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21.
The distribution of several minor and trace elements mainly in fresh (dominating TDS 160–400 mg/l) groundwater of Latvia have
been investigated by the Inductively Coupled Plasma-Mass Spectrometry (ICP-MS) technique. An evaluation of results of about
700 analyses leads to the conclusion that concentrations of these elements is influenced by: pH–Eh conditions, groundwater
residence time and diffuse contamination, whereas the role of water-bearing sediments is of secondary importance. Most trace
elements are characterised by low mobility under alkaline and reducing conditions; concentrations in confined aquifers are
much smaller than the Maximum Permissible Values for drinking water. The strongest anomalies of REE, Al and P were found in
shallow groundwater around the former agrochemical storehouses. 相似文献
22.
Plagioclase ultraphyric basalts (PUBs) with up to 54% plagioclasephenocrysts were dredged in the rift valley and adjacent flanksof the ultraslow-spreading Mohns and Knipovich ridges. The PUBsshow large variations in crystal morphologies and zoning. Thelarge variations suggest that single basalt samples containa mixture of plagioclase crystals that aggregated at differentlevels in the magma conduits. Resorbed crystals and repeatedreverse zones suggest that the magma reservoirs were replenishedand heated several times. Thin concentric zones with melt inclusions,and sharp reductions in the anorthite content of 3–7%,are common between the reverse zones. These zones, and skeletalcrystals with distinctly lower anorthite contents than massivecrystals, are interpreted to be the result of rapid crystalliztionduring strong undercooling. The changes between short periodsof cooling and longer periods with reheating are explained bymultiple advances of crystal-rich magma into cool regions followedby longer periods of gradual magma inflow and temperature increase.The porphyritic basalts are characterizd by more depleted andmore fractionated compositions than the aphyric basalts, withlower (La/Sm)N, K2O and Mg-numbers. This relationship, and theobservation that PUBs are sampled only close to segment centresalong these ridges, suggests that the PUBs formed by higherdegrees of melting and evolved in more long-lived magma reservoirs.We propose that the zoning patterns of plagioclase crystalsand crystal morphologies of these PUBs reflect the developmentand flow of magma through a stacked sill complex-like conduitsystem, whereas the aphyric equivalents represent later flowof magma through the conduit. The formation of voluminous higher-degreemelts may trigger the development of the magma conduits andexplain the generally depleted compositions of PUB magmas. KEY WORDS: basalt; mineral chemistry; MORB; magma mixing; magma chamber; major element 相似文献
23.
Global Correlations of Ocean Ridge Basalt Chemistry with Axial Depth: a New Perspective 总被引:4,自引:0,他引:4
The petrological parameters Na8 and Fe8, which are Na2O andFeO contents in mid-ocean ridge basalt (MORB) melts correctedfor fractionation effects to MgO = 8 wt%, have been widely usedas indicators of the extent and pressure of mantle melting beneathocean ridges. We find that these parameters are unreliable.Fe8 is used to compute the mantle solidus depth (Po) and temperature(To), and it is the values and range of Fe8 that have led tothe notion that mantle potential temperature variation of TP= 250 K is required to explain the global ocean ridge systematics.This interpreted TP = 250 K range applies to ocean ridges awayfrom hotspots. We find no convincing evidencethat calculated values for Po, To, and TP using Fe8 have anysignificance. We correct for fractionation effect to Mg# = 0·72,which reveals mostly signals of mantle processes because meltswith Mg# = 0·72 are in equilibrium with mantle olivineof Fo89·6 (vs evolved olivine of Fo88·1–79·6in equilibrium with melts of Fe8). To reveal first-order MORBchemical systematics as a function of ridge axial depth, weaverage out possible effects of spreading rate variation, local-scalemantle source heterogeneity, melting region geometry variation,and dynamic topography on regional and segment scales by usingactual sample depths, regardless of geographical location, withineach of 22 