Compositions and source apportionments of atmospheric aerosol during Asian dust storm and local pollution in central Taiwan     

Man-Ting Cheng  Wei-Chun Chou  Chia-Pin Chio  Shih-Chieh Hsu  Yi-Ru Su  Pei-Hsuan Kuo  Ben-Jei Tsuang  Shuen-Hsin Lin  Charles C.-K. Chou 《Journal of Atmospheric Chemistry》2008,61(2):155-173

A study has been carried out on water soluble ions, trace elements, as well as PM_2.5 and PM_2.5–10 elemental and organic carbon samples collected daily from Central Taiwan over a one year period in 2005. A source apportionment study was performed, employing a Gaussian trajectory transfer coefficient model (GTx) to the results from 141 sets of PM_2.5 and PM_2.5–10 samples. Two different types of PM₁₀ episodes, local pollution (LOP) and Asian dust storm (ADS) were observed in this study. The results revealed that relative high concentrations of secondary aerosols (NO₃⁻, SO₄²⁻ and NH₄⁺) and the elements Cu, Zn, Cd, Pb and As were observed in PM_2.5 during LOP periods. However, sea salt species (Na⁺ and Cl⁻) and crustal elements (e.g., Al, Fe, Mg, K, Ca and Ti) of PM_2.5–10 showed a sharp increase during ADS periods. Anthropogenic source metals, Cu, Zn, Cd, Pb and As, as well as coarse nitrate also increased with ADS episodes. Moreover, reconstruction of aerosol compositions revealed that soil of PM_2.5–10 elevated approximately 12–14% in ADS periods than LOP and Clear periods. A significantly high ratio of non-sea salt sulfate to elemental carbon (NSS-SO₄²⁻/EC) of PM_2.5–10 during ADS periods was associated with higher concentrations of non-sea-salt sulfates from the industrial regions of China. Source apportionment analysis showed that 39% of PM₁₀, 25% of PM_2.5, 50% of PM_2.5–10, 42% of sulfate and 30% of nitrate were attributable to the long range transport during ADS periods, respectively.  相似文献   

Interdecadal change in the connection between Hadley circulation and winter temperature in East Asia   总被引：5，自引：0，他引：5  

周波涛  王会军 《大气科学进展》2008,25(1):24-30

Based on NCEP/NCAR reanalysis data, the interdecadal variability of Hadley circulation （HC） and its association with East Asian temperature in winter are investigated. Results indicate that the Northern Hemisphere winter HC underwent apparent change in the 1970s, with transition occurring around 1976/77. Along with interdecadal variability of HC, its linkage to surface air temperature （SAT） in East Asia also varied decadally, from weak relations to strong relations. Such a change may be related to the interaction between HC and the atmospheric circulation system over the Philippines, which is associated with the East Asian winter monsoon （EAWM）. Before the 1970s, the connection between HC and the anticyclonic circulation around the Philippines was insignificant, but after the late 1970s their linkage entered a strong regime. The intensification of this connection may therefore be responsible for the strong relations between HC and East Asian winter temperatures after the late 1970s.  相似文献   

Holocene climate evolution of the Ugii Nuur basin,Mongolia     

Wolfgang SCHWANGHART  Brigitta SCH  "UTT  Michael WALTHER 《大气科学进展》2008,25(6):986-998

In order to evaluate the Holocene palaeoenvironmental evolution of the Ugii Nuur basin, central Mongolia, investigations on chemical and mineralogical properties of lacustrine sediments were carried out on a 630 cm sediment core from lake Ugii Nuur. The interpretation of the record is based on a principal component analysis （PCA） of the elemental composition of the samples. The results show that lacustrine deposition started at 10.6 kyr BP. Low lake level conditions were identified during the Early Holocene （10.6-7.9 kyr BP）. The Mid Holocene （7.9-4.2 kyr BP） was characterized by generally higher lake levels and thus higher moisture supply, but it experienced strong climatic fluctuations. Arid conditions prevailed from 4.2-2.8 kyr BP and were followed by a stable, more humid phase until today.  相似文献   

