Quantifying the Response Strength of the Southern Stratospheric Polar Vortex to Indian Ocean Warming in Austral Summer简     

LI Shuanglin  CHEN Xiaoting 《大气科学进展》2014,31(2):492-503

A previous multiple-AGCM study suggested that Indian Ocean Warming （IOW） tends to warm and weaken the southern polar vortex.Such an impact is robust because of a qualitative consistency among the five AGCMs used.However,a significant difference exists in the modeled strengths,particularly in the stratosphere,with those in three of the AGCMs （CCM3,CAM3,and GFS） being four to five times as strong as those in the two other models （GFDL AM2,ECHAM5）.As to which case reflects reality is an important issue not only for quantifying the role of tropical ocean warming in the recent modest recovery of the ozone hole over the Antarctic,but also for projecting its future trend.This issue is addressed in the present study through comparing the models＇ climatological mean states and intrinsic variability,particularly those influencing tropospheric signals to propagate upward and reach the stratosphere.The results suggest that differences in intrinsic variability of model atmospheres provide implications for the difference.Based on a comparison with observations,it is speculated that the impact in the real world may be closer to the modest one simulated by GFDL AM2 and ECHAM5,rather than the strong one simulated by the three other models （CCM3,CAM3 and GFS）.In particular,IOW during the past 50 years may have dynamically induced a 1.0℃ warming in the polar lower stratosphere （～100 hPa）,which canceled a fraction of radiative cooling due to ozone depletion.  相似文献   

北半球平流层臭氧的时空分布特征   总被引：3，自引：0，他引：3  

黄仪方  郭世昌  陈辉  秦瑜  吴涧 《成都信息工程学院学报》2001,16(1):8-11

利用1963－1985年北半球的平流层臭氧观测资料，采用自然平交分解方法，初步分析了北半球、特别是东亚地区大气臭氧层的时空分布特征。结果表明：（1）北半球大气臭氧的空分间分布可能与下垫面的性能有关；（2）东亚地区大气臭氧的时间分布主要具有2年和11年变化的周期特征，这与太阳黑子的准2年和准11年变化有一定的对应关系；（3）北美地区的臭氧变化则主要包含4年和7年的周期变经成分。  相似文献   

武汉市2018年4—9月臭氧及其前体物非线性关系研究     

陈安雄  胡柯  沈龙娇  钟章雄  段佳鹏  汪羽商  陈文泰 《南京气象学院学报》2020,12(6):729-738

近年来武汉市臭氧污染日益严峻,成为影响空气质量达标的瓶颈,弄清臭氧及其前体物非线性关系是臭氧防控的关键和基础.本研究基于武汉中心城区2018年4—9月臭氧及其前体物在线观测数据,分析出武汉市臭氧浓度受前体物和气象条件等因素的共同影响,呈较为明显的季节变化和日变化特征.观测期间武汉市大气挥发性有机物（VOCs）平均体积分数为32.5×10^-9,烷烃是武汉市VOCs的主要组分,其次是含氧VOCs （OVOCs）和卤代烃.利用基于观测的模型定量分析臭氧与前体物之间的关系,发现削减VOCs会引起臭氧生成潜势的显著下降,而削减氮氧化物则会使臭氧生成潜势升高,说明武汉市臭氧生成处于VOCs控制区.在人为源VOCs中,间/对二甲苯和邻二甲苯的相对增量反应活性（RIR）最高,是影响臭氧生成的关键组分.  相似文献   

