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21.
《Chemie der Erde / Geochemistry》2019,79(4):125524
Due to their common occurrence in various types of chondrites, igneous rims formed on pre-existing chondrules throughout chondrule-forming regions of the solar nebula. Although the peak temperatures are thought to reach similar values to those achieved during chondrule formation events, the heating duration in chondrule rim formation has not been well defined. We determined the two-dimensional chemical and oxygen isotopic distributions in an igneous rim of a chondrule within the Northwest Africa 3118 CV3oxA chondrite with sub-micrometer resolution using secondary ion mass spectrometry and scanning electron microscopy. The igneous rim experienced aqueous alteration on the CV parent body. The aqueous alteration resulted in precipitation of the secondary FeO-rich olivine (Fa40–49) and slightly disturbed the Fe-Mg distribution in the MgO-rich olivine phenocrysts (Fa11–22) at about a 1 μm scale. However, no oxygen isotopic disturbances were observed at a scale greater than 100 nm. The MgO-rich olivine, a primary phase of igneous rim formation, has δ17O = −6 ± 3‰ and δ18O = −1 ± 4‰, and some grains contain extreme 16O-rich areas (δ17O, δ18O = ∼−30‰) nearly 10 μm across. We detected oxygen isotopic migration of approximately 1 μm at the boundaries of the extreme 16O-rich areas. Using oxygen self-diffusivity in olivine, the heating time of the igneous rim formation could have continued from several hours to several days at near liquidus temperatures (∼2000 K) in the solar nebula suggesting that the rim formed by a similar flash heating event that formed the chondrules. 相似文献
22.
南辽河群斜长角闪岩的地球化学特征及地质意义:以三家子地区为例 总被引:1,自引:0,他引:1
基于详细的野外地质调查,对南辽河群下部里尔峪组斜长角闪岩进行了岩相学和地球化学研究。岩相学研究表明,南辽河群下部里尔峪组斜长角闪岩属于正变质岩。地球化学研究显示,这些斜长角闪岩原岩属于高铁拉斑玄武岩系列(Nb/Y=0.16~0.4),SiO_2含量为47.27%~50.68%,具有较低的TiO_2含量(0.92%~1.61%),亏损高场强元素(Nb、Ta、Zr、Hf等),表明其原岩形成于岛弧或活动大陆边缘,而非前人所说的大陆裂谷。综合岩相学和地球化学特征,初步认为其岩石成因与活动大陆边缘有关。 相似文献
23.
1992年冲绳海槽地质调查时,在134站(126°56′7″E,27°30′0″N)共采集到3件玄武岩样品,其中1件取自134站表层样,另外2件取自134站柱状样中的118-143cm处和193- 218cm处(刀口位置)。通过对上述3件玄武岩样品的岩相学、岩石化学组成、稀土元素和微量元素和锶同位素比值分析研究,认为本区玄武岩具多期次喷发特征,早期喷发形成的玄武岩中单斜辉石质量分数较低,晚期喷发形成的玄武岩中单斜辉石质量分数相对较高,表明了单斜辉石为晚期结晶堆积产物。本区玄武岩稀土配分模式与岛弧拉斑玄武岩基本一致,其87Sr与86Sr质量分数比值m(87Sr)/m(86Sr)为0.7046,亦与岛弧拉斑玄武岩相当。最后利用Rb-Sr丰度特征确定本区的地壳厚度为19-24 km。 相似文献
24.
Structural parameters and cation ordering are determined for four compositions in the synthetic MgGa2O4-Mg2GeO4 spinel solid solution (0, 8, 15 and 23 mol% Mg2GeO4; 1400 °C, 1 bar) and for spinelloid β-Mg3Ga2GeO8 (1350 °C, 1 bar), by Rietveld refinement of room-temperature neutron diffraction data. Sample chemistry is determined by
XRF and EPMA. Addition of Mg2GeO4 causes the cation distribution of the MgGa2O4 component to change from a disordered inverse distribution in end member MgGa2O4, [4]Ga = x = 0.88(3), through the random distribution, toward a normal cation distribution, x = 0.37(3), at 23 mol% Mg2GeO4. An increase in ao with increasing Mg2GeO4 component is correlated with an increase in the amount of Mg on the tetrahedral site, through substitution of 2 Ga3+⇄ Mg2++Ge4+. The spinel exhibits high configurational entropy, reaching 20.2 J mol−1 (four oxygen basis) near the compositional upper limit of the solid solution. This stabilizes the spinel in spite of positive
enthalpy of disordering over the solid solution, where ΔH
D
= αx + βx
2, α = 22(3), β = −21(3) kJ mol−1. This model for the cation distribution across the join suggests that the empirically determined limit of the spinel solid
solution is correlated with the limit of tetrahedral ordering of Mg, after which local charge-balanced substitution is no
longer maintained.
