全文获取类型
收费全文 | 419篇 |
免费 | 81篇 |
国内免费 | 171篇 |
专业分类
测绘学 | 3篇 |
大气科学 | 221篇 |
地球物理 | 62篇 |
地质学 | 242篇 |
海洋学 | 64篇 |
天文学 | 8篇 |
综合类 | 20篇 |
自然地理 | 51篇 |
出版年
2024年 | 3篇 |
2023年 | 4篇 |
2022年 | 7篇 |
2021年 | 14篇 |
2020年 | 14篇 |
2019年 | 22篇 |
2018年 | 15篇 |
2017年 | 15篇 |
2016年 | 19篇 |
2015年 | 24篇 |
2014年 | 39篇 |
2013年 | 26篇 |
2012年 | 14篇 |
2011年 | 29篇 |
2010年 | 22篇 |
2009年 | 36篇 |
2008年 | 32篇 |
2007年 | 31篇 |
2006年 | 40篇 |
2005年 | 28篇 |
2004年 | 24篇 |
2003年 | 24篇 |
2002年 | 14篇 |
2001年 | 16篇 |
2000年 | 23篇 |
1999年 | 19篇 |
1998年 | 18篇 |
1997年 | 13篇 |
1996年 | 9篇 |
1995年 | 11篇 |
1994年 | 11篇 |
1993年 | 8篇 |
1992年 | 10篇 |
1991年 | 5篇 |
1990年 | 7篇 |
1989年 | 5篇 |
1988年 | 5篇 |
1987年 | 1篇 |
1986年 | 3篇 |
1985年 | 2篇 |
1984年 | 5篇 |
1983年 | 1篇 |
1980年 | 2篇 |
1978年 | 1篇 |
排序方式: 共有671条查询结果,搜索用时 31 毫秒
71.
In this study,the mechanisms underlying the decadal variability of late spring precipitation in South China are investigated by using the latest Community Earth System Model version 1 (CESM1).We aim to unravel the effects of different climate forcing agents such as aerosols and greenhouse gases (GHGs) on the decadal variation of precipitation,based on transient experiments from pre-industry (for year 1850) to present-day (for year 2000).Our results reveal that:(1) CESM1 can reproduce the climatological features of atmospheric circulation and precipitation for the late spring in South China; (2) only simulations including the forcing of anthropogenic aerosols can reproduce the observed decreasing trend of late spring precipitation from 1950-2000 in South China; (3) aerosols affect the decadal change of precipitation mainly by altering the large-scale atmospheric circulation,and to a less extent by increasing the lower-tropospheric stability to inhibit the convective precipitation; and (4) in comparison,other climate forcing agents such as GHGs have much smaller effects on the decadal change of spring precipitation in South China. 相似文献
72.
湿法浸取硫酸镍工艺研究中,净化提纯工艺采取了蒸发浓缩浸液、分步沉淀杂质的技术方案。中试表明,采用此种工艺生产效率很低,还导致生产流水线上的设备匹配性差。为此,作者提出了二次浸取的技术方案。实验室及中试试验表明:采用二次浸取工艺替代蒸发浓缩工艺,行之有效。 相似文献
73.
南海北部海区海底沉积物中孔隙水的Cl~-和SO_4~(2-)浓度异常特征及其对天然气水合物的指示意义 总被引:41,自引:9,他引:32
报道了中国南海北部海区海底沉积物中孔隙水的Cl-和SO42-质量浓度的变化特征, 圈定了孔隙水中Cl-质量浓度的高值异常区。由于水合物形成过程中的排盐效应, 会使其上覆浅表层沉积物中孔隙水的盐度增高, 因此这些氯离子的高值异常区值得进一步的勘查。对孔隙水中SO42-的质量浓度分析表明, 研究区的一些站位表现出随深度增加SO42-的质量浓度梯度发生明显的变化, 计算的硫酸盐甲烷交接带SMI界面深度均在 10m左右, 与ODP164航次和ODP204航次有天然气水合物的钻孔的SMI界面深度基本吻合, 说明这些站位深部有天然气水合物存在的可能性。 相似文献
74.
