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Motivated by detections of nitriles in Titan's atmosphere, cometary comae, and the interstellar medium, we report laboratory investigations of the low-temperature chemistry of acetonitrile, propionitrile, acrylonitrile, cyanoacetylene, and cyanogen (CH3CN, CH3CH2CN, CH2CHCN, HCCCN, and NCCN, respectively). A few experiments were also done on isobutyronitrile and trimethylacetonitrile ((CH3)2CHCN and (CH3)3CCN, respectively). Trends were sought, and found, in the photo- and radiation chemical products of these molecules at 12-25 K. In the absence of water, all of these molecules isomerized to isonitriles, and CH3CN, CH3CH2CN, and (CH3)2CHCN also formed ketenimines. In the presence of H2O, no isonitriles were detected but rather the cyanate ion (OCN−) was seen in all cases. Although isonitriles, ketenimines, and OCN− were the main focus of our work, we also describe cases of hydrogen loss, to make smaller nitriles, and hydrogen addition (reduction), to make larger nitriles. HCN formation also was seen in most experiments. The results are presented in terms of nitrile ice chemistry on Titan, in cometary ice, and in the interstellar medium. Possible connections to prebiotic chemistry are briefly discussed. 相似文献
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Groundwater flooding occurred in the upper parts of many chalk rivers in the UK during the exceptionally wet winter of 2000–01. This provided a rare opportunity to investigate the spatial distribution of groundwater discharge and flooding along the normally dry intermittent headwaters of a chalk catchment. The extent of flooding along the River Pang, upstream of the seasonal head, was mapped using aerial photography, and point measurements of flow and water temperature were used to identify the contributing reaches of the river. The results are discussed in the context of the geological and groundwater conditions. The occurrence of flooding can largely be explained by the regional groundwater flow directions, but increased flow in some locations may be as a result of preferential groundwater flow along lines of geological structure. Published by John Wiley & Sons, Ltd. 相似文献
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Overall properties of heterogeneous material 总被引:1,自引:0,他引:1
J. A. Hudson 《Geophysical Journal International》1991,107(3):505-511
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Problems raised by R CMa are revisited. The theoretical significance of observable period changes is noted. Some recent observations are presented and briefly considered against this background. 相似文献
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Natural Hazards - There is a movement towards the concepts of integrated flood risk management and governance. In these concepts, each stakeholder prone to flooding is tasked with actively limiting... 相似文献
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Xavier Rodó Mercedes Pascual Francisco J. Doblas-Reyes Alexander Gershunov Dáithí A. Stone Filippo Giorgi Peter J. Hudson James Kinter Miquel-Àngel Rodríguez-Arias Nils Ch. Stenseth David Alonso Javier García-Serrano Andrew P. Dobson 《Climatic change》2013,118(3-4):625-640
The next generation of climate-driven, disease prediction models will most likely require a mechanistically based, dynamical framework that parameterizes key processes at a variety of locations. Over the next two decades, consensus climate predictions make it possible to produce forecasts for a number of important infectious diseases that are largely independent of the uncertainty of longer-term emissions scenarios. In particular, the role of climate in the modulation of seasonal disease transmission needs to be unravelled from the complex dynamics resulting from the interaction of transmission with herd immunity and intervention measures that depend upon previous burdens of infection. Progress is also needed to solve the mismatch between climate projections and disease projections at the scale of public health interventions. In the time horizon of seasons to years, early warning systems should benefit from current developments on multi-model ensemble climate prediction systems, particularly in areas where high skill levels of climate models coincide with regions where large epidemics take place. A better understanding of the role of climate extremes on infectious diseases is urgently needed. 相似文献