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121.
Robert E. NovakMichael J. Mumma Michael A. DiSanti Neil Dello Russo Karen Magee-Sauer 《Icarus》2002,158(1):14-23
We present absolute abundances and latitudinal variations of ozone and water in the atmosphere of Mars during its late northern spring (Ls=67.3°) shortly before aphelion. Long-slit maps of the a1Δg state of molecular oxygen (O2) and HDO, an isotopic form of water, were acquired on UT January 21.6 1997 using a high-resolution infrared spectrometer (CSHELL) at the NASA Infrared Telescope Facility. O2(a1Δg) is produced by ozone photolysis, and the ensuing dayglow emission at 1.27 μm is used as a tracer for ozone. Retrieved vertical column densities for ozone above ∼20 km ranged between 1.5 and 2.8 μm-atm at mid- to low latitudes (30°S-60°N) and decreased outside that region. A significant decrease in ozone density is seen near 30°N (close to the subsolar latitude of 23.5°N). The rotational temperatures retrieved from O2(a-X) emissions show a mean of 172±2.5 K, confirming that the sensed ozone lies in the middle atmosphere (∼24 km). The ν1 fundamental band of HDO near 3.67 μm was used as a proxy for H2O. The retrieved vertical column abundance of water varies from 3 precipitable microns (pr-μm) at ∼30°S to 24 pr-μm at ∼60°N. We compare these results with current photochemical models and with measurements obtained by other methods. 相似文献
122.
Margaret A. LeMone Robert L. Grossman Robert T. Mcmillen Kuo-Nan Liou S.C. Ou Stuart Mckeen Wayne Angevine Kyoko Ikeda Fei Chen 《Boundary-Layer Meteorology》2002,104(1):1-52
Aircraft, radiosonde, surface-flux, and boundary-layer windprofiler data from the Cooperative Atmosphere Surface Exchange Study's 1997 field project, CASES-97, are combined with synoptic data to study the evolution of the vertically-averaged mixed-layerpotential temperature []and mixing-ratio [Q] onthree nearly-cloudless days from 1000 CST to 1200CST (local noon is approximately 1230 CST). This was achieved through examination of the terms in the time-tendency (`budget')equations for []and [Q]. We estimate three of the terms –local time rate of change, vertical flux divergence, andhorizontal advection. For the [Q]-budget, vertical flux divergence usually dominates, buthorizontal advection is significant on one of the three days. The [Q]-budget balances for two of the three days to within the large experimental error. For the -budget,vertical flux divergence accounts for most of the morningwarming, with horizontal advection of secondary importance.The residual in the -budget has the same sign for all three days, indicating that not all the heating is accounted for. We can balance the []-budgets to within experimental error on two of the three days by correcting the vertical-flux divergence for apparent low biases in the flux measurements of one of the aircraft and in the surface fluxes, and accounting for direct heating of the mixed layer by radiative flux divergence allowing for the effects of carbonaceous aerosols. The [];-budget with these corrections also balances on the third day if horizontal gradients from synoptic maps are used to estimate the horizontal advection. However, the corrected budget for this day does not balance if the horizontal gradient in the advection term is estimated using CASES-97aircraft and radiosondes; we suggest that persistent mesoscale circulations led to an overestimate of the horizontal gradient andhence horizontal advection. 相似文献
123.
Feature based image processing methods applied to bathymetric measurements from airborne remote sensing in fluvial environments 总被引:1,自引:0,他引:1
Bathymetric maps produced from remotely sensed imagery are increasingly common. However, when this method is applied to fluvial environments, changing scenes and illumination variations severely hinder the application of well established empirical calibration methods used to obtain predictive depth–colour relationships. In this paper, illumination variations are corrected with feature based image processing, which is used to identify areas in an image with a near‐zero water depth. This information can then be included in the depth–colour calibration process, which results in an improved prediction quality. The end product is an automated bathymetric mapping method capable of a 4 m2 spatial resolution with a precision of ±15 cm, which allows for a more widespread application of bathymetric mapping. Copyright © 2006 John Wiley & Sons, Ltd. 相似文献
124.
N. Stuart 《The Photogrammetric Record》2006,21(115):292-293
125.
126.
