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151.
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153.
Katherine?M.?PrimmEmail author Gregory?P.?Schill Daniel?P.?Veghte Miriam?Arak?Freedman Margaret?A.?Tolbert 《Journal of Atmospheric Chemistry》2017,74(1):55-69
Mineral dust particles are known to be efficient ice nuclei in the atmosphere. Previous work has probed heterogeneous ice nucleation on various laboratory dust samples including Arizona Test Dust, kaolinite, montmorillonite, and illite as atmospheric dust surrogates. However, it has recently been suggested that NX illite may be a better representation of atmospheric dust. Hiranuma et al. (2015) performed a laboratory comparison for immersion ice nucleation on NX illite, but here we focus on depositional ice nucleation because of its importance in low temperature cirrus cloud formation. A Raman microscope setup was used to examine the ice-nucleating efficiency of NX illite. Organic coatings on the NX illite particles were also investigated using a mixture of 5 dicarboxylic acids (M5). The ratio of NX illite to M5 was varied from 1:10 to 100:1. It was found that NX illite efficiently nucleates ice with Sice = 1.07 ± 0.01 at ?47 °C, with Sice slightly increasing at lower temperatures. In contrast, pure M5 is a poorer ice nucleus with Sice = 1.30 ± 0.02 at ?40 °C, relatively independent of temperature. Further, it was found that M5 coatings on the order of several monolayers thick hindered the ice nucleating ability of NX illite. Optical images suggest that at colder temperatures (< ?50 °C) 1:1 NX illite:M5 particles and pure M5 particles nucleate ice depositionally, while at warmer temperatures (> ?50 °C) subsaturated immersion ice nucleation dominates. These experiments suggest that mineral dust particles may become less active towards ice nucleation as they age in the atmosphere. 相似文献
154.
Amber J. Roesler Christopher H. Gammons Gregory K. Druschel Harry Oduro Simon R. Poulson 《Aquatic Geochemistry》2007,13(3):211-235
Unlike the majority of the water in the flooded mine complex of Butte Montana, which includes the highly acidic Berkeley pit
lake, groundwater in the flooded West Camp underground mine workings has a circum-neutral pH and contains at least 8 μM aqueous
sulfide. This article examines the geochemistry and stable isotope composition of this unusual H2S-rich mine water, and also discusses problems related to the colorimetric analysis of sulfide in waters that contain FeS(aq) cluster compounds. The West Camp mine pool is maintained at a constant elevation by continuous pumping, with discharge water
that contains elevated Mn (90 μM), Fe (16 μM), and As (1.3 μM) but otherwise low metal concentrations. Dissolved inorganic
carbon in the mine water is in chemical and isotopic equilibrium with rhodochrosite in the mineralized veins. The mine water
is under-saturated with mackinawite and amorphous FeS, but is supersaturated with Cu- and Zn-sulfides. However, voltammetry
studies show that much of the dissolved sulfide and ferrous iron are present as FeS(aq) cluster molecules: as a result, the free
concentration of the West Camp water is poorly constrained. Concentrations of dissolved sulfide determined by colorimetry
were lower than gravimetric assays obtained by AgNO3 addition, implying that the FeS(aq) clusters are not completely extracted by the Methylene Blue reagent. In contrast, the clusters are quantitatively extracted
as Ag2S after addition of AgNO3. Isotopic analysis of co-existing aqueous sulfide and sulfate confirms that the sulfide was produced by sulfate-reducing
bacteria (SRB). The H2S-rich mine water is not confined to the immediate vicinity of the extraction well, but is also present in flooded mine shafts
up to 3 km away, and in samples bailed from mine shafts at depths up to 300 m below static water level. This illustrates that
SRB are well established throughout the southwestern portion of the extensive (>15 km3) Butte flooded mine complex. 相似文献
155.
Stphane Coutu Steven W. Barwick James J. Beatty Amit Bhattacharyya Chuck R. Bower Christopher J. Chaput Georgia A. de Nolfo Michael A. DuVernois Allan Labrador Shawn P. McKee Dietrich Müller James A. Musser Scott L. Nutter Eric Schneider Simon P. Swordy Gregory Tarl Andrew D. Tomasch Eric Torbet 《Astroparticle Physics》1999,11(4):208-435
Galactic cosmic rays consist of primary and secondary particles. Primary cosmic rays are thought to be energized by first order Fermi acceleration processes at supernova shock fronts within our Galaxy. The cosmic rays that eventually reach the Earth from this source are mainly protons and atomic nuclei, but also include electrons. Secondary cosmic rays are created in collisions of primary particles with the diffuse interstellar gas. They are relatively rare but carry important information on the Galactic propagation of the primary particles. The secondary component includes a small fraction of antimatter particles, positrons and antiprotons. In addition, positrons and antiprotons may also come from unusual sources and possibly provide insight into new physics. For instance, the annihilation of heavy supersymmetric dark matter particles within the Galactic halo could lead to positrons or antiprotons with distinctive energy signatures. With the High-Energy Antimatter Telescope (HEAT) balloon-borne instrument, we have measured the abundances of positrons and electrons at energies between 1 and 50 GeV. The data suggest that indeed a small additional antimatter component may be present that cannot be explained by a purely secondary production mechanism. Here we describe the signature of the effect and discuss its possible origin. 相似文献
156.