Spinelloid β-Mg3Ga2GeO8 has cation distribution M1[Mg0.50(2)Ga0.50(2)] M2[Mg0.96(2)Ga0.04(2)] M3[Mg0.77(2) Ga0.23(2)]2 (Ge0.5Ga0.5)2O8 (tetrahedral site occupancies are assumed). Octahedral site size is correlated to Mg distribution, where site volume, site
distortion, and Mg content follow the relation M1<M3<M2. The disordered cation distribution provides local electrical neutrality
in the structure, and stabilization through increased configurational entropy (27.6 J mol−1; eight oxygen basis). Comparison of the crystal structures of Mg1+
N
Ga2−2
N
Ge
N
O4 spinel, β-Mg3Ga2GeO8, and Mg2GeO4 olivine reveals β-Mg3Ga2GeO8 to be a true structural intermediate. Phase transitions across the pseudobinary are necessary to accommodate an increasing
divergence of cation size and valence, with addition of Mg2GeO4 component. Octahedral volume increases while tetrahedral volume decreases from spinel to β-Mg3Ga2GeO8 to olivine, with addition of Mg and Ge, respectively. Furthermore, M-M distances increase regularly across the join, suggesting
that changes in topology reduce cation-cation repulsion.
Received: 9 November 1998 / Revised, accepted: 3 August 1999 相似文献
25.
R. Rinaldi G. Artioli C. C. Wilson G. McIntyre 《Physics and Chemistry of Minerals》2000,27(9):623-629
Crystallographic determinations on natural olivine single crystals of mantle composition and origin, carried out by in situ neutron diffraction at high temperature, show that the octahedrally co-ordinated Fe2+ and Mg cations undergo two successive trends of cation ordering with increasing temperature. An initial slight preference of Fe2+ for site M1, up to a temperature of about 850?°C, is followed by a reverse-ordering reaction with a site preference exchange between the two cations. The cross-over between the two regimes of ordering, corresponding to a situation of complete disorder, occurs at about 900?°C. Above this temperature Fe2+ progressively and strongly segregates into site M2 up to 1300?°C, the practical limit of the experimental setup utilized in the experiments. Care was taken to ensure that no chemical changes occurred in the crystals (i.e. oxidation), as testified by Mössbauer spectroscopy determinations carried out before and after the heat treatment. The cation-ordering behaviour is reflected in temperature-dependent changes of geometrical and atomic displacement parameters occurring in the octahedral sites M1 and M2. A thermodynamical explanation of this behaviour is proposed in terms of a prevailing vibrational contribution to entropy. 相似文献
26.
岩石圈流变实验研究的进展 总被引:2,自引:2,他引:0
岩石高温高压变形实验是了解地球内部物质流动特性的最直接的手段 .本文概述了近年来岩石流变实验研究的一些成果 ,重点总结了水和部分熔融对上地幔顶部橄榄石流变行为的影响 ,以及地壳多相岩石流变实验研究的一些成果 . 相似文献
27.
28.
We present experiments showing that the lower oceanic crust should melt efficiently and quickly when heated by hot ascending
magmas. Average plagioclase–olivine and plagioclase–augite pairs from the lower crust at the Southwest Indian Ridge have melt–mineral
saturation boundaries at 1,190 and 1,154°C, respectively, and melt rapidly (>0.01 mm/h) at 50°C or more above these temperatures.
Melting experiments performed on olivine–plagioclase and augite–plagioclase mineral pairs from actual oceanic lower crustal
rock samples and under conditions applicable to a MOR setting (1,220–1,330°C, 1 atm, quartz–fayalite–magnetite oxygen buffer,
0.25–24 h) indicate that the resulting disequilibrium melts are linear mixes of the mineral compositions. The rates of melting
are slower than the rate of heat-diffusion into a sample and are approximated as:
Our results indicate that great care must be taken in backward models using basalt chemistry alone to explore mantle-melting
processes, assuming only crystallization and fractionation during ascent, as partial melts may mix with intruded hot magma. 相似文献
29.
Zhang Shimin Dou Suqin 《地壳构造与地壳应力文集》1997,(1)
一、引言大同第四纪火山群位于山西省大同县和阳高县境内(图1),包括近5年来在大峪口,秋林地区首次发现的6个小火山。该火山群大、小火山共计31个。大同火山群南以六棱山北麓断裂为界,分布于大同盆地东部的第四纪沉积区范围。火山群南侧的六棱山和北部的小北山是由前寒武花岗片麻岩组成的山地。 相似文献
30.
黔西二叠纪玄武岩及岩浆来源初步分析 总被引:2,自引:0,他引:2
本文以织金熊家场剖面为例进行岩石学及岩浆来源分析研究。岩性和岩石化学特征表明,区内玄武岩为碱性—钙碱性拉斑玄武岩。同位素地球化学和稀土元素分布模式研究资料表明,本区玄武岩原始岩浆来源于地壳和地幔二元组分相混合的体系。通过锶同位素组成的计算,显示了原始岩浆中的幔源和壳源二元组分的混合比例为5.4:1。 相似文献