The provenance of Australian uranium ore concentrates by elemental and isotopic analysis     

Elizabeth Keegan  Stephan Richter  Ian Kelly  Henri Wong  Patricia Gadd  Heinz Kuehn  Adolfo Alonso-Munoz 《Applied Geochemistry》2008

Elemental and isotopic ratio analyses of U ore concentrate samples, from the 3 operating U mining facilities in Australia, were carried out to determine if significant variations exist between their products, thereby allowing the U ore concentrate’s origin to be identified. Elemental analyses were conducted using inductively coupled plasma mass spectrometry (ICP-MS) and X-ray fluorescence spectrometry (XRF). Lead isotope ratios were measured using ICP-MS and U isotope analyses were conducted using thermal ionisation mass spectrometry (TIMS). Minute quantities of sample, such as that obtained from a swipe, were also examined for elemental concentrations using secondary ion mass spectrometry (SIMS). The results of multivariate statistical analysis show clear patterns in the trace elemental composition of the processed U ores, indicating that it is possible to use this feature as a unique identifier of an Australian U ore concentrate’s source. Secondary ion mass spectrometry analyses also allow individual particles to be differentiated using this ‘fingerprinting’ technique. Isotope ratios determined using TIMS reveal that there is a significant difference in the n(²³⁴U)/n(²³⁸U) isotope ratio between the U ore concentrate from each mine.  相似文献   

Changes of cloud microphysical properties during the transition from supercooled to mixed-phase conditions during CIME     

Stephan Mertes  Alfons Schwarzenbck  Paolo Laj  Wolfram Wobrock  Jean-Marc Pichon  Giordano Orsi  Jost Heintzenberg 《Atmospheric Research》2001,58(4)

A ground-based seeding experiment using carbon dioxide and propane sprayed from pressurized bottles was carried out under supercooled cloud conditions on a small spatial and short time scale. Water vapor deposition on the artificially generated dry ice and propane ice germs as the main ice formation process (nucleation and growth) is consistent with the experimental results. After nucleation, diffusional growth of the ice particles, partly at the expense of evaporating small droplets, was identified during the mixing of the seeding line with the ambient supercooled cloud. Within the seeding plume, ice water contents up to 80% of the total condensed water are observed, although the size of the formed ice particles did not exceed 25 μm. From the changes of the ice and supercooled liquid phase with time under mixed-phase conditions, liquid water content (LWC) evaporation, ice water content (IWC) formation, and ice crystal growth rates are estimated, which are not affected by the artificial nucleation process. Thus, these rates are assessed to be applicable for a growing ice phase of small ice particles in a young mixed-phase cloud, where other growth mechanisms, like riming or aggregation, are negligible.  相似文献   

Analyzing Outcrop-Scale Fracture Features to Supplement Investigations of Bedrock Aquifers     

Stephan B. Mabee  Kenneth C. Hardcastle 《Hydrogeology Journal》1997,5(4):21-36

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Interactive Knowledge Generation in Urban Green Building Transitions     

Bérénice Preller  Julia Affolderbach  Christian Schulz  Sebastian Fastenrath  Boris Braun 《The Professional geographer》2017,69(2):214-224

Knowledge coproduction between practitioners and scientists offers promising opportunities for the emerging research field of the geography of sustainability transitions. Drawing on experiences from an international research project on urban green building transitions, this article explores the potentials and challenges of interactive and collaborative knowledge generation methods in understanding sustainability transitions. Our results show that ongoing engagement with local experts and practitioners through interactive World Café workshops and follow-up exchanges allows for a better understanding of the research context and knowledge exchange to all participants involved in the research process.  相似文献   

Two- and three-dimensional inversions of magnetic anomalies in the MARK area (Mid-Atlantic Ridge 23° N)     

Norbert J. Schulz  Robert S. Detrick  Stephen P. Miller 《Marine Geophysical Researches》1988,10(1-2):41-57

