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61.
Regular measurements of the atmospheric ozone in the Brazilian sector were started at Cachoeira Paulista (22.7°S, 45.0°W), and Natal (5.8°S, 35.2°W) in May 1974 and November 1978, respectively. The results of the total ozone measurements carried out at these two stations up to 1981 are presented in this communication and compared with other low-and mid-latitude stations. Although Natal is an equatorial station, it presents a prominent annual variation, and the average total ozone content is high compared to satellite measurements. During 1977–78, abnormally low values of total ozone were observed at Cachoeira Paulista. Some preliminary results about the QBO 9quasi-biennial oscillation) during 1974–81 are also presented. 相似文献
62.
F. C. Fehsenfeld M. J. Bollinger S. C. Liu D. D. Parrish M. McFarland M. Trainer D. Kley P. C. Murphy D. L. Albritton D. H. Lenschow 《Journal of Atmospheric Chemistry》1983,1(1):87-105
The seasonal and diurnal variations of ozone mixing ratios have been observed at Niwot Ridge. Colorado. The ozone mixing ratios have been correlated with the NO
x
(NO+NO2) mixing ratios measured concurrently at the site. The seasonal and diurnal variations in O3 can be reasonably well understood by considering photochemistry and transport. In the winter there is no apparent systematic diurnal variation in the O3 mixing ratio because there is little diurnal change of transport and a slow photochemistry. In the summer, the O3 levels at the site are suppressed at night due to the presence of a nocturnal inversion layer that isolated ozone near the surface, where it is destroyed. Ozone is observed to increase in the summer during the day. The increases in ozone correlate with increasing NO
x
levels, as well as with the levels of other compounds of anthropogenic origin. We interpret this correlation as in-situ or in-transit photochemical production of ozone from these precursors that are transported to our site. The levels of ozone recorded approach 100 ppbv at NO
x
mixing ratios of approximately 3 ppbv. Calculations made using a simple clean tropospheric chemical model are consistent with the NO
x
-related trend observed for the daytime ozone mixing ratio. However, the chemistry, which does not include nonmethane hydrocarbon photochemistry, underestimates the observed O3 production. 相似文献
63.
64.
Data of neutral meridional wind obtained by the meteor radar at Esrange and data of temperature and pressure measured by the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instrument on board the Thermosphere–Ionosphere–Mesosphere Energetics and Dynamics (TIMED) spacecraft were studied with respect to a day-to-day atmospheric variability with periods ranging from 1.5 to 5 days. The detailed analysis was carried out for February 2004. Perturbations of the atmospheric parameters at the examined periods appeared mainly as eastward-propagating waves of zonal wavenumbers 1 and 2. We suggested that these waves excited by the jet instability on both flanks of the polar-night jet in the upper stratosphere and mesosphere interact nonlinearly with each other, and this interaction generates secondary waves. The radar observed both primary and secondary waves at mesospheric heights. The data analysis supports this suggestion. Under conditions of weaker instability observed in February 2003 the perturbations of atmospheric parameters of periods ranging from 1.5 to 5 days had smaller amplitudes at heights of the mesosphere than those in February 2004. It was found that the Eliassen-Palm fluxes calculated for the waves generated by the jet instability were mainly downward directed. This result suggests a possible dynamical influence of the mesospheric layers on the lower atmospheric levels. 相似文献
65.
利用一个三维的冰雹云模式与化学组分输送模块耦合,得到云输送引起大气光化学组分的再分布,然后用一个包含详细气相化学反应机制的箱模式研究了云输送引起的气相体积分数的变化及其对大气化学系统产生的影响。结果表明,云输送后O3体积分数大于无云个例,但其后两天内两者的变化趋势相差不大;HNO3、NO2、NO3、PAN等的体积分数均明显高于无云个例,分别增长了87%、70%、62%和49%,其中NO2体积分数的增加主要由于云输送造成,而NO3、HNO3、PAN主要是输送对化学扰动的结果。两天内OH和HO2自由基体积分数比无云个例平均增长了13%和11%。 相似文献
66.
Two long time series were analysed: the C01 series of the International Earth Rotation Service and the pole series obtained
by re-analysis of the classical astronomical observations using the HIPPARCOS reference frame. The linear drift of the pole
was determined to be 3.31 ± 0.05 milliarcseconds/year towards 76.1 ± 0.80° west longitude. For the least-squares fit the a priori correlations between simultaneous pole coordinates x
p
, y
p
were taken into account, and the weighting function was calculated by estimating empirical variance components. The decadal
variations of the pole path were investigated by Fourier and wavelet analysis. Using sliding windows, the periods and amplitudes
of the Chandler wobble and annual wobble were determined. Typical periods in the variable Chandler wobble and annual wobble
parameters were obtained from wavelet analyses.
Received: 21 January 2000 / Accepted: 28 August 2000 相似文献
67.
NO, NOx, NOy and O3 have been measuredduring the airborne EXPRESSO experiment, November 96,which took place near Bangui (Central Africa) at thebeginning of the dry season. This period correspondsto an intense burning activity. Chemical andphotochemical characteristics of the planetaryboundary layer, which corresponds most of the time tothe monsoon layer, and the Harmattan layer, which issituated above the latter, have been studied forsavanna as well as rain forest areas. These two layersare very different when considering the chemicalcomposition (especially for ozone and NOz) andthe photochemical age.The relationship of photochemical ozone productionversus photochemical NOx oxidation products hasbeen investigated. Results indicate an ozoneproduction efficiency (OPE) ranging from 6.3 to 14.8in the planetary boundary layer. Thus, this layer ischaracteristic of a photochemically young and activeair mass. In this layer, the ozone potentialproduction increases with the air mass photochemicalage. On the other hand, the Harmattan layer shows anOPE ranging from 4.6 to 7.4. These values arecharacteristic of photochemically well-aged airmasses. In this layer, the ozone potential productionseems to be exhausted with values around 4.0 (i.e., 4ozone molecules produced for each NOx moleculeemitted). 相似文献
68.
Mohammed Ilyas Arunsala Pandy Mohd. Suhaimi Jaafar 《Journal of Atmospheric Chemistry》2001,40(2):111-121
The South-East Asian region experienced a haze episode in 1994 which was widely believed to be due to widespread forest fires in Sumatra and Kalimantan (Indonesia). Broadband measurements of the surface level solar ultraviolet-B, UV-A and Global radiation at Penang (Malaysia) are used to study the effect of the 1994 haze on effective UV-B irradiance. We find that during the haze episode, there is enhanced absorption of surface level UV-B radiation. The effect of haze on UV-A and Global radiation is much less. The reduction in absolute noon time UV-B irradiance (mostly cloud free) during the 1994 haze period was 23% relative to the UV-B irradiance during thecorresponding haze-free period in 1995. Even though the noon time radiation data minimizes the cloud effect in the results presented some cloud effect is still present. 相似文献
69.
Simple model flows demonstrating the combined effect of thermobaricity with either salinity variations or nonlinear temperature-dependence in the equation of state of water are investigated. An inviscid flow exhibits a three-layer behaviour, resulting in the formation of a mid-depth temperature maximum, such as is observed in some high-latitude oceans and deep lakes. This may be subsequently overtaken by nonlinear frontogenesis, which in the viscous case is shown to generate a thermal bar. Thermobaricity shifts the thermal bar towards the cold water, and initially produces a slope in the downwelling plume, but this transient feature disappears as the dominant frontogenesis tilts the plume back to the vertical. 相似文献
70.