A Retrospective Analysis of Ozone Formation in the Lower Fraser Valley,British Columbia,Canada. Part II: Influence of Emissions Reductions on Ozone Formation     

B. Ainslie  D. G. Steyn  C. Reuten  P. L. Jackson 《大气与海洋》2013,51(2):170-186

A mechanistic exploration of how ozone formation in the Lower Fraser Valley (LFV) has changed over a 20-year (1985–2005) retrospective period was performed using numerical models, observations, and emissions data from four key episodes selected from the 20-year period. The motivation for this study was the observed differences in trends in summertime episodic ozone concentrations recorded at various monitoring stations within the valley; stations in the western part of the valley have generally shown a noticeable reduction in episodic ozone concentrations whereas stations in the eastern part of the valley have shown little or no improvement in their maximum 8-hour averaged ozone concentrations. Concurrent with these air quality changes, there has been a well-documented reduction in ozone precursor emissions along with an observed shift in the population patterns within the valley over the 20-year period. Ozone formation for four episodes, encompassing the different meteorological regimes that occur during LFV ozone events and spanning the retrospective period, were investigated using the Weather Research and Forecasting (WRF)-Sparse Matrix Operator Kernel Emission (SMOKE)-Community Multiscale Air Quality (CMAQ) modelling system. For each episode, two simulations, intended to isolate the effects of emission changes from meteorological changes, were performed: one with emissions set at the 1985 level and the other with emissions set at the 2005 level. Based on analysis of the model output, observational data, and precursor emission inventories, we find that the Port Moody station in the western LFV remains a volatile organic compound (VOC)-sensitive location; the central part of the LFV around the town of Chilliwack has generally changed from being VOC-limited to being NO_x-limited; the easternmost part of the valley around the town of Hope has been and remains NO_x-limited. Furthermore, based on the observational data and numerical model output, ozone production efficiency as a function of NO has increased noticeably at Chilliwack and likely in the other eastern parts of the valley. This efficiency increase has likely offset some of the benefits resulting from local NO_x emission reductions.

RÉSUMÉ?[Traduit par la rédaction] Nous avons effectué une exploration mécaniste de la façon dont la formation de l'ozone dans la vallée du bas Fraser (VBF) a changé au cours d'une période rétrospective de 20 ans (1985–2005) en nous servant de modèles numériques, d'observations et de données sur les émissions pour quatre épisodes clés choisis dans la période de 20 ans. Ce sont les différences observées entre les tendances dans les concentrations épisodiques d'ozone enregistrées à certaines stations de surveillance dans la vallée qui ont motivé cette étude : les stations dans la partie ouest de la vallée ont généralement affiché une réduction notable des concentrations épisodiques d'ozone alors que les stations dans la partie est de la vallée n'ont montré que peu ou pas d'amélioration dans les valeurs maximales des concentrations moyennes d'ozone sur 8 heures. Concurremment avec ces changements dans la qualité de l'air, il s'est produit une réduction bien documentée dans les émissions de précurseurs de l'ozone en même temps qu'un déplacement observé dans les configurations de population dans la vallée au cours de la période de 20 ans. Nous avons étudié la formation d'ozone au cours de quatre épisodes, englobant les différents régimes météorologiques survenus lors des événements d'ozone dans la VBF et couvrant la période rétrospective, à l'aide du système de modélisation SMOKE (Sparse Matrix Operator Kernel Emissions) – CMAQ (Community Multiscale Air Quality) du WRF (Weather Research and Forecasting). Pour chaque épisode, nous avons effectué deux simulations visant à isoler l'effet des changements dans les émissions de l'effet des changements météorologiques, l'une avec les émissions réglées au niveau de 1985 et l'autre avec les émissions réglées au niveau de 2005. En nous basant sur l'analyse de la sortie du modèle, les données d'observation et les inventaires des émissions de précurseurs, nous trouvons que la stations de Port Moody dans l'ouest de la VBF demeure un endroit sensible aux composés organiques volatiles (COV); la partie centrale de la VBF, autour de la ville de Chilliwack, a généralement changé de « limitée par les COV » à « limitée par les NO_x »; la partie la plus à l'est de la vallée, autour de la ville de Hope, était et est restée « limitée par les NO_x ». De plus, d'après les données d'observation et la sortie du modèle numérique, l'efficacité de la production d'ozone en fonction de NO a notablement augmenté à Chilliwack et vraisemblablement dans les autres parties de l'est de la vallée. Cette augmentation d'efficacité a probablement annulé certains gains provenant des réductions dans les émissions locales de NO_x.  相似文献   

Erratum to: Polar amplification: is atmospheric heat transport important?     

