Modelling of the vertical fluxes of nitric acid,ammonia, and ammonium nitrate     

Gerhard Kramm  Ralph Dlugi 《Journal of Atmospheric Chemistry》1994,18(4):319-357

Results from numerical investigations regarding the exchange of HNO₃, NH₃, and NH₄NO₃ between the atmosphere and the biosphere are presented. The investigations were performed with a modified inferential method which is based on the generally accepted micrometeorological ideas of the transfer of momentum, sensible heat and matter near the Earth's surface and the chemical reactions among these nitrogen compounds. This modified inferential method calculates the micrometeorological quantities (such as the friction velocity and the fluxes of sensible and latent heat), the height-invariant fluxes of the composed chemically conservative trace species with group concentrationsc ₁=[HNO₃]+[NH₄NO₃] (total nitrate),c ₂=[NH₃]+[NH₄NO₃] (total ammonia), andc ₃=[HNO₃]-[NH₃] as well as the fluxes of the individual nitrogen compounds. The parameterization of the fluxes is based on the flux-gradient relationships in the turbulent region of the atmospheric surface layer. The modified inferential method requires only the data of wind velocity, temperature, humidity and concentrations (HNO₃, NH₃, and NH₄NO₃) measured at a reference height by stations of a monitoring network.  相似文献   

On global forces of nature driving the Earth’s climate. Are humans involved?     

L. F. Khilyuk  G. V. Chilingar 《Environmental Geology》2006,50(6):899-910

The authors identify and describe the following global forces of nature driving the Earth’s climate: (1) solar radiation as a dominant external energy supplier to the Earth, (2) outgassing as a major supplier of gases to the World Ocean and the atmosphere, and, possibly, (3) microbial activities generating and consuming atmospheric gases at the interface of lithosphere and atmosphere. The writers provide quantitative estimates of the scope and extent of their corresponding effects on the Earth’s climate. Quantitative comparison of the scope and extent of the forces of nature and anthropogenic influences on the Earth’s climate is especially important at the time of broad-scale public debates on current global warming. The writers show that the human-induced climatic changes are negligible.  相似文献   

青藏高原东部牧区雪灾的环流型及水汽场分析   总被引：10，自引：8，他引：10  

梁潇云  钱正安  李万元 《高原气象》2002,21(4):359-367

冬、春季雪灾是青藏高原东部牧区重要的灾害性天气。本文利用历史天气图和国家气象中心T106L19全球模式的分析值格点资料，分析了青藏高原东部牧区近20年来冬，冬季降雨的天气形势和水汽场。结果表明，北脊南槽型、乌山脊型、阶梯槽型和国境槽型是造成高原东部牧区降雪的四类主要环流型；在高原东部牧区强降雪天气过程时气柱可降水量有明显增加，记要降雪区与水汽通量辐合区吻合，主要水汽来自孟加拉湾地区。  相似文献   

Hindsight and Foresight     

N. E. Busch  L. Kristensen 《Boundary-Layer Meteorology》2002,105(3):369-388

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Determination of Area-Averaged Water Vapour Fluxes with Large Aperture and Radio Wave Scintillometers over a Heterogeneous Surface – Flevoland Field Experiment     

W. M. L. Meijninger  A. E. Green  O. K. Hartogensis  W. Kohsiek  J. C. B. Hoedjes  R. M. Zuurbier  H. A. R. De Bruin 《Boundary-Layer Meteorology》2002,105(1):63-83

A large aperture scintillometer (LAS) andradio wave scintillometer (RWS)were installed over a heterogeneous areato test the applicability of the scintillation method.The heterogeneity in the area, whichconsisted of many plots, was mainly caused bydifferences in thermal properties ofthe crops; the variations in theaerodynamic roughness lengthwere small. The water vapour fluxesderived from the combined LAS-RWSsystem, also known as the two-wavelengthmethod, agreed fairly well with the aggregatedwater vapour fluxes derived from in-situeddy covariance measurements. The water vapourfluxes derived from a stand-alone LASare also presented. It was found that a single LASand an estimate of the area averagedavailable energy (using a simple parameterisationscheme) can provide also reasonablearea-averaged water vapour fluxes.  相似文献   

