金沙本底站空气质量与颗粒物浓度变化特征分析     

吴栋桥  周登 《气象科学进展》2021,(1)

利用华中区域代表性站点金沙国家大气本底站2007—2018年的PM_2.5、PM₁₀颗粒物质量浓度数据,2019年3月—2019年6月反应性气体数据,对华中区域空气质量进行整体评价,并分析了颗粒物浓度的变化特征及其影响因素。结果表明,反应性气体CO、SO₂、NO、NO₂质量浓度其日平均最大值、平均值均达到一级标准,O₃日平均值超标率为10.6%,PM_2.5超标率为18%,PM₁₀超标率为17%。从颗粒物质量浓度多年变化来看,2007—2013年金沙站大气颗粒物质量浓度属于上升趋势,2013年至今质量浓度呈现下降趋势,风向风速也在一定程度上影响颗粒物的来源。  相似文献   

Seasonal variations of atmospheric sulfur dioxide and dimethylsulfide concentrations at Amsterdam Island in the southern Indian Ocean     

J. P. Putaud  N. Mihalopoulos  B. C. Nguyen  J. M. Campin  S. Belviso 《Journal of Atmospheric Chemistry》1992,15(2):117-131

Daily measurements of atmospheric sulfur dioxide (SO₂) concentrations were performed from March 1989 to January 1991 at Amsterdam Island (37°50 S–77°30 E), a remote site located in the southern Indian Ocean. Long-range transport of continental air masses was studied using Radon (²²²Rn) as continental tracer. Average monthly SO₂ concentrations range from less than 0.2 to 3.9 nmol m^-3 (annual average = 0.7 nmol m^-3) and present a seasonal cycle with a minimum in winter and a maximum in summer, similar to that described for atmospheric DMS concentrations measured during the same period. Clear diel correlation between atmospheric DMS and SO₂ concentrations is also observed during summer. A photochemical box model using measured atmospheric DMS concentrations as input data reproduces the seasonal variations in the measured atmospheric SO₂ concentrations within ±30%. Comparing between computed and measured SO₂ concentrations allowed us to estimate a yield of SO₂ from DMS oxidation of about 70%.  相似文献   

The concentration and distribution of different mercury species in the water columns and sediment of Aha Lake     

Weiyang BAI Xinbin FENG Xuewu FU Tianrong HE Guangle QIU 《中国地球化学学报》2006,25(B08):154-154

In order to find out whether Aha Lake was polluted by the acid mining waste water or not, the concentration and distribution of different mercuryspecies in the water columns and sediment profile collected from Aha Lake were investigated. It was found that discernible seasonal variation of different mercury species in water body were obtained in the Aha Reservoir. With regards to the whole sampling periods, the concentrations of HgP in the Aha Reservoir water body were evidently correlated to the concentrations of total mercury, showing that total mercury was mostly associated with particle mercury. The concentrations of methylmercury in water body were also evidently correlated to the concentrations of dissolved mercury. The dissolved mercury evidently affects the distribution and transportation of methylmercury. However, there is no correlation between methylmercury and total mercury. The dissolved mercury, reactive mercury, dissolved methylmercury levels in the water body of high flow period were much higher than those in low flow period. The distribution, speciation and levels of mercury within the Aha Reservoir water body were governed by several factors, such as the output of river, the release of sediment . Discernible seasonal variation of total mercury and methylmercury in porewater was described during the sampling periods, with the concentrations in high flow period generally higher than those in low flow period. The methylmercury in pore water column was evidently correlated to that of the sediment. The results indicated that highly elevated MeHgD concentrations in the porewater were produced at the depths from 2 to 5 cm in the sediment profile, and decreased sharply with depth. A positive correlation has been found between MeHgD formation and sulfate reducing bacterial activity. These highly elevated concentrations of MeHgD at the intersurface between waters and sediments suggest a favorable methylation condition. Moreover,  相似文献   

Response of Ruppia maritima to the reclaimed wastewater in coastal artificial landscape river     