亚洲—太平洋季风区的遥相关研究   总被引：15，自引：6，他引：9  

丁一汇  刘芸芸 《气象学报》2008,66(5):670-682

亚洲-太平洋季风区各季风子系统间的相互作用对季风区甚至全球的气候变化都有非常显著的影响.文中根据国内外相关研究,重点分析和评述了在亚洲-太平洋季风区中4种季节内时间尺度的遥相关关系,清楚地揭示了印度夏季风、东亚夏季风和西北太平洋夏季风之间的相互作用.研究发现:(1) 在亚洲季风爆发初期,印度夏季风的爆发相对于中国长江流域梅雨的开始存在相差大约两周的超前关系,形成从印度西南部经孟加拉湾到达中国长江流域及日本南部的遥相关型,即"南支"遥相关型.(2) 在季风盛行期间,长江流域降水明显受热带西北太平洋夏季风的影响,与西北太平洋夏季风降水呈反相关关系,即当季风减弱时,长江流域夏季降水偏多.(3) 与长江流域降水相反,华北雨季(7月第4候-8月第3候)则与西北太平洋夏季风降水呈正相关关系,当西北太平洋夏季风强时,西太平洋副热带高压异常偏北偏东,副高西南侧的异常东南水汽输送在中国华北地区上空辐合,给该地区降水偏多提供了充足的水汽条件.(4) 华北夏季降水同时还与印度夏季风呈正相关关系,在夏季风盛行期间,形成由印度西北部经青藏高原到中国华北地区的西南-东北走向的遥相关型,即"北支"遥相关型. 上述4种遥相关关系,反映了亚洲夏季风季节北推过程中,印度夏季风、东亚夏季风和西北太平洋夏季风子系统之间的关联.  相似文献   

一个适用于描述中国大陆冬季气温变化的东亚冬季风指数   总被引：16，自引：0，他引：16  

朱艳峰 《气象学报》2008,66(5):781-788

利用1951年1月-2007年2月的NCEP V1格点资料和中国台站观测资料,定义了一个冬季风环流指数(IEAWM),并分析其与中国冬季气温和东亚大气环流变化的联系.结果表明该指数能够很好地反映东亚冬季风系统各成员的变化,兼顾北方和南方的环流状况和东西部热力差异的影响,改进了原有冬季风指数大多针对单一的冬季风环流成员及对中国冬季气温变化反映能力的不足,能够很好地反映中国冬季平均气温的异常变化.分析表明,当该指数为正值时东亚冬季风偏强,对应着地面西伯利亚高压和高空东亚大槽均偏强,东亚地区对流层中层的高-低纬度之间的纬向风经向切变加强,有利于中高纬度冷空气向南侵入,导致中国大陆地区气温偏低,反之亦然.IEAWM的年代际变化表明东亚冬季风在1985年之前偏强,1985年之后明显偏弱,这与1985年之后中国冬季变暖是一致的.  相似文献   

An Assessment on the Performance of IPCC AR4 Climate Models in Simulating Interdecadal Variations of the East Asian Summer Monsoon   总被引：3，自引：0，他引：3       下载免费PDF全文

SUN Ying  DING Yihui 《Acta Meteorologica Sinica》2008,22(4):472-488

Observations from several data centers together with a categorization method are used to evaluate the IPCC AR4 （Intergovernmental Panel on Climate Change, the Fourth Assessment Report） climate models＇ performance in simulating the interdecadal variations of summer precipitation and monsoon circulation in East Asia. Out of 19 models under examination, 9 models can relatively well reproduce the 1979-1999 mean June-July-August （JJA） precipitation in East Asia, but only 3 models （Category-1 models） can capture the interdecadal variation of precipitation in East Asia. These 3 models are： GFDL-CM2.0, MIROC3.2 （hires）, and MIROC3.2 （medres）, among which the GFDL-CM2.0 gives the best performance. The reason for the poor performance of most models in simulating the East Asian summer monsoon interdecadal variation lies in that the key dynamic and thermal-dynamic mechanisms behind the East Asian monsoon change are missed by the models, e.g., the large-scale tropospheric cooling and drying over East Asia. In contrast, the Category-1 models relatively well reproduce the variations in vertical velocity and water vapor over East Asia and thus show a better agreement with observations in simulating the pattern of ＂wet south and dry north＂ in China in the past 20 years.
It is assessed that a single model＇s performance in simulating a particular variable has great impacts on the ensemble results. More realistic outputs can be obtained when the multi-model ensemble is carried out using a suite of well-performing models for a specific variable, rather than using all available models. This indicates that although a multi-model ensemble is in general better than a single model, the best ensemble mean cannot be achieved without looking into each member model＇s performance.  相似文献   

