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91.
A meandering plume model that explicitly incorporates the effects of small-scale structure in the instantaneous plume has been formulated. The model requires the specification of two physically based input parameters; namely, the meander ratio,M, which is dependent on the ratio of the meandering plume dispersion to the instantaneous relative plume dispersion and, a relative in-plume fluctuation measure,k, that is related inversely to the fluctuation intensity in relative coordinates. Simple analytical expressions for crosswind profiles of the higher moments (including the important shape parameters such as fluctuation intensity, skewness, and kurtosis) and for the concentration pdf have been derived from the model. The model has been tested against some field data sets, indicating that it can reproduce many key aspects of the observed behavior of concentration fluctuations, particularly with respect to modeling the change in shape of the concentration pdf in the crosswind direction.List of Symbols C Mean concentration in absolute coordinates - C r Mean concentration in relative coordinates - C0 Centerline mean concentration in absolute coordinates - C r,0 Centerline mean concentration in relative coordinates - f Probability density function of concentration in absolute coordinates - f c Probability density function of plume centroid position - f r Probability density function of concentration in relative coordinates - i Absolute concentration fluctuation intensity (standard deviation to mean ratio) - i r Relative concentration fluctuation intensity (standard deviation to mean ratio) - k Relative in-plume fluctuation measure:k=1/i r 2 - K Concentration fluctuation kurtosis - M Meander ratio of meandering plume variance to relative plume variance - S Concentration fluctuation skewness - x Downwind distance from source - y Crosswind distance from mean-plume centerline - z Vertical distance above ground - Instantaneous (random) concentration - Crosswind dispersion ofnth concentration moment about zero - ny Mean-plume crosswind (absolute) dispersion - y Plume centroid (meandering) dispersion in crosswind direction - y,c Instantaneous plume crosswind (relative) dispersion - Normalized mean concentration in absolute coordinates:C/C 0 - Particular value taken on by instantaneous concentration,   相似文献   
92.
A series of tracer experiments studying the statistical properties of concentration fluctuations in clouds dispersing in the atmospheric surface layer is described and analyzed. Experiments were conducted at downwind fetches between about 200 and 1200 m, under a wide range of atmospheric conditions ranging from very unstable to moderately stable stratification. The present experiments have addressed basic requirements not met by past field experiments involving instantaneously released clouds; namely, the experiments provided repeat realizations of instantaneously released clouds measured with high-resolution concentration detectors, accompanied by the contemporaneous acquisition of high-quality meteorological and turbulence measurements.Extensive analyses are performed on the cloud concentration data in the framework of relative diffusion. Ensembles of cloud concentration realizations have been constructed. From these ensembles, crosswind and time profiles of the ensemble-mean concentration, concentration variance, ensemble-mean dosage, and dosage variance are obtained. The behaviour of the time profiles of the integral time scale of cloud concentration fluctuations is studied. The use of surface-layer similarity theory for the analysis of the downwind variation of a number of cloud quantities (e.g., cloud size and duration, cloud centre ensemble-mean concentration and dosage, cloud centre concentration and dosage variance, cloud centre integral time scale) is shown to be an effective basis for ordering these quantities. Furthermore, a number of approximate universal relationships describing the behavior of these cloud quantities has been derived. Finally, it is shown that the scaled crosswind and time profiles of ensemble-mean concentration and concentration variance as well as the scaled time profiles of the concentration fluctuation integral time scale exhibit self-similar forms that are independent of atmospheric stratification and downwind fetch.  相似文献   
93.
Surface and water column profiles of suspended matter collected during April-May 2002, and satellite images were used to study factors influencing suspended sediment concentrations (SSCs) and dispersal in the northern Andaman Sea and Gulf of Martaban, one of the largest highly turbid areas of the world's oceans. Perennial high SSC in the Gulf of Martaban is due to a combination of factors including resuspension of sediments by strong tidal currents, shallow bathymetry and seasonal sediment influx from rivers. From satellite images, it was observed that in the central portion of the Gulf of Martaban, the turbidity front oscillates about 150 km in phase with spring-neap tidal cycles and the area covered by the turbid zone (SSC>15 mg l−1) increases from less than 15 000 km2 during neap tide to more than 45 000 km2 during spring tide. The sediment discharged by the Ayeyarwady River is transported mainly eastward, along the coast, into the Gulf of Martaban. Occasionally, during the winter monsoon period, sediment plumes are seen heading westward into the Bay of Bengal. Turbidity profiles show that bottom nepheloid layers are actively transporting some of the sediments into the deep Andaman Sea via the Martaban canyon.  相似文献   
