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61.
N. Stuart 《The Photogrammetric Record》2006,21(115):292-293
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Partitioning of volatile chemicals among the gas, liquid, and solid phases during freezing of liquid water in clouds can impact
trace chemical distributions in the troposphere and in precipitation. We describe here a numerical model of this partitioning
during the freezing of a supercooled liquid drop. Our model includes the time-dependent calculation of the coupled processes
of crystallization kinetics, heat transport, and solute mass transport, for a freezing hydrometeor particle. We demonstrate
the model for tracer partitioning during the freezing of a 1000 μm radius drop on a 100 μm ice substrate, under a few ambient
condition scenarios. The model effectively simulates particle freezing and solute transport, yielding results that are qualitatively
and quantitatively consistent with previous experimental and theoretical work. Results suggest that the ice shell formation
time is governed by heat loss to air and not by dendrite propagation, and that the location of ice nucleation is not important
to freezing times or the effective partitioning of chemical solutes. Even for the case of nucleation at the center of the
drop, we found that dendrites propagated rapidly to form surface ice. Freezing then proceeded from the outside in. Results
also indicate that the solid-liquid interfacial surface area is not important to freezing times or the effective partitioning
of chemical solutes, and that the rate aspects of trapping are more important than equilibrium solid-liquid partitioning to
the effective partitioning resulting from freezing. 相似文献
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Microbial ecology of the stratified water column of the Black Sea as revealed by a comprehensive biomarker study 总被引:2,自引:0,他引:2
Stuart G. Wakeham Rudi Amann Katherine H. Freeman Ellen C. Hopmans Bo Barker Jrgensen Isabell F. Putnam Stefan Schouten Jaap S. Sinninghe Damst Helen M. Talbot Dagmar Woebken 《Organic Geochemistry》2007,38(12):2070-2097
The stratified water column of the Black Sea is partitioned into oxic, suboxic, and euxinic zones, each characterized by different biogeochemical processes and by distinct microbial communities. In 2003, we collected particulate matter by large volume in situ filtration at the highest resolution to date for lipid biomarker analysis and bacterioplankton for enumeration of major prokaryotic groups. Abundances of several prokaryotic groups were estimated using CARD-FISH probes specific for Bacteria, Archaea (Crenarchaeota and Euryarchaeota), epsilonproteobacteria (mainly sulfide oxidizers) and sulfate reducing bacteria. We also measured a wide range of bacterial and archaeal lipid biomarkers. Depth distributions of diagnostic biomarkers are matched with zonation of microbial processes, including aerobic bacterial oxidation of methane, oxidation of ammonium by bacteria and archaea, metal reduction, and sulfide oxidation at the chemocline, and bacterial sulfate reduction and anaerobic oxidation of methane by archaea in the anoxic zone. Cell densities for archaea and sulfate reducing bacteria are estimated based on water column biomarker concentrations and compared with CARD-FISH results. 相似文献
66.
Falconer David A. Jordan Stuart D. Brosius Jeffrey W. Davila Joseph M. Thomas Roger J. Andreatta Vicenzo Hara Hirohisa 《Solar physics》1998,180(1-2):179-191
We investigate the possibility that strong EUV lines observed with the Goddard Solar EUV Rocket Telescope and Spectrograph (SERTS) provide good proxies for estimating the total coronal flux over shorter wavelength ranges. We use coordinated SERTS and Yohkoh observations to obtain both polynomial and power-law fits relating the broad-band soft X-ray fluxes to the intensities of Fexvi 335 Ú and 361 Ú, Fexv 284 Ú and 417 Ú, and Mgix 368 Ú measured with SERTS. We found that the power-law fits best cover the full range of solar conditions from quiet Sun through active region, though not surprisingly the cooler Mgix 368 Ú line proves to be a poor proxy. The quadratic polynomial fits yield fair agreement over a large range for all but the Mgix line. However, the linear fits fail conspicuously when extrapolated into the quiet-Sun regime. The implications of this work for the Heii 304 Ú line formation problem are also briefly considered. 相似文献
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Stuart G. Wakeham Christian Schaffner Walter Giger 《Geochimica et cosmochimica acta》1980,44(3):403-413
Polycyclic aromatic hydrocarbons (PAH) in sediment cores from Lake Lucerne, Lake Zürich, and Greifensee, Switzerland, and Lake Washington, northwest U.S.A., have been isolated, identified and quantified by glass capillary gas chromatography and gas chromatography/mass spectrometry. Surface sediment layers are greatly enriched in PAH—up to 40 times—compared to deeper layers. In addition, concentration increases in upper sediments generally correspond to increasing industrialization and urbanization in the catchment basins of the lakes. Few PAH could be detected in pre-industrial revolution sediments, indicating that background levels for most PAH in aquatic sediments are extremely low.These results are consistent with an anthropogenic source for most of the aromatic hydrocarbons present in the modern sediments. A comparison of PAH distributions in the sediments and in possible source materials shows that urban runoff of street dust may be the most important PAH input to these lacustrine sediments. There is evidence that a significant contribution to the PAH content of street dust comes from material associated with asphalt. 相似文献
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