Variations in chemical compositions of the eolian dust in Chinese Loess Plateau over the past 2.5 Ma and chemical weathering in the Asian inland   总被引：5，自引：0，他引：5  

CHEN Jun  LIU Lianwen  JI Junfeng  YANG Jiedong  CHEN Yang 《中国科学D辑(英文版)》2001,44(5):403-413

Major and trace elements as well as strontium isotopic composition have been analyzed on the acid-insoluble (AI) phase of the loess-paleosol sequence from Luochuan, Shaanxi Province, China. Results show that the chemical composition of AI phase of loess and paleosols is distinctive to the average composition of upper continental crust (UCC), characterized by depletion of mobile elements Na, Ca and Sr. The distribution pattern of elements in AI phase reveals that initial dust, derived from a vast area of Asian inland, has suffered from Na- and Ca-removed chemical weathering compared to UCC. Some geochemical parameters (such as CIA values, Na/K, Rb/Sr and⁸⁷Sr/⁸⁶Sr ratios) display a regular variation and evolution, reflecting that the chemical weathering in the source region of loess deposits has decreased gradually since 2.5 Ma with the general increase of global ice volume. This coincidence reflects that the aridity of Asian inland since the Quaternary is a possible regional response to the global climate change.  相似文献   

The aeolian dust accumulation curve     

Dirk Goossens 《地球表面变化过程与地形》2001,26(11):1213-1219

This article presents a simple physical concept of aeolian dust accumulation, based on the behaviour of the subprocesses of dust deposition and dust erosion. The concept is tested in an aeolian dust wind tunnel. The agreement between the accumulation curve predicted by the model and the accumulation curve obtained in the experiments is close to perfect and shows that it is necessary to discriminate between the processes of aeolian dust deposition and aeolian dust accumulation. Two important thresholds determine the accumulation process. For wind speeds below the deflation threshold, the aeolian accumulation of dust increases linearly with the wind speed. For wind velocities between the deflation threshold and the accumulation limit, the sedimentation balance is above unity and there is still accumulation, though it rapidly drops once the deflation threshold has been exceeded. At wind speeds beyond the accumulation limit, the sedimentation balance is below unity and there will no longer be an accumulation of dust. The thresholds have been determined in a wind tunnel test at friction velocity u_* = 0·34 m s^?1 (deflation threshold) and u_* = 0·43 m s^?1 (accumulation limit), but these values are only indicative since they depend heavily on the characteristics of the accumulation surface and of the airborne grains. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献   

Atmospheric pollution assessment near potential source of natural aerosols in the South Gobi Desert region,China     

Mikalai Filonchyk  Volha Hurynovich  Shuwen Yang 《地理信息系统科学与遥感》2020,57(2):227-244

ABSTRACT

Rapid economic growth, a high degree of urbanization and the proximity of a large number of desert and semidesert landscapes can have a significant impact on the atmosphere of adjacent territories, leading to high levels of atmospheric pollution. Therefore, identifying possible sources of atmospheric pollution is one of the main tasks. In this study, we carried out an analysis of spatial and temporal characteristics of five main atmospheric pollutants (PM_2.5, PM₁₀, SO₂, NO₂, and CO) near potential source of natural aerosols, affecting seven cities (Wuhai, Alashan, Wuzhong, Zhongwei, Wuwei, Jinchang, Zhangye), located in immediate proximity to the South Gobi deserts. The results, obtained for the period from 1 January 2016 to 31 December 2018, demonstrate total concentrations of PM_2.5 and PM₁₀ are 38.2 ± 19.5 and 101 ± 80.7 μg/m³ exceeding the same established by the Chinese National Ambient Air Quality Standard (CNAAQS), being 35 and 70 μg/m³, respectively. Based on the data from Moderate Resolution Imaging Spectroradiometer (MODIS) for the whole period, Clean Сontinental (71.49%) and Mixed (22.29%) types of aerosols prevail in the region. In the spring and winter seasons maximum concentrations of pollutants and high values of Aerosol Optical Depth (AOD) in the region atmosphere are observed. PM_2.5 and PM₁₀ ratio shows the presence of coarse aerosols in the total content with value 0.43. The highest concentrations of pollutants were in the period of dust storms activity, when PM_2.5 and PM₁₀ content exceeded 200 and 1000 µg/m³, and AOD value exceeded 1. UV Aerosol Index (UVAI), Aerosol Absorbing Optical Depth (AAOD), and Single Scattering Albedo (SSA), obtained from Ozone Monitoring Instrument (OMI), demonstrate the high content of dust aerosols in the period of sandstorms. Analysis of backward trajectories shows that dust air masses moved from North to Northwest China, affecting large deserts such as Taklamakan, Gurbantunggut, Badain Jaran, Tengger, and Ulan Buh deserts.  相似文献   