Vladimir A. Alexeev  Craig H. Jackson 《Climate Dynamics》2013,41(2):549-549

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Reply to Alves et al. (2022) discussion on “Stratigraphic record of continental breakup,offshore NW Australia” by Reeve et al. (2022)     

Craig Magee  Matthew T. Reeve  Christopher A.-L. Jackson  Rebecca E. Bell  Ian D. Bastow 《Basin Research》2023,35(1):483-486

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Multi-scale groundwater flow modeling during temperate climate conditions for the safety assessment of the proposed high-level nuclear waste repository site at Forsmark,Sweden     

Steven Joyce  Lee Hartley  David Applegate  Jaap Hoek  Peter Jackson 《Hydrogeology Journal》2014,22(6):1233-1249

Forsmark in Sweden has been proposed as the site of a geological repository for spent high-level nuclear fuel, to be located at a depth of approximately 470 m in fractured crystalline rock. The safety assessment for the repository has required a multi-disciplinary approach to evaluate the impact of hydrogeological and hydrogeochemical conditions close to the repository and in a wider regional context. Assessing the consequences of potential radionuclide releases requires quantitative site-specific information concerning the details of groundwater flow on the scale of individual waste canister locations (1–10 m) as well as details of groundwater flow and composition on the scale of groundwater pathways between the facility and the surface (500 m to 5 km). The purpose of this article is to provide an illustration of multi-scale modeling techniques and the results obtained when combining aspects of local-scale flows in fractures around a potential contaminant source with regional-scale groundwater flow and transport subject to natural evolution of the system. The approach set out is novel, as it incorporates both different scales of model and different levels of detail, combining discrete fracture network and equivalent continuous porous medium representations of fractured bedrock.  相似文献   

Friedrich Schwille: an historical appreciation     

Jackson RE 《Ground water》2006,44(5):768-770

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Evaluation of criteria for predicting erosion and accretion on an estuarine sand beach, Delaware Bay, Jew Jersey     

Nancy L. Jackson 《Estuaries and Coasts》1999,22(2):215-223

Predicting erosion and accretion of sand beaches in estuaries is important to managing shoreline development and identifying potential relationships between biological productivity and beach change. Wave, sediment and profile data, gathered over twenty-nine days on an estuarine sand beach in Delaware Bay, New Jersey, were used to evaluate the performance of four criteria that predict beach erosion and accretion due to wave-induced cross-shore sediment movement (Dean 1973; Sunamura and Horikawa 1974; Hattori and Kawamata 1980; Kraus et al. 1991). Each criterion defines a relation, between a wave and sediment parameter, and includes a coefficient that discriminates beach erosion and accretion events. Relations, based on small-scale laboratory and field data, were evaluated for predicting erosion or accretion at the study site. Significant wave heights at the study site, monitored near high water, ranged from 0.08 to 0.52 m with periods of 2.4 to 12.8 s. Median grain sizes of sediments on the beach foreshore, gathered at low water, ranged from 0.33 to 0.73 mm. All four criteria showed a clustering of erosion and accretion events. Relations derived from small-scale laboratory data were better predictors of erosion on the profile at the field site than those derived from field data gathered on exposed ocean environments. The planar profile and dominance of incident waves of low height and short period are similar to laboratory conditions characterized by initial planar beach slopes and monochromatic waves. Decreasing the value of the empirical coefficient to account for the differences in the magnitude of wave energy and grain size increases the performance of the criteria tested to predict erosion of the profile.  相似文献   

Effects of a high rise building on wind flow and beach characteristics at Atlantic City, NJ, USA     

