Bildung bromhaltiger Desinfektionsnebenprodukte nach Chlorung von Bodenseewasser in Abhängigkeit von Aufbereitungsschritten und der Bromidkonzentration     

M. Petri  M. Wilker  H.-H. Stabel  E. Gilbert 《洁净——土壤、空气、水》1997,25(6):319-328

Formation of Brominated Disinfection By-products after Chlorination of Water from Lake Constance Depending on Treatment Steps and Bromide Concentration The formation of halogenated disinfection by-products (DNP) (trihalomethanes (THM), haloacetic acids (HES), haloacetonitriles (HAN), haloketones (HKE) and chloropicrin (TCNM)) was studied after chlorination (0.5 mg/L) of raw water and drinking water from Lake Constance. The objectives of this study were to investigate the effect of bromide ion on the distribution of DNP-species resulting from chlorination and to draw up a bromide mass-balance. The treatment of water from Lake Constance with ozone decreased the formation of DNP about 35% and of total organic halogens (AOX) about 45%. This decline in DNP-formation is mainly due to the formation of chloroform, dichloro- and trichloroacetic acid. Though there is only a small amount of bromide (6.2 μg/L) in water from Lake Constance, about 32% of THM, 16% of HES, and 30% of HAN contained bromine after chlorination of treated water. The addition of bromide ion (up to 1 mg/L) shifted the DNP-composition to more brominated species. The distribution of the DNP-species depends on the initial molar bromide-to-chlorine ratio. A mathematic model showed the same pattern of DNP-species depending on the initial molar bromide-to-chlorine ratio that was observed experimentally in microstrained raw water and drinking water from Lake Constance. After chlorination of microstrained raw water, 27% of the bromide were incorporated in known DNP, 34% in unknown substances, and about 39% of bromide were not converted to organic bromine. After chlorination of treated water, only 16% of the bromide were incorporated in unknown substances, whereas 34% were found in known DNP. About 50% were found as bromide again. After addition of bromide (up to 25 μg/L) to ozonated and treated water from Lake Constance, between 60 and 72% of the bromide that had reacted after chlorination were found in analyzed low-molecular DNP.  相似文献   

大型水域水岩相互作用及其环境效应研究   总被引：26，自引：0，他引：26  

王士天  王思敬 《地质灾害与环境保护》1997,8(1):69-89

以大量实际资料及深入的研究成果，较全面地论述了人工大型水域水岩相作用及其导致的主要地质灾害，包括水库诱发地震，库岸崩滑，水岩作用导致的大坝溃决，以及水库淤积导致的大面积环境恶化等问题。  相似文献   

A Simple Parameterisation for Flux Footprint Predictions   总被引：9，自引：6，他引：9  

N. Kljun  P. Calanca  M. W. Rotach  H. P. Schmid 《Boundary-Layer Meteorology》2004,112(3):503-523

Flux footprint functions estimate the location and relative importance of passive scalar sources influencing flux measurements at a given receptor height. These footprint estimates strongly vary in size, depending on receptor height, atmospheric stability, and surface roughness. Reliable footprint calculations from, e.g., Lagrangian stochastic models or large-eddy simulations are computationally expensive and cannot readily be computed for long-term observational programs. To facilitate more accessible footprint estimates, a scaling procedure is introduced for flux footprint functions over a range of stratifications from convective to stable, and receptor heights ranging from near the surface to the middle of the boundary layer. It is shown that, when applying this scaling procedure, footprint estimates collapse to an ensemble of similar curves. A simple parameterisation for the scaled footprint estimates is presented. This parameterisation accounts for the influence of the roughness length on the footprint and allows for a quick but precise algebraic footprint estimation.  相似文献   

地—空界面天然中子辐射场的扰动及其环境意义     

葛良全  赖万昌  林延畅  黄元清  钟丁生 《地球科学进展》2004,(Z1)

