Seasonal Variations of CH_4 Emissions in the Yangtze River Delta Region of China Are Driven by Agricultural Activities     

Wenjing HUANG  Timothy J. GRIFFIS  Cheng HU  Wei XIAO  Xuhui LEE 《大气科学进展》2021,38(9):1537-1551

Developed regions of the world represent a major atmospheric methane(CH_4) source, but these regional emissions remain poorly constrained. The Yangtze River Delta(YRD) region of China is densely populated(about 16% of China's total population) and consists of large anthropogenic and natural CH_4 sources. Here, atmospheric CH_4 concentrations measured at a 70-m tall tower in the YRD are combined with a scale factor Bayesian inverse(SFBI) modeling approach to constrain seasonal variations in CH_4 emissions. Results indicate that in 2018 agricultural soils(AGS, rice production) were the main driver of seasonal variability in atmospheric CH_4 concentration. There was an underestimation of emissions from AGS in the a priori inventories(EDGAR—Emissions Database for Global Atmospheric Research v432 or v50), especially during the growing seasons. Posteriori CH_4 emissions from AGS accounted for 39%(4.58 Tg, EDGAR v432) to 47%(5.21 Tg, EDGAR v50) of the total CH_4 emissions. The posteriori natural emissions(including wetlands and water bodies) were1.21 Tg and 1.06 Tg, accounting for 10.1%(EDGAR v432) and 9.5%(EDGAR v50) of total emissions in the YRD in2018. Results show that the dominant factor for seasonal variations in atmospheric concentration in the YRD was AGS,followed by natural sources. In summer, AGS contributed 42%(EDGAR v432) to 64%(EDGAR v50) of the CH_4 concentration enhancement while natural sources only contributed about 10%(EDGAR v50) to 15%(EDGAR v432). In addition, the newer version of the EDGAR product(EDGAR v50) provided more reasonable seasonal distribution of CH_4 emissions from rice cultivation than the old version(EDGAR v432).  相似文献   

Radiolarians from the Pohang Basin,Southeast Korea and Paleoceanographic Implications     

Young-Suk BAK  Jong-Deock LEE  Hyesu YUN  Jinyong OH  Seong-Joo LEE 《《地质学报》英文版》2012,86(6):1426-1433

We identified a total of 101 species and two subspecies of radiolarians belonging to 56 genera from 95 samples collected from the Hagjeon and Duho Formations in the Pohang Basin of the southeastern Korean Peninsula. On the basis of the biostratigraphic range of Cyrtocapsella cornuta and Theocorys redondoensis, the depositional period of the upper Hagjeon and lowest Duho Formations was determined to be early to late Middle Miocene. The occurrence of deep-dwelling radiolarians indicates that the paleobathymetry seems to become gradually progressing toward an upper bathyal environment in the middle part of the Hagjeon Formation. However, we prefer to accept another interpretation for the occurrence of deep-sea indicators in the Hagjeon and the lowest part of the Duho Formations, and consider the presence of a region of upwelling cold water that might have simulated a deep-water environment in relatively shallow water. This interpretation is based on the present upwelling of a cold-water mass off the southeast coast of Korea, the occurrence of upwelling microfossils from the Pohang Basin, and the effect of the closing of the Korea Strait approximately 15 Ma. We also considered that the uppermost part of the studied section represents a shallow-water environment.  相似文献   

Improvement in Background Error Covariances Using Ensemble Forecasts for Assimilation of High-Resolution Satellite Data     

Seung-Woo LEE  Dong-Kyou LEE 《大气科学进展》2011,28(4):758-774

Satellite data obtained over synoptic data-sparse regions such as an ocean contribute toward improving the quality of the initial state of limited-area models. Background error covariances are crucial to the proper distribution of satellite-observed information in variational data assimilation. In the NMC (National Meteorological Center) method, background error covariances are underestimated over data-sparse regions such as an ocean because of small differences between different forecast times. Thus, it is necessary to reconstruct and tune the background error covariances so as to maximize the usefulness of the satellite data for the initial state of limited-area models, especially over an ocean where there is a lack of conventional data. In this study, we attempted to estimate background error covariances so as to provide adequate error statistics for data-sparse regions by using ensemble forecasts of optimal perturbations using bred vectors. The background error covariances estimated by the ensemble method reduced the overestimation of error amplitude obtained by the NMC method. By employing an appropriate horizontal length scale to exclude spurious correlations, the ensemble method produced better results than the NMC method in the assimilation of retrieved satellite data. Because the ensemble method distributes observed information over a limited local area, it would be more useful in the analysis of high-resolution satellite data. Accordingly, the performance of forecast models can be improved over the area where the satellite data are assimilated.  相似文献   

