluxes, the source of 3He is estimated to be between 0.14 and 1.2 nmol s− 1. In either case, the 3He source is significantly lower than expected from the spreading rate of the Mid-Atlantic Ridge. From the inventory of methane in the rift valley adjacent to the vent, it appears that the average specific rate of oxidation is 2.6 to 23 yr− 1, corresponding to a turnover time between 140 and 16 days. Vertical profiles of methane in the surrounding region often exhibited Gaussian-like distributions, and the variances appear to increase with distance from the vent. Using a Gaussian plume model, we obtained a range of vertical eddy diffusivities between 0.009 and 0.08 m2m2 s− 1. These high values may be due to tidally driven internal waves across the promontory on which the vent is located. 相似文献
106.
107.
Probabilistic seismic hazard analysis: Early history 总被引:1,自引:0,他引:1
Robin K. McGuire 《地震工程与结构动力学》2008,37(3):329-338
Probabilistic seismic hazard analysis (PSHA) is the evaluation of annual frequencies of exceedence of ground motion levels (typically designated by peak ground acceleration or by spectral accelerations) at a site. The result of a PSHA is a seismic hazard curve (annual frequency of exceedence vs ground motion amplitude) or a uniform hazard spectrum (spectral amplitude vs structural period, for a fixed annual frequency of exceedence). Analyses of this type were first conceived in the 1960s and have become the basis for the seismic design of engineered facilities ranging from common buildings designed according to building codes to critical facilities such as nuclear power plants. This Historical Note traces the early history of PSHA. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
108.
109.
Estimating suspended sediment concentrations from turbidity measurements and the calibration problem 总被引:1,自引:0,他引:1
In situ turbidity meters are being increasingly used to generate continuous records of suspended sediment concentration in rivers. However, the usefulness of the information obtained depends heavily on the existence of a close relationship between fluctuations in suspended sediment concentration and turbidity and the calibration procedure that relates suspended sediment concentration to the turbidity meter's signal. This study assesses the relationship between suspended sediment concentration and turbidity for a small (1·19 km2) rural catchment in southern Brazil and evaluates two calibration methods by comparing the estimates of suspended sediment concentration obtained from the calibrated turbidity readings with direct measurements obtained using a USDH 48 suspended sediment sampler. With the first calibration method, the calibration relationship is derived by relating the turbidity readings to simultaneous measurements of concentration obtained from suspended sediment samples collected from the vicinity of the turbidity probe during flood events. With the second method, the calibration is based on the readings obtained from the turbidity meter when the probe immersed in samples of known concentration prepared using soils collected from the catchment. Overall, there was a close link between fluctuations in suspended sediment concentration and turbidity in the stream at the outlet of the catchment, and the estimates of sediment concentration obtained using the first calibration method corresponded closely with the conventionally measured sediment concentrations. However, use of the second calibration method introduced appreciable errors. When the estimated sediment concentrations were compared with the measured values, the mean errors were ± 122 mg l?1 and + 601 mg l?1 for the first and second calibration procedures respectively. Copyright © 2007 John Wiley & Sons, Ltd. 相似文献
110.
Claude Robin Jean-Philippe Eissen Pablo Samaniego Hervé Martin Minard Hall Joseph Cotten 《Bulletin of Volcanology》2009,71(3):233-258
The Mojanda–Fuya Fuya Volcanic Complex consists of two nearby volcanoes, Mojanda and Fuya Fuya. The older one, Mojanda volcano
(0.6 to 0.2 Ma), was first constructed by andesites and high-silica andesites forming a large stratovolcano (Lower Mojanda).
This edifice was capped by a basaltic andesite and andesitic cone (Upper Mojanda), which collapsed later to form a 3-km-wide
summit caldera, after large phreatomagmatic eruptions. The Lower Fuya Fuya edifice was constructed by the extrusion of viscous
Si-rich andesitic lavas and dacitic domes, and the emission of a thick sequence of pyroclastic-flow and fallout deposits which
include two voluminous rhyolitic layers. An intermediate construction phase at Fuya Fuya is represented by a mainly effusive
cone, andesitic in composition (San Bartolo edifice), the construction of which was interrupted by a major sector collapse
in the Late Pleistocene. Finally, a complex of thick siliceous lavas and domes was emplaced within the avalanche amphitheatre,
forming the Upper Fuya Fuya volcanic centre. This paper shows that the general evolution from an effusive to an explosive
eruptive style is related to a progressive adakitic contribution to the magma source. Although all the rocks of the complex
are included in the medium-K field of continental arcs, the Fuya Fuya suite (61–75 wt.% SiO2) shows depletion in Y and HREE and high Sr/Y and La/Yb values, compared to the less silicic Mojanda suite (55–66.5 wt.% SiO2). The Mojanda calc-alkaline suite was generated by partial melting of an adakite-metasomatised mantle source that left a
residue with 2% garnet, followed by fractional crystallization of dominant plagioclase + pyroxene + olivine at shallow, intra-crustal
depths. For Fuya Fuya, geochemical and mineralogical data suggest either (1) partial melting of a similar metasomatised mantle
with more garnet in the residue (4%), followed by fractional crystallization involving plagioclase, amphibole and pyroxene,
or (2) mixing of mafic mantle-derived magma from the Mojanda suite and slab melts, followed by the same fractional crystallization
process. 相似文献