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91.
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Sulfur Isotope Fractionation in Magmatic Systems:Models of Rayleigh Distillation and Selective Flux 总被引:2,自引:0,他引:2
郑永飞 《中国地球化学学报》1990,9(1):27-45
The effect of Rayleigh distillation by outgassing of SO2 and H2S on the isotopic composition of sulfur remaining in silicate melts is quantitatively modelled.A threshold mole fraction of sulfur in sulfide component of the melts is reckoned to be of critical importance in shifting the δ^34S of the melts mith respect to the original magmas.The partial equilibrium fractionation in a magmatic system is evaluated by assuming that a non-equilibrium flux of sulfur occurs between magmatic volatiles and the melts,while an equilibrium fractionation is approached between sulfate and sulfide within the melts.The results show that under high fo2 conditions,the sulfate/sulfide ratio in a melt entds to increase,and the δ^34S value of sulfur in a solidified rock might then be shifted in the positive direction.This may either be due to Rayleigh outgassing in case the mole fraction of sulfide is less than the threshold,or due to a unidirectional increase in δ^34S value of the sulfate with decreaing temperature,Conversely,at low fo2,the sulfate/sulfide ratio tends to decrease and the δ^34S value of total sulfur could be driven in the negative direction,either because of the Rayleigh outgassing in case the mole fraction of sulfide is greater than the threshold,or because of a unidirectional decrease inδ^34S value of the sulfide.To establish isotopic equilibrium between sulfate and sulfide,the HM,QFM or WM buffers in the magmatic system are suggested to provide the redox couple that could simultaneously reduce the sulfate and oxidize the sulfide.CaO present in the silicatte Melts is also called upon to participate in the chemical equilibrium between sulfate and sulfide,Consequently,the δ^34S value of an igneous rock could considerably deviate from that of its original magma due to the influence of oxygen fugacity and temperature at the time of magma solidification. 相似文献
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Franco Tassi Orlando Vaselli Elena Lognoli Fabrizio Cuccoli Barbara Nisi Elena Ramaldi Sandro Moretti Luca Lombardi Bruno Capaccioni 《中国地球化学学报》2006,25(B08):70-71
Mt. Amiata (Southern Tuscany, Central Italy) is an extinct Quaternary volcano located in an area still marked by high heat-flow that is caused by deep seated (6-10 km) hot masses related to Pliocene magmatic activity. The anomalous geothermal gradient gives rise, within the Mesozoic limestone formation (Tuscan series), to geothermal systems that fed the Ca-SO4 thermal springs characterizing this area. Besides of thermal fluids, several cold, dry CO2-rich gas emissions seep out on the NE flank of the volcano. These gas vents mostly consist of large sub-circular craters at variable depth and diameter (5-15 m and 10-50 m, respectively), and represent a serious hazard for the local population, as testified by the several asphyxia casualties that have been repeatedly occurred within these morphological depressions. In this work, the chemical and isotopic compositions of the Mt. Amiata "CO2-rich gas vents" and the estimation of both the CO2 flux from the soil and the CO2 distribution in air of their surroundings, has been carried out in order to: (1) assess the origin of gases, (2) recognize the mechanism of formation for these gas emissions and their relationship with local tectonics, and (3) to evaluate the CO2 hazard in the high flux emanations. The chemical composition of the gases is largely dominated by CO2 (up to 98 % by vol) and shows relatively high concentrations of N2, CH4 and H2S (up to 1.1%, 0.9% and 3.9 % by vol, respectively). These features, coupled with the carbon and nitrogen isotopic signatures, suggest that the origin of the main gas compounds may be related to the contribution of deep (i.e., thermometamorphic processes on carbonate formations for CO2) and shallow (i.e. thermal decomposition of organic material for CH4, N2 and H2S) sources. 相似文献
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界牌岭锡多金属矿床是一个大型隐伏矿床,找矿工作采用了化探次生晕、原生晕、地质调查等多种方法和手段.含铍条纹状蚀变岩的发现在找矿预测中起到了致关重要的作用,为找矿工作开拓了新的思路. 相似文献
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近年来在新疆巴喀勒萨依地区发现一套含少量火山碎屑岩的含铜砂岩地层,由于该地层位于近东西向的断裂夹块中,其含矿层位的确定就成了难题。在该地层中发现了一些腕足类、珊瑚、腹足类、植物化石,经中国科学院南京地质古生物研究所鉴定,时代属晚石炭世晚期。介绍了巴喀勒萨依地区晚石炭世伊什基里克组含铜砂岩剖面及铜矿特征,并获得铜资源量19 797 t,银铜资源量371 t,提出了该区铜、银富集在红色含铜砂岩中有机质聚集处的新观点。 相似文献
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延边地区中生代火山岩的岩浆源区:来自Sr-Nd同位素和深源捕虏体(晶)的证据 总被引:6,自引:0,他引:6
延边地区中侏罗世和早白垩世火山岩中包含有较多的辉石岩捕虏体和角闪石捕虏晶,前者为普通辉石变种,其化学成分类似于中国东部新生代玄武岩中单斜辉石巨晶的成分,具有岩浆堆积成因特征;后者为韭闪石和镁质绿钠闪石变种,其成分类似于中生代晚期玄武岩中角闪二辉石岩包体里的角闪石和新生代玄武岩中的角闪石巨晶.矿物温压计算结果显示,它们形成深度介于25~37km.延边地区中生代火山岩的(87Sr/86Sr)i值介于0.704 3~0.705 0,εNd(t)值介于2.33~4.71,表明岩浆源区应是一套具有亏损性质的新增生的地幔物质.综合上述结果,可以判定延边地区中生代火山岩的原始岩浆应来源于新增生的壳幔过渡带物质的部分熔融,地壳增生事件的时间为新元古代. 相似文献
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红旗岭镁铁-超镁铁岩侵入体及铜镍硫化物矿床的成岩成矿机制 总被引:7,自引:0,他引:7
红旗岭铜镍矿床地处华北地台与吉黑地槽系接触带--辉发河断裂北侧.区内出露30多个镁铁-超镁铁质岩体,其中1、7号超镁铁岩体中赋存铜镍硫化物矿(床)体.含矿岩体分相明显,各类岩石均具堆积结构.铜镍矿体呈似板状、脉状、透镜状及囊状赋存于超镁铁岩体底部橄榄辉岩相中.岩石学和地球化学研究表明,7号岩体形成以流动分异为主,1号岩体为重力分异;原始岩浆属拉斑玄武质,块状矿石系压滤作用产物,后续岩浆的补给和混合补充了成矿物质,硫化物不混溶程度受挥发分制约,矿床属岩浆深部熔离分异成因,成矿时代为印支期. 相似文献
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