具有尘带的椭圆星系的红外辐射特性     

胡景耀  王钢 《中国天文和天体物理学报》1988,(1)

IRAS在12,25,60和100μm的巡天,给我们提供了研究各类星系红外辐射特性的可能。为了研究具有尘带的E和SO星系的红外辐射特性,我们利用了E.Sadler给出的完备的E和SO星系表。在该星系表中共列出248个夭体,其中38个被证记为IRAS点源,且又有确切的60和100μm的流量值。在这38个天体中有6个被列在K.Ebneter和B.Balik最新发表的具有全带的椭圆星系表中。我们以这6个星系作为具有尘带的E和SO星系的样本,其它32个没有尘带的E和SO星系即作为对照样本。为了讨论具有尘带的椭圆星系的红外辐射特性,我们利用非参数Mann-Whitney检验,对这两个样本的LIR和FIR/FB的分布作了讨论,结果是在对于置信度α=0.05的水平上,我们不能拒绝另一假设:这两个样本的LIR和FIR/FB的分布是相同的。对于同时具有25,60和100μm确切流量的E和SO星系我们讨论了它们的双色图,结果发现,不具尘带的E和SO星系都处于Rowan-Robinson.et al所指出的正常星系区,而一些具有尘和带的ESO星系,则远离这一区域,它们是LINER和SEYFERT星系。  相似文献   

Gas and Particulate Products Distribution from the Photooxidation of α-Humulene in the Presence of NOx, Natural Atmospheric Air and Sunlight     

M. Jaoui  R. M. Kamens 《Journal of Atmospheric Chemistry》2003,46(1):29-54

The photooxidation of -humulene in the presence of NO_x, natural sunlight, and rural background air was investigated using a combination of gas chromatography-mass spectrometry (GC-MS) and high performance liquid chromatography (HPLC). Identification and quantification of gas and particulate reaction products were reported over the course of the reaction. The daytime photooxidation was carried out in a large outdoor smog chamber (190 m³). A wide range of ring retaining and ring opening products in the gas and particle phase are reported. On average, measured gas and particle phase products accounted for 44% of the reacted -humulene carbon. Measurements show that a number of reaction products with low vapor pressures (e.g. 3-seco--humulone aldehyde, 7-seco--humulone aldehyde, -humulal aldehyde, -humulene 3-oxide or -humulene 7-oxide, -humulaic/alic acid isomers, and 3-seco--14-hydroxyhumulone aldehyde) were found in the early stage of the reaction and may play an important role in the early formation of secondary organic aerosol. A detailed mechanism is proposed to account for most products observed in this investigation.  相似文献   

平流层和中层大气研究的进展   总被引：16，自引：4，他引：12  

吕达仁  陈洪滨 《大气科学》2003,27(4):750-769

平流层和中层大气研究是20世纪70年代以来持续得到大气科学界和日地物理界共同关注的研究前沿.中国科学界在文化大革命结束后立即抓住这一前沿作为发展重点之一.20多年来,中国科学院大气物理研究所等单位较为系统地开展了这一方向的研究,并在一些方面进行了前沿性的工作.作者着重介绍以下几方面的进展:(1)平流层和中层大气探测设施与探测方法;(2)大气臭氧、平流层气溶胶的监测与分析;(3)行星波在中层大气环流与大气臭氧分布中的作用;(4)重力波在中层大气的传播特征与作用;(5)平流层-对流层交换的动力物理与化学问题.  相似文献   