Partitioning of volatile chemicals among the gas, liquid, and solid phases during freezing of liquid water in clouds can impact
trace chemical distributions in the troposphere and in precipitation. We describe here a numerical model of this partitioning
during the freezing of a supercooled liquid drop. Our model includes the time-dependent calculation of the coupled processes
of crystallization kinetics, heat transport, and solute mass transport, for a freezing hydrometeor particle. We demonstrate
the model for tracer partitioning during the freezing of a 1000 μm radius drop on a 100 μm ice substrate, under a few ambient
condition scenarios. The model effectively simulates particle freezing and solute transport, yielding results that are qualitatively
and quantitatively consistent with previous experimental and theoretical work. Results suggest that the ice shell formation
time is governed by heat loss to air and not by dendrite propagation, and that the location of ice nucleation is not important
to freezing times or the effective partitioning of chemical solutes. Even for the case of nucleation at the center of the
drop, we found that dendrites propagated rapidly to form surface ice. Freezing then proceeded from the outside in. Results
also indicate that the solid-liquid interfacial surface area is not important to freezing times or the effective partitioning
of chemical solutes, and that the rate aspects of trapping are more important than equilibrium solid-liquid partitioning to
the effective partitioning resulting from freezing. 相似文献
127.
A regional geochemical survey using soils, stream sediment and stream water sampling revealed multi-element geochemical anomalies, though of low environmental mobility, associated with Mesozoic sedimentary ironstones in Lincolnshire, UK. The most prominent of these anomalies were of As and V in soils and sediments, but elevated levels of elements such as Cr, La, Ce and Th were also observed. These were initially thought to be part of a residual resistate element or heavy-mineral suite, but careful examination suggests that these too may be primarily associated with the process of Fe oxide precipitation during the initial formation of the ironstones. 相似文献
128.
129.
An 18 million year record of the Ca isotopic composition (δ44/42Ca) of planktonic foraminiferans from ODP site 925, in the Atlantic, on the Ceara Rise, provides the opportunity for critical analysis of Ca isotope-based reconstructions of the Ca cycle. δ44/42Ca in this record averages +0.37 ± 0.05 (1σ SD) and ranges from +0.21‰ to +0.52‰. The record is a good match to previously published Neogene Ca isotope records based on foraminiferans, but is not similar to the record based on bulk carbonates, which has values that are as much as 0.25‰ lower. Bulk carbonate and planktonic foraminiferans from core tops differ slightly in their δ44/42Ca (i.e., by 0.06 ± 0.06‰ (n = 5)), while the difference between bulk carbonate and foraminiferan values further back in time is markedly larger, leaving open the question of the cause of the difference. Modeling the global Ca cycle from downcore variations in δ44/42Ca by assuming fixed values for the isotopic composition of weathering inputs (δ44/42Caw) and for isotope fractionation associated with the production of carbonate sediments (Δsed) results in unrealistically large variations in the total mass of Ca2+ in the oceans over the Neogene. Alternatively, variations of ±0.05‰ in the Ca isotope composition of weathering inputs or in the extent of fractionation of Ca isotopes during calcareous sediment formation could entirely account for variations in the Ca isotopic composition of marine carbonates. Ca isotope fractionation during continental weathering, such as has been recently observed, could easily result in variations in δ44/42Caw of a few tenths of permil. Likewise a difference in the fractionation factors associated with aragonite versus calcite formation could drive shifts in Δsed of tenths of permil with shifts in the relative output of calcite and aragonite from the ocean. Until better constraints on variations in δ44/42Caw and Δsed have been established, modeling the Ca2+ content of seawater from Ca isotope curves should be approached cautiously. 相似文献
130.
Microbial ecology of the stratified water column of the Black Sea as revealed by a comprehensive biomarker study 总被引:2,自引:0,他引:2
Stuart G. Wakeham Rudi Amann Katherine H. Freeman Ellen C. Hopmans Bo Barker Jrgensen Isabell F. Putnam Stefan Schouten Jaap S. Sinninghe Damst Helen M. Talbot Dagmar Woebken 《Organic Geochemistry》2007,38(12):2070-2097
The stratified water column of the Black Sea is partitioned into oxic, suboxic, and euxinic zones, each characterized by different biogeochemical processes and by distinct microbial communities. In 2003, we collected particulate matter by large volume in situ filtration at the highest resolution to date for lipid biomarker analysis and bacterioplankton for enumeration of major prokaryotic groups. Abundances of several prokaryotic groups were estimated using CARD-FISH probes specific for Bacteria, Archaea (Crenarchaeota and Euryarchaeota), epsilonproteobacteria (mainly sulfide oxidizers) and sulfate reducing bacteria. We also measured a wide range of bacterial and archaeal lipid biomarkers. Depth distributions of diagnostic biomarkers are matched with zonation of microbial processes, including aerobic bacterial oxidation of methane, oxidation of ammonium by bacteria and archaea, metal reduction, and sulfide oxidation at the chemocline, and bacterial sulfate reduction and anaerobic oxidation of methane by archaea in the anoxic zone. Cell densities for archaea and sulfate reducing bacteria are estimated based on water column biomarker concentrations and compared with CARD-FISH results. 相似文献