介绍了地—空界面天然中子流的来源和轻便型天然中子流测量仪器。论述了地—空界面天然中子辐射场的扰动。理论与长期观测表明,在地—空界面上天然中子流注量率随高程的增加而呈指数规律增加,而在近地表(20m内)却随距地面高度的增加而呈指数规律减少;天然中子流注量率与大气压力呈负相关关系,气压系数为(-0.060～-0.064)中子计数/30min/kPa;地—空界面天然中子流的纬度效应与高空中更显著;天然中子流注量率异常与气象的变化密切相关;地表介质的含水率增高,则地—空界面上升快中子流明显降低。通过对地一空界面天然中子流测量,可以揭示气象的瞬态变化、确定地表介质的含水率的关系,以及在地震预报与环境电离辐射评价方面具有重要的科学意义与实用价值。  相似文献   

三江源地区水资源的涵养和保护   总被引：1，自引：0，他引：1  

马致远 《地球科学进展》2004,(Z1)

分析了三江源区水资源现状,论述了建立水资源三级保护区的意义、作用和划分方案,实施林草植被的保护和恢复的水文生态效益及健全水资源补偿机制的必要性。  相似文献   

Water exchange between Tokyo Bay and the Pacific Ocean during winter     

Tetsuo Yanagi  Hirofumi Hinata 《Ocean Dynamics》2004,54(3-4):452-459

Variability in water-exchange time between Tokyo Bay and the Pacific Ocean during winter is investigated based on the results of intensive field observation from November 2000 to March 2001. Water-exchange time between Tokyo Bay and the Pacific Ocean during winter mainly depends on the strength of northerly monsoon, being about 16 days under the weak monsoon and about 12 days under the strong monsoon. Moreover, it becomes longer by about 1 day in spring tide and shorter in neap tide due to the coupling effect of estuarine circulation and vertical mixing. Water-exchange time also varies depending on the open-ocean condition. When the warm water mass approaches from the Pacific Ocean to the mouth of Tokyo Bay through the eastern channel of Sagami Bay, which connects Tokyo Bay and the Pacific Ocean, water-exchange time becomes longer by about 2 days because the warm water mass is blocked in the surface layer at the bay mouth. On the other hand, when the warm water mass approaches to the mouth of Tokyo Bay through the western channel of Sagami Bay, water-exchange time becomes shorter by about 1 day because the warm water mass intrudes into the middle or lower layers of Tokyo Bay. Such different behavior of warm water mass at the mouth of Tokyo Bay is due to the difference in density of approaching warm water masses, that is, the density of the warm water mass through the eastern channel is smaller than that of the warm water mass through the western channel of Sagami Bay.Responsible Editors: Yens Kappenberg  相似文献   

Type-specific and indicator taxa of phytoplankton as a quality criterion for assessing the ecological status of Finnish boreal lakes   总被引：6，自引：0，他引：6  

Liisa Lepist  Anna-Liisa Holopainen  Heidi Vuoristo 《Limnologica》2004,34(3):236-248

Key issues in the implementation of the Water Framework Directive are classification of lakes using biological quality parameters and type-specific reference conditions. This work is one of three studies considering different metrics of phytoplankton in the classification of ecological status. Phytoplankton was studied in a total of 55 Finnish boreal lakes, including 32 reference lakes. We tested the suitability of taxonomic composition and abundance of phytoplankton groups for biological classification. We also preliminarily determined the type-specific taxa for the studied lakes. The type-specific taxa for reference conditions are coincidently the indicator species/taxa for high ecological status. Interestingly, some taxa type-specific for impacted oligo-humic lakes proved to be the type-specific taxa for humic reference lakes. The pressure of human impact was observed not only as increase of biomass but also as changes in the species composition. The phytoplankton composition indicated the ecological status of impacted lakes moderately well. There was some variation in the indications given by different algal groups, probably due to the preliminary class boundaries used. However, the preliminary combination of indicative parameters to estimate the ecological status of the studied impacted lakes was in general in accordance with earlier classification of water quality in Finnish lakes.  相似文献   

Influence of water level fluctuation on the spatial dynamic of the water chemistry at Lake Fertõ/Neusiedler See     

Mria Dinka  Edit goston-Szab  rpd Berczik  Gyula Kutrucz 《Limnologica》2004,34(1-2):48

