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21.
P. P. Sujith D. Ramanan P. A. LokaBharathi 《Marine Georesources & Geotechnology》2017,35(8):1158-1167
The different mineral phases of the ferromanganese (Fe–Mn) crusts stem from the interaction of biotic and abiotic components. It is therefore vital to study the activity of these components to decipher their contribution to the enrichment/depletion of metals in the crust. Thus, the present study examined sorption and release of Co and Ni by Fe-Mn crusts with associated microbial communities in the presence and absence of the metabolic poison sodium azide (15?mM). The study was conducted in the presence (G+) and absence (G?) of added glucose (0.1%) at temperatures of 4?±?1°C and 28?±?2°C. Results showed that the microbial community had maximal sorption of Co of 66.12?µg?g?1 at 4?±?1°C in the absence of added glucose and 479.75?µg?g?1 at 28?±?2°C in the presence of added glucose. Maximum sorption of Ni in the absence of added glucose was 1.89?µg?g?1 at 4?±?1°C and release of Ni was 51.28?µg?g?1 in the presence of added glucose. Under abiotic conditions with 15?mM sodium azide as a metabolic inhibitor, significant amounts of Co and Ni were released in the G+ medium. Total cell counts on the Fe-Mn crust in the presence of added glucose increased by an order of magnitude from 106 to 107 cells g?1 and in the absence of added glucose remained within the order of 106 cells?g?1 irrespective of temperature of incubation. Microscopic observation of the samples from biotic incubations showed numerous bacterial cells, exopolysaccharides, and structures resembling secondary minerals formed by bacteria. The results indicate that bacteria promote the enrichment of Co and Ni on the hydrogenetic Fe-Mn crusts by sorption processes and release of Ni by reductive dissolution of the oxides. The higher enrichment of Co than Ni is attributed to the way in which microbes interact with the metals. 相似文献
22.
煤岩吸附二氧化碳气体的CT实验研究 总被引：1，自引：0，他引：1
利用工业CT技术及应变测量研究不同气压下煤岩的二氧化碳气体吸附性质。研究发现：煤样的应变随吸附时间和气体压力的增加而增加,且在不同方向是不同的,吸附气体导致煤样孔隙率增加;煤样CT图像的灰度均值和灰度标准差随吸附时间和气体压力的增长都表现出增加的趋势。结果表明：吸附二氧化碳导致煤样总体发生膨胀变形,这为吸附提供更多的孔隙表面积而使吸附气体量增加,含气煤样的密度也因此而增大;气体吸附导致的煤样密度均值增加的效应大于体积膨胀导致的煤样密度均值减小的效应;吸附使煤样内部物质分布不均匀程度增加。 相似文献
23.
A series of batch tests have been presented to investigate the effects of solid-solution contact time, solid:solution ratio, and pH of solution on sorption of Cd2+ and Pb2+ on Ariake clay from Kyushu region of Japan. The results show that, among the three investigated factors, solid:solution ratio (SD/SN) seems to be the crucial controlling factor. The Freundlich sorption parameters determined from the batch tests were applied to a typical field landfill in which the Ariake clay was used as soil barrier. The impacts of the landfill were assessed by numerical analysis. Based on the analysis result, the significance of selecting proper solid:solution ratio for determining sorption parameters from batch test has been discussed. 相似文献
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粘土矿物的掺杂对沉积物吸持Cu、Zn能力的影响 总被引：3，自引：0，他引：3
通过考察粘土矿物及掺杂粘土矿物前后沉积物的吸附/解吸特性,分析了伊利石与蒙脱石对重金属污染沉积物中Cu与Zn稳定固定化的可行性。结果表明：伊利石与蒙脱石的掺杂均降低了沉积物吸持Cu的能力（最大下降量分别为5.4%和3.8%）,伊利石的掺杂同样降低了沉积物吸持Zn的能力（最大下降量为4.4%）,但蒙脱石掺杂后沉积物吸持Zn的能力明显增强,最高增加5.7%。因此,蒙脱石具有固定污染沉积物中Zn的能力,但不能提高污染沉积物中Cu的稳定性。 相似文献
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Soil contamination by radioactive Cs from Fukushima Daiichi Nuclear Power Plant accident was investigated. Absorption and desorption experiments of Cs were conducted for several phyllosillicates (kaolinite, sericite, montmorillonite, vermiculite, chrysotile and biotite), zeolite and solid organic matter (dead and green leaves). The results confirmed the characteristic sorption and desorption of Cs by these materials. The 2:1 type phyllosilicate, especially, vermiculite and montmorillonite absorbed Cs well. Heated vermiculite for agricultural use and weathered montmorillonite also adsorbed Cs. Leaves also absorbed Cs considerably but easily desorbed it. In summary, the relative capacity and strength of different materials for sorption of Cs followed the order: zeolite (clinoptilolite) > 2:1 type clay mineral > 1:1 type clay mineral > dead and green leaves. Culture experiments using bacteria of both naturally living on dead leaves in Iitate village, Fukushima Pref. and bacterial strains of Bacillus subtillis, Rhodococus erythropolis, Streptomyces aomiensis and Actinomycetospora chlora were carried out. Non-radioactive 1% Cs solution (CsCl) was added to the culture media. Two types of strong or considerable bacterial uptakes of Cs were found in bacterial cells. One is that Cs was contained mainly as globules inside bacteria and the other is that Cs was absorbed in the whole bacterial cells. The globules consisted mainly of Cs and P. Based on all these results, future diffusion and re-circulation behavior of Cs in the surface environment was discussed. 相似文献
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29.
Hakan Sirin Miguel A. Mariño 《Stochastic Environmental Research and Risk Assessment (SERRA)》2008,22(4):551-565
The laboratory-scale ground water transport equation with nonequilibrium sorption reaction subjected to unsteady, nondivergence-free,
and nonstationary velocity fields is up-scaled to the field-scale by using the ensemble-averaged equations obtained from the
cumulant expansion ensemble-averaging method. It is found that existing ensemble-averaged equations obtained with the help
of the cumulant expansion method for the system of linear partial differential equations are not second-order exact. Although
the cumulant expansion methodology is designed for noncommuting operators, it is found that there are still commudativity
requirements that need to be satisfied by the functions and constants exist in the coefficient matrix of the system of ordinary/partial
differential equations. A reversibility requirement, which covers the commudativity requirements, is also proposed when applying
the cumulant expansion method to a system of partial differential equations/a partial differential equation. The significance
of the new velocity correction obtained in this study due to the applied second-order exact cumulant expansion is investigated
on a numerical example with a linear trend in the distribution coefficient. It is found that the effect of the new velocity
correction can be significant enough to affect the maximum concentration values and the plume center of mass in the case of
a trending distribution coefficient in a physically heterogeneous environment. 相似文献
30.