Evaluating the mobility of137Cs,239+240Pu and210Pb from their distributions in laminated lake sediments   总被引：1，自引：0，他引：1  

John Crusius  Robert F. Anderson 《Journal of Paleolimnology》1995,13(2):119-141

Post-depositional mobility of¹³⁷Cs,^239+240Pu and²¹⁰Pb was assessed in six small lake basins by comparing sedimentary nuclide profiles with their known fallout history. Laminae couplets, when present, were determined to be varves because the¹³⁷Cs and^239+240Pu 1963 fallout peaks are present in laminae couplets corresponding to years 1962–1964. There is no evidence of mobility of²¹⁰Pb, because 1) mass accumulation rates based on²¹⁰Pb agree with those based on¹³⁷Cs and^239+240Pu peak depths and with those based on varve counts, and 2)²¹⁰Pb ages agree with varve ages. Significant mobility of¹³⁷Cs is evident from the penetration of¹³⁷Cs to depths 15–20 cm deeper than^239+240Pu. Deep penetration of¹³⁷Cs in spite of a sharp gradient below the peak is interpreted by a numerical model to suggest that¹³⁷Cs is present in two distinct forms in these sediments, 67–82% as an immobile form and 18–33% reversibly adsorbed with a K _d of approximately 5000. The profiles can be interpreted equally well assuming a small portionof the total¹³⁷Cs was present as an extremely mobile phase (K _d 5000) in the months to years following peak fallout, slowly becoming more strongly adsorbed. High NH ₄ ⁺ concentrations in porewaters may enhance diffusion of the mobile form of¹³⁷Cs, but not of the immobile form of¹³⁷Cs that defines the sharp gradient. Mobility of¹³⁷Cs is likely also enhanced by the low clay content and the high porosity of these sediments. Thus the first detection of¹³⁷Cs in the sediments cannot automatically be assumed to correspond to a date of 1952 (initial testing of thermonuclear weapons), although the depth of the peak can be assumed to correspond to 1963 (the year of maximum fallout from testing of thermonuclear weapons).^239+240Pu is a more reliable sediment chronometer than¹³⁷Cs because it is significantly less mobile.This is the sixth of a series of papers to be published by this journal following the 20 ^th anniversary of the first application of²¹⁰Pb dating of lake sediments. Dr P.G. Appleby is guest editing this series.  相似文献   

Cosmic ray ionization of the Jovian atmosphere     

Louis A. Capone  John Dubach  Robert C. Whitten  Sheo S. Prasad 《Icarus》1979,39(3):433-449

An approximate form of the Boltzmann equation has been used to obtain local ionization rates due to the absorption of galactic cosmic rays in the Jovian atmosphere. It is shown that the muon flux component of the cosmic ray-induced cascade may be especially importannt in ionizing the atmosphere at levels where the total number density exceeds 10¹⁹ cm^?3 (well below the ionospheric layers produced by solar euv). A model containing both positive and negative ion reactions has been employed to compute equilibrium electron and ion number densities. Peak electron number densities on the order of 10³ cm^?3 may be expected even at relatively low magnetic latitudes. The dominant positive ions are NH₄⁺ and C_nH_m⁺ cluster ions, with n ? 2; it is suggested that the absorption of galactic cosmic ray energy at such relatively high pressures in the Jovian atmosphere $\text{(M ? 10}{}^{18}\text{to}\text{10}{}^{20}\text{cm}{}^{\mathrm{?3}}\text{)}$ and the subsequent chemical reactions may be instrumental in the local formation of complex hydrocarbons.  相似文献   

Spectral reflectance change and luminescence of selected salts during 2–10 KeV proton bombardment: Implications for Io     

Robert M. Nelson  Douglas B. Nash 《Icarus》1979,39(2):277-285

Radiation damage and luminescence, caused by magnetospheric charged particles, have been suggested by several authors as mechanisms for explaining some of the peculiar spectral/albedo features of Io. We have pursued this possibility by measuring the uv-visual spectral reflectance and luminescent efficiency of several proposed Io surface constituents during 2 to 10-keV proton irradiation at room temperature and at low temperature (120 < T < 140°K). The spectral reflectance of NaCl and KCl during proton irradiation exhibits the well-known F-center absorption bands at 4580 and 5560 Å. Na₂SO₄ shows a generalized darkening which increases toward longer wavelengths. NaNO₃ shows a spectral reflectance change indicative of the partial alteration of NaNo₃ to NaNo₂. NaNO₂ shows no change. The luminescent efficiencies of NaCl and KCl are ～10^?4 at 300°K and increase by one-half order of magnitude at ～130°K. The efficiencies of K₂CO₃, Na₂CO₃, Na₂SO₄, and NaNO₃ are 10^?4, 10^?4, 10^?5 and 10^?6, respectively, at 300°K and they all decrease by one-half order of magnitude at ～130°K. These results indicate that magnetospheric proton irradiation of Io could cause spectral features in its observed ultraviolet and visible reflection spectrum if salts such as those studied here are present on its surface. However, because the magnitude of these spectral effects is dependent on competing factors such as surface temperature, incident particle energy flux, solar bleaching effects, and trace element abundance, we are unable at this time to make a quantitative estimate of the strength of these spectral effects on Io. The luminescent efficiencies of pure samples that we have studied in the laboratory suggest that charged-particle induced luminescence from Io's surface might be observable by a spacecraft such as Voyager when viewing Io's dark side.  相似文献   

Spectropolarimetry of the methane and ammonia bands of Jupiter between 6800 and 8200 Å     

