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941.
西太平洋富钴结壳元素组合特征及其地质意义 总被引:10,自引:0,他引:10
海山富钴结壳是一种重要的海底固体矿产。对西太平洋海山的56个结壳样品进行了23种化学组分分析,并利用R型聚类分析和R型因子分析,分别提取四组元素组合和四个主因子。综合特征表明.富钴结壳在形成过程中,经历了一次强度较大的锰矿物相成矿作用,Co、Ni等元素的富集与此有关;铁矿物相的成矿作用强度较小,但表现出多期次的特点;锰、铁矿物是不同成矿作用的产物;结壳形成过程中,可能遭受了二次磷酸盐化作用,结壳中磷酸盐矿物的形成对铁矿物相的形成可能有抑制作用。 相似文献
942.
锆基柱撑蒙脱石是近年来多孔材料研究的热点之一。由于大的比表面积、层间距以及孔容积,而具有良好的吸附与催化性能。近年来,锆基柱撑蒙脱石的研究进展主要集中在多种复合柱撑蒙脱石的制备,其应用多在有机物、重金属吸附和催化有机反应等方面,而对柱撑机理、层间结构的研究较少,有待深入。 相似文献
943.
944.
丝光沸石/TiO2复合体的特征及对甲苯光催化降解研究 总被引:5,自引:2,他引:3
在TiO2光催化剂的制备过程中加入一定比例的丝光沸石制备了丝光沸石/TiO2复合体光催化剂.对含甲苯废气进行光催化降解实验.同时运用X射线粉末衍射技术、红外光谱、激光拉曼光谱和紫外一可见漫反射光谱等技术对丝光沸石/TiO2复合体的结构特征和光催化性能进行研究结果表明:丝光沸石的加入能够显著地降低复合光催化剂中TiO2的纳米颗粒粒径、增强其对紫外光的吸收,同时复合光催化剂中TiO2与丝光沸石的结构羟基发生反应形成键合,从而增强了复合体的光催化活性。在丝光沸石和TiO2复合的质量配比为1:5时.复合光催化剂对甲苯的光催化降解率最高.达94.58%。 相似文献
945.
Zhou Tianjun Zhang Wenxia Zhang Lixia Zhang Xuebin Qian Yun Peng Dongdong Ma Shuangmei Dong Buwen 《中国科学:地球科学(英文版)》2020,63(7):919-933
Changes in monsoon precipitation have profound social and economic impacts as more than two-thirds of the world's population lives in monsoon regions. Observations show a significant reduction in global land monsoon precipitation during the second half of the 20 th century. Understanding the cause of this change, especially possible anthropogenic origins, is important.Here, we compare observed changes in global land monsoon precipitation during 1948–2005 with those simulated by 5 global climate models participating in the Coupled Model Inter-comparison Project-phase 5(CMIP5) under different external forcings.We show that the observed drying trend is consistent with the model simulated response to anthropogenic forcing and to anthropogenic aerosol forcing in particular. We apply the optimal fingerprinting method to quantify anthropogenic influences on precipitation and find that anthropogenic aerosols may have contributed to 102%(62–144% for the 5–95% confidence interval)of the observed decrease in global land monsoon precipitation. A moisture budget analysis indicates that the reduction in precipitation results from reduced vertical moisture advection in response to aerosol forcing. Since much of the monsoon regions,such as India and China, have been experiencing rapid developments with increasing aerosol emissions in the past decedes, our results imply a further reduction in monsoon precipitation in these regions in the future if effective mitigations to reduce aerosol emissions are not deployed. The observed decline of aerosol emission in China since 2006 helps to alleviate the reducing trend of monsoon precipiptaion. 相似文献
946.
Science China Earth Sciences - Oxygen fugacity (fO2) is an intensive variable that describes the redox state of a system. By controlling the valence state of multivalent elements, fO2 affects the... 相似文献
947.
Xu Yigang Wang Qiang Tang Gongjian Wang Jun Li Hongyan Zhou Jinsheng Li Qiwei Qi Yue Liu Pingping Ma Lin Fan Jingjing 《中国科学:地球科学(英文版)》2020,63(12):1969-1991
Science China Earth Sciences - Whether arc magmatism occurs above oceanic subduction zones is the forefront of studies on convergent plate margins. The most important petrologic issue related to... 相似文献
948.
采用ABAQUS有限元分析软件,分别对基于刚性地基假定的环板基础、考虑土-结构动力相互作用的环板基础和桩基础超大型冷却塔模型进行了模态分析、弹性和弹塑性时程分析,研究了土-结构动力相互作用和基础形式对超大型冷却塔结构动力特性和地震反应的影响。结果表明:当考虑相同阶数的振型时,刚性地基模型的振型参与质量系数最小。地震作用下,刚性地基模型和桩基础模型的加速度响应、支柱内力、塔壳混凝土主应力等一般比考虑土-结构动力相互作用的环板基础模型偏大,但塔顶水平位移偏小。土-结构动力相互作用比基础形式对冷却塔动力特性以及地震反应的影响更大,且二者对冷却塔竖向振动的影响比水平向大。三种模型计算所获得的冷却塔薄弱部位均集中于支柱,且支柱最大侧移角相差不大。 相似文献
949.
950.
Zircon is one of the most commonly used accessory minerals rich in U and Th for(U-Th)/He dating system. Compared with apatite, zircon has a higher He closure temperature (~190℃), which gives it more advantages in solving the problem of source material and thermal history reconstruction in sedimentary basins. However, the crystals of zircons often have U and Th zoning development, with obvious differences in concentration. Even the standard sample of FCT(Fish Canyon Tuff)zircon which is widely used in (U-Th)/He dating has an average age dispersion of about 10%. In this study, the Alphachron He isotope mass spectrometer is used for laser melting of a batch of single grains of FCT zircon(11 grains)to determine their 4He content. The contents of U and Th of parent isotopes are accurately determined by automatic injection of Agilent 7900 ICP-MS and isotope diluent method. The Th/U ratios of the 10 FCT zircons calculated with (U-Th)/He average age in this paper range from 0.52 to 0.67, which are consistent with the Th/U ratios of 186 reported so far. According to the Th/U ratios of 189 FCT zircons published in the statistical literature, we found that only three of them had high Th/U ratios, namely, 1.12, 1.16 and 1.5, the other 186 FCT zircons(occupy>98%) had a Th/U ratio less than 1. Based on previous results and the 10 Th/U ratios measured in this paper, 196 FCT zircons have a normal Th/U ratio ranging from 0.27 to 1.00, with an average ratio of 0.56(n=196). Excluding one abnormally old age, the(U-Th)/He ages of the remaining FCT zircons in this study range from 26.61 to 31.91Ma, with a weighted mean age of (28.8±3.1)Ma (2SD, n=10), which is consistent with the mean age ((28.3±3.1)Ma, 2σ, n=127) or (28.29±2.6)Ma(2σ external error, 9.3%, n=114)obtained by several other international laboratories. This indicates that the zircon single particle(U-Th)/He dating process established by our laboratory is reliable. For the zircon samples with U, Th banding and concentration differences prevailing, determining the distribution of U, Th elements in the crystal prior to the (U-Th)/He experiment is essential for understanding effects of geometry and elemental zoning on nuclear recoil and diffusion and the interpretation of (U-Th)/He age data. 相似文献