Karl F. Nordstrom  Nancy L. Jackson 《Ocean & Coastal Management》1998,39(3):245-263

This study assesses the effects of a high rise building on the beach and dune at an intensively developed shoreline through field investigation of geomorphological and sedimentological characteristics and wind tunnel investigation of wind speed and direction. Results indicate that wind speed is increased close to the building, where wind is often deflected to a more onshore direction. Obliquely offshore northwesterly winds are the most dramatically altered and cause onshore flows (with pronounced upward flows) in the landward portion of the beach near the building. Onshore deflections in wind direction cause besanding of the boardwalk and create highly localized scour and deposition zones. A dune on the backbeach breaks up zones of sediment transport and scour and diminishes the likelihood that scour areas will cause increased hazard to landward buildings as a result of flooding. Generic large-scale studies are required to develop criteria for communities to use to specify optimum dimensions, locations and shapes of landforms that are modified or created by high rise structures.  相似文献   

High-Resolution Characterization of a Chlorinated Solvent Impacted Aquifer Using a Passive Profiler     

Haley A. Schneider  W. Andrew Jackson Ph.D.  P.E.  Paul B. Hatzinger Ph.D  Charles E. Schaefer Ph.D 《Ground Water Monitoring & Remediation》2020,40(4):27-43

A direct-drive high-resolution passive profiler (HRPP) was developed to quantify and delineate concentrations of chlorinated volatile organic compounds (CVOCs), geochemical indicators and CVOC-degrading microorganisms/genes, as well as to perform compound-specific stable isotope analysis (CSIA) of CVOCs and estimate interstitial velocity at <30-cm resolution. The profilers can be coupled together to provide a continuous sample interval and advanced to depths up to approximately 9 m below-ground surface (bgs) within saturated media where direct-push techniques are feasible. The HRPP was field tested in a previous dense nonaqueous phase liquid (DNAPL) source zone at the former Naval Air Station in Alameda, CA. HRPP data sets were compared to the following traditional groundwater data sets: CVOC and anion concentrations in standard and multilevel monitoring well water samples, CVOC concentrations in soil core samples, qualitative contaminant profiles delineated with a membrane interface probe (MIP), microbial community and CSIA profiles from Bio-Traps® deployed in wells, groundwater velocity from passive flux meters (PFMs), lithologic profiles correlated with MIP electrical conductivity (EC), and velocity estimates based on permeability profiles measured with a Geoprobe hydraulic profiling tool (HPT). In some cases, the HRPP data were equivalent to traditional techniques and, in other cases, the HRPP data were more representative of local variability rather than bulk aquifer conditions. Overall the results support the use of the HRPP to provide high-resolution data on concentrations, velocity, and microbial activity in temporary direct-push deployments without well installation, providing a new tool to better assess source zones and contaminated groundwater plumes, even in low permeability media, and to increase the fidelity of site transport models.  相似文献   

Beach recovery from extreme storm activity during the 2013–14 winter along the Atlantic coast of Europe     

Guillaume Dodet  Bruno Castelle  Gerd Masselink  Timothy Scott  Mark Davidson  France Floc'h  Derek Jackson  Serge Suanez 《地球表面变化过程与地形》2019,44(1):393-401

The storm sequence of the 2013–14 winter left many beaches along the Atlantic coast of Europe in their most eroded state for decades. Understanding how beaches recover from such extreme events is essential for coastal managers, especially in light of potential regional increases in storminess due to climate change. Here we analyse a unique dataset of decadal beach morphological changes along the west coast of Europe to investigate the post-2013–14 winter recovery. We show that the recovery signature is site specific and multi-annual, with one studied beach fully recovered after 2 years, and the others only partially recovered after 4 years. During the recovery phase, winter waves primarily control the timescales of beach recovery, as energetic winter conditions stall the recovery process whereas moderate winter conditions accelerate it. This inter-annual variability is well correlated with climate indices. On exposed beaches, an equilibrium model showed significant skill in reproducing the post-storm recovery and thus can be used to investigate the recovery process in more detail. © 2018 John Wiley & Sons, Ltd.  相似文献