Application of Plutonium Isotopes to the Sediment Geochronology of Coarse-Grained Sediments from Englebright Lake,California (USA)     

Christina R. Pondell  Aaron J. Beck  Steven A. Kuehl  Elizabeth A. Canuel 《Aquatic Geochemistry》2016,22(2):97-115

The determination of sediment accumulation rates in environments with temporal variations in texture is challenging using traditional radioisotope methods, largely due to low activities associated with coarse sediments. This study used Englebright Lake, an impoundment in northern California, as a model system to examine the application of plutonium isotopes in lacustrine environments where the interlayering of coarse and fine sediments complicates the geochronology. Inductively coupled plasma mass spectrometry was used to quantify plutonium isotopes and low limits of detection allowed for the measurement of plutonium in sand, clay, and silt fractions. Although measurable levels of plutonium were found in sand fractions, over 75 % of the total plutonium activity was found in fine-grain-size fractions (<63 μm). Correlations between cesium-137 and plutonium activities in fine-grained sediments (r = 0.81–0.98, p < 0.005) suggest that plutonium isotopes may be substituted for cesium isotopes in coarse-grained sediments where cesium is typically below detectable levels. Sediment accumulation rates calculated from grain-size normalized plutonium activity profiles ranged from 6 to 145 cm year^?1 in Englebright Lake and identified a sediment depocenter at the delta front upstream of Englebright Dam. Progradation of the delta front reflected changes in sediment supply from the watershed in response to flood events, whereas average annual accumulation responded to human impacts. This study extends the application of plutonium isotopes for sediment geochronology to aquatic environments dominated by coarse sediments and provides new information that contributes to a better understanding of the processes influencing sediment deposition in Englebright Lake.  相似文献   

Cartographies of Stalin: Place,Scale, and Reputational Politics     

Alexi Gugushvili  Peter Kabachnik  Aaron H. Gilbreath 《The Professional geographer》2016,68(3):356-367

In this article we explore the spatial variation of support for former Soviet leader Joseph Stalin in his home country, Georgia. This research contributes to the literature on reputational politics by highlighting the role of spatial, rather than only social, factors in the construction of public opinion about Stalin. We illustrate how geographic factors impact Georgians' perceptions of the Soviet dictator by examining various aspects of place at various scales—including distance to Gori, Stalin's birthplace, the history of urbanization, and economic and political indices. To this end we map attitudes toward the Soviet dictator and use a multilevel spatial regression technique to explain variance in support for Stalin across forty-seven districts of Georgia. This enables us to explore the impact of place on people's attitudes by examining (1) whether there are local and regional hotspots of Stalin admiration and, if so, (2) what the contextual explanations of these attitudes are.  相似文献   

Influences of Natural and Anthropogenic Factors and Tidal Restoration on Terrestrial Arthropod Assemblages in West Coast North American Estuarine Wetlands     

Aaron T. David  Pascale A. L. Goertler  Stuart H. Munsch  Brittany R. Jones  Charles A. Simenstad  Jason D. Toft  Jeffery R. Cordell  Emily R. Howe  Ayesha Gray  Michael P. Hannam  William Matsubu  Erin E. Morgan 《Estuaries and Coasts》2016,39(5):1491-1504

Compared to benthic and water-column invertebrate assemblages, considerably less is known about terrestrial arthropods inhabiting estuarine wetlands despite their importance to tidal wetland biodiversity and productivity. We also need to know more about how human modification of estuaries, including efforts to restore estuarine wetlands, affects these assemblages. To address this knowledge gap, we assembled data from multiple studies on terrestrial arthropod assemblages from 87 intertidal wetland sites in 13 estuaries along the west coast of North America. Arthropods were sampled between 1998 and 2013 with fallout traps deployed in wetlands for 1 to 3 days at a time. We describe patterns in the abundance and taxonomic composition of terrestrial arthropods and evaluate the relative ability of natural and anthropogenic factors to explain variation in abundance and composition. Arthropod abundance was highly variable. Vegetation assemblage, precipitation, and temperature best explained variation in arthropod abundance, while river discharge, latitude, and developed and agricultural land cover surrounding sampling sites were less important. Arthropod abundance rapidly achieved levels of reference wetlands after the restoration of tidal influence to leveed wetlands, regardless of surrounding land cover. However, arthropod assemblage composition was affected by the amount of developed land cover as well as restoration age. These results suggest that restoration of tidal influence to leveed wetlands can rapidly restore some components of estuarine wetland ecosystems but that recovery of other components will take longer and may depend on the extent of anthropogenic modification in the surrounding landscape.  相似文献   

