Establishment of an assessment method for site-scale suitability of CO2 geological storage     

ZHANG Wei 《地下水科学与工程》2014,2(4):19-25

Geological storage of CO2 (known as geological sequestration) is increasingly seen as a viable strategy to reduce the release of greenhouse gases into the atmosphere. China has become one of the largest emitters of CO2 in the world. Therefore, alongside other emissions reductions measures, the deployment of geological storage projects to capture CO2 in China is essential. This paper focuses on the establishment of qualitative and quantitative assessment methods for site-scale suitability of CO2 geological storage in deep saline formation systems. This is based on numerical modelling prior to the development a specific geological storage project, providing a more accurate selection of preferential sites from a list of potential storage locations. However, the detailed design of specific geological storage projects was not con?sidered.  相似文献   

Impact of Urbanization on Local Air Quality: Differences in Urban and Rural Areas of Balikesir,Turkey          下载免费PDF全文

Lokman Hakan Tecer  Sermin Tagil 《洁净——土壤、空气、水》2014,42(11):1489-1499

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一次能源消费导致的二氧化碳排放量变化   总被引：12，自引：4，他引：8  

郭义强  郑景云  葛全胜 《地理研究》2010,29(6):1027-1036

从不同燃料和不同地区入手,分析了我国1995~2006年间一次能源消费导致的二氧化碳排放量变化情况。结果表明:1995~2006年间,我国一次能源消费导致的二氧化碳年总排放量呈现"先减少后增加"的发展态势,其拐点出现在2000年,而且2001年后各个省(区、市)的二氧化碳年排放量较前期均有大幅度的增加,总排放量由1995年的78678万t碳增长到2006年的146919万t碳,年均增长率5.84％,人均二氧化碳年排放量也由0.62t碳/人增加到1.12t碳/人;煤炭消费导致的二氧化碳排放量占全国二氧化碳年总排放量的79%~85％;我国七大区和大部分省(区、市)二氧化碳年排放量与全国总排放量有类似的发展态势,其中华北、华东地区二氧化碳排放量居全国首位,山西省的二氧化碳排放量位居全国第一。  相似文献   

BOOK REVIEWS     

《The Professional geographer》1984,36(4):498-530

Book reviewed is the article: Small-State Security in the Balkans . Aurel Braun. South American Development: A Geographical Introduction . Rosemary D. F. Bromley and Ray Bromley. Interregional Migration, National Policy and Social Justice . Gordon L. Clark. Marketing Architectural and Engineering Services . Weld Coxe. A Geography of the Third World . J. P. Dickenson, C. G. Clarke, W. T. S. Gould, R. M. Prothero, D. J. Siddle, C. T. Smith, E. M. Thomas-Hope, and A. G. Hodgkiss. Wildlife and Man in Texas: Environmental Change and Conservation . Robin W. Doughty. At the Sea's Edge . William T. Fox. Englewood Cliffs Geography and Ecology . I. P. Gerasimov. Urbanization in Contemporary Latin America. Critical Approaches to the Analysis of Urban Issues . Alan Gilbert in association with Jorge E. Hardoy and Ronaldo Ramírez, eds. The Coming of the Transactional City . Jean Gottmann. College Park Visions of City and Country: Prints and Photographs of Nineteenth-Century France . Bonnie L. Grad and Timothy A. Riggs. Worcester Soviet Geography Today: Physical Geography . N. A. Gvozdetskiy, ed. Adaptive Responses of Native Amazonians . Raymond B. Hames and William T. Vickers, eds. Urban and Regional Industrial Research: The Changing UK Data Base . Michael Healey, ed. Cuando se Acaban los Montes . Stanley Heckadon Moreno. A Panama Forest and Shore: Natural History and Amerindian Culture in Bocas del Toro . Burton L. Gordon. Pacific Grove Mozambique: From Colonialism to Revolution, 1900–1982 . Allen Isaacman and Barbara Isaacman. Soviet Natural Resources in the World Economy . Robert G. Jensen, Theodore Shabad, and Arthur W. Wright, eds. The Changing Geography of the United Kingdom . R. J. Johnston and J. C. Doornkamp, eds. Pluralism and Political Geography—People, Territory and State . Nurit Kliot and Stanley Waterman, eds. Landmarks Preservation and the Property Tax . David Listokin. Irrigation Horticulture in Highland Guatemala: The Tablón System of Panajachel . Kent Mathewson. Her Space, Her Place: A Geography of Women . Mary Ellen Mazey and David R. Lee. Man, A Geomorphological Agent . Dov Nir. Dordrecht The Book of America: Inside the 50 States Today . Neal R. Peirce and Jerry Hagstrom. Rivers . Geoffrey E. Petts. Proceedings, United States/Australia Workshop on Design and Implementation of Computer-Based Geographic Information Systems . Donna Peuquet and John O'Callaghan, eds. Outdoor Recreational and Resource Management . John Pigram. Remaking the City: Social Science Perspectives on Urban Design . John S. Pipkin, Mark La Gory and Judith R. Blau, eds. The Crust of Our Earth: An Armchair Traveler's Guide to the New Geology . Chet Raymo. Englewood Cliffs Concepts and Themes in the Regional Geography of Canada J. Lewis Robinson. Vancouver Secondary Cities in Developing Countries: Policies for Diffusing Urbanization . Dennis A. Rondinelli. Beverly Hills Legal Foundations of Environmental Planning , Vol 1. J. G. Rose. Can We Delay a Greenhouse Warming? Stephen Seidel and Dale Keyes. Mobilizing Human Resources in the Arab World . R. Paul Shaw. Prairie Mosaic: An Ethnic Atlas of Rural North Dakota . William C. Sherman. The Future of Conflict in the 1980s . William J. Taylor, Jr. and Steven A. Maaranen, eds. The Visual Display of Quantitative Information . Edward R. Tufte. U.S. 40 Today: Thirty Years of landscape Change in America . Thomas R. Vale and Geraldine R. Vale. Madison Silent Violence: Food, Famine and Peasantry in Northern Nigeria . Michael Watts. Readings in Historic Preservation: Why? What? How? Norman Williams Jr., Edmund Kellogg and Frank Gilbert, eds.  相似文献   

