天然气水合物体系动态演化研究（I）：地质历史演变     

宋海斌 《地球物理学进展》2003,18(2):188-196

1995年Dickens对55．5Ma前古新世末增温事件进行了研究，提出天然气水合物作为全球环境变化重要因子的假说．认为古新世末增温事件溶解无机碳-2～-3‰的^13δC位移可以用水合物所含甲烷的释放与随后氧化成二氧化碳来解释．此后，地质历史演变中的天然气水合物演化研究蓬勃发展，本文总结古新世末增温事件、新元古代末期雪球事件、第四纪千年尺度事件等最新进展，为天然气水合物动态演化研究提供基础．开展天然气水合物-天然气体系动态演化过程数值模拟与特征分析，可望促进天然气水合物在全球变化与碳循环中作用的深入认识．  相似文献   

Monitoring volcanic hazard using eddy covariance at Solfatara volcano, Naples, Italy     

C Werner  G Chiodini  D Voigt  S Caliro  R Avino  M Russo  T Brombach  J Wyngaard  S Brantley 《Earth and Planetary Science Letters》2003,210(3-4):561-577

An eddy covariance (EC) station was deployed at Solfatara crater, Italy, June 8–25, 2001 to assess if EC could reliably monitor CO₂ fluxes continuously at this site. Deployment at six different locations within the crater allowed areas of focused gas venting to be variably included in the measured flux. Turbulent (EC) fluxes calculated in 30-min averages varied between 950 and 4460 g CO₂ m⁻² d⁻¹; the highest measurements were made downwind of degassing pools. Comparing turbulent fluxes with chamber measurements of surface fluxes using footprint models in diffuse degassing regions yielded an average difference of 0% (±4%), indicating that EC measurements are representative of surface fluxes at this volcanic site. Similar comparisons made downwind of degassing pools yielded emission rates from 12 to 27 t CO₂ d⁻¹ for these features. Reliable EC measurements (i.e. measurements with sufficient and stationary turbulence) were obtained primarily during daytime hours (08:00 and 20:00 local time) when the wind speed exceeded 2 m s⁻¹. Daily average EC fluxes varied by ±50% and variations were likely correlated to changes in atmospheric pressure. Variations in CO₂ emissions due to volcanic processes at depth would have to be on the same order of magnitude as the measured diurnal variability in order to be useful in predicting volcanic hazard. First-order models of magma emplacement suggest that emissions could exceed this rate for reasonable assumptions of magma movement. EC therefore provides a useful method of monitoring volcanic hazard at Solfatara. Further, EC can monitor significantly larger areas than can be monitored by previous methods.  相似文献   

鄂尔多斯盆地苏里格庙与靖边天然气单体碳同位素特征及其成因   总被引：7，自引：1，他引：7  

付锁堂  冯乔  张文正 《沉积学报》2003,21(3):528-532,538

苏里格庙上古生界砂岩气藏天然气重烃含量高,干燥系数低,为湿气;靖边奥陶系风化壳气藏天然气重烃含量低,干燥系数高,属干气。苏里格庙天然气的正构烷烃碳同位素具有δ13 C₁<δ13 C₃ <δ13 C₂ <δ13 C4的规律,靖边天然气具有δ13 C₁<δ13 C₂ <δ13 C₃ 的规律。二者高碳数烷烃的同位素差别较大,尤其是苏里格庙的乙烷碳同位素比靖边平均重 3.6‰。根据天然气单体碳同位素及其含量变化,苏里格庙天然气属煤成气,靖边天然气属煤成气与油型气的混合气。苏里格庙和靖边天然气中均含少量CO₂ 气,其碳同位素表明苏里格庙除苏 5井为无机CO₂ 气外,均为有机CO₂ 气;靖边林 1、林 5井为无机CO₂ 气,陕参 1井为有机CO₂ 气。结合烷烃气和CO₂ 气,苏里格庙天然气可以分为含有机CO₂ 煤成气和含无机CO₂ 煤成气。碳同位素比值与Ro 关系分析认为,苏里格庙的天然气成熟度处于成熟到高成熟阶段,其相应气源岩的平均Ro 为 1.2 9%～ 1.39%,这一结果与该区二叠系煤岩的成熟度符合较好。  相似文献   

