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31.
Martha Riherd Weller Marian Furst T.A. Tombrello D.S. Burnett 《Geochimica et cosmochimica acta》1978,42(7):999-1009
We have analyzed B in carbonaceous chondrites in order to clarify a factor of 100 difference between the solar system B abundance derived from the solar photosphere and that inferred from previous meteorite data. Consistent results were obtained from two instrumental methods for B analysis: (a) counting of the high energy betas from 12B produced by the 11B(d,p) reaction, and (b) measurement of particle track densities from 10B(n,α)7Li in a plastic track detector affixed to a homogenized meteorite sample. Contamination is a major problem in B analyses, but extensive testing showed that our results were not seriously affected. Our B concentrations are typically 1–2 ppm and are a factor of 2–6 lower than previous carbonaceous chondrite measurements. Our data for the Cl chondrites Ivuna and Orgueil would indicate a solar system B/Si atomic abundance ratio of 58 × 10?6, but this is still a factor of 2–10 higher than the photospheric estimates. It may be that B is depleted in the sun by thermonuclear processes; however, the similarity of photospheric and meteoritic Be abundances is a problem for this point of view. Alternatively, B may be enhanced in carbonaceous chondrites, but this would make B a cosmochemically unique element. A mm-sized (Fe,Mn,Mg)CO3 crystal from Orgueil shows no B enrichment. We find 10B ≤ 1016 atoms/g in two Allende fine-grained inclusions suggesting that B is not a refractory element under solar nebula conditions. This 10B limit, when taken as a limit on 10Be when the inclusion formed, puts constraints on the possibility of a solar system synthesis of 26Al. For a proton spectrum of E?a, a must be ≥ 3 if a solar gas is irradiated or a ≥1.5 if dust of solar composition is irradiated. 相似文献
32.
Polished sections of 5 enstatite chondrites have been irradiated with 30 MeV 4He ions to produce the alpha-radioactive nuclei 211At and 210Po from 209Bi and 208Pb, respectively. The distribution of alpha activity can be mapped, using cellulose nitrate as an alpha track detector, to give the corresponding Bi or Pb distributions in the meteorite. No strong localization of Bi or 208Pb was found; relatively uniform track distributions were observed. In particular, metal or sulfide grains are not enriched in Bi or Pb (relative to bulk), which is in agreement with the predictions of nebular condensation calculations. While the track distributions appear uniform, the results of detailed, track-by-track mappings of the Bi detectors indicate that the Bi is not totally randomly distributed; the statistical fluctuations in the observed track density are different for the cases where the Bi is totally randomly distributed and where the Bi is localized in point sources. Assuming that the Bi in a given sample is localized in identical point sources which are uniformly distributed throughout the sample, the observed relative population densities of clusters (‘stars’) of small numbers of tracks (2–5) corresponds to Bi being localized, with ~90% in grains with about 10?16g-Bi (~3 × 105Biatoms), and with ~10% in 4 × 10?14 g-Bi sources. If these are elemental Bi, as predicted theoretically, they are ~ 102 Å and 103 Å in size, respectively. 相似文献
33.
34.
An analysis of Apollo lunar soil samples 12070,889, 12030,187, and 12070,891: Basaltic diversity at the Apollo 12 landing site and implications for classification of small‐sized lunar samples 下载免费PDF全文
Louise Alexander Joshua F. Snape Katherine H. Joy Hilary Downes Ian A. Crawford 《Meteoritics & planetary science》2016,51(9):1654-1677
Lunar mare basalts provide insights into the compositional diversity of the Moon's interior. Basalt fragments from the lunar regolith can potentially sample lava flows from regions of the Moon not previously visited, thus, increasing our understanding of lunar geological evolution. As part of a study of basaltic diversity at the Apollo 12 landing site, detailed petrological and geochemical data are provided here for 13 basaltic chips. In addition to bulk chemistry, we have analyzed the major, minor, and trace element chemistry of mineral phases which highlight differences between basalt groups. Where samples contain olivine, the equilibrium parent melt magnesium number (Mg#; atomic Mg/[Mg + Fe]) can be calculated to estimate parent melt composition. Ilmenite and plagioclase chemistry can also determine differences between basalt groups. We conclude that samples of approximately 1–2 mm in size can be categorized provided that appropriate mineral phases (olivine, plagioclase, and ilmenite) are present. Where samples are fine‐grained (grain size <0.3 mm), a “paired samples t‐test” can provide a statistical comparison between a particular sample and known lunar basalts. Of the fragments analyzed here, three are found to belong to each of the previously identified olivine and ilmenite basalt suites, four to the pigeonite basalt suite, one is an olivine cumulate, and two could not be categorized because of their coarse grain sizes and lack of appropriate mineral phases. Our approach introduces methods that can be used to investigate small sample sizes (i.e., fines) from future sample return missions to investigate lava flow diversity and petrological significance. 相似文献
35.