Atmospheric nitrogen inputs into the North Sea: effect on productivity     

Gerrit de Leeuw  Lucinda Spokes  Tim Jickells  Carsten Ambelas Skjth  Ole Hertel  Elisabetta Vignati  Susanne Tamm  Michael Schulz  Lise-Lotte Srensen  Britta Pedersen  Laura Klein  K. Heinke Schlünzen 《Continental Shelf Research》2003,23(17-19):1743

The ANICE (Atmospheric Nitrogen Inputs into the Coastal Ecosystem) project addressed the atmospheric deposition of nitrogen to the North Sea, with emphasis on coastal effects. ANICE focused on quantifying the deposition of inorganic nitrogen compounds to the North Sea and the governing processes. An overview of the results from modelling and experimental efforts is presented. They serve to identify the role of the atmosphere as a source of biologically essential chemical species to the marine biota. Data from the Weybourne Atmospheric Observatory (UK) are used to evaluate the effect of short episodes with very high atmospheric nitrogen concentrations. One such episode resulted in an average deposition of 0.8 mmol N m⁻² day⁻¹, which has the potential to promote primary productivity of 5.3 mmol C m⁻² day⁻¹. This value is compared to long-term effects determined from model results. The total calculated atmospheric deposition to the North Sea in 1999 is 948 kg N km⁻¹, i.e. 0.19 mmol N m⁻² day⁻¹ which has the potential to promote primary productivity of 1.2 mmol C m⁻² day⁻¹. Detailed results for August 1999 show strong gradients across the North Sea due to adjacent areas where emissions of NO_x and NH₃ are among the highest in Europe. The average atmospheric deposition to the southern part of the North Sea in August 1999 could potentially promote primary production of 2.0 mmol C m⁻² day⁻¹, i.e. 5.5% of the total production at this time of the year in this area of the North Sea. For the entire study area the atmospheric contribution to the primary production per m² is about two-third of this value. Most of the deposition occurs during short periods with high atmospheric concentrations. This atmospheric nitrogen is almost entirely anthropogenic in origin and thus represents a human-induced perturbation of the ecosystem.  相似文献   

Simulation of marine boundary layer characteristics using a 1-D PBL model over the Bay of Bengal during BOBMEX-99     

N. V. Sam  U. C. Mohanty  A. N. V. Satyanarayana 《Journal of Earth System Science》2003,112(2):185-204

The characteristic features of the marine boundary layer (MBL) over the Bay of Bengal during the southwest monsoon and the factors influencing it are investigated. The Bay of Bengal and Monsoon Experiment (BOBMEX) carried out during July–August 1999 is the first observational experiment under the Indian Climate Research Programme (ICRP). A very high-resolution data in the vertical was obtained during this experiment, which was used to study the MBL characteristics off the east coast of India in the north and south Bay of Bengal. Spells of active and suppressed convection over the Bay were observed, of which, three representative convective episodes were considered for the study. For this purpose a one-dimensional multi-level PBL model with a TKE-ε closure scheme was used. The soundings, viz., the vertical profiles of temperature, humidity, zonal and meridional component of wind, obtained onboard ORV Sagar Kanya and from coastal stations along the east coast are used for the study. The temporal evolution of turbulent kinetic energy, marine boundary layer height (MBLH), sensible and latent heat fluxes and drag coefficient of momentum are simulated for different epochs of monsoon and monsoon depressions during BOBMEX-99.The model also generates the vertical profiles of potential temperature, specific humidity, zonal and meridional wind. These simulated values compared reasonably well with the observations available from BOBMEX.  相似文献   