The Heterogeneous Reaction of NO<Subscript>2</Subscript> with NH<Subscript>4</Subscript>Cl: A Molecular Diffusion Tube Study     

Norimichi?TakenakaEmail author  Michel?J.?Rossi 《Journal of Atmospheric Chemistry》2005,50(2):171-194

The heterogeneous interaction of nitrogen dioxide with ammonium chloride was investigated in a molecular diffusion tube experiment at 295–335 K and interpreted using Monte Carlo trajectory calculations. The surface residence time (τ_surf) of NO₂ on NH₄Cl is equal to 15 μs at 295 K, increases with temperature up to 323 K (τ_surf = 45 μs) and probably decreases beyond 323 K. The same experiment also yields uptake coefficients, γ, which are derived from the absolute number of surviving molecules effusing out of the diffusion tube. The rate of uptake of NO₂ on NH₄Cl followed a rate law first order in [NO₂] and the uptake coefficient γ is equal to 7 × 10⁻⁵ at 295 K, increases with temperature up to 323 K (γ = 2.1 × 10⁻⁴) and probably decreases beyond 323 K. Nitrous acid, water and nitrogen were detected as products. From these products, it is concluded that the reaction of NO₂ with NH₄Cl is a reverse disproportionation reaction where two moles of NO₂ result in ammonium nitrite, NH₄NO₂, as an intermediate, and nitryl chloride, NO₂Cl. NH₄NO₂ decomposes in two pathways, one to nitrous acid, HONO and NH₃, the other to nitrogen and water. The branching ratio for the production of HONO + NH₃ to that of N₂ + H₂O is approximately 20 at 298 K and increases with increasing temperature.  相似文献   

Transformation of Aerosol Chemical Properties due to Transport Over a City     

Gerhard?LammelEmail author  Thomas?Engelhardt  Adrian?Leip  Christian?Neusü?  Andreas?R?hrl  Birgit?Wehner  Alfred?Wiedensohler  Paul?Wieser 《Journal of Atmospheric Chemistry》2005,51(1):95-117

The change of the chemical composition of the near-ground level atmospheric aerosol was studied during two summer episodes by a Lagrangian type of experimental approach. Bulk and single-particle chemical analyses of ions and elements in the particulate phase were deployed. N(-III) and N(V) components were also measured in the gas-phase. The measurements were completed by particle size distributions.Secondary inorganic aerosols (SIA) and fine particles of ≈0.2–0.4 μm size were still elevated 50 km downwind of the city. The direct comparison of transport over the city in contrast to transport over the surrounding areas showed that SIA was formed from emission from the city within less than 3 h. Relative increases, i.e., enrichment during transport were observed for primary and secondary aerosol components. The degree of mixing on the individual particle level increased significantly during transport in the area. In particular, newly emitted carbonaceous particles became internally mixed within hours with pre-existing sulphate particles. Mostly due to secondary aerosol formation the average particle size (mass median diameter) of major constituents of the aerosol was significantly decreased while being transported over 13 h. Given recent insights which link fine particles number and mass concentrations with health risks, the results suggest that rural populations in areas which frequently are located within an urban plume might run an elevated health risk relative to populations in areas not affected by urban plumes.  相似文献   

Comparative soil CO2 flux measurements and geostatistical estimation methods on Masaya volcano, Nicaragua     

Jennifer L. Lewicki  Deborah Bergfeld  Carlo Cardellini  Giovanni Chiodini  Domenico Granieri  Nick Varley  Cynthia Werner 《Bulletin of Volcanology》2005,68(1):76-90