Oxygen isotope compositions of quartz grains (4–16 μm) from Chinese eolian deposits and their implications for provenance     

Shengshan?HouEmail author  Shiling?Yang  Jimin?Sun  Zhongli?Ding 《中国科学D辑(英文版)》2003,46(10):1003-1011

Oxygen isotope compositions were measured in quartz grains extracted from a 7.0 Ma red clay-loess sequence at Lingtai and six late Pleistocene loess sediments (Malan loess). Results show that the changes in oxygen isotope compositions of Malan loess are basically controlled by the geochemical characteristics of the source materials, while the effect of weathering process after dust deposition could be minor. The oxygen isotope distribution of quartz grains from red clay at Lingtai is similar to that of the overlying loess-paleosol sequence, thus indicating that the red clay at Lingtai has the same eolian origin as the loess-paleosol deposits. Furthermore, the oscillations of the isotope compositions in 4–16 μm-sized quartz grains may reflect the changes, to some extent, of the climatic systems of the source region.  相似文献   

Solar ultraviolet transfer in the Martian atmosphere: biological and geological implications     

C Córdoba-Jabonero  L.M LaraA.M Mancho  A MárquezR Rodrigo 《Planetary and Space Science》2003,51(6):399-410

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Aging of Titan's Aerosols     

Vasili DimitrovAkiva Bar-Nun 《Icarus》2002,156(2):530-538

Titan's haze is composed of aerosols containing long chain polymers of acetylene with some hydrogen cyanide. These polymers have alternating double/single and triple/single bonds, which can open spontaneously or under the action of UV radiation or particle impact. Once opened, they can induce the opening of a double or triple bond in an adjacent chain and link to it. This cross-linking and chain elongation hardens or “ages” the polymer particles, making them less sticky. As observed experimentally and calculated theoretically, newly formed polymer particles grow by collecting other polymer chains and by complete merging into symmetrical spheres. However, when aged, they merely adhere to each other and do not merge. Eventually, when hard enough, they do not even adhere to each other. In this paper we calculate the spontaneous aging process as applied to Titan's atmospheric conditions and find that the surface tension and viscosity of the aerosols below H∼570 km are one order of magnitude harder than when the aerosols formed. Furthermore, UV irradiation and particle impacts reduce both viscosity and surface tension by an additional factor of 10-100. Thus, the aerosol particles expected to be encountered by the descending Huygens probe will, most likely, be quite hard.  相似文献   

Biomass Burning in Southern Africa: Individual Particle Characterization of Atmospheric Aerosols and Savanna Fire Samples   总被引：2，自引：0，他引：2  

Xiande Liu  Piet Van Espen  Freddy Adams  Jan Cafmeyer  Willy Maenhaut 《Journal of Atmospheric Chemistry》2000,36(2):135-155

Ambient atmospheric aerosols and savanna fireparticulate emission samples from southern Africa werecharacterised in terms of particle classes and theirnumber abundance by electron probe X-ray microanalysis(EPXMA). About ten particle classes were identifiedfor each sample. The major classes werealuminosilicates and sea salts for ambient coarse(2–10 m equivalent aerodynamic diameter (EAD))samples, and K-S and S-only particles for ambient fine(<2 m EAD) samples. The K-S particles are oneof the major products of biomass burning. The EPXMAresults were found to be consistent with the resultsfrom bulk analyses on a sample by sample basis. Forsavanna fire fine samples, quantitative EPXMA revealedthat many particles had a composition of simple saltssuch as KCl. Some particles had a deviatingcomposition in the sense that more ionic species wereinvolved in sustaining the balance between cations andanions, and they were composite or mixed salts.Because of extensive processing during the atmospherictransport, the composition of the K-S particles in theambient samples was different from K₂SO₄,and such particles were enriched with S. The finepyrogenic KCl particles and the fine sea-saltparticles were much depleted in chlorine.  相似文献