Magnetic data collected in conjunction with a Sea Beam bathymetric survey of the Mid-Atlantic Ridge south of the Kane Fracture Zone are used to constrain the spreading history of this area over the past 3 Ma. Two-dimensional forward modeling and inversion techniques are carried out, as well as a full three-dimensional inversion of the anomaly field along a 90-km-long section of the rift valley. Our results indicate that this portion of the Mid-Atlantic Ridge, known as the MARK area, consists of two distinct spreading cells separated by a small, zero-offset transform or discordant zone near 23°10′ N, The youngest crust in the median valley is characterized by a series of distinct magnetization highs which coalesce to form two NNE-trending bands of high magnetization, one on the northern ridge segment which coincides with a large constructional volcanic ridge, and one along the southern ridge segment that is associated with a string of small axial volcanos. These two magnetization highs overlap between 23° N and 23°10° N forming a non-transform offset that may be a slow spreading ridge analogue of the small ridge axis discontinuities found on the East Pacific Rise. The crustal magnetizations in this overlap zone are generally low, although an anomalous, ESE-trending magnetization high of unknown origin is also present in this area. The present-day segmentation of spreading in the MARK area was inherited from an earlier ridge-transform-ridge geometry through a series of small (∼ 10 km) eastward ridge jumps. These small ridge jumps were caused by a relocation of the neovolcanic zone within the median valley and have resulted in an overall pattern of asymmetric spreading with faster rates to the west (14 mm yr⁻¹) than to the east (11 mm yr⁻¹). Although the detailed magnetic survey described in this paper extends out to only 3 Ma old crust, a regional compilation of magnetic data from this area by Schoutenet al. (1985) indicates that the relative positions and dimensions of the spreading cells, and the pattern of asymmetric spreading seen in the MARK area during the past 3 Ma, have characterized this part of the Mid-Atlantic Ridge for at least the past 36 Ma.  相似文献   

The end of trend estimation for extreme floods under climate change?          下载免费PDF全文

Karsten Schulz  Matthias Bernhardt 《水文研究》2016,30(11):1804-1808

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Astrophysical smooth particle hydrodynamics     

Stephan Rosswog   《New Astronomy Reviews》2009,53(4-6):78-104

The paper presents a detailed review of the smooth particle hydrodynamics (SPH) method with particular focus on its astrophysical applications. We start by introducing the basic ideas and concepts and thereby outline all ingredients that are necessary for a practical implementation of the method in a working SPH code. Much of SPH’s success relies on its excellent conservation properties and therefore the numerical conservation of physical invariants receives much attention throughout this review. The self-consistent derivation of the SPH equations from the Lagrangian of an ideal fluid is the common theme of the remainder of the text. We derive a modern, Newtonian SPH formulation from the Lagrangian of an ideal fluid. It accounts for changes of the local resolution lengths which result in corrective, so-called “grad-h-terms”. We extend this strategy to special relativity for which we derive the corresponding grad-h equation set. The variational approach is further applied to a general-relativistic fluid evolving in a fixed, curved background space-time. Particular care is taken to explicitly derive all relevant equations in a coherent way.  相似文献   

The Scaling Behaviour of a Turbulent Kinetic Energy Closure Model for Stably Stratified Conditions   总被引：2，自引：1，他引：1  

Peter Baas  Stephan R. de Roode  Geert Lenderink 《Boundary-Layer Meteorology》2008,127(1):17-36

We investigate the scaling behaviour of a turbulent kinetic energy (TKE) closure model for stably stratified conditions. The mixing length scale for stable stratification is proportional to the ratio of the square root of the TKE and the local Brunt–Väisälä frequency, which is a commonly applied formulation. We analyze the scaling behaviour of our model in terms of traditional Monin–Obukov Similarity Theory and local scaling. From the model equations, we derive expressions for the stable limit behaviour of the flux–gradient relations and other scaling quantities. It turns out that the scaling behaviour depends on only a few model parameters and that the results obey local scaling theory. The analytical findings are illustrated with model simulations for the second GABLS intercomparison study. We also investigate solutions for the case in which an empirical correction function is used to express the eddy diffusivity for momentum as a function of the Richardson number (i.e. an increasing turbulent Prandtl number with stability). In this case, it seems that for certain parameter combinations the model cannot generate a steady-state solution. At the same time, its scaling behaviour becomes unrealistic. This shows that the inclusion of empirical correction functions may have large and undesired consequences for the model behaviour.  相似文献   