Weihong WANG Min JI Yuwei XUE 《中国地球化学学报》2006,25(B08):167-168

In recent years, reclaimed wastewater as a water source for urban artificial landscape rivers is being rapidly developed in some coastal cities with limited water resource available in China. However, eutrophication occurs more often in the landscape waterbody with reclaimed wastewater than in natural rivers and lakes. The study of restoration and reconstruction of macrophytes, especially the submerged aquatic vegetation, is essential to inhibit eutrophication of reclaimed wastewater. This study investigated the seasonal variation of biomass of Ruppia maritima in the artificial landscape river using reclaimed wastewater as the only water source in Tianjin, China. It was found that there were two seasonal growth peaks of Ruppia maritima each year in the coastal reclaimedwastewater. The contents of nitrogen and phosphorus of Ruppia maritima varied with the season.  相似文献   

Tin mineralization in the Dajing tin–polymetallic deposit, Inner Mongolia, China     

Y.W. Wang  J.B. Wang  L.J. Wang  Y.Z. Chen 《Journal of Asian Earth Sciences》2006,28(4-6):320-331

Dajing is a large-scale tin–polymetallic deposit that hosts the largest tin mine in North China. It is a hydrothermal vein-type deposit containing Sn, Cu, Pb, Zn, Ag, and minor components Co and In. The deposit consists of more than 690 veins hosted within Upper Permian sedimentary rocks.Three mineralization stages and six ore types are recognized with cassiterite constituting the dominant tin mineral. The SnO₂ content of cassiterite increases in the sequence of mineralization stages shear-deformation→cassiterite–quartz→cassiterite–sulfide (or chalcopyrite–pyrite) stage, while the content of FeO, TiO₂, Nb₂O₅, Ta₂O₅, and In₂O₅ tends to decrease with increases in NiO and Ga₂O₅. It is considered that the negative correlation between SnO₂ and FeO, Nb₂O₅, Ta₂O₅, and In₂O₅ results from elemental substitutions. The early stage cassiterite is much richer in Ta and the later stage cassiterite is much poorer in Ti and Fe than is usual in hydrothermal vein type tin deposits. This is interpreted to indicate that the component of early stage cassiterite reflects a granitic magma source while the composition of later stage cassiterite has a more obvious strata source. The compositional variation of cassiterite corresponds to decreasing crystallization temperatures within each stage and between sequential stages with time. The characteristics of REE in cassiterite from two stages are in accord with that of subvolcanic rocks and the Linxi formation. It suggests that tin transported during the cassiterite–quartz stage may have originated from subvolcanic dikes (e.g., dacite porphyry), while in the cassiterite–sulfide stage, tin may have been derived from wallrock (e.g. siltstone) of the Upper Permian-age Linxi Formation.  相似文献   

A comparative error analysis of manual versus automated methods of data acquisition for algebraic strain estimation   总被引：1，自引：0，他引：1  

Kingshuk Roy Choudhury  Kieran Mulchrone   《Tectonophysics》2006,421(3-4):209-230

This paper presents a statistical analysis of the algebraic strain estimation algorithm of Shimamoto and Ikeda [Shimamoto, T., Ikeda, Y., 1976. A simple algebraic method for strain estimation from deformed eillipsoidal objects: 1. Basic theory. Tectonophysics 36, 315–337]. It is argued that the error in their strain estimation procedure can be quantified using an expected discrepancy measure. An analysis of this measure demonstrates that the error is inversely proportional to the number of clasts used. The paper also examines the role of measurement error, in particular that incurred under (i) a moment based and (ii) manual data acquisition methods. Detailed analysis of these two acquisition methods shows that in both cases, the effect of measurement error on the expected discrepancy is small relative to the effect of the sample size (number of objects). Given their relative speed advantage, this result favours the use of automated measurement methods even if they incur more measurement error on individual objects. Validation of these results is carried out by means of a simulation study, as well as by reference to studies appearing in previous literature. The results are also applied to obtain an upper bound on the error of strain estimation for various studies published in the literature on strain analysis.  相似文献   

