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11.
Assessment of alternative adsorption models and global sensitivity analysis to characterize hexavalent chromium loss from soil to surface runoff 下载免费PDF全文
We investigate our ability to assess transfer of hexavalent chromium, Cr(VI), from the soil to surface runoff by considering the effect of coupling diverse adsorption models with a two‐layer solute transfer model. Our analyses are grounded on a set of two experiments associated with soils characterized by diverse particle size distributions. Our study is motivated by the observation that Cr(VI) is receiving much attention for the assessment of environmental risks due to its high solubility, mobility, and toxicological significance. Adsorption of Cr(VI) is considered to be at equilibrium in the mixing layer under our experimental conditions. Four adsorption models, that is, the Langmuir, Freundlich, Temkin, and linear models, constitute our set of alternative (competing) mathematical formulations. Experimental results reveal that the soil samples characterized by the finest grain sizes are associated with the highest release of Cr(VI) to runoff. We compare the relative abilities of the four models to interpret experimental results through maximum likelihood model calibration and four model identification criteria (i.e., the Akaike information criteria [AIC and AICC] and the Bayesian and Kashyap information criteria). Our study results enable us to rank the tested models on the basis of a set of posterior weights assigned to each of them. A classical variance‐based global sensitivity analysis is then performed to assess the relative importance of the uncertain parameters associated with each of the models considered, within subregions of the parameter space. In this context, the modelling strategy resulting from coupling the Langmuir isotherm with a two‐layer solute transfer model is then evaluated as the most skilful for the overall interpretation of both sets of experiments. Our results document that (a) the depth of the mixing layer is the most influential factor for all models tested, with the exception of the Freundlich isotherm, and (b) the total sensitivity of the adsorption parameters varies in time, with a trend to increase as time progresses for all of the models. These results suggest that adsorption has a significant effect on the uncertainty associated with the release of Cr(VI) from the soil to the surface runoff component. 相似文献
12.
盐水沟北铜矿区位于新疆库车县北部,其大地构造位置处于塔吉克-塔里木陆块区、塔里木陆块、塔里木北缘隆起、库车前陆盆地,区内构造活动强烈。铜矿床赋存于新近纪中新统康村组第一岩性段,矿体呈层状,严格受地层控制。区内共圈定10个铜矿体,矿石矿物主要为孔雀石、赤铜矿、水胆矾、自然铜等,矿体内无夹石,顶、底板围岩均为褐红色及浅红色粉质泥岩。该矿床为砂岩型铜矿床。 相似文献
13.
全球气候变化下南海诸岛保护优先区识别分析 总被引:3,自引:1,他引:2
全球变化下,珊瑚礁保护区是保护生物多样性、增强珊瑚礁对气候变暖抵抗力的有效方式,而维持珊瑚礁弹性是其核心内容。针对珊瑚礁最具有威胁性的热压力因子,基于南海1982—2009年卫星观测海表面温度(SST)数据和CMIP5加拿大地球系统模式CanESM2模型预估的2006—2100年南海SST数据构建热压力强度模型,从维持珊瑚礁弹性的角度识别IPCC RCP 4.5和RCP 8.5情景下南海诸岛保护优先区。结果表明:RCP 4.5和RCP 8.5情景下13%左右的南海诸岛珊瑚礁识别为保护优先区。根据热压力强度与珊瑚抵抗力及避难所关系,西沙群岛七连屿和晋卿岛近年观测与未来预估的热压力强度均比较低,在保障其服务功能的基础上建议实施完全保护;东沙群岛东沙环礁和中沙环礁排洪滩近年观测急性热压力强度较高但未来预估热压力强度较低,建议实施50%禁止利用保护;中沙群岛黄岩岛近年观测和未来预估的急性热压力强度均比较低,建议实施50%多用途保护。南沙群岛有14%左右的珊瑚礁识别为保护优先区,根据其热压力强度可实施30%~100%禁止利用保护或30%~50%多用途保护。RCP 4.5和RCP 8.5情景下的南海诸岛保护优先区及保护对策,可为维持珊瑚礁生态弹性及应对全球气候变化提供重要的参考价值。 相似文献
14.