36.
Katherine H. Joy Ian A. Crawford Hilary Downes Sara S. Russell Anton T. Kearsley 《Meteoritics & planetary science》2006,41(7):1003-1025
Abstract— LaPaz Icefield (LAP) 02205, 02226, and 02224 are paired stones of a crystalline basaltic lunar meteorite with a low‐Ti (3.21–3.43% TiO2) low‐Al (9.93–10.45% Al2O3), and low‐K (0.11–0.12% K2O) composition. They consist mainly of zoned pyroxene and plagioclase grains, with minor ilmenite, spinel, and mesostasis regions. Large, possibly xenocrystic, forsteritic olivine grains (<3% by mode) contain small trapped multiphase melt inclusions. Accessory mineral and mesostasis composition shows that the samples have experienced residual melt crystallization with silica oversaturation and late‐stage liquid immiscibility. Our section of LAP 02224 has a vesicular fusion crust, implying that it was at one time located sufficiently close to the lunar surface environment to have accumulated solar‐wind‐implanted gases. The stones have a comparable major element composition and petrography to low‐Ti, low‐Al basalts collected at the Apollos 12 and 15 landing sites. However, the LAP stones also have an enriched REE bulk composition and are more ferroan (Mg numbers in the range of 31 to 35) than similar Apollo samples, suggesting that they represent members of a previously unsampled fractionated mare basalt suite that crystallized from a relatively evolved lunar melt. 相似文献
37.
Ian A. Crawford Sarah A. Fagents Katherine H. Joy M. Elise Rumpf 《Earth, Moon, and Planets》2010,107(1):75-85
One of the principal scientific reasons for wanting to resume in situ exploration of the lunar surface is to gain access to
the record it contains of early Solar System history. Part of this record will pertain to the galactic environment of the
Solar System, including variations in the cosmic ray flux, energetic galactic events (e.g., supernovae and/or gamma-ray bursts),
and passages of the Solar System through dense interstellar clouds. Much of this record is of astrobiological interest as
these processes may have affected the evolution of life on Earth, and perhaps other Solar System bodies. We argue that this
galactic record, as for that of more local Solar System processes also of astrobiological interest, will be best preserved
in ancient, buried regolith (‘palaeoregolith’) deposits in the lunar near sub-surface. Locating and sampling such deposits
will be an important objective of future lunar exploration activities. 相似文献
38.
Preservation potential of implanted solar wind volatiles in lunar paleoregolith deposits buried by lava flows 总被引:1,自引:0,他引:1
The lunar surface is bathed in a variety of impacting particles originating from the solar wind, solar flares, and galactic cosmic rays. These particles can become embedded in the regolith and/or produce a range of other molecules as they pass through the target material. The Moon therefore contains a record of the variability of the solar and galactic particle fluxes through time. To obtain useful temporal snapshots of these processes, discrete regolith units must be shielded from continued bombardment that would rewrite the record over time. One mechanism for achieving this preservation is the burial of a regolith deposit by a later lava flow. The archival value of such deposits sandwiched between lava layers is enhanced by the fact that both the under- and over-lying lava can be dated by radiometric techniques, thereby precisely defining the age of the regolith layer and the geologic record contained therein. The implanted volatile species would be vulnerable to outgassing by the heat of the over-lying flow, at temperatures exceeding 300-700 °C. However, the insulating properties of the finely particulate regolith would restrict significant heating to shallow depths. We have therefore modeled the heat transfer between lunar mare basalt lavas and the regolith in order to establish the range of depths below which implanted volatiles would be preserved. We find that the full suite of solar wind volatiles, consisting predominantly of H and He, would survive at depths of ∼13-290 cm (for 1-10 m thick lava flows, respectively). A substantial amount of CO, CO2, N2 and Xe would be preserved at depths as shallow as 3.7 cm beneath meter-thick flows. Given typical regolith accumulation rates during mare volcanism, the optimal localities for collecting viable solar wind samples would involve stacks of thin mare lava flows emplaced a few tens to a few hundred Ma apart, in order for sufficient regolith to develop between burial events. Obtaining useful archives of Solar System processes would therefore require extraction of regolith deposits buried at quite shallow depths beneath radiometrically-dated mare lava flows. These results provide a basis for possible lunar exploration activities. 相似文献
39.