From the editors     

George C.LEE 《地震工程与工程振动(英文版)》2011,10(1):I0001-I0001

Dear Contributors,Readers and Friends: 2011 milestones the tenth anniversary of the Journal of Earthquake Engineering and Engineering Vibration.we first want to take this opportunity to express our gratitude to those retiring members of the Editorial Board for their valuable contributions in the past,and to welcome those who joined the Editorial Board this year. As we mentioned in our message to you in December 2010,effective 20ll,the journal is officially co-sponsored by the Huixian Earthquake  相似文献   

Geochemistry of ultramafic xenoliths in Cenozoic alkali basalts from Jiangsu province, eastern China and their geological implication     

SHAO-WEI HUANG  YUNG-TAN LEE  JU-CHIN CHEN  KUNG-SUAN HO  MENG-LUNG LIN  YEN-TSUI HU  REN-YI HUANG 《Journal of Earth System Science》2013,122(3):777-793

  相似文献   

大兴安岭中生代两类流纹岩与玄武岩的成因联系   总被引：2，自引：0，他引：2  

林强  葛文春  孙德有  吴福元  元钟宽  李文远  尹成孝  陈明植  闵庚德  权致纯 《吉林大学学报(地球科学版)》2000,30(4):322-328

根据地质产状和地球化学特征大兴安岭中生代流纹岩类可划分为高Ti流纹岩和低Ti流纹岩。高Ti流纹岩类与亚碱性系列玄武岩类紧密伴生 ,两者在地球化学上构成连续变异系列。低Ti流纹岩类则与碱性系列玄武岩类构成地球化学双峰态。岩相学和地球化学研究表明 ,这两类流纹岩与该区同期玄武岩类有着密切的成因联系 :起源于地幔柱亏损成分的亚碱性系列玄武岩浆经过单斜辉石、斜长石、磷灰石、锆石的分离结晶 ,形成亚碱性系列低钾玄武岩→高钾玄武岩→高Ti流纹岩演化系列 ;起源于地幔柱富集成分的碱性系列玄武岩浆侵入下地壳 ,使下地壳岩石发生部分熔融 ,形成碱性系列玄武岩 -低Ti流纹岩双峰态组合  相似文献   

沙尘分析及等离子空气清洁系统沙尘去除效果的评价     

LEE Jae-keun  KIM Seong-chan  NOH Hyung-soo  董旭辉  狄一安 《中国沙漠》2003,23(3):316-321

本研究对在中国和韩国采集的沙尘的粒径分布及质量浓度进行了测定,使用黄沙标准物质对基于静电沉降原理的等离子空气清洁系统的去除沙尘效率进行了评价。本研究所使用的黄沙采集于北京和汉城,其粒径中值在7.0~80μm之间,浓度范围为300~1462μg·m^-3。在单通道测试中,沙尘去除效果随粒径增大和流速降低而增加。系统速度为1.0m·s^-1时,去除率大于80%。在27m2的房间中,进行多通道测试时,浓度为300μg·m^-3的大气颗粒物仅用10min即可降至150μg·m^-3。因此,等离子空气清洁系统能够有效地去除沙尘及保持室内空气质量。  相似文献   

A comparison of scavenging and deposition processes in global models: results from the WCRP Cambridge Workshop of 1995   总被引：2，自引：1，他引：1  

P. J. RASCH  J. FEICHTER  K LAW  N. MAHOWALD  J. PENNER  C. BENKOVITZ  C. GENTHON  C. GIANNAKOPOULOS  P. KASIBHATLA  D. KOCH  H. LEVY  T. MAKI  M. PRATHER  D. L. ROBERTS  G.&#;J. ROELOFS  D. STEVENSON  Z. STOCKWELL  S. TAGUCHI  M. KRITZ  M. CHIPPERFIELD  D. BALDOCCHI  P. McMURRY  L. BARRIE  Y. BALKANSKI  R. CHATFIELD  E. KJELLSTROM  M. LAWRENCE  H. N. LEE  J. LELIEVELD  K. J. NOONE  J. SEINFELD  G. STENCHIKOV  S. SCHWARTZ  C. WALCEK  D. WILLIAMSON 《Tellus. Series B, Chemical and physical meteorology》2000,52(4):1025-1056