ridge depth intervals of 250 m on a global scale.These depth-interval averages give Fe72 = 7·5–8·5,which would give TP = 41 K (vs 250 K based on Fe8) beneathglobal ocean ridges. The lack of Fe72–Si72 and Si72–ridgedepth correlations provides no evidence that MORB melts preservepressure signatures as a function of ridge axial depth. We thusfind no convincing evidence for TP > 50 K beneath globalocean ridges. The averages have also revealed significantcorrelations of MORB chemistry (e.g. Ti72, Al72, Fe72,Mg72, Ca72, Na72 and Ca72/Al72) with ridge axial depth. Thechemistry–depth correlation points to an intrinsic linkbetween the two. That is, the 5 km global ridge axial reliefand MORB chemistry both result from a common cause: subsolidusmantle compositional variation (vs TP), which determines themineralogy, lithology and density variations that (1) isostaticallycompensate the 5 km ocean ridge relief and (2) determine thefirst-order MORB compositional variation on a global scale.A progressively more enriched (or less depleted) fertileperidotite source (i.e. high Al2O3 and Na2O, and low CaO/Al2O3)beneath deep ridges ensures a greater amount of modal garnet(high Al2O3) and higher jadeite/diopside ratios in clinopyroxene(high Na2O and Al2O3, and lower CaO), making a denser mantle,and thus deeper ridges. The dense fertile mantle beneath deepridges retards the rate and restricts the amplitude of the upwelling,reduces the rate and extent of decompression melting, givesway to conductive cooling to a deep level, forces melting tostop at such a deep level, leads to a short melting column,and thus produces less melt and probably a thin magmatic crustrelative to the less dense (more refractory) fertile mantlebeneath shallow ridges. Compositions of primitive MORB meltsresult from the combination of two different, but geneticallyrelated processes: (1) mantle source inheritance and (2) meltingprocess enhancement. The subsolidus mantle compositional variationneeded to explain MORB chemistry and ridge axial depth variationrequires a deep isostatic compensation depth, probably in thetransition zone. Therefore, although ocean ridges are of shalloworigin, their working is largely controlled by deep processesas well as the effect of plate spreading rate variation at shallowlevels. KEY WORDS: mid-ocean ridges; mantle melting; magma differentiation; petrogenesis; MORB chemistry variation; ridge depth variation; global correlations; mantle compositional variation; mantle source density variation; mantle potential temperature variation; isostatic compensation 相似文献
24.
海水中234Th的超低水平液闪谱仪测定 总被引:2,自引:1,他引:2
本文提出了利用超低水平液闪谱仪测定海水中234Th的方法.海水经氢氧化铁吸附共沉淀富集后,接着用阴离子交换和TBP/煤油萃取进行Th同位素的分离与纯化.对一系列测定条件进行了详细的研究,提出了测定海水中234Th的适宜程序,即在含有234Th和产额示踪剂230Th的纯化后的5mol/dm3HNO3溶液中加入TBP/煤油进行萃取,然后用0.1mol/dm3HNO3反萃取,后者是先用契伦柯夫计数法测量234Th(通过234mPa),后加入闪烁液Hisafe 3用α/β模式测量α放射体230Th.对于α和β放射体液闪谱仪的计数效率分别为100%和55.7%±2.7%.234Th的化学回收率和总探测效率分别为70%~80%和30%~45%.该法测定海水中的234Th快速、简便和高效. 相似文献
25.
于1995—1996年在厦门海域采集了28种鱼类样品,用ICP—MS法测定了15种稀土元素(REE)的含量,研究了鱼体稀土元素的组成和分布模式及与海水环境之间的关系。结果表明,厦门海域鱼体REE总量介于12.4—596.5ng/g,平均为(77.5l2.8)岭g。鱼体明显官集轻稀土,同时轻、重稀土之间则存在较大的分馏作用,说明轻稀土的生物学效应比重稀土更为显著。鱼类稀土元素分布模式总体上与海水REE分布模式接近,并且鱼类REE含量与近岸陆架海水REE含量之间有很好的相关性,说明海洋鱼类对稀土元素的利用遵从丰度规律。鱼类对稀土元素的富集系数在103以上。稀土元素沿厦门海域食物链的迁移传递没有表现出明显的生物放大作用。 相似文献
26.
Based on the recent research results on dry and wet deposition of nutrient elements and sulphate,we estimate the atmospheric flux of nutrient elements and sulphate to the southern Yellow Sea and the East China Sea in each season.The results suggest that the concentrations of nutrient elements and sulphate in aerosol and precipitation show an apparent seasonal cycle with the maximum values in winter and the minimum values in summer.Depositions of nitrate and sulphate are dominated by wet deposition,while the deposition for phosphate is mainly dry deposition.Moreover,compared with the riverine inputs,the atmospheric deposition may be the main source of dissolved inorganic nutrients in the southern Yellow Sea and the East China Sea. 相似文献
27.
九龙江河口区水体中的226Ra和228Ra 总被引:8,自引:0,他引:8
用MnO2-纤维富集大体积水样中的Ra同位素,并用直接射气法测定226Ra和228Ac的β计数法测定228Ra的方法,研究了九龙江河口区226Ra,228Ra的行为,结果表明:在该河口区226Ra,228Ra均呈非保守行为,226Ra,228Ra的最高值分别在盐度为19和9处测得。228Ra/226Ra)A.R.值在盐度小于19的区域约为3左右。与世界其他河口区相比,九龙江河口区的226Ra,22 相似文献
28.