喜马拉雅山地区地气间物质交换及其与南亚夏季风的联系   总被引：2，自引：1，他引：1  

周立波  邹捍  马舒坡  李鹏  朱金焕  霍翠萍 《气候与环境研究》2010,15(3):289-294

喜马拉雅山是青藏高原的重要组成部分,是大型山地的代表。该地区陡峭的地形和复杂的地表状态在强烈太阳辐射条件下形成了特殊的局地环流系统。该特殊局地环流系统所导致的地气交换过程可能不同于平坦地形和其他山区。喜马拉雅山毗邻南亚季风区,该地区的地气交换过程也可能受到南亚季风活动的影响。为正确认识喜马拉雅山地区的地气交换过程,利用2006年夏季喜马拉雅山北侧绒布河谷地区获得大气观测资料,结合同期的大气环流资料,对绒布河谷地区地气间的物质交换进行研究。结果表明:1)该地区的地气间物质交换以午后至次日凌晨强烈的向下输送为主;观测期间平均向下输送强度为7.9×106m3.s-1,相当于每天将整个封闭河谷内大气置换约38次;2)该地区地气间的物质输送与南亚夏季风存在密切关系,南亚夏季风活动弱(季风中断期)则物质交换量大(9.7×106m3.s-1),季风活动强(季风活跃期)则物质交换量小(6.6×106m3.s-1);3)南亚夏季风可能主要通过改变局地大气辐射状况进而影响该地区地气间的物质交换过程。  相似文献   

东亚大气环流由冬向夏的转变时间及其特征   总被引：4，自引：0，他引：4  

何金海  祁莉  刘丹妮  朱占云 《气象科学》2010,30(5):591-596

利用NCEP/NCAR再分析数据集及CMAP降水资料分析了东亚大气环流由冬转夏的可能时间及其特征。结果表明,3月底4月初,东亚与西太平洋对流层纬向热力差异由东暖西冷转为东冷西暖,对流层低层大陆高压东移,使得纬向气压梯度发生逆转。与此同时,对流层低层偏南风建立,经向垂直环流也发生季节逆转。同时,3月底4月初华南已出现持续性降水雨带。所有这些特征都表明东亚大气环流可能在3月底4月初已经由冬季型开始转为夏季型。  相似文献   

夏季亚洲季风区对流层向平流层输送的源区、路径及其时间尺度的模拟研究   总被引：9，自引：4，他引：5  

陈斌  徐祥德  卞建春 《大气科学》2010,34(3):495-505

基于NCEP/NCAR分析资料和拉格朗日轨迹输送模式FLEXPART, 通过气块轨迹计算, 对2005年夏季亚洲季风区对流层向平流层输送 (Troposphere to Stratosphere Transport, 简称TST) 的近地层源区、 输送路径及其时间尺度问题进行了一些初步探讨。结果表明: (1) 夏季亚洲季风区TST两个主要的边界层源区, 一个是热带西太平洋地区; 另一个是青藏高原南部、 孟加拉湾以及印度半岛中北部等地区, 上述两个区域与夏季强对流的分布相一致。在对流层顶高度附近 (约16 km高度), 两个近地层源区的垂直输送贡献相当。但进一步分析发现, 穿越对流层顶高度的质量输送只有约10％能够进入20～22 km高度的平流层中, 且主要源于以青藏高原南侧为代表的南亚季风区 (约贡献75%), 这进一步强调了青藏高原及其周边区域在全球TST过程中的重要地位。 (2) 轨迹分析显示, 夏季亚洲季风区对流层进入平流层的 “入口区” 主要在 (25°N～35°N, 90°E～110°E) 区域的青藏高原及其周边区域。TST路径受对流层上层南亚高压闭合环流、 北半球副热带西风急流和赤道东风急流的共同控制。 (3) 亚洲季风区TST两个主要的过程, 一个是和夏季湿对流抬升直接联系的快速输送过程, 它可以使近地层大气在1～2天内输送到平流层中, 贡献了整个TST的10%～30%; 另一个是大气辐射加热所致的大尺度垂直输送, 该输送是一个相对的慢过程, 时间尺度一般为5～30天。此结果意味着, 源于地表的短生命周期的大气污染物可通过光化学反应过程对该区域平流层臭氧及其他大气痕量成分平衡产生重要影响。  相似文献   

亚洲夏季风区中尺度地形降水结构及分布特征   总被引：4，自引：0，他引：4  

朱素行  徐海明  徐蜜蜜 《大气科学》2010,34(1):71-82

采用高分辨率TRMM、AIRS卫星实测资料, 从气候态的降水微物理过程角度分析了亚洲夏季风期间中尺度山脉对不同性质降水垂直结构和水平分布的影响。研究表明, 中尺度山脉迎风、背风坡均以层云降水为主, 层云降水强度在迎风坡强于背风坡; 对流降水在迎风坡主要为浅对流, 背风坡主要为深对流, 对流降水强度在背风坡强于迎风坡。沿西南季风推进方向依次经过的中尺度山脉, 其两侧发生降水像素个数、 降水微物理特征等差异逐渐减小, 其中, 对流降水迎风坡向背风坡转变明显, 而层云降水背风坡向迎风坡转变明显。大气稳定度与对流降水在迎风、背风坡的分布相一致。另外, 对中尺度地形降水的研究为区域气候模式模拟高精度地形降水分布提供了实测依据。  相似文献