We report on results from a World Climate Research Program workshop on representations of scavenging and deposition processes in global transport models of the atmosphere. 15 models were evaluated by comparing simulations of radon, lead, sulfur dioxide, and sulfate against each other, and against observations of these constituents. This paper provides a survey on the simulation differences between models. It identifies circumstances where models are consistent with observations or with each other, and where they differ from observations or with each other. The comparison shows that most models are able to simulate seasonal species concentrations near the surface over continental sites to within a factor of 2 over many regions of the globe. Models tend to agree more closely over source (continental) regions than for remote (polar and oceanic) regions. Model simulations differ most strongly in the upper troposphere for species undergoing wet scavenging processes. There are not a sufficient number of observations to characterize the climatology (long‐term average) of species undergoing wet scavenging in the upper troposphere. This highlights the need for either a different strategy for model evaluation (e.g., comparisons on an event by event basis) or many more observations of a few carefully chosen constituents.  相似文献   

淡水双壳类壳体碳同位素研究:以河蚬(corbicula fluminea,Müller 1774)为例   总被引：2，自引：0，他引：2  

闫慧  李心清  周会 《地球化学》2008,37(3)

双壳类壳体碳酸盐(文石)稳定同位素组成已被广泛地用于古气候和古环境重建研究中,但是双壳类壳体碳同位素组成所指示的气候和环境意义一直是争议的问题.对双壳类河蚬(corbicula fluminea)进行了室内养殖,并选取两个壳体样品(壳高,A=13 mm,B=9mm),测定其生长部分壳体和生长期间水体碳同位素,研究表明,随着水体碳同位素的升高(δ13CDIC由-5.24‰升至1.41‰),两壳体碳同位素也随之升高,表明水体对壳体碳同位素的影响;δ13CA分布范围为-4.76‰～2.09‰,δ13CB为-8.49‰～2.89,壳体A和B碳同位素均比预测平衡值偏负,表明壳体在形成过程中利用了新陈代谢产生的富集12C的CO2.根据计算壳体A在实验中沉淀部分壳体利用新陈代谢碳的比例(M值)为24%～43%,平均值为33%;壳体B为33%～75%,平均值为58%.M值随生物的生长呈下降变化,这说明在实验中河蚬主要是通过增加对DIC的吸收和利用来满足壳体生长对物质量增加的需求.  相似文献   

针式微萃取结合GC-IRMS测定水溶液中甲酸、乙酸的稳定碳同位素组成     

李心清  黄代宽  章炎麟  江伟  安宁  胡璐  徐刚 《地球化学》2008,37(6)

甲酸和乙酸稳定碳同位素组成（δ^13C）的分析对环境、食品、制药和自然产品等的研究具有重要的应用价值。但目前尚缺乏有效的测定方法。本研究利用最近出现的针式固相微萃取技术（NeedlEX）,以吹扫．捕集方式对水溶液中的有机酸进行了萃取,然后利用气相色谱．同位素比值质谱联用仪（GC—IRMS）对所萃取的有机酸分子进行了占δ^13C的测定。结果显示,质谱计的信号强度与水溶液中有机酸的浓度存在显著的线性相关关系（R^2〉0．99,P〈0．05）,表明Needl EX对水溶液中有机酸具有稳定的萃取能力。在甲酸与乙酸含量分别不低于300μg／mL与200μg／mL的水溶液中,1000mL的吹扫体积可以使两者δ^13C多次分析结果的相对误差分别保持在3％和1％左右,且整个实验流程没有造成可检测的碳同位素分馏作用。低于这两个浓度界线,则分析误差随浓度的降低迅速增加。本研究虽然是针对水溶液中有机酸δ^13C的测定,其萃取方法对其他水溶性挥发和半挥发有机物δ^13C的分析也同样具有应用价值。  相似文献