Lake Fertõ/Neusiedler See is a steppe lake situated on the Hungarian-Austrian border with a surface area of 309 km². It is an extremely shallow lake with regulated outflow. 54% of the whole lake and 85% of the Hungarian part (75 km²) is covered by reed. There are numerous reedless areas (inner ponds) of variable size within the reed belt, which is enmeshed with canals connecting the inner ponds with the open water areas. Fundamental differences were recorded in the water chemistry of the three water type areas, open water, canals and inner ponds. The degree of these differences is basically determined by the distance from the open water areas and the water level of the actual years. An extremely high, an average and an extremely low water level year was examined, in order to present the spatial and temporal differences in the water chemistry of the investigated water bodies. Differences due to the water level fluctuation between years in the three different water types are discussed on the basis of electrical conductivity, cation, and anion concentration changes of the water. Our results support the concept of high instability of Lake Fertõ and describe habitats with remarkable temporal and spatial variability. The high influence of water level on habitat conditions at different sites of the lake recommend a carefull water level regulation strategy.  相似文献   

Toxic Cyanobacteria in Greek Freshwaters, 1987—2000: Occurrence,Toxicity, and Impacts in the Mediterranean Region     

Catherine M. Cook  Elisabeth Vardaka  Tom Lanaras 《洁净——土壤、空气、水》2004,32(2):107-124

In a survey in Greece from 1987 to 2000 hepatotoxic cyanobacterial blooms were observed in 9 out of 33 freshwaters. Microcystins (MCYSTs) were detected by HPLC in 7 of these lakes, and the total MCYST concentration per scum dry weight ranged from 50.3 to 1638 ± 464 μg g^—1. Cyanobacterial genera (Microcystis, Anabaena, Anabaenopsis, Aphanizomenon, Cylindrospermopsis) with known toxin producing taxa were present in 31 freshwaters. From our data and a review of the literature, it would appear that Mediterranean countries are more likely 1) to have toxic cyanobacterial blooms consisting of Microcystis spp. and 2) to have higher intracellular MCYST concentrations. A case study in Lake Kastoria is used to highlight seasonal patterns of cyanobacterial and MCYST‐LR occurrence and to assess cyanotoxin risk. Cyanobacterial biovolume was high (> 11 μL L^—1) throughout the year and was in excess of Guidance Level 2 (10 μL L^—1) proposed by WHO for recreational waters and Alert Level 2 for drinking water. Further, surface water samples from April to November exceeded Guidance Level 3, with the potential for acute cyanobacterial poisoning. Intracellular MCYST‐LR concentrations (max 3186 μg L^—1) exceeded the WHO guideline for drinking water (1 μg L^—1) from September to November with a high risk of adverse health effects. Preliminary evidence indicates that in 3 lakes microcystins are accumulated in some aquatic organisms. Generally, a high risk level can be deduced from the data for the Mediterranean region.  相似文献   

2002年6月21～24日梅雨锋暴雨过程中的水汽羽特征   总被引：4，自引：2，他引：4  

覃丹宇  江吉喜  方宗义 《气象学报》2004,62(3):329-337

利用GMS 5水汽图像和NCAR/NCEP再分析资料 ,分析了 2 0 0 2年 6月 2 1～ 2 4日长江中下游梅雨锋暴雨过程中水汽图像上水汽羽的特征。结果表明 :日平均水汽图像上显示了这次暴雨过程中对流层中上部的主要水汽型 ,是一条热带水汽羽从孟加拉湾经过青藏高原东部向偏东方向伸展至江淮地区 ,并与中纬度水汽羽相互作用 ,暴雨云团在热带水汽羽中连续生成。这条热带水汽羽是一条深厚暖湿输送带 ,反映了中高层水汽从孟加拉湾向长江下游的输送 ,以及通过大尺度上升运动造成的水汽自下而上的垂直输送 ,并且水汽羽与对流层上层的负涡度和正散度区域有很好的对应关系。水汽羽的北部边界附近的暗带与一条强涡度梯度和高空急流轴相关 ,具有明显的斜压性  相似文献