Nanogeochemistry of hydrothermal magnetite     

Artur?P.?DeditiusEmail author  Martin?Reich  Adam?C.?Simon  Alexandra?Suvorova  Jaayke?Knipping  Malcolm?P.?Roberts  Sergey?Rubanov  Aaron?Dodd  Martin?Saunders 《Contributions to Mineralogy and Petrology》2018,173(6):46

Magnetite from hydrothermal ore deposits can contain up to tens of thousands of parts per million (ppm) of elements such as Ti, Si, V, Al, Ca, Mg, Na, which tend to either structurally incorporate into growth and sector zones or form mineral micro- to nano-sized particles. Here, we report micro- to nano-structural and chemical data of hydrothermal magnetite from the Los Colorados iron oxide–apatite deposit in Chile, where magnetite displays both types of trace element incorporation. Three generations of magnetites (X–Z) were identified with concentrations of minor and trace elements that vary significantly: SiO₂, from below detection limit (bdl) to 3.1 wt%; Al₂O₃, 0.3–2.3 wt%; CaO, bdl–0.9 wt%; MgO, 0.02–2.5 wt%; TiO₂, 0.1–0.4 wt%; MnO, 0.04–0.2 wt%; Na₂O, bdl–0.4 wt%; and K₂O, bdl–0.4 wt%. An exception is V₂O₃, which is remarkably constant, ranging from 0.3 to 0.4 wt%. Six types of crystalline nanoparticles (NPs) were identified by means of transmission electron microscopy in the trace element-rich zones, which are each a few micrometres wide: (1) diopside, (2) clinoenstatite; (3) amphibole, (4) mica, (5) ulvöspinel, and (6) Ti-rich magnetite. In addition, Al-rich nanodomains, which contain 2–3 wt% of Al, occur within a single crystal of magnetite. The accumulation of NPs in the trace element-rich zones suggest that they form owing to supersaturation from a hydrothermal fluid, followed by entrapment during continuous growth of the magnetite surface. It is also concluded that mineral NPs promote exsolution of new phases from the mineral host, otherwise preserved as structurally bound trace elements. The presence of abundant mineral NPs in magnetite points to a complex incorporation of trace elements during growth, and provides a cautionary note on the interpretation of micron-scale chemical data of magnetite.  相似文献   

Groundwater recharge in a confined paleovalley setting,Northeast British Columbia,Canada     

Goetz  A. Maximilian  Beckie  Roger D.  Cahill  Aaron G. 《Hydrogeology Journal》2021,29(5):1797-1812

Hydrogeology Journal - Ancient river channels or subglacial drainage networks infilled with younger sediments can include significant deposits of highly permeable sands and gravels. Despite being...  相似文献   

Use of fallout tracers 7Be, 210Pb and 137Cs to distinguish the form of sub‐surface soil erosion delivering sediment to rivers in large catchments          下载免费PDF全文

Gary J. Hancock  Scott N. Wilkinson  Aaron A. Hawdon  Rex J. Keen 《水文研究》2014,28(12):3855-3874

