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11.
Homogeneous 129I / 127I ratios from 6.51 ± 1.36 × 10− 14 to 12.6 ± 1.49 × 10− 14 were measured in formation brine at the Pol-Chuc, Abkatún, Taratunich–Batab off-shore oil reservoirs, Bay of Campeche in S-Mexico. Cosmogenic production could account for a homogeneous, Late Cretaceous/Paleocene time period (71.3 ± 5.3 to 56.3 ± 2.9 Ma) for the sedimentation and burial of organic material in the source formation. As the actual reservoir column is formed by Paleocene to Kimmeridgian sediments, the lower part of the lithological column must have received hydrocarbons that migrated downward from an initial source rock (Upper Cretaceous?) during a post-Paleocene event, probably during Miocene. Cosmogenic production from Tithonian shales can be excluded, as 129I would have been decayed. As an alternative or complementary process, the subsurface, radiogenic production of 129I / 127I by 238U-fission in Uranium-enriched sediments should also be considered to explain the present, low 129I / 127I ratios. 相似文献
12.
Water sampling during the 1993 IV Russian–US Joint Expedition to the Bering and Chukchi Seas (BERPAC) indicates that Pacific Ocean burdens of the long-lived radionuclide 129I are relatively low in the Pacific-influenced Arctic, particularly compared to high latitude waters influenced by the North Atlantic. These low concentrations occur despite the presence of potential submerged anthropogenic sources in the East Sea (Sea of Japan), and in the northwest Pacific Ocean, east of the Kamchatka Peninsula. The concentration of 129I entering the Arctic Ocean through Bering Strait, 0.7×108 atoms kg−1, is only slightly higher than observed in deep Pacific waters. Similar concentrations (0.44–0.76×108 atoms kg−1) measured in Long Strait indicate no significant transfer of 129I eastward into the Chukchi Sea in the Siberian Coastal Current from the Siberian marginal seas to the west. However, the concentrations reported here are more than an order of magnitude higher than the Bering Strait input concentration estimated (1.0×106 atoms kg−1) from bomb fallout mass balances, which supports other existing evidence for a significant atmospheric deposition term for this radionuclide in surface ocean waters. Near-bottom water samples collected in productive waters of the Bering and Chukchi Seas also suggest that sediment regeneration may locally elevate 129I concentrations, and impact its utility as a water mass tracer. As part of this study, two deep 129I profiles were also measured in the East Sea in 1993–1994. The near-surface concentration of 129I ranged from 0.12 to 0.31×108 atoms kg−1. The 129I concentration showed a steady decrease with depth, although because of active deep water ventilation, the entire 3000 m water column exceeded natural concentrations of the radionuclide. Atom ratios of 129I/137Cs in the East Sea also suggest an excess of 129I above bomb fallout estimates, also possibly resulting from atmospheric deposition ultimately originating from nuclear facilities. 相似文献
13.
本研究建立了AMS(Accelerator mass spectrum,加速器质谱)测定海水中129 I的气载分离制样方法:对加入载体的海水样品进行氧化还原处理,在加热的条件下将生成的单质碘吹出,并使用吸收装置吸收,后经阴离子交换树脂富集纯化,最后生成用于AMS分析的AgI沉淀,本方法全程回收率50%~70%,在相对密闭的体系中进行,减少了碘的损失,相对于萃取-反萃取的制样方法具有可操作性强,避免有机试剂使用等优点,可用于固态、液态和气态样品中129 I的AMS分析制样。 相似文献
14.
BAT99-129 is a rare, short-period eclipsing Wolf-Rayet binary in the Large Magellanic Cloud. We present here medium-resolution NTT/EMMI spectra that allow us to disentangle the spectra of the two components and find the orbital parameters of the binary. We also present VLT/FORS1 spectra of this binary taken during the secondary eclipse, i.e. when the companion star passes in front of the Wolf-Rayet star. With these data we are able to extract, for the first time in absolute units for a WR + O binary, the sizes of the line emitting regions.Based on observations obtained at the La Silla and Paranal Observatories, European Southern Observatory (Chile). 相似文献
15.
本文讨论了~(129)Ⅰ的三个起源:大气起源、地下起源和人工起源,通过三个实例,介绍了~(129)Ⅰ在石油勘探、水文地质研究和环境监测中的应用进展,并且指出了未来研究方向。 相似文献
16.
Hitoshi Tomaru Udo Fehn Zunli Lu Rika Takeuchi Fumio Inagaki Hiroyuki Imachi Ryosuke Kotani Ryo Matsumoto Kan Aoike 《Resource Geology》2009,59(4):359-373
Iodine concentration and radioisotopic composition (129I/I) were measured in the pore waters from the gas hydrate occurrence in the forearc basin offshore Shimokita Peninsula, north-eastern Japan, to determine the source formation of I and accompanying hydrocarbons. Iodine concentrations correlate well with the alkalinity and SO4 patterns, reflecting degradation stages of I-rich buried organic matter, rapidly increasing in the sulfate reduction interval, and becoming constant below 250 meters below the seafloor with an upwelling flux of 1.5 × 10−11 µmol cm−2 year−1. The 129I/I ratios of 300 × 10−15–400 × 10−15 in deep pore waters suggest ages for iodine and hydrocarbon sources as old as 40 Ma. These ages correlate well with the coaly source formations of the Eocene age thought to be responsible for the conventional natural gas deposits underlying the gas hydrate stability zone. Similar profiles are observed in 129I/I ratios of pore waters in the gas hydrate stability zone from the forearc basin in the eastern Nankai Trough, offshore central Japan, where pore waters are enriched in I and reach ages as old as ∼50 Ma through the sediment column. At the outer ridge site along the trough, on the other hand, relatively younger I are more frequently delivered probably through thrusts/faults associated with subduction. The nature of source formations of I and hydrocarbons in the offshore Shimokita Peninsula has a more terrestrial contribution compared with those in the Nankai Trough, but these formations are also considerably older than the host sediments, suggesting long-term transport of I and hydrocarbons for the accumulation of gas hydrates in both locations. 相似文献
17.