Ramon D. Wolstencroft  Robert J. Smith 《Icarus》1979,38(2):155-165

Spectropolarimetry of Jupiter at resolutions between 22 and 35 Å reveals a strong increase of linear polarization in the 7250-$\text{A}\text{?}$ CH₄ band. This is very probably due to the decreasing contribution toward the band center of the higher orders of scattering, which have a smaller net polarization than the first few orders. The linear polarization is also enhanced in the band at 7900 $\text{A}\text{?}$ comprising the 7920-$\text{A}\text{?}$ NH₃ and 7600- to 8200-$\text{A}\text{?}$ CH₄ bands. The normalized circular polarization shows a feature at 7250 $\text{A}\text{?}$ with a dispersion shape. This is most probably produced in a double-scattering process involving either a solid or liquid aerosol with an absorption at 7250 $\text{A}\text{?}$. Methane aerosols, the obvious candidates from a spectroscopic point of view, are, however, forbidden if current estimates of the Jovian atmospheric temperature are correct.  相似文献   

An improved transformation-elimination technique for the solution of perturbed Hamiltonian systems     

Robert A. Howland Jr. 《Celestial Mechanics and Dynamical Astronomy》1979,19(1):95-110

A Lie transformation technique proposed by the author (1977) utilizing an approach due to Kolmogorov and Arnol'd is modified to eliminate the calculation of unproductive terms. Special features of the original method — the ability to eliminate simultaneously both short- and long-period terms, and [formal] quadratic convergence for non-degenerate system sand nearly quadratic convergence for degenerate systems—are retained in an even more efficient technique. Comparisons of the new method with other available Lie transform techniques is made.  相似文献   

A search for natural or artificial objects located at the Earth-Moon libration points     

Robert A. Freitas  Francisco Valdes 《Icarus》1980,42(3):442-447

Photographs in the vicinity of the Earth-Moon triangular libration points L4 and L5, and of the solar-synchronized positions in the associated halo orbits (A. A. Kamel, 1969, Ph.D. dissertation, Stanford University), were made during August–September 1979, using the 30-in Cassegrain telescope at Leuschner Observatory, Lafayette, California. An effective 2° square field was covered at each position. No discrete objects, either natural or artificial, were found. The detection limit was about 14th magnitude. The present work extends traditional SETI observations to include the search for interstellar probes (R. A. Freitas, Jr., 1980a, J. Brit. Interplanet. Soc.33, 95–100).  相似文献   

Solar gravitational redshift     

James C. Lopresto  Robert D. Chapman  Elizabeth A. Sturgis 《Solar physics》1980,66(2):245-249

Wavelengths of solar spectrum lines should be shifted toward the red by the Sun's gravitational field as predicted by metric theories of gravity according to the principle of equivalence. Photographic wavelengths of 738 solar Fe i lines and their corresponding laboratory wavelengths have been studied. The measured solar wavelength minus the laboratory wavelength (_observed) averaged for the strong lines agrees well with the theoretically predicted shift (_theoretical). Studies show that the departures depend on line strength. No dependence of the departures on wavelength was found within the existing data.By studying strong lines over a wide spectral range, velocity shifts caused by the complex motions in the solar atmosphere seem to affect the results in a minimal fashion.  相似文献   

Venus mesosphere and thermosphere temperature structure: II. Day-night variations     

Robert E. Dickinson  E.C. Ridley 《Icarus》1977,30(1):163-178

A two-dimensional nonlinear hydrodynamic model has been developed for studying the global scale winds, temperature, and compositional structure of the mesosphere and thermosphere of Venus. The model is driven by absorption of solar radiation. Ultraviolet radiation produces both heating and photodissociation. Infrared solar heating and thermal cooling are also included with an accurate NLTE treatment. The most crucial uncertainty in determining the solar drive is the efficiency by which $\text{λ < 1080}\text{A}\text{?}$ solar radiation is converted to heat. This question was analyzed in Part I, where it was concluded that essentially all hot atom and O(¹D) energy may be transferred to vibrational-rotational energy of CO₂ molecules. If this is so, the minimum possible euv heating occurs and is determined by the quenching of the resulting excess rotational energy. The hydrodynamic model is integrated with this minimum heating and neglecting any small-scale vertical eddy mixing. The results are compared with predictions of another model with the same physics except that it assumes that 30% of $\text{λ < 1080}\text{A}\text{?}$ radiation goes into heat and that the heating from longer-wavelength radiation includes the O(¹D) energy. For the low-efficiency model, exospheric temperatures are ?300°K on the dayside and drop to < 180°K at the antisolar point. For the higher-efficiency model, the day-to-night temperature variation is from ?600°K to ?250°K. Both versions of the model predict a wind of several hundred meters per second blowing across the terminator and abruptly weakening to small values on the nightside with the mass flow consequently going into a strong tongue of downward motion on the nightside of the terminator. The presence of this circulation could be tested observationally by seeing if its signature can be found in temperature measurements. Both versions of the model indicate that a self-consistent large-scale circulation would maintain oxygen concentrations with ?5% mixing ratios near the dayside F-1 ionospheric peak but ?40% at the antisolar point at the same pressure level.  相似文献   

FLOWER COLOR AND ENVIRONMENT: THE CASE OF BUTTERFLY WEED IN OKLAHOMA     

Lawrence J. Watson  Robert Q. Hanham 《The Professional geographer》1977,29(4):374-377

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AN EFFICIENCY EVALUATION OF FOUR DRAINAGE BASIN SHAPE RATIOS*     

David S. McArthur  Robert Ehrlich 《The Professional geographer》1977,29(3):290-295

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