Fallout radionuclides (FRNs) ¹³⁷Cs and ²¹⁰Pb are well established as tracers of surface and sub‐surface soil erosion contributing sediment to river systems. However, without additional information, it has not been possible to distinguish sub‐surface soil erosion sources. Here, we use the FRN ⁷Be (half‐life 53 days) in combination with ¹³⁷Cs and excess ²¹⁰Pb to trace the form of erosion contributing sediment in three large river catchments in eastern Australia; the Logan River (area 3700 km²), Bowen River (9400 km²) and Mitchell River (4700 km²). We show that the combination of ¹³⁷Cs, excess ²¹⁰Pb and ⁷Be can discriminate horizontally aligned sub‐surface erosion sources (rilled and scalded hillslopes and the floors of incised drainage lines and gully ‘badland’ areas) from vertical erosion sources (channel banks and gully walls). Specifically, sub‐surface sources of sediment eroded during high rainfall and high river flow events have been distinguished by the ability of rainfall‐derived ⁷Be to label horizontal soil surfaces, but not vertical. Our results indicate that in the two northern catchments, erosion of horizontal sub‐surface soil sources contributed almost as much fine river sediment as vertical channel banks, and several times the contribution of hillslope topsoils. This result improves on source discrimination provided previously and indicates that in some areas erosion of hillslope soils may contribute significantly to sediment yield, but not as topsoil loss. We find that in north‐eastern Australia, scalded areas on hillslopes and incising drainage lines may be sediment sources of comparable importance to vertical channel banks. Previous studies have used the combination of ¹³⁷Cs, excess ²¹⁰Pb and ⁷Be to estimate soils losses at the hillslope scale. Here, we show that with timely and judicious sampling of soil and sediment during and immediately after high flow events ⁷Be measurements can augment fallout ¹³⁷Cs and ²¹⁰Pb to provide important erosion source information over large catchments. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

Hierarchical livelihood outcomes among co-managed fisheries     

M. Aaron MacNeil  Joshua E. Cinner 《Global Environmental Change》2013,23(6):1393-1401

Collaborative management arrangements are increasingly being used in fisheries, yet critical questions remain about the conditions under which these are most successful. Here, we conduct one of the first comprehensive tests of Elinor Ostrom's diagnostic framework for analyzing social–ecological systems to examine how 16 socioeconomic and institutional conditions are related the livelihood outcomes in 42 co-management arrangements in five countries across the Indo-Pacific. We combine recent developments in both theory and modeling to address three key challenges among comparative studies of social–ecological systems: the presence of a large number of explanatory mechanisms, variables operating at multiple scales, and the potential for interactions among socio-economic and institutional factors. We find that resource users were more likely to perceive benefits from co-management when they are more involved in decisions, were aware that humans are causal agents of change in marine systems, were wealthier, were not migrants, were in villages with smaller populations and older co-management arrangements, and had clearly established boundaries. Critically, we quantify a number of key interactions between: wealth, dependence on marine resources, involvement in decision-making, and population size that have strong implications for co-management success in terms of livelihood benefits. This study demonstrates that context plays a critical but identifiable role in co-management success.  相似文献   

A NanoSIMS and Auger Nanoprobe investigation of an isotopically primitive interplanetary dust particle from the 55P/Tempel‐Tuttle targeted stratospheric dust collector     

Christine FLOSS  Frank J. STADERMANN  Aaron F. MERTZ  Thomas J. BERNATOWICZ 《Meteoritics & planetary science》2010,45(12):1889-1905

Abstract– An IDP nicknamed Andric, from a stratospheric dust collector targeted to collect dust from comet 55P/Tempel‐Tuttle, contains five distinct presolar silicate and/or oxide grains in 14 ultramicrotome slices analyzed, for an estimated abundance of approximately 700 ppm in this IDP. Three of the grains are ¹⁷O‐enriched and probably formed in low‐mass red giant or asymptotic giant branch (AGB) stars; the other two grains exhibit ¹⁸O enrichments and may have a supernova origin. Carbon and N isotopic analyses show that Andric also exhibits significant variations in its N isotopic composition, with numerous discrete ¹⁵N‐rich hotspots and more diffuse regions that are also isotopically anomalous. Three ¹⁵N‐rich hotspots also have statistically significant ¹³C enrichments. Auger elemental analysis shows that these isotopically anomalous areas consist largely of carbonaceous matter and that the anomalies may be hosted by a variety of components. In addition, there is evidence for dilution of the isotopically heavy components with an isotopically normal endmember; this may have occurred either as a result of extraterrestrial alteration or during atmospheric entry. Isotopically primitive IDPs such as Andric share many characteristics with primitive meteorites such as the CR chondrites, which also contain isotopically anomalous carbonaceous matter and abundant presolar silicate and oxide grains. Although comets are one likely source for the origin of primitive IDPs, the presence of similar characteristics in meteorites thought to come from the asteroid belt suggests that other origins are also possible. Indeed the distinction between cometary and asteroidal sources is somewhat blurred by recent observations of icy comet‐like planetesimals in the outer asteroid belt.  相似文献   