塔里木河源区冰川系统变化趋势预测   总被引：1，自引：0，他引：1  

王欣  谢自楚  刘时银  上官冬辉  陶建军  阳岳龙 《山地学报》2006,24(6):641-646

塔里木河源区是我国冰川分布最集中的地区之一,总面积达17 745.51 km2,占全国冰川总面积的30%;同时本区又属于我国升温幅度最大的地区之一。应用冰川系统变化的功能模型,对塔里木河源区冰川系统在本世纪对气候变化的趋势进行预测。结果表明:到2050年,如气温比1961~1990年高出1.9~2.3℃,本区冰川面积将减少4%~6%,冰川径流将增加22%~34%,零平衡线将上升62~94 m;如此升温率持续到本世纪末,则本区冰川面积将减少10%~16%,冰川径流将会回落,但仍比本世纪初多11%~13%,零平衡线将上升156~233 m。  相似文献   

Centennial to millennial geomagnetic secular variation     

M. Korte  C. G. Constable 《Geophysical Journal International》2006,167(1):43-52

A time-varying spherical harmonic model of the palaeomagnetic field for 0–7 ka is used to investigate large-scale global geomagnetic secular variation on centennial to millennial scales. We study dipole moment evolution over the past 7 kyr, and estimate its rate of change using the Gauss coefficients of degree 1 (dipole coefficients) from the CALS7K.2 field model and by two alternative methods that confirm the robustness of the predicted variations. All methods show substantial dipole moment variation on timescales ranging from centennial to millennial. The dipole moment from CALS7K.2 has the best resolution and is able to resolve the general decrease in dipole moment seen in historical observations since about 1830. The currently observed rate of dipole decay is underestimated by CALS7K.2, but is still not extraordinarily strong in comparison to the rates of change shown by the model over the whole 7 kyr interval. Truly continuous phases of dipole decrease or increase are decadal to centennial in length rather than longer-term features. The general large-scale secular variation shows substantial changes in power in higher spherical harmonic degrees on similar timescales to the dipole. Comparisons are made between statistical variations calculated directly from CALS7K.2 and longer-term palaeosecular variation models: CALS7K.2 has lower overall variance in the dipole and quadrupole terms, but exhibits an imbalance between dispersion in   g ¹₂  and   h ¹₂  , suggestive of long-term non-zonal structure in the secular variations.  相似文献   

韧性剪切变形对岩石地球化学行为的制约——以北阿尔金巴什考供韧性剪切带为例   总被引：6，自引：0，他引：6  

戚学祥李海兵  吴才来陈松永 《地质通报》2005,24(3):252-257

韧性剪切变形对岩石地球化学行为的制约一直是地质学家们探讨的课题。本文以构成北阿尔金红柳沟——拉配泉俯冲碰撞杂岩带与北阿尔金地块边界的巴什考供斜向逆冲型韧性剪切带为例，通过对韧性剪切带内花岗岩变形前后不同变形强度构造岩的地球化学组成进行对比，确定等比线斜率，探讨韧性变形对岩石体积和成分变异的影响。计算结果表明，在糜棱岩化过程中，糜棱岩化花岗岩体积亏损21％，花岗质糜棱岩体积亏损31％。质量平衡计算结果和等比线图表明，韧；陛剪切作用导致SiO2，流失量最大，A12O3、K2O及Ba、Rb、Sr等都有不同程度的丢失，显示出较强的活动性，MnO、P2O5、Sc位于等比线上或附近，表现出相对的稳定性。岩石中活动组分的变异是流体渗滤作用引起的，不活动组分的变异是体．积亏损造成的。  相似文献   

黄土坡面侵蚀产沙时空演变的REE示踪技术研究   总被引：2，自引：0，他引：2       下载免费PDF全文

薛亚洲  刘普灵  杨明义  琚彤军 《水科学进展》2005,16(2):174-180

室内交叉布设不同的稀土氧化物,通过人工模拟次降雨,在同一试验条件下,对坡面侵蚀沿顺坡方向和深度方向的演变过程同时展开研究。结果表明:REE示踪技术对定量研究土壤侵蚀具有较高的精度;降雨前期,片蚀与细沟侵蚀发育程度基本相当;后期细沟侵蚀占据坡面侵蚀的主导地位,其侵蚀平均加速度和平均侵蚀率分别是片蚀的15倍、9倍;试验结束,细沟侵蚀占据坡面总侵蚀的90%;本试验条件下,坡面下1/3区域为侵蚀活跃带。  相似文献