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91.
92.
Wooyong Um Jonathan P. Icenhower R. Jeffery Serne Cleveland J. Dodge Arokiasamy J. Francis 《Geochimica et cosmochimica acta》2010,74(4):1363-6031
The concentration and distribution of uranium (U) in sediment samples from three boreholes recovered near radioactive waste storage tanks at Hanford, Washington, USA, were determined in detail using bulk and micro-analytical techniques. The source of contamination was a plume that contained an estimated 7000 kg of dissolved U that seeped into the subsurface as a result of an accident that occurred during filling of tank BX-102. The desorption character and kinetics of U were also determined by experiment in order to assess the mobility of U in the vadose zone. Most samples contained too little moisture to obtain quantitative information on pore water compositions. Concentrations of U (and contaminant phosphate—P) in pore waters were therefore estimated by performing 1:1 sediment-to-water extractions and the data indicated concentrations of these elements were above that of uncontaminated “background” sediments. Further extraction of U by 8 N nitric acid indicated that a significant fraction of the total U is relatively immobile and may be sequestered in mobilization-resistant phases. Fine- and coarse-grained samples in sharp contact with one another were sub-sampled for further scrutiny and identification of U reservoirs. Segregation of the samples into their constituent size fractions coupled with microwave-assisted digestion of bulk samples showed that most of the U contamination was sequestered within the fine-grained fraction. Isotope exchange (233U) tests revealed that ∼51% to 63% of the U is labile, indicating that the remaining fund of U is locked up in mobilization-resistant phases. Analysis by Micro-X-ray Fluorescence and Micro-X-ray Absorption Near-Edge Spectroscopy (μ-XRF and μ-XANES) showed that U is primarily associated with Ca and is predominately U(VI). The spectra obtained on U-enriched “hot spots” using Time-Resolved Laser-Induced Fluorescence Spectroscopy (TRLIFS) provide strong evidence for uranophane-type [Ca(UO2)2(SiO3OH)2(H2O)5] and uranyl phosphate [Ca(UO2)2(PO4)2(H2O)10-12] phases. These data show that disseminated micro-precipitates can form in narrow pore spaces within the finer-grained matrix and that these objects are likely not restricted to lithic fragment environments. Uranium mobility may therefore be curtailed by precipitation of uranyl silicate and phosphate phases, with additional possible influence exerted by capillary barriers. Consequently, equilibrium-based desorption models that predict the concentrations and mobility of U in the subsurface matrix at Hanford are unnecessarily conservative. 相似文献
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95.
Pradeep Adhikari Yang Hong Kimberly R. Douglas Dalia Bach Kirschbaum Jonathan Gourley Robert Adler G. Robert Brakenridge 《Natural Hazards》2010,55(2):405-422
Floods have profound impacts on populations worldwide in terms of both loss of life and property. A global inventory of floods
is an important tool for quantifying the spatial and temporal distribution of floods and for evaluating global flood prediction
models. Several global hazard inventories currently exist; however, their utility for spatiotemporal analysis of global floods
is limited. The existing flood catalogs either fail to record the geospatial area over which the flood impacted or restrict
the types of flood events included in the database according to a set of criteria, limiting the scope of the inventory. To
improve upon existing databases, and make it more comprehensive, we have compiled a digitized Global Flood Inventory (GFI)
for the period 1998–2008 which also geo-references each flood event by latitude and longitude. This technical report presents
the methodology used to compile the GFI and preliminary findings on the spatial and temporal distributions of the flooding
events that are contained in the inventory. 相似文献
96.
Jonathan J. Liberda Jeroen W. Thompson W. Jack Rink Federico Bernaldo de Quirs Rohit Jayaraman Kailash Selvaretinam Kerry Chancellor‐Maddison Vito Volterra 《Geoarchaeology》2010,25(4):467-474
Nine faunal teeth from layer 20 of El Castillo cave in Cantabrian Spain were dated using electron spin resonance (ESR). Two teeth were rejected due to inconsistent subsample ages, while the remaining teeth yielded a mean age that is consistent with the stratigraphic expectations: 42.7±3.5. Uncertainty in the external γ dose rate results in a potential systematic uncertainty of±6.4ka that should affect all samples equally. The results provide independent confirmation of previously reported 14C ages for layer 20. © 2010 Wiley Periodicals, Inc. 相似文献
97.
Mapping block-and-ash flow hazards based on Titan 2D simulations: a case study from Mt. Taranaki,NZ 总被引:1,自引:0,他引:1
Jonathan N. Procter Shane J. Cronin Thomas Platz Abani Patra Keith Dalbey Michael Sheridan Vince Neall 《Natural Hazards》2010,53(3):483-501
Numerical models for simulation of mass flows are typically focussed upon accurately predicting the paths, travel times and
inundation from a single flow or collapse event. When considering catchment-based hazards from a volcano, this is complicated
by often being faced with several possible scenarios. Over the last 800 years at Mt. Taranaki/Egmont, a number of dome growth
and collapse events have resulted in the genesis and emplacement of block-and-ash flows (BAFs). Each BAF was directed northwestward
by a breach in the crater rim. The latest dome collapse events in the AD 1880s and AD 1755 inundated the northwestern flank
and had run-out lengths 10 km from source. Future activity of this type could have a devastating effect on the Taranaki region’s
communities, infrastructure and economy. Hazard planning has involved constructing volcanic hazard maps based upon the areas
inundated by past volcanic flows, with little consideration of present-day topography. Here, a numerical geophysical mass
flow modelling approach is used to forecast the hazards of future comparable BAF events on NW Mt. Taranaki. The Titan2D programme
encompasses a “shallow water”, continuum solution-based, granular flow model. Flow mechanical properties needed for this approach
include estimates of internal and basal friction as well as the physical dimensions of the initial collapse. Before this model
can be applied to Taranaki BAFs, the input parameters must be calibrated by simulating a range of past collapse events. By
using AD 1860 and AD 1755 scenarios, initial collapse volumes can be well constrained and internal and basal friction angles
can be evaluated through an iterative approach from previous run-out lengths. A range of possible input parameters was, therefore,
determined to produce a suite of potentially inundated areas under present-day terrain. A suite of 10 forecasts from a uniformly
distributed range were combined to create a map of relative probabilities of inundation by future BAF events. These results
were combined in a GIS package to produce hazard zones related to user-specified hazard thresholds. Using these input parameter
constraints, future hazard forecasts for this scale and type of event can also take into account changing summit and topographic
configurations following future eruptive or collapse events. 相似文献
98.