未来甲烷排放增加对平流层水汽和全球臭氧的影响   总被引：3，自引：0，他引：3  

谢飞  田文寿  李建平  张健恺  商林 《气象学报》2013,71(3):555-567

利用一个耦合的大气化学-气候模式(WACCM3)研究了地表甲烷排放增加对平流层水汽和全球臭氧变化的影响.结果表明,如果地表甲烷的排放量在2000年的基础上增加50%(达到政府间气候变化专门委员会A1B排放情景中2050年的值),平流层水汽体积分数将平均增加约0.8×10^-6.南半球平流层甲烷转化为水汽的效率比北半球高.在北半球平流层中,1mol甲烷分子可以转化为约1.63mol的水汽分子,而在南半球1mol甲烷分子大概可以转化为约1.82mol的水汽分子.甲烷排放增加50%将使全球中低纬度地区以及北半球高纬度地区的臭氧柱总量增加1%-3%,使南半球高纬度地区臭氧柱总量增加近8%,而秋季(南半球春季)南极地区臭氧柱总量增加幅度可高达20%,南极臭氧的这种显着增加主要是由于甲烷增加造成的化学反馈所致.在北半球中高纬度地区,甲烷增加引起的臭氧变化主要与甲烷氧化导致的水汽增加有关.研究还表明,未来甲烷排放增加对臭氧的恢复作用其实与溴化物排放的减少一样重要.  相似文献   

An intercomparison of two rawinsonde systems     

G.A. McBean  D.J. Phillips  J.R. Mathieson 《大气与海洋》2013,51(1):42-51

Abstract

An intercomparison of the Väisälä MicroCora system used in the Automated Shipboard Aerological Program (ASAP) and the Atmospheric Environment Service upper‐air system (GMD/ADRES) was conducted in May‐June 1983. Thirty‐three paired ascents were made. The ASAP system dry‐bulb temperatures averaged 0.3°C warmer. For the lowest 100 mb, the dew‐point temperature difference (ASAP ‐ GMD/ADRES) was near ‐1°C whereas for the 780–500 mb layer, the difference was 1°C. The wind component mean differences averaged were small but with a 4 m s^?1 standard deviation.  相似文献   

Numerical Simulation Study on the Impacts of Tropospheric O3 and CO2 Concentration Changes on Winter Wheat.Part I: Model Description          下载免费PDF全文

ZHENG Changling  WANG Chunyi 《Acta Meteorologica Sinica》2006,20(1):109-116

Ozone is well documented as the air pollutant most damaging to agricultural crops and other plants.It is reported that tropospheric O3 concentration increases rapidly in recent 20 years. Evaluating and predicting impacts of ozone concentration changes on crops are drawing great attention in the scientific community. In China, main study method about this filed is controlled experiments, for example, Open Top Chambers. But numerical simulation study about impacts of ozone on crops with crop model was developed slowly, what is more, the study about combined impacts of ozone and carbon dioxide has not been reported.The improved agroecosystem model is presented to evaluate simultaneously impacts of tropospheric O3 and CO2 concentration changes on crops in the paper by integrating algorithms about impacts of ozone on photosynthesis with an existing agroecosystem biogeochemical model (named as DNDC). The main physiological processes of crop growth (phenology, leaf area index, photosynthesis, respiration, assimilated allocation and so on) in the former DNDC are kept. The algorithms about impacts of ozone on photosynthesis and winter wheat leaf are added in the modified DNDC model in order to reveal impacts of ozone and carbon dioxide on growth, development, and yield formation of winter wheat by coupling the simulation about impacts of carbon dioxide on photosynthesis of winter wheat which exists in the former DNDC. In the paper, firstly assimilate allocation algorithms and some genetic parameters (such as daily thermal time of every development stage) were modified in order that DNDC can be applicable in North China. Secondly impacts of ozone on crops were simulated with two different methods-one was impacts of ozone on light use efficiency , and the other was direct effects of ozone on leaves photosynthesis. The latter simulated results are closer to experiment measurements through comparing their simulating results. At last the method of direct impacts of ozone on leaf growth is adopted and the coe cients about impacts of ozone on leaf growth and death are ascertained. Effects of climate changes, increasing ozone, and carbon dioxide concentration on agroecosystem are tried to be simulated numerically in the study which is considered to be advanced and credible.  相似文献   

Some observations on the effect of ozone treatment on suspended particulate matter in seawater     

Hasong Pak  James Kitchen  Percy Donaghay  J. Ronald  V. Zaneveld 《Estuarine, Coastal and Shelf Science》1981,13(3):327-336