Submarine landslides at the eastern Sunda margin: observations and tsunami impact assessment     

Brune  Sascha  Ladage  Stefan  Babeyko  Andrey Y.  Müller  Christian  Kopp  Heidrun  Sobolev  Stephan V. 《Natural Hazards》2010,54(2):547-562

Our analysis of new bathymetric data reveals six submarine landslides at the eastern Sunda margin between central Java and Sumba Island, Indonesia. Their volumes range between 1 km3 in the Java fore-arc basin up to 20 km3 at the trench off Sumba and Sumbawa. We estimate the potential hazard of each event by modeling the corresponding tsunami and its run-up on nearby coasts. Four slides are situated remarkably close to the epicenter of the 1977 tsunamigenic Sumba M _w  = 8.3 earthquake. However, comparison of documented tsunami run-up heights and arrival times with our modeling results neither allows us to confirm nor can we falsify the hypothesis that the earthquake triggered these submarine landslides.  相似文献   

Boninites as windows into trace element mobility in subduction zones   总被引：3，自引：0，他引：3  

Stephan König  Carsten Münker  Stephan Schuth  Ambre Luguet  Jonathan Kuduon 《Geochimica et cosmochimica acta》2010,74(2):684-338

Boninites are subduction-related rocks originating from re-melting of highly depleted mantle sources left after extraction of tholeiitic melts. Due to their depleted nature, the incompatible trace element inventory of boninites is virtually entirely inherited from slab components without a significant contribution from the refractory mantle wedge. Thus, boninites constitute an excellent window into processes controlling trace element mobilization at the slab-mantle wedge interface. In order to constrain the behaviour of trace elements in subduction zones with a special emphasis on high field strength elements, we analyzed low-Ca boninites and associated tholeiitic basalts from Cape Vogel, Papua New Guinea (PNG) and compare them with compositions of high-Ca boninites and associated tholeiitic basalts from Cyprus. High-precision HFSE (Nb, Ta, Zr, Hf, W) concentration data of the boninites and associated tholeiitic basalts were obtained by isotope dilution. Major, trace element, and Sr-Nd-Hf-Pb isotope compositions clearly document a significant contribution of slab-derived melts involved in the petrogenesis of the PNG boninites, whereas only fluid-like subduction components were involved in the petrogenesis of the PNG basalts and the Cyprus suite. Low-Ca boninites from PNG are derived from a more refractory mantle source (∼21% depletion) than the high-Ca boninites from Cyprus (∼11% depletion) and their respective tholeiitic precursors (<10% depletion). In agreement with the more depleted nature of their mantle source, boninites exhibit a significantly stronger overprint by slab components. High-precision HFSE data indicate that, in comparison to LILE, a somewhat lower but measurable mobilization of all investigated HFSE in both slab-derived fluids and melts is evident. Modelling calculations demonstrate that the subduction components dominate the LILE budget and also largely control LREE and HFSE abundances in the boninite sources. Notably, the increasing influence of slab-derived fluids results in a decrease of the negative Nb-Ta anomaly, most likely reflecting a similar mobility of Nb-Ta and LREE at higher pressures near the critical point of fluid-melt miscibility. Ratios of Zr/Hf and Nb/Ta in the melt-like slab components dominating in the sources of the PNG boninites were probably fractionated in equilibrium with garnet-amphibolitic mafic oceanic crust. HFSE ratios in the Cyprus boninites are best explained by dehydration of subducted pelagic sediments in the absence of Ti-rich phases such as rutile. Our results also confirm previous assertions that the mobility of HFSE decreases in the order Sb > W-Mo > Nb-Ta > Zr-Hf. Furthermore, Mo-W systematics may provide a potential novel tracer for the amount, composition and redox state of subducted pelagic sediments that contribute to the geochemical budget of intra-oceanic arc systems.  相似文献