地表非均匀性对区域平均水分通量参数化的影响   总被引：3，自引：3，他引：3  

刘晶淼  丁裕国  周秀骥  汪方 《气象学报》2003,61(6):712-717

次网格尺度地表非均匀性对于网格区平均通量具有重要影响。若将网格区视为均一地表 ,并不能真实描述地 气通量交换过程 ,且可造成很大误差。文中从理论上证明 ,区域平均水分通量的变化率可分解为两部分 :第一部分为区域水分通量的算术平均变化率 ;第二部分为非均匀性所引起的水分通量变化率扰动 ,它与区域内土壤水分空间分布的变差系数有关。数值试验表明 ,地表土壤水分的水平空间变差系数集中反映了区域内土壤水分分布的非均匀程度 ,不同土壤对同样的非均匀程度其敏感性是不同的。变差系数愈大 ,非均匀性愈强 ,在相同的土壤水分平均值下 ,不同土壤类型对地表非均匀程度的敏感性并不相同。例如沙土和粘土受非均匀性的影响就可相差数十倍。  相似文献   

A Case Study Of An On-Ice Air Flow Over The Arctic Marginal Sea-Ice Zone     

Timo Vihma  Jörg Hartmann  Christof Lüpkes 《Boundary-Layer Meteorology》2003,107(1):189-217

A case study of warm air advection over the Arctic marginalsea-ice zone is presented, based on aircraft observations with direct flux measurements carriedout in early spring, 1998. A shallow atmospheric boundary layer (ABL) was observed, which wasgradually cooling with distance downwind of the ice edge. This process was mainly connected with astrong stable stratification and downward turbulent heat fluxes of about 10–20 W m^-2, but wasalso due to radiative cooling. Two mesoscale models, one hydrostatic and the other non-hydrostatic,having different turbulence closures, were applied. Despite these fundamental differences betweenthe models, the results of both agreed well with the observed data. Various closure assumptions had amore crucial influence on the results than the differences between the models.Such an assumption was, for example,the parameterization of the surface roughness for momentum (z₀) and heat (z_T). This stronglyaffected the wind and temperature fields not only close to the surface but also within and abovethe temperature inversion layer. The best results were achieved using a formulation for z₀ that took intoaccount the form drag effect of sea-ice ridges together withz_T = 0.1z₀. The stability within theelevated inversion strongly depended on the minimum eddy diffusivity K_min. A simple ad hocparameterization seems applicable, where K_min is calculated as 0.005 timesthe neutral eddy diffusivity. Although the longwave radiative cooling was largest within the ABL, theapplication of a radiation scheme was less important there than above the ABL. This was related to theinteraction of the turbulent and radiative fluxes. To reproduce the strong inversion, it wasnecessary to use vertical and horizontal resolutions higher than those applied in most regional andlarge-scale atmospheric models.  相似文献   

Modelling of the OASIS Energy Flux Measurements Using Two Canopy Concepts     

K. Finkele  J.J. Katzfey  E.A. Kowalczyk  J.L. McGregor  L. Zhang  M.R. Raupach 《Boundary-Layer Meteorology》2003,107(1):49-79

Two land surface schemes, SCAM and CSIRO9, were used to model the measured energy fluxes during the OASIS (Observations At Several Interacting Scales) field program. The measurements were taken at six sites along a 100 km rainfall gradient. Two types of simulations were conducted: (1) offline simulations forced with measured atmospheric input data at each of the six sites, and (2) regional simulations with the two land surface schemes coupled to the regional climate model DARLAM.The two land surface schemes employ two different canopy modelling concepts: in SCAM the vegetation is conceptually above the ground surface, while CSIRO9 employs the more commonly used `horizontally tiled' approach in which the vegetation cover is modelled by conceptually placing it beside bare ground. Both schemes utilize the same below-ground components (soil hydrological and thermal models) to reduce the comparison to canopy processes only. However, the ground heat flux, soil evaporation and evapotranspiration are parameterised by the two canopy treatments somewhat differently.Both canopy concepts reproduce the measured energy fluxes. SCAM has a slightly higher root-mean standard error in the model-measurement comparison for the ground heat flux. The mean surface radiative temperature simulated by SCAM is approximately 1K lower than in the CSIRO9 simulations. However, the soil and vegetation temperatures (which contribute to the radiative temperature) varied more in the CSIRO9 simulations. These larger variations are due to the absence of a representation of the aerodynamic interactions between vegetation and ground.  相似文献