地史过程中烃源岩有机质丰度和生烃潜力变化的模拟计算   总被引：17，自引：0，他引：17  

卢双舫薛海涛  钟宁宁 《地质论评》2003,49(3):292-297

在同时考察源岩中有机质因生、排烃而损失和无机质因成岩作用而失重的基础上，模拟计算了地史过程中，随有机质类型、初始有机质丰度、成熟度及排烃效率的改变，烃源岩有机质丰度和生烃潜力的变化，探讨了有机碳恢复系数及生烃潜力损失率的可能变化范围。结果表明，地史过程中，有机质生烃潜力和有机质丰度的变化主要取决于源岩的生、排烃效率，对性质偏差的有机质，有机质的实测丰度随演化程度的增高不降反升；而对位于高成熟阶段的优质有机质，有机碳的恢复系数可达2以上；随有机质类型变好和成熟度升高，生烃潜力损失率增高；一般情况下，有机质生烃潜力的恢复幅度比有机质丰度的恢复大得多。  相似文献   

黑土的水土流失及其保育治理   总被引：10，自引：2，他引：10  

王其存  齐晓宁  王洋  刘兆永  鲍强 《地理科学》2003,23(3):361-365

黑土因其肥沃而闻名，但其退化和水土流失问题往往易被忽略。虽然在人类影响下的现代环境过程开始较晚，但黑土区的环境已发生了较大的变化。对黑土水土流失的现状进行了评价，指出了黑土保育治理的必要性与紧迫性，提出了治理保育措施。  相似文献   

Origin and Formational Environment of Noda-Tamagawa Manganese Ore, Northeast Japan: Constraints from Isotopic Studies     

Mohammed El Rhazi  Ken-ichiro Hayashi 《Chemie der Erde / Geochemistry》2003,63(2):149-162

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GMS卫星遥感中国地区气溶胶光学厚度   总被引：20，自引：2，他引：20       下载免费PDF全文

张军华  斯召俊  毛节泰  王美华 《大气科学》2003,27(1):23-35

讨论了利用GMS卫星遥感湖面上空气溶胶光学厚度的方法,根据在5个湖面附近与多波段光度计遥感结果的比较,对卫星遥感的方法和结果进行了检验,然后利用该方法遥感了中国大陆25个湖面上空气溶胶光学厚度.结果显示,利用卫星反演湖面光学厚度可以提供大陆上空气溶胶的信息,是研究大陆上空气溶胶光学厚度一个可行的方法.  相似文献   

The Global Distribution of Secondary Particulate Matter in a 3-D Lagrangian Chemistry Transport Model     

R. G. Derwent  W. J. Collins  M. E. Jenkin  C. E. Johnson  D. S. Stevenson 《Journal of Atmospheric Chemistry》2003,44(1):57-95

A global 3-D Lagrangian chemistry-transport model STOCHEM is used to describe the tropospheric distributions of four components of the secondary atmospheric aerosol: nitrate, sulphate, ammonium and organic compounds. The model describes the detailed chemistry of the formation of the acid precursors from the oxidation of SO₂, DMS, NO_x, NH₃ and terpenes and their uptake into the aerosol. Model results are compared in some detail with the available surface observations. Comparisons are made between the global budgets and burdens found in other modelling studies. The global distributions of the total mass of secondary aerosols have been estimated for the pre-industrial, present day and 2030 emissions and large changes have been estimated in the mass fractions of the different secondary aerosol components.  相似文献   

MODELING THE EFFECTS OF ANTHROPOGENIC SULFATE IN CLIMATE CHANGE BY USING A REGIONAL CLIMATE MODEL   总被引：3，自引：2，他引：3  

高学杰  林一骅  赵宗慈 《热带气象学报(英文版)》2003,9(2):173-180

1 INTRODUCTION Being an important composition of the atmosphere, aerosol attracts increasing attention from the scientific community in recent years, together with the radiative forcing it causes and effects it imposes on the climate system. The anthropogenic aerosol affects the climate both directly and indirectly. The climate is directly affected when solar shortwave radiation is scattered and absorbed in what is known as the 搖mbrella effect? which can be dated back to as early as mor…  相似文献   

大气气溶胶光学厚度的宽带消光遥感方法及其应用   总被引：6，自引：1，他引：6  

邱金桓 《遥感学报》1997,1(1):15-23

该文发展了遥感气溶胶光学厚度的一个宽带消光遥感方法 ,它应用地面上太阳直射表探测的宽波段太阳直射信息反演 0 75 μm大气柱光学厚度。这方法的主要误差因子是气溶胶谱的不确定性。数值试验表明 ,气溶胶谱分布的误差所引起光学厚度解的误差一般小于 5 %。 1995年 1— 10月进行的 12 6 7组对比实验表明 ,由本方法探测的气溶胶光学厚度与光度计探测的气溶胶光学厚度的标准差为 10 5 % ,两者平均结果的偏差只有 0 7%。该文还应用这个方法 ,从气象台站辐射观测资料反演得到北京、沈阳等 10个地方 1980— 1994年间晴天气溶胶光学厚度资料 ,并分析其变化规律  相似文献