Guangyou?ZhuEmail author Shuichang?Zhang Yingbo?Liang Jinxing?Dai Jian?Li 《中国科学D辑(英文版)》2005,48(11):1960-1971
The northeastern area of Sichuan Basin, southwestern China, is the area with the maximal reserve of natural gas containing
higher hydrogen sulphide (H2S) that has been found among the petroliferous basins of China, with the proven and controlled gas reserve of more than 200
billion cubic meters. These gas pools, with higher H2S contents averaging 9%, some 17%, are mainly distributed on structural belts of Dukouhe, Tieshanpo, Luojiazhai, Puguang,
etc., while the oolitic-shoal dolomite of the Triassic Feixianguan Fm. (T1f) is the reservoir. Although many scholars regard the plentiful accumulation of H2S within the deep carbonate reservoir as the result of Thermochemical Sulfate Reduction (TSR), however, the process of TSR
as well as its residual geological and geochemical evidence is still not quite clear. Based on the carbon isotopic analysis
of carbonate strata and secondary calcite, etc., together with the analysis of sulfur isotopes within H2S, sulphur, gypsum, iron pyrites, etc., as well as other aspects including the natural gas composition, carbon isotopes of
hydrocarbons reservoir petrology, etc., it has been proved that the above natural gas is a product of TSR. The H2S, sulphur and calcite result from the participation of TSR reactions by hydrocarbon gas. During the process for hydrocarbons
being consumed due to TSR, the carbons within the hydrocarbon gas participate in the reactions and finally are transferred
into the secondary calcite, and become the carbon source of secondary calcite, consequently causing the carbon isotopes of
the secondary calcite to be lower (−18.2‰). As for both the intermediate product of TSR, i.e. sulfur, and its final products,
i.e. H2S and iron pyrites, their sulfur elements are all sourced from the sulfate within the Feixianguan Fm. During the fractional
processes of sulfur isotopes, the bond energy leads to the 32S being released firstly, and the earlier it is released, the lower δ 34S values for the generated sulphide (H2S) or sulfur will be. However, for the anhydrite that participates in reactions, the higher the reaction degree, the more
32S is released, while the less 32S remains and the more δ 34S is increased. The testing results have proved the process of the dynamic fractionation of sulfur isotopes. 相似文献
75.
R. K. R. Vupputuri 《Natural Hazards》1984,5(1):1-16
A coupled one-dimensional radiative-convective-photochemical diffusion model, which takes into account the influence of ocean inertia on global radiative perturbations is used to investigate the possible climatic and other atmospheric effects of a major volcanic eruption, thought to be similar in magnitude to that of the Tambora eruption, Indonesia, which took place in 1815. A volcanic cloud was introduced in the model stratosphere between 20–25 km and the global average peak aerosol optical thickness was assumed to be 0.25. Both the aerosol optical thickness and aerosol composition, which determine the optical properties, were allowed to vary in the model atmosphere during the life cycle of the volcanic cloud. The results indicate that the global average surface temperature decreases steadily from the date of eruption (7–12 April 1815) with maximum cooling of 1° K occurring in the spring of 1816. The calculations also show significant warming of the stratosphere, with temperature increasing up to 15° K at 25 km in less than six months after the date of eruption. The important effects of the Tambora eruption on stratospheric ozone and UV-B radiation at the surface are also mentioned. 相似文献
76.
77.
The potential resources on the ion-stimulated syntheses effects of aerosol particles of lower troposphere in test sites in the arctic, mountain, arid and forest areas as the function of irradiation time and gas-precursor concentration were experimentally and theoretically evaluated. The dust-free outdoor air was irradiated with an ionization current of 10− 6 A by α-rays from isotope 239Pu. The total output of radiolytic aerosols (RA) with a diameter of 3–1000 nm was found to be 0.05–0.1 molecules per 1 eV of absorbed radiation, while the physical upper limit is 0.25–0.4 molecules/eV. In an interval of exposition time from 6 to 800 s (adsorbed energy is 3 · 1012–1014 eV/cm3) the RA mass concentration at different sites was increased from 1–10 to 50–500 μg/m3. According to the liquid chromatography data the major RA material is the H2O/HNO3 solution with acid concentration 25%. The used physical model presents new aerosols as a product from small and intermediate ion association through formation of neutral clusters and describes adequately some of the peculiarities in field experiment data. Introducing SO2, NH3, and also hydrochloric, nitric and sulphuric acid vapours with concentration 0.1–1 mg/m3 in the irradiated air stimulated an increase of mass aerosol concentration by a factor of 8–30. The mean size also decreased by a factor of 3–5. These facts allowed us to expect that the chemical composition of radiolytic aerosols generated in outdoor air would noticeably differ after addition of the gas-precursors. 相似文献
78.