Fangli Zhang 《International journal of geographical information science》2019,33(10):1984-2010
High-performance simulation of flow dynamics remains a major challenge in the use of physical-based, fully distributed hydrologic models. Parallel computing has been widely used to overcome efficiency limitation by partitioning a basin into sub-basins and executing calculations among multiple processors. However, existing partition-based parallelization strategies are still hampered by the dependency between inter-connected sub-basins. This study proposed a particle-set strategy to parallelize the flow-path network (FPN) model for achieving higher performance in the simulation of flow dynamics. The FPN model replaced the hydrological calculations on sub-basins with the movements of water packages along the upstream and downstream flow paths. Unlike previous partition-based task decomposition approaches, the proposed particle-set strategy decomposes the computational workload by randomly allocating runoff particles to concurrent computing processors. Simulation experiments of the flow routing process were undertaken to validate the developed particle-set FPN model. The outcomes of hourly outlet discharges were compared with field gauged records, and up to 128 computing processors were tested to explore its speedup capability in parallel computing. The experimental results showed that the proposed framework can achieve similar prediction accuracy and parallel efficiency to that of the Triangulated Irregular Network (TIN)-based Real-Time Integrated Basin Simulator (tRIBS). 相似文献
15.
16.
《Sedimentology》2018,65(6):2055-2087
This study, conducted in the Catalan Coastal Ranges, north‐east Spain, describes the Upper Devonian Kellwasser event in a shallowing‐upward sequence of black shales, siltstones and quartz arenites. This sequence was deposited in a progradational and regressive coastal system where the sedimentary environment evolved from the inner shelf to a lagoonal pond located landward of the shoreline. Three anomalous succeeding steps have been identified by geochemical analysis. The first one, detected on the inner shelf, was characterized by oxygen depletion and high organic productivity. The second, detected in the nearshore, was caused by hydrothermal activity occurring under normal oxic conditions. The third and most intense step was identified in the muds of the lagoonal pond and has been linked to strong anoxic conditions, elevated clastic input derived from changes in the weathering regime at the source area and moderate hydrothermal activity. The Kellwasser event is thus defined in the study area as stepwise and multi‐causal. This is the first time that the Kellwasser event has been identified in a sedimentary environment behind the shoreline. It is also the first time that it has been reported in the Catalan Coastal Ranges. 相似文献
17.
为了得出雾霾气象成因机制、影响因素和时空分布特征,以石家庄市区与郊县为研究区域,将2013年9月至2016年12月石家庄市各市区、郊县的PM2.5历史监测数据中的有效数据进行了数据分析处理得到雾霾浓度数据,还有温度、降水、风速、地形和人口密度等数据,运用GIS分析的方法,模拟绘制石家庄雾霾的时空分布图、雾霾与各影响因子的专题对比图,得到雾霾形成机制的因子、雾霾的时空分布规律、雾霾季节变化特征、雾霾与地形间的关系等;运用数据分析软件OriginPro8.SR3分析雾霾浓度与风速数据、降雨数据、温度数据间的相关性。 相似文献
18.
利用 2000—2015 年的 EOS/MODIS 数据,采用趋势分析、Hurst 指数、变异系数法对伊犁河 谷植被时空变化及未来趋势进行分析,结果显示:空间分布上,伊犁河谷植被覆盖度呈北部、南部、 东部偏高,西部、中部偏低的分布特征;时间变化上,2000—2015 年,伊犁河谷植被覆盖度波动减 小,减速为 6.25%·(10 a)-1;区域分布上,伊犁河谷植被表现为低波动变化,波动程度中等以及下占 73.16%,波动程度高的区域占 26.84%。未来预测表明,伊犁河谷植被覆盖呈退化趋势,其中,持续 退化的面积占 57.55%,持续改善的面积占 13.51%。 相似文献
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采用香港11个GPS测站的观测资料进行1 h、2 h、3 h和4h静态PPP解算,获得4组PPP坐标序列,利用调和分析求取11个测站处8个主要分潮的负荷位移参数(振幅和相位),将其与海潮模型计算的负荷位移参数进行对比,并比较分析PPP反演值与海潮模型值改正海潮负荷信号的效果。结果表明,垂直和水平方向上,不同PPP结果反演8个分潮的负荷位移分别具有约5 mm和7 mm的差异;PPP反演8个分潮垂向负荷位移优于全球海潮模型,但水平方向上的反演效果稍弱。 相似文献