Iron isotope compositions of carbonatites record melt generation, crystallization, and late-stage volatile-transport processes   总被引：2，自引：0，他引：2  

Clark M. Johnson  Keith Bell  Brian L. Beard  Aaron I. Shultis 《Mineralogy and Petrology》2010,98(1-4):91-110

Carbonatites define the largest range in Fe isotope compositions yet measured for igneous rocks, recording significant isotopic fractionations between carbonate, oxide, and silicate minerals during generation in the mantle and subsequent differentiation. In contrast to the relatively restricted range in δ⁵⁶Fe values for mantle-derived basaltic magmas (δ⁵⁶Fe?=?0.0?±?0.1‰), calcite from carbonatites have δ⁵⁶Fe values between ?1.0 and +0.8‰, similar to the range defined by whole-rock samples of carbonatites. Based on expected carbonate-silicate fractionation factors at igneous or mantle temperatures, carbonatite magmas that have modestly negative δ⁵⁶Fe values of ~ ?0.3‰ or lower can be explained by equilibrium with a silicate mantle. More negative δ⁵⁶Fe values were probably produced by differentiation processes, including crystal fractionation and liquid immiscibility. Positive δ⁵⁶Fe values for carbonatites are, however, unexpected, and such values seem to likely reflect interaction between low-Fe carbonates and Fe³⁺-rich fluids at igneous or near-igneous temperatures; the expected δ⁵⁶Fe values for Fe²⁺-bearing fluids are too low to produced the observed positive δ⁵⁶Fe values of some carbonatites, indicating that Fe isotopes may be a valuable tracer of redox conditions in carbonatite complexes. Further evidence for fluid-rock or fluid-magma interactions comes from the common occurrence of Fe isotope disequilibrium among carbonate, oxide, silicate, and sulfide minerals in the majority of the carbonatites studied. The common occurrence of Fe isotope disequilibrium among minerals in carbonatites may also indicate mixing of phenocyrsts from distinct magmas. Expulsion of Fe³⁺-rich brines into metasomatic aureols that surround carbonatite complexes are expected to produce high-δ⁵⁶Fe fenites, but this has yet to be tested.  相似文献   

Radiometric and stratigraphic constraints on terminal Ediacaran (post-Gaskiers) glaciation and metazoan evolution     

Craig L. Hebert  Alan J. Kaufman  Sarah C. Penniston-Dorland  Aaron J. Martin 《Precambrian Research》2010

Radiometric constraints on mid-Ediacaran Period glaciation (Gaskiers) in Newfoundland narrowed the known temporal gap between widespread ice ages and the evolution of complex metazoans to several million years. To further evaluate this claim we studied an Ediacaran glacial diamictite at the base of the Fauquier Formation of northern Virginia, and discovered a conformable relationship between the post-glacial cap carbonate and overlying volcanic rocks of the Catoctin Formation. U/Pb zircon age constraints for the rift-related volcanic flows suggest initial emplacement around 571 million years ago. Application of the Catoctin age to the Fauquier succession indicates the occurrence of an ice age about 10 million years younger than the 582 Ma Gaskiers event, supporting the view of multiple Ediacaran Period glaciations. Furthermore, the age constraint from eastern Laurentia falls within radiometric uncertainty of fossiliferous strata in Avalonia, indicating that the Fauquier glaciation was coincident with early metazoan evolution.  相似文献