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The kinetics of the reactions of C2H radical with ethane (k1), propane (k2), and n-butane (k3) are studied over the temperature range of T = 96-296 K with a pulsed Laval nozzle apparatus that utilizes a pulsed laser photolysis-chemiluminescence technique. The C2H decay profiles in the presence of both the alkane reactant and O2 are monitored by the CH(A2Δ) chemiluminescence tracer method. The results, together with available literature data, yield the following Arrhenius expressions: k1(T) = (0.51 ± 0.06) × 10−10 exp[(−76 ± 30)K/T] cm3 molecule−1 s−1 (T = 96-800 K), k2(T) = (0.98 ± 0.32) × 10−10exp[(−71 ± 60)K/T] cm3 molecule−1 s−1 (T = 96-361 K), and k3(T) = (1.23 ± 0.26) × 10−10 cm3 molecule−1 s−1 (T = 96-297 K). At T = 296 K, k1 is measured as a function of total pressure and has little or no pressure dependence. The results from this work support a direct hydrogen abstraction mechanism for the title reactions. Implications to the atmospheric chemistry of Titan are discussed. 相似文献
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Mars Global Surveyor accelerometer observations of the martian upper atmosphere revealed large variations in density with longitude during northern hemisphere spring at altitudes of 130-160 km, all latitudes, and mid-afternoon local solar times (LSTs). This zonal structure is due to tides from the surface. The zonal structure is stable on timescales of weeks, decays with increasing altitude above 130 km, and is dominated by wave-3 (average amplitude 22% of mean density) and wave-2 (18%) harmonics. The phases of these harmonics are constant with both altitude and latitude, though their amplitudes change significantly with latitude. Near the South Pole, the phase of the wave-2 harmonic changes by 90° with a change of half a martian solar day while the wave-3 phase stays constant, suggesting diurnal and semidiurnal behaviour, respectively. We use a simple application of classical tidal theory to identify the dominant tidal modes and obtain results consistent with those of General Circulation Models. Our method is less rigorous, but simpler, than the General Circulation Models and hence complements them. Topography has a strong influence on the zonal structure. 相似文献
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1 IntroductionAccordingtogeologicalstructure ,theGansu Ningxia Qinghaiareabelongstothenortheastmar ginofQinghai Tibetblock .Thisareahasbeenpaidmuchattentionby geo specialistsinChinaandabroadbecauseofitssignificanttectonicmovement,itsintensiveseismicity ,anditsimportanceinearth quakehazardmitigation .IntheDevelopmentPro gramonNationalKeyBasicResearchesundertheProject“MechanismandPredictionofContinentalStrongEarthquakes”,themechanismsofcontinen talstrongearthquakesarestudied ,usinghypo… 相似文献
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本文简要介绍了陆地系列地球资源卫星的轨道特征,并以陆地—5号资源卫星为例,根据南山站的座标计算出该站对陆地—5号资源卫星的可观测范围及以该站为中心的卫星的覆盖区域。 相似文献
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Xue-Fei Chen Zhan-Wen HanNational Astronomical Observatories Yunnan Observatory Chinese Academy of Sciences. Kunming Graduate School of the Chinese Academy of Sciences Beijing 《中国天文和天体物理学报》2005,5(1):65-76
We have studied the influence of different choices of core-envelope transition point on the final merger of contact binaries with two main-sequence components. A binary of 1.00 + 0.90M⊙ with an initial orbital period of 0.35d is examined. The mass fraction of the primary mixed with the matter of the secondary, qmix, determined by the chosen core-envelope transition point, ranges from 0.04 to 1.00 in our analysis. If as qmix< 0.8, none of the 相似文献
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ENVIRONMENTAL SUSTAINABILITY AND SCENARIOS OF URBANIZATION IN ARID AREA——A Case Study in Wuwei City of Gansu Province 总被引:1,自引:0,他引:1
YOUFei LIYu DONGSuo-cheng 《中国地理科学(英文版)》2005,15(2):120-130
1IN T R O D U C T IO N The western China isfacinggrowing problems of eco- logicaland economic development. The disparitiebse- tween the socio-economy of the western and eastern China were enlarging, and the major ecologicalprob- lems stilelvolve as past(H… 相似文献
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