Weather in the North Gulf of Alaska is characterized by a high frequency of deep synoptic-scale low-pressure systems, especially during the cold season. The strong pressure gradients of these storms interact with the extremely rugged terrain of the coastal mountains to produce a variety of channeled flows. These surface wind regimes are not well documented in the scientific community, due to the paucity of observations. Modeling of these phenomena in regions of complex terrain is of great interest to those working with hydrodynamic, wave, and pollutant transport models in coastal and shelf areas. Such models, when coupled with ocean and coastal-ecology counterparts, give a broad view of the role surface winds play in shaping local coastal marine ecosystem in this region. This paper presents a climatology of simulated low-level wind jets over the domain of Cook Inlet and Shelikof Strait along Alaska's south-central coast. Daily simulations using the RAMS model were conducted in a 36-h forecast mode for the cold-season period 10/1/03 to 3/31/04. Systematic analysis of the resulting simulated low-level wind field makes it possible to characterize these jets and gap flows in spatial and temporal detail. The comparison between the RAMS winds and the Synthetic Aperture Radar (SAR)-derived winds when available verifies the existence of these wind jets and the capability of the model to simulate these cases. Clearly, the results of a study in this region depend on the fidelity of the model at these scales (O[5 km]). The SAR comparisons attempt to help establish this. From the 6 months of simulations over Cook Inlet and Shelikof Strait, the low-level wind jets are classified into 10 different regimes by location and orientation. These regimes are categorized into four more general groups: cross-channel westerly, easterly, and up and down Inlet flows. The nature of a particular regime is largely a function of pressure gradient orientation and local topography. Jets in the same group have a similar occurrence distribution with time. Some form of jet occurred in the study region almost daily each month of the period, with December 2003 having the highest frequency of wind jets. 相似文献
29.
对1999年9~10月采自北太平洋亚热带环流区的19份表层海水样品的Ra同位素分析表明。研究海域表层水中的^226Ra、^228Ra放射性比度分别介于0.67~0.92、0.08~0.30Bq/m^3之间,平均值分别为0.74、0.11Bq/m^3.^226Ra/^228Ra)A.R.活度比的变化范围为0.11~0.44,平均值为0.19.上述数值明显低于近岸海域水体的相应值,表现为典型的开阔大洋水的特征.从空间分布的特征看,研究海域Ra同位素含量与^226Ra/^228Ra)A.R.值均呈均匀分布态势.将本研究结果与历史数据进行对比后发现,本研究获得的^226Ra、^228Ra放射性比度比20世纪60~80年代得到的数据来得低,可能与水体层化作用加强导致的Ra补充量的减少以及生物生产力升高导致的Ra迁出量的增加有关.北太平洋亚热带环流区表层水中Ra同位素的时间变化与文献报道的该海域叶绿素a、硅酸盐、磷酸盐含量与初级生产力的历史变化趋势相吻合. 相似文献
30.
Atmospherically-promoted photosynthetic activity in a well-mixed ecosystem: Significance of wet deposition events of nitrogen compounds 总被引:1,自引:0,他引:1
C. Boulart P. Flament V. Gentilhomme K. Deboudt C. Migon F. Lizon M. Schapira A. Lefebvre 《Estuarine, Coastal and Shelf Science》2006,69(3-4):449
Wet atmospheric deposition of dissolved N, P and Si species is studied in well-mixed coastal ecosystem to evaluate its potential to stimulate photosynthetic activities in nutrient-depleted conditions. Our results show that, during spring, seawater is greatly depleted in major nutrients: Dissolved Inorganic Nitrogen (DIN), Dissolved Inorganic Phosphorus (DIP) and Silicic acid (Si), in parallel with an increase of phytoplanktonic biomass. In spring (March–May) and summer (June–September), wet atmospheric deposition is the predominant source (>60%, relative to riverine contribution) for nitrates and ammonium inputs to this N-limited coastal ecosystem. During winter (October–February), riverine inputs of DIN predominate (>80%) and are annually the most important source of DIP (>90%). This situation allows us to calculate the possibility for a significant contribution to primary production in May 2003, from atmospheric deposition (total input for DIN ≈300 kg km−2 month−1). Based on usual Redfield ratios and assuming that all of the atmospheric-derived N (AD-N) in rainwater is bioavailable for phytoplankton growth, we can estimate new production due to AD-N of 950 mg C m−2 month−1, during this period of depletion in the water column. During the same episode (May 2003), photosynthetic activity rate, considered as gross primary production, was estimated to approximately 30 300 mg C m−2 month−1. Calculation indicates that new photosynthetic activity due to wet atmospheric inputs of nitrogen could be up to 3%. 相似文献