94.
Mechanisms and kinetics of aqueous Fe+2Fe+3 oxidation-reduction and dissolved O2 interaction in the presence of augite, biotite and hornblende were studied in oxic and anoxic solutions at pH 1–9 at 25°C. Oxidation of surface iron on the minerals coincided with both surface release of Fe+2 and by reduction of Fe+3 in solution. Reaction with iron silicates consumed dissolved oxygen at a rate that increased with decreasing pH. Both Fe+3 and O2 consumption were shown to be controlled by coupled electron-cation transfer reactions of the form;
[Fe+2, 1zM+z]silicate + Fe+3 → [Fe+3]silicate + Fe+2 + 1zM+z
and
[Fe+2, 1zM+z]silicate + H+ + 14O2 → [Fe+3]silicate + 1zM+z + 12H2O
where M is a cation of charge +z. The spontaneous reduction of aqueous Fe+3in the presence of precipitated Fe(OH)3bracketed the surface oxidation standard half cell between +0.33 and +0.52 volts. Concurrent hydrolysis reactions involving cation release from the iron silicates were suppressed by the above reactions. Calculated oxidation depths in the minerals varied between 12 and 80Å and were apparently controlled by rates of solid-state cation diffusion.  相似文献   
95.
Measurements have been made of concentration fluctuations in a dispersing plume from an elevated point source in the atmospheric surface layer using a recently developed fast-response photoionization detector. This detector, which has a frequency response (–6 dB point) of about 100 Hz, is shown to be capable of resolving the fluctuation variance contributed by the energetic subrange and most of the inertial-convective subrange, with a reduction in the fluctuation variance due to instrument smoothing of the finest scales present in the plume of at most 4%.Concentration time series have been analyzed to obtain the statistical characteristics of both the amplitude and temporal structure of the dispersing plume. We present alongwind and crosswind concentration fluctuation profiles of statistics of amplitude structure such as total and conditional fluctuation intensity, skewness and kurtosis, and of temporal structure such as intermittency factor, burst frequency, and mean burst persistence time. Comparisons of empirical concentration probability distributions with a number of model distributions show that our near-neutral data are best represented by the lognormal distribution at shorter ranges, where both plume meandering and fine-scale in-plume mixing are equally important (turbulent-convective regime), and by the gamma distribution at longer ranges, where internal structure or spottiness is becoming dominant (turbulent-diffusive regime). The gamma distribution provides the best model of the concentration pdf over all downwind fetches for data measured under stable stratification. A physical model is developed to explain the mechanism-induced probabilistic schemes in the alongwind development of a dispersing plume, that lead to the observed probability distributions of concentration. Probability distributions of concentration burst length and burst return period have been extracted and are shown to be modelled well with a powerlaw distribution. Power spectra of concentration fluctuations are presented. These spectra exhibit a significant inertial-convective subrange, with the frequency at the spectral peak decreasing with increasing downwind fetch. The Kolmogorov constant for the inertial-convective subrange has been determined from the measured spectra to be 0.17±0.03.  相似文献   
96.
REDD+ was designed globally as a results-based instrument to incentivize emissions reduction from deforestation and forest degradation. Over 50 countries have developed strategies for REDD+, implemented pilot activities and/or set up forest monitoring and reporting structures, safeguard systems and benefit sharing mechanisms (BSMs), offering lessons on how particular ideas guide policy design. The implementation of REDD+ at national, sub-national and local levels required payments to filter through multiple governance structures and priorities. REDD+ was variously interpreted by different actors in different contexts to create legitimacy for certain policy agendas. Using an adapted 3E (effectiveness, efficiency, equity and legitimacy) lens, we examine four common narratives underlying REDD+ BSMs: (1) that results-based payment (RBP) is an effective and transparent approach to reducing deforestation and forest degradation; (2) that emphasis on co-benefits risks diluting carbon outcomes; (3) that directing REDD+ benefits predominantly to poor smallholders, forest communities and marginalized groups helps address equity; and (4) that social equity and gender concerns can be addressed by well-designed safeguards. This paper presents a structured examination of eleven BSMs from within and beyond the forest sector and analyses the evidence to variably support and challenge these narratives and their underlying assumptions to provide lessons for REDD+ BSM design. Our findings suggest that contextualizing the design of BSMs, and a reflexive approach to examining the underlying narratives justifying particular design features, is critical for achieving effectiveness, equity and legitimacy.