含铬废水具有有机物含量高,难降解物质浓度高,色度大,悬浮物多,水质、水量变化大,含有微量毒性物质等特点。本文探讨了在不同参数条件下,硫酸亚铁、铁、硫化亚铁三种还原剂对含铬废水处理效果的影响,实验表明:硫酸亚铁具有明显的优越性,在同等条件下其去除率达到99%以上。 相似文献
79.
P. D. Safai S. Kewat G. Pandithurai P. S. Praveen K. Ali S. Tiwari P. S. P. Rao K. B. Budhawant S. K. Saha P. C. S. Devara 《Journal of Atmospheric Chemistry》2008,61(2):101-118
Simultaneous measurements on physical, chemical and optical properties of aerosols over a tropical semi-arid location, Agra
in north India, were undertaken during December 2004. The average concentration of total suspended particulates (TSP) increased
by about 1.4 times during intense foggy/hazy days. Concentrations of SO4
2−, NO3
−, NH4
+ and Black Carbon (BC) aerosols increased by 4, 2, 3.5 and 1.7 times, respectively during that period. Aerosols were acidic
during intense foggy/hazy days but the fog water showed alkaline nature, mainly due to the neutralizing capacity of NH4 aerosols. Trajectory analyses showed that air masses were predominantly from NW direction, which might be responsible for
transport of BC from distant and surrounding local sources. Diurnal variation of BC on all days showed a morning and an evening
peak that were related to domestic cooking and vehicular emissions, apart from boundary layer changes. OPAC (Optical properties
of aerosols and clouds) model was used to compute the optical properties of aerosols. Both OPAC-derived and observed aerosol
optical depth (AOD) values showed spectral variation with high loadings in the short wavelengths (<1 μm). AOD value at 0.5 μm
wavelength was significantly high during intense foggy/hazy days (1.22) than during clear sky or less foggy/hazy days (0.63).
OPAC-derived Single scattering albedo (SSA) was 0.84 during the observational period, indicating significant contribution
of absorbing aerosols. However, the BC mass fraction to TSP increased by only 1% during intense foggy/hazy days and thereby
did not show any impact on SSA during that period. A large increase was observed in the shortwave (SW) atmospheric (ATM) forcing
during intense foggy/hazy days (+75.8 W/m2) than that during clear sky or less foggy/hazy days (+38 W/m2), mainly due to increase in absorbing aerosols. Whereas SW forcing at surface (SUF) increased from −40 W/m2 during clear sky or less foggy/hazy days to −76 W/m2 during intense foggy/hazy days, mainly due to the scattering aerosols like SO4
2-. 相似文献
80.
中国区域气溶胶对东亚夏季风的可能影响(Ⅱ):黑碳气溶胶及其与硫酸盐气溶胶的综合影响 总被引:8,自引:0,他引:8
利用NCAR的新一代GCM CAM3.0模式耦合一个气溶胶同化系统,研究了中国区域黑碳气溶胶的直接气候效应。结果显示,中国区域黑碳气溶胶引起全球平均辐射强迫为0.13 W/m2,导致除了青藏高原和广西以外的中国大部分地区降温,其中东北、四川和内蒙古中北部降温最显著。由此造成海陆温差缩小,气压差降低,从而总体上使东亚夏季风减弱。但与硫酸盐气溶胶的影响相比,黑碳气溶胶使季风减弱的程度较小,长江中下游地区的降水有所增加。黑碳气溶胶加强了中国东南部地区的对流活动,这与硫酸盐气溶胶的作用相反。同时,探讨了中国区域硫酸盐和黑碳气溶胶的综合直接气候效应。结果表明,硫酸盐和黑碳气溶胶的综合作用与仅有硫酸盐气溶胶的情形十分相似,降水变化的区域也和硫酸盐的保持一致。 相似文献