  相似文献   

Urban Atmospheric Chemistry During the PUMA Campaign 2: Radical Budgets for OH,HO<Subscript>2</Subscript> and RO<Subscript>2</Subscript>   总被引：1，自引：0，他引：1  

K.?M.?Emmerson  N.?CarslawEmail author  M.?J.?Pilling 《Journal of Atmospheric Chemistry》2005,52(2):165-183

A detailed photochemical box model was used to investigate the key reaction pathways between OH, HO₂ and RO₂ radicals during the summer and winter PUMA field campaigns in the urban city-centre of Birmingham in the UK. The model employed the most recent version of the Master Chemical Mechanism and was constrained to 15-minute average measurements of long-lived species determined in situ at the site. The results showed that in the summer, OH initiation was dominated by the reactions of ozone with alkenes, nitrous acid (HONO) photolysis and the reaction of excited oxygen atoms atoms with water. In the winter, ozone+alkene reactions were the primary initiation route, with a minor contribution from HONO photolysis. Photolysis of aldehydes was the main initiation route for HO₂, in both summer and winter. RO₂ initiation was dominated by the photolysis of aldehydes in the summer with a smaller contribution from ozone+alkenes, a situation that was reversed in the winter. At night, ozone+alkene reactions were the main radical source. Termination, under all conditions, primarily involved reactions with NO (OH) and NO₂ (OH and RCO₃). These results demonstrate the importance of ozone+alkene reactions in urban atmospheres, particularly when photolysis reactions were less important during winter and at nighttime. The implications for urban atmospheric chemistry are discussed.  相似文献   

The Tambora eruption in 1815 provides a test on possible global climatic and chemical perturbations in the past     

R. K. R. Vupputuri 《Natural Hazards》1984,5(1):1-16

A coupled one-dimensional radiative-convective-photochemical diffusion model, which takes into account the influence of ocean inertia on global radiative perturbations is used to investigate the possible climatic and other atmospheric effects of a major volcanic eruption, thought to be similar in magnitude to that of the Tambora eruption, Indonesia, which took place in 1815. A volcanic cloud was introduced in the model stratosphere between 20–25 km and the global average peak aerosol optical thickness was assumed to be 0.25. Both the aerosol optical thickness and aerosol composition, which determine the optical properties, were allowed to vary in the model atmosphere during the life cycle of the volcanic cloud. The results indicate that the global average surface temperature decreases steadily from the date of eruption (7–12 April 1815) with maximum cooling of 1° K occurring in the spring of 1816. The calculations also show significant warming of the stratosphere, with temperature increasing up to 15° K at 25 km in less than six months after the date of eruption. The important effects of the Tambora eruption on stratospheric ozone and UV-B radiation at the surface are also mentioned.  相似文献   

NO<Subscript><Emphasis Type="Italic">x</Emphasis></Subscript> change over China and its influences   总被引：2，自引：0，他引：2  

LIU Yu  I. S. A. ISAKSEN  J. K. SUNDET  HE Jinhai  YAN Peng 《大气科学进展》2004,21(1):132-140

A 3-D chemical transport model (OSLO CTM2) is used to investigate the impact of the increase of NOx emission over China. The model is capable to reproduce basically the seasonal variation of surface NOx and ozone over eastern China. NOx emission data and observations reveal that NOx over eastern China increases quite quickly with the economic development of China. Model results indicate that NOx concentration over eastern China increasingly rises with the increase of NOx emission over China, and accelerates to increase in winter. When the NOx emission increases from 1995 to its double, the ratio of NO2/NOx abruptly drops in winter over northern China. Ozone at the surface decreases in winter with the continual enhancement of the NOx level over eastern China, but increases over southern China in summertime. It is noticeable that peak ozone over northern China increases in summer although mean ozone changes little. In summer, ozone increases in the free troposphere dominantly below 500 hPa.Moreover, the increases of total ozone over eastern China are proportional to the increases of NOx emission.In a word, the model results suggest that the relationship between NOx and ozone at the surface would change with NOx increase.  相似文献