Key policy insights

  • A results-based payment approach does not guarantee an effective REDD+; the contexts in which results are defined and agreed, along with conditions enabling social and political acceptance, are critical.

  • A flexible and reflexive approach to designing a benefit-sharing mechanism that delivers emissions reductions at the same time as co-benefits can increase perceptions of equity and participation.

  • Targeting REDD+ to smallholder communities is not by default equitable, if wider rights and responsibilities are not taken into account

  • Safeguards cannot protect communities or society without addressing underlying power and gendered relations.

  • The narratives and their underlying generic assumptions, if not critically examined, can lead to repeated failure of REDD+ policies and practices.

  相似文献   
97.
98.
During 1990–2007, there were 894 lidar observations of nocturnal mesopause region temperatures over Fort Collins, Colorado. In an earlier analysis with data to April 1997, an unexpected episodic warming, peaking in 1993 with a maximum value over 10 K, was reported and attributed to the Mount Pinatubo eruption in June 1991. With all data, long-term temperature trends from a 7-parameter linear regression analysis including solar cycle effect and long-term trends leads to a cooling of as much as 6.8 K/decade at 100 km, consistent with some reported observations but larger than model predictions. Including the observed episodic warming response in an 11-parameter nonlinear regression analysis reduces the maximum long-term cooling trends to 1.5 K/decade at 91 km, with magnitude and altitude dependences consistent with the prediction of two models, Spectral Mesosphere/Lower Thermosphere Model (SMLTM) and Hamburg Model of the Neutral and Ionized Atmosphere (HAMMONIA). In addition, the mid-latitude middle-atmospheric response to solar flux variability in Thermosphere–Ionosphere-Energetics and Dynamics (TIMED)/Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) temperatures is presented.  相似文献   
99.
Exposure to 7 MPa of helium at room temperature alters the texture of Upper Freeport coal in a lump form. The differences in texture and porosity between coal powder and lumps may affect the transport and interaction of fluids and coal. In this work, the information about the coal texture and micro- and meso-porosity was obtained via the BET, BJH, and Dubinin–Astakhov analyses. We further investigated the free-fluid-phase volume (free-volume) effects due to helium interaction with the powder and the lumps. During the manometric experiment, helium penetration into the dry coal matrix resulted in slow relaxation of pressure. After exposure of coal to helium, there have been no significant changes of the macroscopic dimensions observed and the relaxation process can be attributed to microscopic ‘free-volume’ effects. Evolution of the sorption–desorption rates indicates that exposure to helium may change the texture and apparent (helium) density of dry coal.  相似文献   
100.
We address the inverse problem of source reconstruction for the difficult case of multiple sources when the number of sources is unknown a priori. The problem is solved using a Bayesian probabilistic inferential framework in which Bayesian probability theory is used to derive the posterior probability density function for the number of sources and for the parameters (e.g., location, emission rate, release time and duration) that characterize each source. A mapping (source–receptor relationship) that relates a multiple source distribution to the concentration measurements made by an array of detectors is formulated based on a forward-time Lagrangian stochastic model. A computationally efficient methodology for determination of the likelihood function for the problem, based on an adjoint representation of the source–receptor relationship and realized in terms of a backward-time Lagrangian stochastic model, is described. An efficient computational algorithm based on a parallel tempered Metropolis-coupled reversible-jump Markov chain Monte Carlo (MCMC) method is formulated and implemented to draw samples from the posterior probability density function of the source parameters. This methodology allows the MCMC method to initiate jumps between the hypothesis spaces corresponding to different numbers of sources in the source distribution and, thereby, allows a sample from the full joint posterior distribution of the number of sources and the parameters for each source to be obtained. The proposed methodology for source reconstruction is tested using synthetic concentration data generated for cases involving two and three unknown sources.  相似文献   
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