We present a comparative study of soil CO₂ flux () measured by five groups (Groups 1–5) at the IAVCEI-CCVG Eighth Workshop on Volcanic Gases on Masaya volcano, Nicaragua. Groups 1–5 measured using the accumulation chamber method at 5-m spacing within a 900 m² grid during a morning (AM) period. These measurements were repeated by Groups 1–3 during an afternoon (PM) period. Measured ranged from 218 to 14,719 g m⁻² day⁻¹. The variability of the five measurements made at each grid point ranged from ±5 to 167%. However, the arithmetic means of fluxes measured over the entire grid and associated total CO₂ emission rate estimates varied between groups by only ±22%. All three groups that made PM measurements reported an 8–19% increase in total emissions over the AM results. Based on a comparison of measurements made during AM and PM times, we argue that this change is due in large part to natural temporal variability of gas flow, rather than to measurement error. In order to estimate the mean and associated CO₂ emission rate of one data set and to map the spatial distribution, we compared six geostatistical methods: arithmetic and minimum variance unbiased estimator means of uninterpolated data, and arithmetic means of data interpolated by the multiquadric radial basis function, ordinary kriging, multi-Gaussian kriging, and sequential Gaussian simulation methods. While the total CO₂ emission rates estimated using the different techniques only varied by ±4.4%, the maps showed important differences. We suggest that the sequential Gaussian simulation method yields the most realistic representation of the spatial distribution of , but a variety of geostatistical methods are appropriate to estimate the total CO₂ emission rate from a study area, which is a primary goal in volcano monitoring research.Editorial responsibility: H Shinohara  相似文献   

Coring experiments with cryogenic water and carbon dioxide ices—toward planetary surface operations     

J.R.C Garry  I.P Wright 《Planetary and Space Science》2004,52(9):823-831

As a prelude to the design of sampling devices able to extract materials from the icy surfaces of comets, outer-planet satellites, and the martian poles, it is necessary to understand some of the physical properties of these ices. To this end we have investigated the mechanical resistance displayed by two ices subjected to coring operations at low temperatures and under vacuum. The ices used in this study were water ice, frozen from liquid water, and carbon dioxide ice grown from its vapour. The coring tool employed had dimensions and required power levels that were comparable to a sample extraction system designed for a present-day spacecraft lander. The specific cutting strength, a parameter that measures the toughness of the material, has been measured while coring these two ices. For water ice this property rose from at an ice temperature of , to at . At the lower temperature of , pore-free carbon dioxide ice has also been measured to have a specific cutting strength approximately half that of water ice at the same temperature. These laboratory-based measurements may be used as guides for the power levels needed to core solid water and CO₂ ices at certain rates.  相似文献   

南极昭和站大气中CO_2浓度变化          下载免费PDF全文

曲绍厚  山内恭 《极地研究》1991,3(1):54-58

本文作者于1987～1988年由国家南极考察委员会派遣随JARE29赴日本南极昭和站、瑞穗站和阿斯加等站进行考察,根据日本同行提供的1984～1988年昭和站大气中二氧化碳浓度连续变化资料以及相应年份该站年平均气温资料进行研究,结果表明:从1984年到1988年该站大气中二氧化碳浓度变化趋势与该站年平均气温变化趋势是相当一致的,二者呈明显正相关。此外,还给出该地区从1984年到1988年大气中二氧化碳浓度变化的年增长率,其值分别为1.21ppmV/年(1984～1985年)、1.35ppmV/年(1985～1986年)、1.68ppmV/年(1986～1987年)和1.99ppmV/年(1987～1988年)。  相似文献   

Phosphorus and dissolved silicon dynamics in the River Swale catchment,UK: a mass‐balance approach     

M. J. Bowes  W. A. House 《水文研究》2001,15(2):261-280

The internal riverine processes acting upon phosphorus and dissolved silicon were investigated along a 55 km stretch of the River Swale during four monitoring campaigns. Samples of river water were taken at 3 h intervals at sites on the main river and the three major tributaries. Samples were analysed for soluble reactive phosphorus, total dissolved phosphorus, total phosphorus, dissolved silicon and suspended solid concentration. Mass‐balances for each determinand were calculated by comparing the total load entering the river with the total load measured at the downstream site. The difference, i.e. the residual load, showed that there was a large retention of phosphorus and silicon within the system during the March 1998 flood event, but the other three campaigns produced net‐exports. Cumulative residual loads were calculated for each determinand at 6 h intervals throughout each campaign. This incremental approach showed that the mass‐balance residuals followed relatively consistent patterns under various river discharges. During stable low‐flow, there was a retention of particulate phosphorus within the system and also a retention of total dissolved phosphorus and soluble reactive phosphorus, most likely caused by the sorption of soluble phosphorus by bed‐sediments. In times of high river‐discharge, there was a mobilization and export of stored bed‐sediment phosphorus. During overbank flooding, there was a large retention (58% of total input) of particulate phosphorus within the system, due to the mass deposition of phosphorus‐rich sediment onto the floodplain. Soluble phosphorus was also retained within the system by sequestration from the water column by the high concentration of suspended solids. The dissolved silicon mass‐balance residuals had a less consistent pattern in relation to river discharge. There was a large retention of dissolved silicon during overbank flooding, possibly due to sorption onto floodplain soil, and net‐exports during periods of both stable low‐flow and rising limbs of hydrographs, due to release of dissolved silicon from pore‐waters. Copyright © 2001 John Wiley & Sons, Ltd.  相似文献