Gregory D. Bierly 《The Professional geographer》1999,51(3):340-349
Although previous climatological studies have investigated the relationship between cyclone frequency and trajectory and regional weather, analyses of structural airflow features and precipitation have been confined to meteorological case studies. In the following paper, the influence of Colorado cyclone airstreams on Midwestern snowfall is investigated using isentropic streamline maps for five cold season months. Results indicate that Colorado cyclones account for a minor percentage of Midwestern snowfall events and amounts. When snowfall is induced by Colorado cyclogenesis, diffluence and instability in the cold sector portions of the cyclone are the dominant lifting mechanisms. 相似文献
157.
M. A. Gregory R. C. George D. J. Marshall A. Anandraj T. P. McClurg 《Marine pollution bulletin》1999,39(1-12):116-121
This study investigated the possibility that changes in the surface morphology of mussel (Perna perna) gill filaments may be used to indicate the relative toxicity of pollutants in the marine environment. Healthy, adult P. perna were collected and immersed in 2 free-flow tanks. Mercury was added to seawater as it entered tank 1 to achieve a constant level of 50 μg/l−1 over 24 days. Uncontaminated seawater was circulated over the mussels in tank 2 (control) for the same period. A 25 mm2 area of gill filament was removed from each of the 5 specimens before and after 24 days immersion in tank 2, and after immersion for 1, 2, 4, 8, 16 and 24 days in tank 1. These were examined using a scanning electron microscope. The remaining soft tissues from each animal were analysed for mercury using an atomic absorption spectrometer. Mercury concentration increased from 0.13 (pre-immersion) to 87 μg/g after day 24. Surface morphology remained normal for all animals in tank 2 and for those exposed to Hg for up to 8 days. However, from 16 to 24 days exposure there was a gradual increase in the diameters of microvilli, a depletion of abfrontal cilia, an increase in abnormal, perhaps necrotic cells and an unusual increase in the number of cilia on the lateral surfaces. These results confirm that P. perna is an efficient bio-accumulator and suggest that their gill pathomorphology may be a useful indicator of toxicity. 相似文献
158.
159.
Hierarchically nested river landform sequences. Part 2: Bankfull channel morphodynamics governed by valley nesting structure
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Gregory B. Pasternack Dastagir Baig Matthew D. Weber Rocko A. Brown 《地球表面变化过程与地形》2018,43(12):2519-2532
River corridors exhibit landforms nested within landforms repeatedly down spatial scales. In Pasternack et al. ( 2018 ), a new, scale‐independent, hierarchical river classification was developed that uses five landform types to map the domains of a single fluvial process – flow convergence routing – at each of three–five spatial scales. Given those methods, this study investigated the details of how flow convergence routing organizes nested landform sequences. The method involved analyzing landform abundance, sequencing, and hierarchical nesting along the 35 km gravel/cobble lower Yuba River in California. Independent testing of flow convergence routing found that hydraulic patterns at every flow matched the essential predictions from classification, substantiating the process–morphology link. River width and bed elevation sequences exhibit large, nonrandom, and linked oscillations structured to preferentially yield wide bars and constricted pools at base flow and bankfull flow. At a flow of 8.44 times bankfull, there is still an abundance of wide bar and constricted pool landforms, but larger topographic drivers also yield an abundance of nozzle and oversized landforms. The nested structure of flow convergence routing landforms reveals that base flow and bankfull landforms are nested together within specific floodprone valley landform types, and these landform types control channel morphodynamics during moderate to large floods. As a result, this study calls into question the prevailing theory that the bankfull channel of a gravel/cobble river is controlled by in‐channel, bankfull, and/or small flood flows. Such flows may initiate sediment transport, but they are too small to control landform organization in a gravel/cobble river with topographic complexity. Copyright © 2018 John Wiley & Sons, Ltd. 相似文献
160.
Gregory M. Reznik 《Ocean Dynamics》2018,68(8):987-1000
Theory of wave boundary layers (WBLs) developed by Reznik (J Mar Res 71: 253–288, 2013, J Fluid Mech 747: 605–634, 2014, J Fluid Mech 833: 512–537, 2017) is extended to a rotating stratified fluid. In this case, the WBLs arise in the field of near-inertial oscillations (NIOs) driven by a tangential wind stress of finite duration. Near-surface Ekman layer is specified in the most general form; tangential stresses are zero at the lower boundary of Ekman layer and viscosity is neglected below the boundary. After the wind ceases, the Ekman pumping at the boundary becomes a linear superposition of inertial oscillations with coefficients dependent on the horizontal coordinates. The solution under the Ekman layer is obtained in the form of expansions in the vertical wave modes. We separate from the solution a part representing NIO and demonstrate development of a WBL near the Ekman layer boundary. With increasing time t, the WBL width decays inversely proportional to \( \sqrt{t} \) and gradients of fields in the WBL grow proportionally to \( \sqrt{t} \); the most part of NIO is concentrated in the WBL. Structure of the WBL depends strongly on its horizontal scale L determined by scale of the wind stress. The shorter the NIO is, the thinner and sharper the WBL is; the short-wave NIO with L smaller than the baroclinic Rossby scale LR does not penetrate deep into the ocean. On the contrary, for L?≥?LR, the WBL has a smoother vertical structure; a significant long-wave NIO signal is able to reach the oceanic bottom. An asymptotic theory of the WBL in rotating stratified fluid is suggested. 相似文献