Yasuyuki Muramatsu Yukari Takada Hiroyuki Matsuzaki Satoshi Yoshida 《Quaternary Geochronology》2008,3(3):291-297
Analytical procedures in the determination of iodine-129 (half-life: 1.6×107 y) have been studied using accelerator mass spectrometry (AMS), with special references to the separation procedures of iodine from soil samples for the AMS measurement. Iodine was successfully volatilized from soil samples by pyrohydrolysis at 1000 °C and collected in a trap solution. Iodine was purified from the matrix by solvent extraction. Finally, it was precipitated as silver iodide to make a target for AMS. In order to obtain information on the 129I/127I ratio in a chemical blank (or iodine carrier), we have determined the ratios in several iodine reagents and found that the ratios fell in a narrow range around 1.7×10−13. The detection limit for soil sample (1 g material) by the present method was about 0.01 mBq/kg or 4×10−11 as the ratio of stable iodine (129I/127I ratio), i.e. these values were much better than that by neutron activation analysis (NAA) used in our previous studies. We have applied this method in the analysis of soil samples collected from different places in Japan. We could successfully determine 129I in soil samples with low 129I concentrations, which could not be detected by NAA. Sample size necessary for the soil analysis by AMS was only about 0.5 g or less, whereas about 100 g of the sample were required for NAA [Muramatsu, Y., Ohmomo, Y., 1986. Iodine-129 and iodine-127 in environmental samples collected from Tokaimura/ Ibaraki, Japan. Sci. Total Environ. 48, 33-43]. Using this method, new data were obtained for the 129I levels in 20 soil samples collected from background areas far from nuclear facilities, and the ranges were 1.4×10−5−4.5×10−3 Bq/kg as 129I concentrations and 3.9×10−11−2.2×10−8 as 129I/127I ratios. These values are useful in understanding the 129I levels in Japanese environments. Higher 129I concentrations were observed in forest soils than those in field and rice paddy soils should be related to the interception effect of atmospheric 129I due to tree canopies. Relatively high 129I/127I ratios found in rice paddy soils could be explained by their low stable iodine concentrations which were caused by the desorption of stable iodine from the rice paddies during the cultivation. 相似文献
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19.
The cluster 3C 129 is classified as a rich cluster. An analysis of the properties of the cluster 3C 129 from ROSAT PSPC and HRI, Einstein IPC, and EXOSAT ME observations is presented. The mean temperature from a joint fit of the ROSAT PSPC and EXOSAT ME data is 5.5(±0.2) keV. The luminosity is 0.6×1044 erg s−1 in 0.2–2.4 keV and 2.7×1044 erg s−1 in 0.2–10 keV. We find a cooling flow with a rate of ∼84 M⊙ yr−1 . The central gas density is 6×10−3 cm−3 , and the ICM mass is 3.6×1013 M⊙ . The total cluster mass is ∼5×1014 M⊙ . The X-ray morphology shows an east–west elongation, which is evidence for a recent merger event. The radio source 3C 129.1 is located near the X-ray centre. Another cluster member galaxy (the radio galaxy 3C 129) is a prototype of head-tailed radio galaxies, and is located in the west part of the cluster. The tail points along the gradient of intracluster gas pressure. There are no significant point X-ray sources associated with the AGNs of the two radio galaxies. 相似文献
20.
JI Lihong LIU Guangshan CHEN Zhigang HUANG Yipu XING N JIANG Shan HE Ming 《海洋学报(英文版)》2015,34(10):31-35
In the present study,the analytical method for 129iodine(129I) in ferromanganese crusts is developed and129iodine/127iodine(129I/127I) ratio in ferromanganese crusts is measured by the accelerator mass spectrometry(AMS).The developed method is applied to analyze 129I/127 I ratio in two ferromanganese crusts MP5D44 and CXD08-1 collected from the Mid-Pacific Ocean.The results show that 129I/127 I ratio in MP5D44 and CXD08-1crusts varies from 7×10–14 to 1.27×10–12,with the lowest value falling on the detection limit level of AMS reported by previous literatures.For the depth distribution of 129I/127 I,it is found that both MP5D44 and CXD08-1 crusts have two growth generations,and the 129I/127 I profiles in two generations all displayed an approximate exponential decay.According to the 129I/127 I ratio,the generate age of bottom layer of MP5D44 and CXD08-1 was estimated to be 54.77 and 69.69 Ma,respectively. 相似文献