The state of knowledge and resources available to issue alerts of precipitation-induced landslides vary across the USA. Federal
and state agencies currently issue warnings of the potential for shallow, rapidly moving landslides and debris flows in a
few areas along the Pacific coast and for areas affected by Atlantic hurricanes. However, these agencies generally lack resources
needed to provide continuous support or to expand services to other areas. Precipitation thresholds that form the basis of
landslide warning systems now exist for a few areas of the USA, but the threshold rainfall amounts and durations vary over
three orders of magnitude nationwide and over an order of magnitude across small geographic areas such as a county. Antecedent
moisture conditions also have a significant effect, particularly in areas that have distinct wet and dry seasons. Early warnings
of shallow landslides that include specific information about affected areas, probability of landslide occurrence, and expected
timing are technically feasible as illustrated by a case study from the Seattle, WA area. The four-level warning scheme (Null,
Outlook, Watch, Warning) defined for Seattle is based on observed or predicted exceedance of a cumulative precipitation threshold
and a rainfall intensity–duration threshold combined with real-time monitoring of soil moisture. Based on analysis of historical
data, threshold performance varies according to precipitation characteristics, and threshold exceedance corresponds to a given
probability of landslide occurrence. Experience in Seattle during December 2004 and January 2005 illustrates some of the challenges
of providing landslide early warning on the USA West Coast. 相似文献
99.
The state of knowledge and resources available to issue alerts of precipitation-induced landslides vary across the USA. Federal and state agencies currently issue warnings of the potential for shallow, rapidly moving landslides and debris flows in a few areas along the Pacific coast and for areas affected by Atlantic hurricanes. However, these agencies generally lack resources needed to provide continuous support or to expand services to other areas. Precipitation thresholds that form the basis of landslide warning systems now exist for a few areas of the USA, but the threshold rainfall amounts and durations vary over three orders of magnitude nationwide and over an order of magnitude across small geographic areas such as a county. Antecedent moisture conditions also have a significant effect, particularly in areas that have distinct wet and dry seasons. Early warnings of shallow landslides that include specific information about affected areas, probability of landslide occurrence, and expected timing are technically feasible as illustrated by a case study from the Seattle, WA area. The four-level warning scheme (Null, Outlook, Watch, Warning) defined for Seattle is based on observed or predicted exceedance of a cumulative precipitation threshold and a rainfall intensity–duration threshold combined with real-time monitoring of soil moisture. Based on analysis of historical data, threshold performance varies according to precipitation characteristics, and threshold exceedance corresponds to a given probability of landslide occurrence. Experience in Seattle during December 2004 and January 2005 illustrates some of the challenges of providing landslide early warning on the USA West Coast. 相似文献
100.
Stanislav S. Shabala Jonathan G. Rogers Jamie N. McCallum Oleg A. Titov Jay Blanchard James E. J. Lovell Christopher S. Watson 《Journal of Geodesy》2014,88(6):575-586
We examine the relationship between source position stability and astrophysical properties of radio-loud quasars making up the International Celestial Reference Frame (ICRF2). Understanding this relationship is important for improving quasar selection and analysis strategies, and therefore reference frame stability. We construct flux density time series, known as light curves, for 95 of the most frequently observed ICRF2 quasars at both the 2.3 and 8.4 GHz geodetic very long baseline interferometry (VLBI) observing bands. Because the appearance of new quasar components corresponds to an increase in quasar flux density, these light curves alert us about potential changes in source structure before they appear in VLBI images. We test how source position stability depends on three astrophysical parameters: (1) flux density variability at X band; (2) time lag between flares in S and X bands; (3) spectral index root-mean-square (rms), defined as the variability in the ratio between S and X band flux densities. We find that the time lag between S and X band light curves provides a good indicator of position stability: sources with time lags $<$ 0.06 years are significantly more stable ( $>$ 20 % improvement in weighted rms) than sources with larger time lags. A similar improvement is obtained by observing sources with low $(<$ 0.12) spectral index variability. On the other hand, there is no strong dependence of source position stability on flux density variability in a single frequency band. These findings can be understood by interpreting the time lag between S and X band light curves as a measure of the size of the source structure. Monitoring of source flux density at multiple frequencies therefore appears to provide a useful probe of quasar structure on scales important to geodesy. The observed astrometric position of the brightest quasar component (the core) is known to depend on observing frequency. We show how multi-frequency flux density monitoring may allow the dependence on frequency of the relative core positions along the jet to be elucidated. Knowledge of the position–frequency relation has important implications for current and future geodetic VLBI programs, as well as the alignment between the radio and optical celestial reference frames. 相似文献