Heather Katherine Handley Colin G. Macpherson Jon P. Davidson 《Contributions to Mineralogy and Petrology》2010,159(6):885-908
The Gede Volcanic Complex (GVC) of the Sunda island arc (West Java, Indonesia) consists of multiple volcanic centres and eruptive
groups with complex magmatic histories. We present new petrological, mineralogical, whole-rock major and trace element and
Sr–O isotopic data to provide constraints on the relative importance of fractional crystallisation and magma mixing in petrogenesis,
as well as on the role and nature of the arc crust. Banded juvenile scoria from Young and Old Gede provide unequivocal evidence
for the (late-stage) interaction of distinct magmas at Gede volcano. However, the relatively small-degree compositional zoning
observed in plagioclase phenocrysts of all eruptive groups (up to ~20 mol% An) may be attributed to physical changes in magma
properties (e.g. P, T, and PH2O) rather than changes in melt composition. Major element and trace element variations within each eruptive series are inconsistent
with magmatic evolution through simple mixing processes. Instead, mixing of variably fractionated magma batches is suggested
to account for the significant scatter in some element variation diagrams. No correlation is observed between textural complexity
and/or mineral disequilibrium and whole-rock geochemistry. REE data and geochemical modelling indicate that fractional crystallisation
involving amphibole in the mid- to lower crust, and fractionation of plagioclase, clinopyroxene, Fe–Ti oxide ± olivine ± orthopyroxene
provide strong control on the geochemical evolution of GVC rocks. Two-pyroxene geothermobarometry provides pre-eruption crystallisation
temperatures of 891–1,046°C and pressures of 3.4–6.5 kbar, equivalent to ~13–24 km depth beneath the volcanoes (mid- to lower
crust). Low, mantle-like clinopyroxene δ18O values of GVC lavas and poor correlation of Sr isotope ratios with indices of differentiation precludes significant assimilation
of isotopically distinct crust during magmatic differentiation. Therefore, we suggest that the geochemical character of the
moderately thick West Javan arc crust is relatively immature compared to typical continental crust. Trace element ratios and
strontium isotopes show that the magmatic source composition of the older geographical units, Gegerbentang and Older Quaternary,
is distinct from the other GVC groups. 相似文献
40.
Bernard Marty Laurent Zimmermann Rainer Wieler Donald L. Burnett Peter Bochsler 《Geochimica et cosmochimica acta》2010,74(1):340-19141
We have analyzed nitrogen, neon and argon abundances and isotopic ratios in target material exposed in space for 27 months to solar wind (SW) irradiation during the Genesis mission. SW ions were extracted by sequential UV (193 nm) laser ablation of gold-plated material, purified separately in a dedicated line, and analyzed by gas source static mass spectrometry. We analyzed gold-covered stainless steel pieces from the Concentrator, a device that concentrated SW ions by a factor of up to 50. Despite extensive terrestrial N contamination, we could identify a non-terrestrial, 15N-depleted nitrogen end-member that points to a 40% depletion of 15N in solar-wind N relative to inner planets and meteorites, and define a composition for the present-day Sun (15N/14N = [2.26 ± 0.67] × 10−3, 2σ), which is indistinguishable from that of Jupiter’s atmosphere. These results indicate that the isotopic composition of nitrogen in the outer convective zone of the Sun has not changed through time, and is representative of the protosolar nebula. Large 15N enrichments due to e.g., irradiation, low temperature isotopic exchange, or contributions from 15N-rich presolar components, are therefore required to account for inner planet values. 相似文献